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The digital economy is crucial to promoting green technology innovation and development. However, there needs to be more research on the relationship between the digital economy, digital talent aggregation (DTA), and green technology innovation (GTI). Therefore, based on the data from 30 provinces, municipalities, and autonomous regions in mainland China (excluding Tibet) from 2011 to 2020, this paper uses fixed effect, threshold effect, moderating effect model, and spatial econometric model to make an empirical analysis of this research direction. The results show that (1) there is a nonlinear relationship between the digital economy and green technology innovation (GTI). This effect has regional heterogeneity effects. In the central and western regions, the digital economy is more prominent in promoting green technology innovation (GTI). (2) Digital talent aggregation (DTA) has a negative moderating effect on the influence of the digital economy on promoting green technology innovation (GTI). (3) The negative spillover effect of the digital economy on local green technology innovation (GTI) will be intensified at the spatial level due to the accumulation of digital talents. Therefore, this paper suggests that the government should actively and reasonably develop the digital economy to promote green technology innovation (GTI). In addition, the government can implement a flexible talent introduction policy, strengthen talent quality education and talent service station construction. [ABSTRACT FROM AUTHOR]