Search

A scintillating bolometer based on a large cubic Li$_{2}$$^{100}$MoO$_4$crystal (45 mm side) and a Ge wafer (scintillation detector) has been operatedin the CROSS cryogenic facility at the Canfranc underground laboratory inSpain. The dual-readout detector is a prototype of the technology that will beused in the next-generation $0\nu2\beta$ experiment CUPID. The measurementswere performed at 18 and 12 mK temperature in a pulse tube dilutionrefrigerator. This setup utilizes the same technology as the CUORE cryostatthat will host CUPID and so represents an accurate estimation of the expectedperformance. The Li$_{2}$$^{100}$MoO$_4$ bolometer shows a high energyresolution of 6 keV FWHM at the 2615 keV $\gamma$ line. The detection ofscintillation light for each event triggered by the Li$_{2}$$^{100}$MoO$_4$bolometer allowed for a full separation ($\sim$8$\sigma$) between$\gamma$($\beta$) and $\alpha$ events above 2 MeV. The Li$_{2}$$^{100}$MoO$_4$crystal also shows a high internal radiopurity with $^{228}$Th and $^{226}$Raactivities of less than 3 and 8 $\mu$Bq/kg, respectively. Taking also intoaccount the advantage of a more compact and massive detector array, which canbe made of cubic-shaped crystals (compared to the cylindrical ones), this testdemonstrates the great potential of cubic Li$_{2}$$^{100}$MoO$_4$ scintillatingbolometers for high-sensitivity searches for the $^{100}$Mo $0\nu2\beta$ decayin CROSS and CUPID projects.

A scintillating bolometer based on a large cubic Li$_{2}$$^{100}$MoO$_4$crystal (45 mm side) and a Ge wafer (scintillation detector) has been operatedin the CROSS cryogenic facility at the Canfranc underground laboratory inSpain. The dual-readout detector is a prototype of the technology that will beused in the next-generation $0u2\beta$ experiment CUPID. The measurementswere performed at 18 and 12 mK temperature in a pulse tube dilutionrefrigerator. This setup utilizes the same technology as the CUORE cryostatthat will host CUPID and so represents an accurate estimation of the expectedperformance. The Li$_{2}$$^{100}$MoO$_4$ bolometer shows a high energyresolution of 6 keV FWHM at the 2615 keV $\gamma$ line. The detection ofscintillation light for each event triggered by the Li$_{2}$$^{100}$MoO$_4$bolometer allowed for a full separation ($\sim$8$\sigma$) between$\gamma$($\beta$) and $\alpha$ events above 2 MeV. The Li$_{2}$$^{100}$MoO$_4$crystal also shows a high internal radiopurity with $^{228}$Th and $^{226}$Raactivities of less than 3 and 8 $\mu$Bq/kg, respectively. Taking also intoaccount the advantage of a more compact and massive detector array, which canbe made of cubic-shaped crystals (compared to the cylindrical ones), this testdemonstrates the great potential of cubic Li$_{2}$$^{100}$MoO$_4$ scintillatingbolometers for high-sensitivity searches for the $^{100}$Mo $0u2\beta$ decayin CROSS and CUPID projects.

An organic glass scintillator developed by Sandia National Laboratories was characterized in terms of its light output and pulse shape discrimination (PSD) properties and compared to commercial liquid (EJ-309) and plastic (EJ-276) organic scintillators. The electron light output was determined through relative comparison of the 137Cs Compton edge location. The proton light yield was measured using a double time-of-flight technique at the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory. Using a tunable broad-spectrum neutron source and an array of pulse-shape-discriminating observation scintillators, a continuous measurement of the proton light yield was performed for EJ-309 (200 keV–3.2 MeV), EJ-276 (170 keV–4.9 MeV), and the organic glass (50 keV–20 MeV). Finally, the PSD properties of the organic glass, EJ-309, and EJ-276 were evaluated using an AmBe source and compared via a figure-of-merit metric. The organic glass exhibited a higher electron light output than both EJ-309 and EJ-276. Its proton light yield and PSD performance were comparable to EJ-309 and superior to that of EJ-276. With these performance characteristics, the organic glass scintillator is well poised to replace current state-of-the-art PSD-capable scintillators in a range of fast neutron detection applications.

Medical imaging instrumentation is mostly based on the use of luminescent materials coupled to optical sensors. These materials are employed in the form of granular screens, structured crystals, single transparent crystals, ceramics, etc. Storage phosphors are also incorporated in particular X-ray imaging systems. The physical properties of these materials should match the criteria required by the detective systems employed in morphological and functional biomedical imaging. The systems are analyzed based on theoretical frameworks emanating from the linear cascaded systems theory as well as the signal detection theory. Optical diffusion has been studied by different methodological approaches, such as experimental measurements and analytical modeling, including geometrical optics and Monte Carlo simulation. Analysis of detector imaging performance is based on image quality metrics, such as the luminescence emission efficiency (LE), the modulation transfer function (MTF), the noise power spectrum (NPS), and the detective quantum efficiency (DQE). Scintillators and phosphors may present total energy conversion on the order of 0.001–0.013 with corresponding DQE in the range of 0.1–0.6. Thus, the signal-to-noise ratio, which is crucial for medical diagnosis, shows clearly higher values than those of the energy conversion.

We report on the development of scintillating bolometers based on lithium molybdate crystals that contain molybdenum that has depleted into the double- β active isotope 100 Mo (Li 2 100 depl MoO 4 ). We used two Li 2 100 depl MoO 4 cubic samples, each of which consisted of 45-millimeter sides and had a mass of 0.28 kg; these samples were produced following the purification and crystallization protocols developed for double- β search experiments with 100 Mo-enriched Li 2 MoO 4 crystals. Bolometric Ge detectors were utilized to register the scintillation photons that were emitted by the Li 2 100 depl MoO 4 crystal scintillators. The measurements were performed in the CROSS cryogenic set-up at the Canfranc Underground Laboratory (Spain). We observed that the Li 2 100 depl MoO 4 scintillating bolometers were characterized by an excellent spectrometric performance (∼3–6 keV of FWHM at 0.24–2.6 MeV γ s), moderate scintillation signal (∼0.3–0.6 keV/MeV scintillation-to-heat energy ratio, depending on the light collection conditions), and high radiopurity ( 228 Th and 226 Ra activities are below a few µBq/kg), which is comparable with the best reported results of low-temperature detectors that are based on Li 2 MoO 4 using natural or 100 Mo-enriched molybdenum content. The prospects of Li 2 100 depl MoO 4 bolometers for use in rare-event search experiments are briefly discussed. [ABSTRACT FROM AUTHOR]

Lutetium oxyorthosilicate Lu2SiO5 (LSO) and pyrosilicate Lu2Si2O7 (LPS) activated by Ce3+ or Pr3+ are known to be effective and fast scintillation materials for the detection of X-rays and γ-rays. Their performances can be further improved by co-doping with aliovalent ions. Herein, we investigate the Ce3+(Pr3+) → Ce4+(Pr4+) conversion and the formation of lattice defects stimulated by co-doping with Ca2+ and Al3+ in LSO and LPS powders prepared by the solid-state reaction process. The materials were studied by electron paramagnetic resonance (EPR), radioluminescence spectroscopy, and thermally stimulated luminescence (TSL), and scintillation decays were measured. EPR measurements of both LSO:Ce and LPS:Ce showed effective Ce3+ → Ce4+ conversions stimulated by Ca2+ co-doping, while the effect of Al3+ co-doping was less effective. In Pr-doped LSO and LPS, a similar Pr3+ → Pr4+ conversion was not detected by EPR, suggesting that the charge compensation of Al3+ and Ca2+ ions is realized via other impurities and/or lattice defects. X-ray irradiation of LPS creates hole centers attributed to a hole trapped in an oxygen ion in the neighborhood of Al3+ and Ca2+. These hole centers contribute to an intense TSL glow peak at 450–470 K. In contrast to LPS, only weak TSL peaks are detected in LSO and no hole centers are visible via EPR. The scintillation decay curves of both LSO and LPS show a bi-exponential decay with fast and slow component decay times of 10–13 ns and 30–36 ns, respectively. The decay time of the fast component shows a small (6–8%) decrease due to co-doping. [ABSTRACT FROM AUTHOR]

Two-photon excitation in light-sheet microscopy advances applications to live imaging of multicellular organisms. In a previous study, we developed a two-photon Bessel beam light-sheet microscope with a nearly 1-mm field of view and less than 4-μm axial resolution, using a low magnification (10×), middle numerical aperture (NA 0.5) detection objective. In this study, we aimed to construct a light-sheet microscope with higher resolution imaging while maintaining the large field of view, using low magnification (16×) with a high NA 0.8 objective. To address potential illumination and detection mismatch, we investigated the use of a depth of focus (DOF) extension method. Specifically, we used a stair-step device composed of five-layer annular zones that extended DOF two-fold, enough to cover the light-sheet thickness. Resolution measurements using fluorescent beads showed that the reduction in resolutions was small. We then applied this system to in vivo imaging of medaka fish and found that image quality degradation at the distal site of the beam injection could be compensated. This demonstrates that the extended DOF system combined with wide-field two-photon light-sheet microscopy offers a simple and easy setup for live imaging application of large multicellular organism specimens with sub-cellular resolution. [ABSTRACT FROM AUTHOR]

Free-space optical (FSO) communication has been studied for next-generation network systems. Because an FSO system establishes point-to-point communication links, maintaining alignment among the transceivers is a critical challenge. In addition, atmospheric turbulence causes significant signal loss in FSO vertical links. Even in clear weather conditions, transmitted optical signals suffer significant scintillation losses due to random variations. Thus, the effect of atmospheric turbulence should be considered in vertical links. In this paper, we analyze the relationship between pointing error and scintillation from the aspect of beam divergence angle. Furthermore, we propose an adaptive beam that optimizes its divergence angle according to the pointing error between the communicating optical transceivers to mitigate the effect of scintillation due to pointing error. We performed a beam divergence angle optimization and compared it with adaptive beamwidth. The proposed technique was demonstrated using simulations, which revealed an enhanced signal-to-noise ratio and the mitigation of the scintillation effect. The proposed technique would be useful in minimizing the scintillation effect in vertical FSO links. [ABSTRACT FROM AUTHOR]

The green-emitting plastic scintillators with high transparence, short decay time and high quantum yield were fabricated by the modified thermal polymerization procedure. The effects of different concentrations of primary and secondary fluorescent dopants on photoluminescence performance, such as fluorescence intensity, decay time and absolute quantum yield, were investigated through orthogonal experiments. The optimal formula ratio for the plastic scintillator was that the primary dopant concentration was 0.25 wt.% and the secondary dopant concentration was 0.03 wt.%. The photoluminescence decay time of the optimal sample was 3.37 ns, which was faster than that of EJ-260 (6.57 ns) and its corresponding quantum yield was 91.57%, compared to that of EJ-260 (98.59%). [ABSTRACT FROM AUTHOR]

Xenon is a widely used detector target material due to its excellent scintillation properties in the ultraviolet (UV) spectrum. The additional use of infrared (IR) scintillation light could improve future detectors. However, a comprehensive characterization of the IR component is necessary to explore its potential. We report on the first measurement of the time profile of the IR scintillation response of gaseous xenon. Our setup consists of a gaseous xenon target irradiated by an alpha particle source and is instrumented with one IR- and two UV-sensitive photomultiplier tubes. Thereby, it enables IR timing measurements with nanosecond resolution and simultaneous measurement of UV and IR signals. We find that the IR light yield is in the same order of magnitude as the UV yield. We observe that the IR pulses can be described by a fast and a slow component and demonstrate that the size of the slow component decreases with increasing levels of impurities in the gas. Moreover, we study the IR emission as a function of pressure. These findings confirm earlier observations and advance our understanding of the IR scintillation response of gaseous xenon, which could have implications for the development of novel xenon-based detectors. [ABSTRACT FROM AUTHOR]

Within the framework of an interionic potential model, electrostatic and repulsive energies, lattice self-potentials for distinct ions, and the Madelung constant were calculated for several technologically important layered alkaline-earth fluorohalide scintillators belonging to the matlockite family and crystallizing with the PbFCl-type structure. The Coulombic term was computed using the conventional Ewald method, where the formulas were adjusted to optimize the computer calculation, and the overlap repulsive term was computed by means of an empirical approach based on the compressible ionic theory. The dispersive contribution was quantified using well-known formulations, and the polarization contribution was determined purely by geometric considerations based on both the size and anisotropic coordination of the highly polarizable halogen atom. In general, the obtained results were found to be in close agreement with the available data, except for the contribution of short-range interactions in the lattice. A quantitative explanation has been proposed to elucidate the differences detected. It was pointed out that the structural stability of these lamellar structures can be understood in terms of the anisotropic coordination of halogen anions, especially the high coordination of metal cations combined with their sizes. Our calculations led to an accurate evaluation of the cohesive energy, which, to the best of our knowledge, has never been measured before. Finally, the corresponding results will be useful for a better understanding of the chemical bonds and structural behavior of PbFCl-type compounds at high pressures. [ABSTRACT FROM AUTHOR]

Mg4Ta2O9 single crystals doped with 0.01, 0.1, and 1% Er were grown using the floating zone method, and their photoluminescence and scintillation properties were studied. X-ray diffraction analysis confirmed that all samples had a hexagonal structure of Mg4Ta2O9. The samples showed that the emission peak at 1550 nm was due to 4f−4f transitions of Er3+ ions, with quantum yields of 32.9, 46.6, and 18.0% for 0.01, 0.1, and 1% doping concentrations, respectively. All samples showed scintillation with a broad emission band at 350 nm due to charge transfer from Ta5+ to O2− ions and emission peak at 1550 nm due to 4f−4f transition of Er3+ ions. The dose rate response functions showed that the detection limit for all samples was 0.06 Gy/h for scintillation detector applications. [ABSTRACT FROM AUTHOR]

Digital spectroscopy with Silicon Photomultiplier (SiPM) array coupled on CsI(Tl) crystal, needs some consideration to achieve desirable energy resolution. an array of SiPMs must be used with large scintillation crystal, therewithal signal from whole SiPMs is not ideal. Also silicon pixels are arranged in arrays at regular intervals. The distances between the pixels and the interference of the cross-talk of adjacent pixels are undesirable factors for energy resolution when the light is received by the crystal and transmitted to the SiPM array. On the other hand, due to the advantages of the SiPM array, there is a need to improve the energy resolution in order to be able to be applied. In this paper, an attempt is made to obtain the desired energy resolution by using the digital spectroscopy method and digital filters and properly shaping the output pulse of the preamplifier by the trapezoidal filter method. In this case, it will be possible to use it in different applications such as spectroscopy by the detector. [ABSTRACT FROM AUTHOR]

In the present study, radon concentration has been estimated in drinking water samples of different locations of Lolab in Kupwara district of Kashmir valley. A scintillation based detector, (Smart RnDuo) has been used to evaluate the radon concentration in collected drinking water samples. In addition, the surface contamination of gamma radiations at each location was detected using portable gamma ray detector (PM 1405, Polimaster Inc., USA). The radon concentration in drinking water samples has been found to vary from 3.27 to 59.50 BqL-1, with an average of 23.65 BqL-1.The annual inhalation dose varied from 0.01 to 0.15 mSvy-1. The average annual inhalation dose was found to be 0.06 mSvy-1 and it lies well within the permissible limits. [ABSTRACT FROM AUTHOR]

Radon-resistant materials are of great importance for High Background Radiation Areas. Depending on the radon diffusion coefficient, waterproofing and radon-resistant materials with thicknesses ranging from a few microns to several centimeters are used in various parts of the world. The cost of installation of an effective radon mitigation system varied with material properties, i.e., thickness and diffusion coefficient. The present study is concerned with the measurement of the radon diffusion coefficient through single and multilayer homogeneous and heterogeneous stacks of various waterproofing materials. One, two, and three layers of polyethylene, printing paper, mica sheets, PVC sheets, Mylar sheets and aluminum foil of varying thicknesses are tested for determination of diffusion length by the two-chamber method and the active scintillation radon monitor. The radon diffusion coefficient of materials varies from 10-13m²/s to 10-8m²/s for PVC sheet to paper sheet when a single layer is used and 10-11 m²/s to 10-13 m²/s for aluminum and polyethylene sheets in multilayer stack arrangement. The radon diffusion coefficient for most of the materials reduces with increasing layers in the stack. By the use of these materials, 85-90 % of radon can be reduced by using single or multi-layer stack combination. [ABSTRACT FROM AUTHOR]

β-Ga2O3 is a well-known semiconductor material for power devices and other applications. Recently, β-Ga2O3 has also been reported as a scintillator material with a light yield of approximately 8400 ph./MeV, scintillation decay time of <1 μs, and density of 6.44 g/cm3. In this study, 45 cm diameter β-Ga2O3 single crystals were prepared via oxide crystal growth using the cold crucible (OCCC) method under various oxygen partial pressures. In the OCCC method, as in the cold crucible method, a high frequency is applied directly to the oxide materials, which are heated and melted, and the melt is held by the outermost solid material itself that is cooled by water using a copper hearth. In the OCCC method, crystal growth is performed while rotating the seed crystal, as in the Czochralski method, to increase the crystal diameter. The optical properties and radiation responses of the crystals grown under various oxygen partial pressures were evaluated. [ABSTRACT FROM AUTHOR]

Scintillating materials that convert ionizing radiation into low‐energy photons hold great potential for radiation detection, nondestructive inspection, medical radiography, and space exploration. However, organic scintillators are characterized by low radioluminescence, while bulky inorganic scintillators are not suitable for the development of flexible detectors. Here, high‐resolution X‐ray imaging using solution‐processable lanthanide‐based metal–organic frameworks as microscale scintillators is demonstrated. Mechanistic studies suggest that lanthanide ions absorb X‐rays to generate high‐density molecular triplet excitons, and excited linkers subsequently sensitize lanthanide ions via nonradiative resonance energy transfer. Furthermore, the crystalline nature offers a delocalized electronic feature rather than isolated subunits, which enables direct trapping of charge carriers by lanthanide emitters. By controlling the concentration ratio between Tb3+ and Eu3+ ions, efficient and color‐tunable radioluminescence of lanthanide ions can be achieved. When coupled with elastic, transparent polymer matrices, these metal–organic framework‐based microscintillators allow the fabrication of flexible X‐ray detectors. Such detectors feature a detection limit of 23 nGy s−1, which is 240 times lower than the typical radiation dose for medical diagnosis. X‐ray imaging with resolution higher than 16.6 line pairs per millimeter is further demonstrated. These findings provide insight into the future design of hybrid scintillators for optoelectronics and X‐ray sensing and imaging. [ABSTRACT FROM AUTHOR]

Luminescence clusters composed of organic ligands and metals have gained significant interests as scintillators owing to their great potential in high X-ray absorption, customizable radioluminescence, and solution processability at low temperatures. However, X-ray luminescence efficiency in clusters is primarily governed by the competition between radiative states from organic ligands and nonradiative cluster-centered charge transfer. Here we report that a class of Cu4I4 cubes exhibit highly emissive radioluminescence in response to X-ray irradiation through functionalizing biphosphine ligands with acridine. Mechanistic studies show that these clusters can efficiently absorb radiation ionization to generate electron-hole pairs and transfer them to ligands during thermalization for efficient radioluminescence through precise control over intramolecular charge transfer. Our experimental results indicate that copper/iodine-to-ligand and intraligand charge transfer states are predominant in radiative processes. We demonstrate that photoluminescence and electroluminescence quantum efficiencies of the clusters reach 95% and 25.6%, with the assistance of external triplet-to-singlet conversion by a thermally activated delayed fluorescence matrix. We further show the utility of the Cu4I4 scintillators in achieving a lowest X-ray detection limit of 77 nGy s−1 and a high X-ray imaging resolution of 12 line pairs per millimeter. Our study offers insights into universal luminescent mechanism and ligand engineering of cluster scintillators. X-ray luminescence efficiency of copper halide clusters is limited by nonradiative charge transfer. Here, Zhang et al. report highly emissive radioluminescence of Cu4I4 cubes by functionalizing biphosphine ligands with acridine, unlocking the potential use as low-cost and eco-friendly scintillators. [ABSTRACT FROM AUTHOR]

Highlights: The classification of 2D perovskite is summarized, and the preparation methods of 2D perovskite according to the requirements of X-ray detection materials are introduced. We analyzed the advantages and insufficiency of different devices and introduced improvement measures, including ion migration, charge transfer performance, stability, and 2D/3D heterojunctions. Finally, we introduced the potential preponderances of 2D perovskite in the scintillation detection field; meanwhile, the main challenges facing the practical application of 2D perovskite X-ray detectors are analyzed. Metal halide perovskites have recently emerged as promising candidates for the next generation of X-ray detectors due to their excellent optoelectronic properties. Especially, two-dimensional (2D) perovskites afford many distinct properties, including remarkable structural diversity, high generation energy, and balanced large exciton binding energy. With the advantages of 2D materials and perovskites, it successfully reduces the decomposition and phase transition of perovskite and effectively suppresses ion migration. Meanwhile, the existence of a high hydrophobic spacer can block water molecules, thus making 2D perovskite obtain excellent stability. All of these advantages have attracted much attention in the field of X-ray detection. This review introduces the classification of 2D halide perovskites, summarizes the synthesis technology and performance characteristics of 2D perovskite X-ray direct detector, and briefly discusses the application of 2D perovskite in scintillators. Finally, this review also emphasizes the key challenges faced by 2D perovskite X-ray detectors in practical application and presents our views on its future development. [ABSTRACT FROM AUTHOR]

The article describes the combination of experimental measurements with mathematical–physics analyses in flow investigation in the chambers of the scintillator detector, which is a part of the environmental scanning electron microscope. The chambers are divided with apertures by small openings that keep the desirable pressure differences between three chambers: The specimen chamber, the differentially pumped intermediate chamber, and the scintillator chamber. There are conflicting demands on these apertures. On the one hand, the diameter of the apertures must be as big as possible so that they incur minimal losses of the passing secondary electrons. On the other hand, it is possible to magnify the apertures only to a certain extent so the rotary and turbomolecular vacuum pump can maintain the required operating pressures in separate chambers. The article describes the combination of experimental measurement using an absolute pressure sensor and mathematical physics analysis to map all the specifics of the emerging critical supersonic flow in apertures between the chambers. Based on the experiments and their tuned analyses, the most effective variant of combining the sizes of each aperture concerning different operating pressures in the detector is determined. The situation is made more difficult by the described fact that each aperture separates a different pressure gradient, so the gas flow through each aperture has its own characteristics with a different type of critical flow, and they influence each other, thereby influencing the final passage of secondary electrons detected by the scintillator and thus affecting the resulting displayed image. [ABSTRACT FROM AUTHOR]

In positron emission tomography (PET), parallax errors degrade spatial resolution. The depth of interaction (DOI) information provides the position in the depth of the scintillator interacting with the γ-rays, thus reducing parallax errors. A previous study developed a Peak-to-Charge discrimination (PQD), which can separate spontaneous alpha decay in LaBr3:Ce. Since decay constant of GSO:Ce depends on Ce concentration, the PQD is expected to discriminate GSO:Ce scintillators with different Ce concentration. In this study, the PQD-based DOI detector system was developed, which can be processed online and implemented in PET. A detector was composed of four layers of GSO:Ce crystals and a PS-PMT. The four crystals were obtained from both the top and bottom of ingots with a nominal Ce concentration of 0.5 mol% and 1.5 mol%. The PQD was implemented on the Xilinx Zynq-7000 SoC board with 8ch Flash ADC to gain real-time processing, flexibility, and expandability. The results showed that the mean Figure of Merits in 1D between four scintillators are 1.5, 0.99, 0.91 for layers between 1st–2nd, 2nd–3rd, and 3rd–4th respectively, and the mean Error Rate in 1D between four scintillators are 3.50%, 2.96%, 13.3%, and 1.88% for layers 1, 2, 3, and 4, respectively. In addition, the introduction of the 2D PQDs resulted in the mean Figure of Merits in 2D greater than 0.9 and the mean Error Rate in 2D less than 3% in all layers. [ABSTRACT FROM AUTHOR]

Scintillator glasses have the potential for X-ray imaging owing to their low production cost, controllable shape and size, and uniform ion-doping concentration. In this study, Tb3+-doped and Ce3+/Tb3+-co-doped oxyfluoride scintillator (C4T9) glass samples were fabricated by high-temperature melting and quenching. In addition, the luminescence properties of the glass samples and the discrepancy in the energy transfer mechanism between Ce3+ and Tb3+ under ultraviolet (UV) light and X-ray excitation were investigated. The C4T9 glass sample showed excellent integral scintillation efficiency of 84.1% for commercial Bi 4 Ge 3 O 12 (BGO) crystals. The spatial resolution of the C4T9 glass sample was higher than that of the commercial BGO crystal with 42.29 mGy s−1 X-ray irradiation, reaching 16 lp·mm−1. C4T9 glass is expected to become a key material in medical imaging, safety inspection, industrial inspection, and other fields. [ABSTRACT FROM AUTHOR]

Lead halide perovskites have recently emerged as promising X/γ-ray scintillators. However, the small Stokes shift of exciton luminescence in perovskite scintillators creates problems for the light extraction efficiency and severely impedes their applications in hard X/γ-ray detection. Dopants have been used to shift the emission wavelength, but the radioluminescence lifetime has also been unwantedly extended. Herein, we demonstrate the intrinsic strain in 2D perovskite crystals as a general phenomenon, which could be utilized as self-wavelength shifting to reduce the self-absorption effect without sacrificing the radiation response speed. Furthermore, we successfully demonstrated the first imaging reconstruction by perovskites for application of positron emission tomography. The coincidence time resolution for the optimized perovskite single crystals (4 × 4 × 0.8 mm3) reached 119 ± 3 ps. This work provides a new paradigm for suppressing the self-absorption effect in scintillators and may facilitate the application of perovskite scintillators in practical hard X/γ-ray detections. Efficient light extraction in perovskite X/γ-ray scintillators is hindered by the small Stokes shift of exciton luminescence. Here, Jin et al. exploit the intrinsic strain in 2D perovskite as "self-wavelength shifting" to reduce the self-absorption effect without sacrificing the device response speed. [ABSTRACT FROM AUTHOR]

Scintillation crystals Gd3Al2Ga3O12 (GAGG) are an excellent candidate for application in ionizing-radiation detectors because of their high radiation resistance, density and light yield. These crystals can be used in combination with lead tungstate (PbWO4 or PWO) crystals for the development of a new generation of electromagnetic calorimeter with advanced spatial and energy resolutions in a broad energy range. PWO crystals enable the accurate detection of high-energy photons, while GAGG crystals provide the possibility of precisely measuring photon energies, down to a few MeV. Different options for a composite electromagnetic calorimeter based on PWO and GAGG crystals are considered to optimize spatial and energy resolutions in a broad energy range (from 1 MeV to 100 GeV). In particular, different lengths of the GAGG section of the calorimeter are considered, from 0.5 to 10 cm. The separation of signals from photons and hadrons is also taken into consideration through the study of shower shape in the calorimeter. The optimization is based on Geant4 simulations, considering light collection as well as the use of different photodetectors and electronic noise. Simulations are verified with light yield measurements of GAGG samples obtained using radioactive sources and test beam measurements of the prototype of the PWO-based Photon Spectrometer of the ALICE experiment at CERN. [ABSTRACT FROM AUTHOR]

The present study introduces the heterogeneous quasi-continuous spiking cortical model (HQC-SCM) method as a novel approach for neutron and gamma-ray pulse shape discrimination. The method utilizes specific neural responses to extract features in the falling edge and delayed fluorescence parts of radiation pulse signals. In addition, the study investigates the contributions of HQC-SCM's parameters to its discrimination performance, leading to the development of an automatic parameter selection strategy. As HQC-SCM is a chaotic system, a genetic algorithm-based parameter optimization method was proposed to locate local optima of HQC-SCM's parameter solutions efficiently and robustly in just a few iterations of evolution. The experimental results of this study demonstrate that the HQC-SCM method outperforms traditional and state-of-the-art pulse shape discrimination algorithms, including falling edge percentage slope, zero crossing, charge comparison, frequency gradient analysis, pulse-coupled neural network, and ladder gradient methods. The outstanding discrimination performance of HQC-SCM enables plastic scintillators to compete with liquid and crystal scintillators' neutron and gamma-ray pulse shape discrimination ability. Additionally, the HQC-SCM method outperforms other methods when dealing with noisy radiation pulse signals. Therefore, it is an effective and robust approach that can be applied in radiation detection systems across various fields. [ABSTRACT FROM AUTHOR]

Cerium-doped lutetium-yttrium oxyorthosilicate (Ce:LYSO) is a well-known single crystal scintillator used in medical imaging and security scanners. Recent development of high power UV LED, matching its absorption band, questions the possibility to use Ce:LYSO in a new way: as LED-pumped solid-state light source. Since Ce:LYSO is available in large size crystals, we investigate its potential as a luminescent concentrator. This paper reports an extensive study of the performance in close relation to the spectroscopic properties of this crystal. It gives the reasons why the Ce:LYSO crystal tested in this study is less efficient than Ce:YAG for luminescent concentration: limited quantum efficiency and high losses coming from self-absorption and from excited-state absorption are playing key roles. However, we demonstrate that a Ce:LYSO luminescent concentrator is an innovative source for solid-state lighting. Pumped by a peak power of 3400 W in quasi-continuous wave regime (40 µs, 10 Hz), a rectangular (1 × 22 × 105 mm3) Ce:LYSO crystal delivers a broadband spectrum (60 nm FWHM) centered at 430 nm. At full output aperture (20 × 1 mm2), it emits a peak power of 116 W. On a squared output surface (1 × 1 mm2) it emits 16 W corresponding to a brightness of 509 W cm–2 sr–1. This combination of spectrum power and brightness is higher than blue LEDs and opens perspectives for Ce:LYSO in the field of illumination namely for imaging. [ABSTRACT FROM AUTHOR]

Gallium nitride is a wide-direct-bandgap semiconductor suitable for the creation of modern optoelectronic devices and radiation tolerant detectors. However, formation of dislocations is inevitable in MOCVD GaN materials. Dislocations serve as accumulators of point defects within space charge regions covering cores of dislocations. Space charge regions also may act as local volumes of enhanced non-radiative recombination, deteriorating the photoluminescence efficiency. Surface etching has appeared to be an efficient means to increase the photoluminescence yield from MOCVD GaN materials. This work aimed to improve the scintillation characteristics of MOCVD GaN by a wet etching method. An additional blue photo-luminescence (B-PL) band peaking at 2.7–2.9 eV and related to dislocations was discovered. This B-PL band intensity appeared to be dependent on wet etching exposure. The intensity of the B-PL was considerably enhanced when recorded at rather low temperatures. This finding resembles PL thermal quenching of B-PL centers. The mechanisms of scintillation intensity and spectrum variations were examined by coordinating the complementary photo-ionization and PL spectroscopy techniques. Analysis of dislocation etch pits was additionally performed by scanning techniques, such as confocal and atomic force microscopy. It was proved that this blue luminescence band, which peaked at 2.7–2.9 eV, is related to point defects those decorate dislocation cores. It was shown that the intensity of this blue PL band was increased due to enhancement of light extraction efficiency, dependent on the surface area of either single etch-pit or total etched crystal surface. [ABSTRACT FROM AUTHOR]

Cerium-doped gadolinium aluminum gallium garnet (Ce3+:Gd3Al3Ga2O12, Ce3+:GAGG) ceramic is a promising scintillation material. In this study, Ce3+:Gd3Al3Ga2O12 scintillation ceramics were prepared by the one-step sintering of commercially available Gd2O3, Al2O3, Ga2O3, and CeO2 powders in a flowing oxygen atmosphere at 1600 °C by solid-phase reaction sintering. For all the Ce3+:Gd3Al3Ga2O12 ceramic samples doped with different amounts of Ce3+ doping, dense ceramics were obtained. The structure, photoluminescence, and scintillation properties of the Ce3+:Gd3Al3Ga2O12 ceramics have been investigated. The average grain size of samples sintered at 1600 °C is about 2 μm. The X-ray excitation luminescence peak is around 560 nm, which is consistent with that of Ce3+:Gd3Al3Ga2O12 single crystals, matching well with the computed tomography X-ray detector's response sensitivity. The light yield is higher compared to the standard reference sample—lutetium yttrium orthosilicate single crystal. [ABSTRACT FROM AUTHOR]

The occurrence probability of equatorial plasma bubbles and the associated spread F (ESF) irregularities have been derived from ground-based and space-borne measurements. In general, ESF occurrence depends on season and longitude and is high in equinoctial months and low around June solstice. In the West Pacific sector, previous statistical results show that the ESF occurrence probability increases gradually and continuously from March to August. In this study, we use trans-ionospheric VHF data received at Kwajalein Atoll in 2012 to derive the occurrence characteristics of scintillation. It is found that the occurrence probability of strong scintillation had two maxima in June and September and a minimum in July in the evening and midnight sector but only one maximum in June in the post-midnight sector. The monthly variations of scintillation occurrence at Kwajalein are different from almost all previous studies on ESF and scintillation at or near this longitude. To identify the cause for the June peak and the July minimum of scintillation, the ion density and velocity data measured by the Communication/Navigation Outage Forecasting System (C/NOFS) satellite in 2011–2012 are used to derive the ESF occurrence and the post-sunset vertical ion drift near Kwajalein. The ESF occurrence probability and the ion drift measured by the C/NOFS satellite showed two maxima in May/June and August/September and a minimum in July, verifying that the June peak and the July minimum of the VHF scintillation are realistic and caused by the similar variations in the ionospheric ion drift and density. [ABSTRACT FROM AUTHOR]

Energy nonlinearity and resolution in liquid scintillator (LS) detectors are correlated and particle-dependent. A unified energy response model for liquid scintillator detectors has been presented in details. This model has advanced a data-driven approach to calibrate the particle-dependent energy response, using both the monoenergetic γ -ray sources and the continuous β spectra of 12 B and Michel e - induced by cosmic muons. Monte Carlo studies have demonstrated the effectiveness and robustness of the proposed model, in particular, the positron energy resolution can be extracted in the absence of positron sources. This work will provide a feasible approach of simultaneous calibration of energy nonlinearity and resolution for the running and future LS detectors. [ABSTRACT FROM AUTHOR]

Random coincidences of events could be one of the main sources of background in the search for neutrino-less double-beta decay of 100 Mo with macro-bolometers, due to their modest time resolution. Scintillating bolometers as those based on Li 2 MoO 4 crystals and employed in the CROSS and CUPID experiments can eventually exploit the coincident fast signal detected in a light detector to reduce this background. However, the scintillation provides a modest signal-to-noise ratio, making difficult a pile-up pulse-shape recognition and rejection at timescales shorter than a few ms. Neganov–Trofimov–Luke assisted light detectors (NTL-LDs) offer the possibility to effectively increase the signal-to-noise ratio, preserving a fast time-response, and enhance the capability of pile-up rejection via pulse shape analysis. In this article we present: (a) an experimental work performed with a Li 2 MoO 4 scintillating bolometer, studied in the framework of the CROSS experiment, and utilizing a NTL-LD; (b) a simulation method to reproduce, synthetically, randomly coincident two-neutrino double-beta decay events; (c) a new analysis method based on a pulse-shape discrimination algorithm capable of providing high pile-up rejection efficiencies. We finally show how the NTL-LDs offer a balanced solution between performance and complexity to reach background index ∼ 10 - 4 counts/keV/kg/year with 280 g Li 2 MoO 4 ( 100 Mo enriched) bolometers at 3034 keV, the Q β β of the double-beta decay, and target the goal of a next generation experiment like CUPID. [ABSTRACT FROM AUTHOR]

Terahertz (THz) technology has great potential for applications in various fields, such as security imaging detection, optical communication, environmental quality monitoring, and life sciences. Most of these applications require THz detectors with high sensitivity, fast response, and a miniaturized size that can operate at room temperature. In this study, we present a graphene THz detector integrated with an asymmetric bowtie antenna. The asymmetric antenna confines the incident THz waves into the graphene active layer, leading to photocurrent generation and its directional flow. The maximum responsivity of this device can reach 19.6 V/W at 2.52 THz, with a noise–equivalent power (NEP) of 0.59 nW /Hz0.5. Additionally, the response time is less than 21 μs, with an active area of less than 1500 μm2. Such a small device enables THz imaging with a spatial resolution as small as 200 μm. These results provide a feasible way to design miniaturized and integrable two–dimensional material–based THz detectors. [ABSTRACT FROM AUTHOR]

The linear response of a photomultiplier tube (PMT) is a required property for photon counting and reconstruction of the neutrino energy. The linearity valid region and the saturation response of a PMT were investigated using a linear-alkylbenzene (LAB)-based liquid scintillator. A correlation was observed between the two different saturation responses, with pulse-shape distortion and pulse-area decrease. The observed pulse shape provides useful information for the estimation of the linearity region relative to the pulse area. This correlation-based diagnosis allows an in situ estimation of the linearity range, which was previously challenging. The measured correlation between the two saturation responses was employed to train an artificial neural network (ANN) to predict the decrease in pulse area from the observed pulse shape. The ANN-predicted pulse-area decrease enables a prediction of the ideal number of photoelectrons regardless of the saturation behavior. This pulse-shape-based machine-learning technique offers a novel method for restoring the saturation response of PMTs. [ABSTRACT FROM AUTHOR]

High-resolution imaging of alpha particles is required in the detection of alpha radionuclides in cells or small organs for the development of radio-compounds for targeted alpha-particle therapy or other purposes. We developed an ultrahigh resolution, real time alpha-particle imaging system for observing the trajectories of alpha particles in a scintillator. The developed system is based on a magnifying unit and a cooled electron multiplying charge-coupled device (EM-CCD) camera, combined with a 100-µm-thick Ce-doped Gd3Al2Ga3O12 (GAGG) scintillator plate. Alpha particles from an Am-241 source were irradiated to the GAGG scintillator and imaged with the system. Using our system, we measured the trajectories of the alpha particles having different shapes in real time. In some of these measured trajectories, the line shapes of the alpha particles that flew in the GAGG scintillator were clearly observed. The lateral profiles of the alpha-particle trajectories were imaged with widths of ~ 2 µm. We conclude that the developed imaging system is promising for research on targeted alpha-particle therapy or other alpha particle detections that require high spatial resolution. [ABSTRACT FROM AUTHOR]

A compact back-end interface for silicon photomultipliers (SiPMs) implementing Zener diode-based temperature compensation has been developed for the remote detection of beta and gamma radiation. Remote detection is facilitated by the development of an efficient data management system utilising MySQL database storage for recording periodic spectra data for wireless access over a private Wi-Fi network. A trapezoidal peak shaping algorithm has been implemented on an FPGA for the continuous conversation of pulses from the SiPM, signifying the detection of a radiological particle, into spectra. This system has been designed to fit within a 46 mm cylindrical diameter for in situ characterization, and can be attached to one or more SiPMs used in conjunction with a range of scintillators. LED blink tests have been used to optimise the trapezoidal shaper coefficients to maximise the resolution of the recorded spectra. Experiments with an array of SiPMs integrated with a NaI(Tl) scintillator exposed to sealed sources of Co-60, Cs-137, Na-22 and Am-241 have shown that the detector achieves a peak efficiency of 27.09 ± 0.13% for a gamma peak at 59.54 keV produced by Am-241, and a minimum energy resolution (Delta E/E) of 4.27 ± 1.16% for the 1332.5 keV gamma peak from Co-60. [ABSTRACT FROM AUTHOR]

Synthesis in the radiation field is a promising direction for the development of materials transformation processes, especially those differing in melting temperature. It has been established that the synthesis of yttrium–aluminum ceramics from yttrium oxides and aluminum metals in the region of a powerful high-energy electron flux is realized in 1 s, without any manifestations that facilitate synthesis, with high productivity. It is assumed that the high rate and efficiency of synthesis are due to processes that are realized with the formation of radicals, short-lived defects formed during the decay of electronic excitations. This article presents descriptions of the energy-transferring processes of an electron stream with energies of 1.4, 2.0, and 2.5 MeV to the initial radiation (mixture) for the production of YAG:Ce ceramics. YAG:Ce (Y3Al5O12:Ce) ceramics samples in the field of electron flux of different energies and power densities were synthesized. The results of a study of the dependence of the morphology, crystal structure, and luminescence properties of the resulting ceramics on the synthesis modes, electron energy, and electron flux power are presented. [ABSTRACT FROM AUTHOR]

Micron/sub-micron hard X-ray imaging is an important development direction of X-ray detection technology. Scintillation screens with excellent X-ray stopping power and high light output are desired to obtain good imaging quality. Europium-doped lutetium oxide (Lu 2 O 3 :Eu) film with micro-columnar structure is an ideal candidate for this application. In this study, micro-columnar structured Lu 2 O 3 :Eu films were prepared on quartz glass substrates by laser chemical vapor deposition (LCVD) method. The influences of preparation conditions on structure and morphology properties of films were investigated by X-ray diffraction (XRD) and scanning electron microscopy (SEM). Photoluminescence and scintillation properties of the films, including photoluminescence excitation (PLE), photoluminescence (PL), PL decay, X-ray excitation luminescence (XEL), and afterglow curves, were recorded. The relationships between structure, morphology, luminescence properties of films, and preparation conditions were investigated and discussed as well. The preparation conditions include laser power, oxygen flow rate, and precursor evaporation temperature. In addition, dual-layer Lu 2 O 3 :Eu film was prepared for the first time by just turning off the laser. [ABSTRACT FROM AUTHOR]

Background: The Jagiellonian Positron Emission Tomograph is the 3-layer prototype of the first scanner based on plastic scintillators, consisting of 192 half-metre-long strips with readouts at both ends. Compared to crystal-based detectors, plastic scintillators are several times cheaper and could be considered as a more economical alternative to crystal scintillators in future PETs. JPET is also a first multi-photon PET prototype. For the development of multi-photon detection, with photon characterized by the continuous energy spectrum, it is important to estimate the efficiency of J-PET as a function of energy deposition. The aim of this work is to determine the registration efficiency of the J-PET tomograph as a function of energy deposition by incident photons and the intrinsic efficiency of the J-PET scanner in detecting photons of different incident energies. In this study, 3-hit events are investigated, where 2-hits are caused by 511 keV photons emitted in e + e - annihilations, while the third hit is caused by one of the scattered photons. The scattered photon is used to accurately measure the scattering angle and thus the energy deposition. Two hits by a primary and a scattered photon are sufficient to calculate the scattering angle of a photon, while the third hit ensures the precise labeling of the 511 keV photons. Results: By comparing experimental and simulated energy distribution spectra, the registration efficiency of the J-PET scanner was determined in the energy deposition range of 70–270 keV, where it varies between 20 and 100 % . In addition, the intrinsic efficiency of the J-PET was also determined as a function of the energy of the incident photons. Conclusion: A method for determining registration efficiency as a function of energy deposition and intrinsic efficiency as a function of incident photon energy of the J-PET scanner was demonstrated. This study is crucial for evaluating the performance of the scanner based on plastic scintillators and its applications as a standard and multi-photon PET systems. The method may be also used in the calibration of Compton-cameras developed for the ion−beam therapy monitoring and simultaneous multi-radionuclide imaging in nuclear medicine. [ABSTRACT FROM AUTHOR]

LIDAL (Light Ion Detector for ALTEA, Anomalous Long-Term Effects on Astronauts) is a radiation detector designed to measure the flux, the energy spectra and, for the first time, the time-of-flight of ions in a space habitat. It features a combination of striped silicon sensors for the measurement of deposited energy (using the ALTEA device, which operated from 2006 to 2012 in the International Space Station) and fast scintillators for the time-of-flight measurement. LIDAL was tested and calibrated using the proton beam line at TIFPA (Trento Institute for Fundamental Physics Application) and the carbon beam line at CNAO (National Center for Oncology Hadron-therapy) in 2019. The performance of the time-of-flight system featured a time resolution (sigma) less than 100 ps. Here, we describe the detector and the results of these tests, providing ground calibration curves along with the methodology established for processing the detector's data. LIDAL was uploaded in the International Space Station in November 2019 and it has been operative in the Columbus module since January 2020. [ABSTRACT FROM AUTHOR]

Radioactivity is a form of natural radiation, and it is measured in becquerels (Bq) using the SI system. Both human activities and natural processes can produce radioactivity. For this study, three regions on the South Tamilnadu coastline in India, namely Manavalakurichi, Colachel, and Kudankulam, were chosen. A dual-channel alpha-beta counter was used to measure gross alpha and beta activity based on the scintillation principle. The radioactive nuclide activity concentrations in soil and water were measured, and the levels were considered acceptable. The alpha and beta radiation levels in soil and water samples did not significantly differ. The study's results suggest that the risk of radiation danger in the study area is not significantly increased because the values obtained are within the generally accepted limits. The ANOVA experiments also revealed that there was no significant difference in the gross alpha and beta activity of soil and water samples. Moreover, the alpha and beta activity in drinking water was lower in all three areas than what is recommended by the WHO. Therefore, it can be concluded that the drinking water in these three regions is safe for consumption. [ABSTRACT FROM AUTHOR]

Recent progress in the field of scintillators and silicon photomultipliers (SiPM) has allowed development of new scintillation detectors capable of detecting low-energy X- and gamma-ray sources that are widely used in medicine, security and industry. Such scintillation detectors are compact, insensitive to magnetic fields, have low operation voltages and are functional at room temperature. These advantages of SiPM are considered to solve the main problems facing scintillation detectors in medicine and industry today. Development of detectors of low-energy electromagnetic radiation is relevant now. Scintillation detectors based on lutetium fine silicate, LaBr3(Ce), NaI and silicon avalanche photomultipliers offer a great potential for use for X- and gamma-ray detection. The present work demonstrates the gamma-ray detection performance of a new micropixel avalanche photodiode (MAPD) array (16 (4×4) elements - 15×15 cm) with a LaBr3(Ce) scintillator (15×15×30 mm) using 177Lu and 133Ba isotopes as the gamma-ray sources. [ABSTRACT FROM AUTHOR]

The study deals with the use of different amounts of MgO or tetraethyl orthosilicate (C 8 H 20 O 4 Si, TEOS), from 0.04 wt %, 0.06 wt %, 0.08 wt %, 0.4 wt %, 0.6 wt % to 0.8 wt %, respectively, as additional sintering aids during the vacuum sintering of transparent Ce3+ doped Y 3 Al 5 O 12 (Ce:YAG) ceramics to investigate their effect on microstructure and luminescence properties. A comparative study was carried out by using X - ray diffraction, scanning electron microscopy/energy dispersive X - ray spectroscopy, optical and photo-luminesce spectra, as well as electroluminescent spectra. The dominant garnet phase was obtained even when adding 0.8 wt % of MgO or TEOS, while adding MgO led to finer average grain size (∼ 5 - 10 μm) and more homogenous distribution compared to TEOS (∼ 20 - 25 μm) in Ce:YAG ceramics. Adding a large amount of MgO was found to result in the segregation of MgO in Ce:YAG ceramics, while an excess of TEOS led to the segregation of Al 2 O 3. A strong absorption peak at 308 nm was observed in Ce:YAG ceramics with MgO sintering aids, which was ascribed to the existence of Ce4+ induced by a charge compensation effect of Mg2+. The optimum transmittance reached 80% @ 800 nm in Ce:YAG ceramics when adding 0.6 wt % TEOS, which also exhibited a maximum luminous efficacy of 106 lm/W. Si4+ was experimentally proved to have a better optimization effect on luminous efficacy compared to Mg2+. • MgO or TEOS (C 8 H 20 O 4 Si) was added as additional sintering aids in a wide amount range. • MgO proves to have distinct inhibit effect on the grain growth. • Better luminous efficacy were observed in ceramics with TEOS additives. [ABSTRACT FROM AUTHOR]

Sesquioxides of lanthanides, yttrium, and scandium are promising hosts for laser and scintillation materials; however, the crystallization of such compounds is complicated by very high melting temperatures, as well as polymorph transitions. This work reports for the first time the growth of Y2O3 and Y2−xScxO3 crystals by the Vertical Gradient Freezing method from tungsten crucibles, proposing an alternative to extremely expensive rhenium and iridium crucibles. Translucent Y2O3 samples are obtained, and their luminescent and scintillation parameters are evaluated. The main issues of Y2O3 crystallization under the proposed conditions are discussed, as well as ways of enhancing the crystal quality. Finally, polymorph transitions are avoided by decreasing the average radius of the rare earth cation by Y3+/Sc3+ substitution, providing transparent Y2−xScxO3 crystals with a cubic structure. [ABSTRACT FROM AUTHOR]

We investigate scintillation linearity of a commercial high pressure 4He gas detector using monoenergetic 2.8 MeV neutrons from a deuterium-deuterium fusion neutron generator. The scintillation response of the detector was measured for a range of recoil energies between 83 keV and 626 keV by tagging neutrons scattering into fixed angles with a far-side organic scintillator detector. Detailed Monte Carlo simulations were compared to experimental data to determine the linearity of the detector response by comparing the scaling of the energy deposits in the simulations to the detector output. In this analysis, a linear scintillation response corresponds to a consistent value for the scaling factor between simulated energy deposits and experimental data for several different scattering angles. We demonstrate that the detector can be used to detect fast neutron interactions down to 83 keV recoil energies and can be used to characterize low-energy neutron sources, one of its potential applications.

Simultaneous measurement of phonon and light signatures is an effective way to reduce the backgrounds and increase the sensitivity of CUPID, a next-generation bolometric neutrinoless double-beta decay (0νββ) experiment. Light emission in tellurium dioxide (TeO2) crystals, one of the candidate materials for CUPID, is dominated by faint Cherenkov radiation, and the high refractive index of TeO2 complicates light collection. Positive identification of 0νββ events therefore requires high-sensitivity light detectors and careful optimization of light transport. A detailed microphysical understanding of the optical properties of TeO2 crystals is essential for such optimization. We present a set of quantitative measurements of light production and transport in a cubic TeO2 crystal, verified with a complete optical model and calibrated against a UVT acrylic standard. We measure the optical surface properties of the crystal, and set stringent limits on the amount of room-temperature scintillation in TeO2 for β and α particles of 5.3 and 8 photons/MeV, respectively, at 90% confidence. The techniques described here can be used to optimize and verify the particle identification capabilities of CUPID.

Abstract Copper-based metal halides have become important materials in the field of X-ray and photodetection due to their excellent optical properties, good environmental stability and low toxicity. This review presents the progress of research on crystal structure/morphology, photophysics/optical properties and applications of copper-based metal halides. We also discuss the challenges of copper-based metal halides with a perspective of their future research directions. Graphical Abstract

Thermal neutron detection is a key subject for nuclear physics research and also in a wide variety of applications from homeland security to nuclear medicine. In this work, it is proposed a novel flexible and conformable composite thermal neutron scintillator based on a fully enriched Lithium Tetraborate preparation ( 6 Li 2 10 B 4 O 7 ) combined with a phosphorescent inorganic scintillator powder (ZnS:Ag), and is then distributed into a polydimethylsiloxane matrix. The proposed scintillator shows a good neutron detection efficiency (max. ∼ 57% with respect to the commercial EJ-420), an average light output of ∼ 9000 ph/neutron-capture, a remarkable insensitivity to γ -rays (Gamma Rejection Ratio <10 - 11 ), and an extraordinary flexibility, so as to reach extremely small curvature radii, down to 1.5 mm, with no signs of cracking or tearing. Its characteristics make it suitable to be employed in scenarios where non-standard geometries are needed, for example, to optimize the detector performance and/or maximize the detection efficiency. Finally, the response of a hybrid detector made of a plastic scintillator, wrapped with the proposed scintillator, coupled to a silicon photomultiplier array is described, and the excellent discrimination between γ -rays, fast and thermal neutrons resulting from data processing is demonstrated. [ABSTRACT FROM AUTHOR]

The occurrence of plasma irregularities and ionospheric scintillation over the Caribbean region have been reported in previous studies, but a better understanding of the source and conditions leading to these events is still needed. In December 2021, three ground-based ionospheric scintillation and Total Electron Content monitors were installed at different locations over Puerto Rico to better understand the occurrence of ionospheric irregularities in the region and to quantify their impact on transionospheric signals. Here, the findings for an event that occurred on March 13–14, 2022 are reported. The measurements made by the ground-based instrumentation indicated that ionospheric irregularities and scintillation originated at low latitudes and propagated, subsequently, to mid-latitudes. Imaging of the ionospheric F-region over a wide range of latitudes provided by the GOLD mission confirmed, unequivocally, that the observed irregularities and the scintillation were indeed caused by extreme equatorial plasma bubbles, that is, bubbles that reach abnormally high apex heights. The joint ground- and space-based observations show that plasma bubbles reached apex heights exceeding 2600 km and magnetic dip latitudes beyond 28°. In addition to the identification of extreme plasma bubbles as the source of the ionospheric perturbations over low-to-mid latitudes, GOLD observations also provided experimental evidence of the background ionospheric conditions leading to the abnormally high rise of the plasma bubbles and to severe L-band scintillation. These conditions are in good agreement with the theoretical hypothesis previously proposed. [ABSTRACT FROM AUTHOR]