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NOX (NOX = NO + NO2) emissions measurements in Beijing are of great significance because they can aid in understanding how NOX pollution develops in mega-cities throughout China. However, NOX emissions in mega-cities are difficult to measure due to changes in wind patterns and moving sources on roads during measurement. To obtain good spatial coverage on different ring roads in Beijing over a short amount of time, two mobile differential optical absorption spectroscopy (DOAS) instruments were used to measure NOX emission flux from April 18th to 26th, 2018. In addition, a wind profile radar provided simultaneous wind field measurements for altitudes between 50 m and 1 km for each ring road measurement. We first determined NOX emission flux of different ring roads using wind field averages from measured wind data. The results showed that the NOX emission flux of Beijing's fifth ring road, which represented the urban part, varied from (19.29 ± 5.26) × 1024 molec./s to (36.46 ± 12.86) × 1024 molec./s. On April 20th, NOX emission flux for the third ring was slightly higher than the fourth ring because the two ring roads were measured at different time periods. We then analyzed the NOX emission flux error budget and error sensitivity. The main error source was the wind field uncertainty. For some measurements, the main emission flux error source was either wind speed uncertainty or wind direction uncertainty, but not both. As Beijing's NOX emissions came from road vehicle exhaust, we found that emission flux error had a more diverse sensitivity to wind direction uncertainty, which improved our knowledge on this topic. The NOX emission flux error sensitivity study indicated that more accurate measurements of the wind field are crucial for effective NOX emission flux measurements in Chinese mega-cities. Obtaining actual time and high resolved wind measurements is an advantage for mega-cities' NOX emission flux measurements. The emission flux errors caused by wind direction and wind speed uncertainties were clearly distinguished. Other sensitivity studies indicated that NOX/NO2 ratio uncertainty dominated flux errors when the NOX/NO2 ratio uncertainty was >0.4. Using two mobile-DOAS and wind profile radars to measure NOx emission flux improved the quality of the emission flux measuring results. This approach could be applied to many other mega-cities in China and in others countries. [ABSTRACT FROM AUTHOR]

Clouds are significant in the global radiation budget, atmospheric circulation, and hydrological cycle. However, knowledge regarding the observed climatology of the cloud vertical structure (CVS) over Beijing is still poor. Based on high-resolution radiosonde observations at Beijing Nanjiao Weather Observatory (BNWO) during the period 2010–2017, the method for identifying CVS depending on height-resolved relative humidity thresholds is improved, and CVS estimation by radiosonde is compared with observations by millimeter-wave cloud radar and ceilometer at the same site. Good consistency is shown between the three instruments. Then, the CVS climatology, including the frequency distribution and seasonal variation, is investigated. Overall, the occurrence frequency (OF) of cloudy cases in Beijing is slightly higher than that of clear-sky cases, and the cloud OF is highest in summer and lowest in winter. Single-layer clouds and middle-level clouds are dominant in Beijing. In addition, the average cloud top height (CTH), cloud base height (CBH), and cloud thickness in Beijing are 6.2 km, 4.0 km, and 2.2 km, respectively, and show the trend of reaching peaks in spring and minimums in winter. In terms of frequency distribution, the CTH basically resides below an altitude of 16 km, and approximately 43% of the CBHs are located at altitudes of 0.5–1.5 km. The cloud OF has only one peak located at altitudes of 4–8 km in spring, whereas it shows a trimodal distribution in other seasons. The height at which the cloud OF reaches its peak is highest in summer and lowest in winter. To the best of our knowledge, the cloud properties analyzed here are the first to elucidate the distribution and temporal variation of the CVS in Beijing from a long-term sounding perspective, and these results will provide a scientific observation basis for improving the atmospheric circulation model, as well as comparisons and verifications for measurements by ground-based remote sensing equipment. [ABSTRACT FROM AUTHOR]

Based on application of the atomic filter technology in a signal detection system of lidar, the diurnal observation of sodium lidar were obtained using the system at the National Space Science Center of the Chinese Academy of Sciences at Beijing Yanqing station (40.5° N, 116° E) in April 2014. During the lidar observation period, among the 103 cases of continuous daytime observations, the longest time was 181 h. In the case of a continuous observation period of 5 days (13–18 October 2014), the signal-to-noise ratio reached to 19:1 at 12:00–13:00 Local Time of the daytime, when the spatial and time resolutions were respectively set to 96 m of 167 s. The improvements resulted in the highest detection level of any existing diurnal lidars in China. Some interesting phenomena such as the sporadic sodium layer have also been observed during the daytime. The daytime capability extended the observing time range of the earlier systems that were limited to only nighttime observations. This innovation provides a useful method for the studies of diurnal tides, photochemistry, gravity waves, and correlative modeling studies. [ABSTRACT FROM AUTHOR]