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In the work, a composite cooling system coupled with PCM (phase change material) and liquid cooling was designed. The influence of parameters such as spacing, EG (expanded graphite) content, battery direction, coolant flow rate and pipe diameter on the cooling performance was analyzed. The results revealed that: (1) The increase of spacing makes the temperature of the pack decrease, but the effect degree of increasing the spacing on temperature performance decreases when the spacing exceeds 14 mm. At the same time, CPCM formed by the added high thermal conductivity material expanded graphite and paraffin can effectively improve the temperature control performance of the pack, which can control the temperature at 313.15K under the condition of an ambient temperature of 308.15K (2) By comparing the maximum temperature and the temperature difference of the pack under different discharge methods, it is concluded that the poles facing inward can reduce the accumulation of the interior heat. (3) The convective heat transfer coefficient and Nu number of the pack are increasing as the flow rate increases, but the slope of the temperature versus flow rate decreasing slowly. After increasing the inlet size, the inner wall surface area of the pipe increases and the average convective heat transfer coefficient of the pack reduces. However, the Nu number increases with the increase of the pipe diameter, indicating that the growth of the pipe diameter can enhance the heat transfer rate. (4) Orthogonal experiment and fuzzy correlation analysis were combined to analyze the parameters that affect the thermal performance of the BTMS. It was determined that using a proper coolant flow rate can maximize the thermal performance of the pack. • A composite cooling system coupled with PCM and liquid cooling is designed. • Influences of the key parameters on the cooling performance are analyzed. • Orthogonal experiment and fuzzy correlation analysis are used to analyze affecting parameters. • Some results for enhancing cooling performance are obtained. [ABSTRACT FROM AUTHOR]

• Composite PCM is designed by in-situ constructing phase changeable framework in PEG. • The novel composite PCM possesses dual phase change temperature regions (PCTRs). • The two PCTRs are precisely tailored at 31.7–42.1 ℃ and 42.1–51.2 ℃, respectively. • The lower PCTR ensures suitable working temperature for battery at normal operation. • The higher PCTR prevents thermal hazards of battery under high ambient temperature. The phase change material (PCM)-based battery thermal management technology still remains a contradiction of guaranteeing a suitable operating temperature (20–40 ℃) of the batteries under regular working conditions, while avoiding the malfunction of the PCM under high ambient temperature (>40 ℃). Therefore, a novel composite PCM (CPCM) possessing dual phase change temperature regions (PCTRs) is designed herein by in-situ constructing a phase-changeable polymer (PCP) framework in the polyethylene glycol (PEG)/expanded graphite (EG) slurry. As prepared, the lower PCTR at 31.7–42.1 ℃ from the PCP framework provides a latent heat of 35.0 J g−1, while the higher PCTR at 42.1–51.2 ℃ from the PEG offers a latent heat of 68.3 J g−1. Additionally, the nanoscaled PCP framework strongly adsorbs the PEG, preventing the leakage phenomenon (mass loss < 1%), and the uniformly dispersed EG endows the CPCM with a high thermal conductivity of 1.98 W m−1 K−1. In consequence, under the normal ambient temperature of 25 ℃, the lower PCTR effectively keeps the battery module operating within the suitable temperature range of 25.9–34.9 ℃ and with a low temperature difference (ΔT) of 2.4 ℃ at the discharge rate of 1C. For comparison, the battery module adopting classical CPCM with a single PCTR at 40.9–55.1 ℃ demonstrates a much higher temperature range and maximum ΔT at 28.0–40.9 ℃ and 4.8 ℃, respectively. Under the high ambient temperature of 40 ℃, the higher PCTR starts to work like the single PCTR of traditional CPCMs, and controls the T max and ΔT of the module below 49.2 and 2.2 ℃ at the discharge rate of 1C, respectively, preventing thermal hazards. [ABSTRACT FROM AUTHOR]

Lithium-ion batteries (LIBs) are extremely sensitive to their temperature and therefore, require a battery thermal management system (BTMS). BTMS is commonly employed to prevent thermal runaway of the LIB pack by controlling their operating temperature. This review paper provides various cooling strategies, including active and passive approaches, utilized in BTMSs. Air-cooled, liquid-based, and PCM-cooled techniques are first reviewed. This article presents an assessment of the application of nanofluids and nano-phase change materials (nano-PCMs) in BTMSs to improve heat dissipation from the LIB pack. This work emphasizes the utilization of these materials to intensify their thermal conductivity and suggests further investigations on their application in BTMSs. • Lithium-ion batteries are extremely sensitive to their temperature. • BTMS is employed to prevent battery thermal runaway by controlling its temperature. • Providing various cooling strategies for BTMS: active and passive approaches. • Presenting an assessment of the application of nanofluids and nano-PCMs) in BTMSs. [ABSTRACT FROM AUTHOR]

The optimal performance of a Li-ion battery is directly impacted by temperature. In order to control the temperature rise and provide even temperature distributions in the battery pack, a thermal management scheme comprises thin heat sinks with multiple phase change materials (PCMs) and air channels is investigated in this paper. The cooling performance and temperature homogenization of the battery thermal management (BTM) system are carefully studied under various configurations of PCMs. The results show that increasing the air inlet velocity has less effect in suppressing the temperature rise at early discharge stage, but ameliorates as the discharge prolonged to 3600 s. The standard deviation of the temperature (STDV) and maximum temperature of the batteries can be decreased by arranging PCMs with a lower melting temperature at the midsection and a higher melting temperature at the air outlet region of the heat sinks. In addition, for volume fraction of PCMs, Case IV, having a PCM with a higher melting point adjacent to the air outlet region and occupying one-half the height of the heat sink, illustrates a lower temperature rise and decreases the maximum temperature in the battery module by 1.024 K, 2.186 K, and 2.553 K, compared to Case I, II, and III, respectively. • Multiple PCMs incorporated thin heat sinks for battery thermal management is proposed. • The thermal performance of the battery based on maximum temperature upsurge is investigated. • The distributions of PCMs based on melting point and latent heat were carefully explored. • The optimal design for the distribution of PCMs is obtained for the proposed battery. [ABSTRACT FROM AUTHOR]