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Future space-based interferometers offer an unprecedented opportunity to detect signals from the stochastic gravitational wave background originating from a first-order phase transition at the electroweak scale. The phase transition is accompanied by a change of the equation of state from that of pure radiation. In this work we study the effect of this change on the power spectrum of gravitational waves generated by the sound waves in the plasma during the acoustic phase of the transition. We carry out an analytic calculation assuming that the sound speed and the fluid shear-stress that sources tensor perturbations remain approximately constant during the acoustic phase. The effect of a softer equation of state is twofold: (i) a scale-independent suppression of the power spectrum at all scales, due to the modified propagation of both sound and gravitational waves and (ii) the peak of the spectrum moves to smaller frequencies as the equation of state becomes softer. The power-law indices of the spectrum at small and large scales are unaffected by the softening of the equation of state. Our work improves the current estimation of the gravitational waves power spectrum from first order phase transitions and expands the possible scenarios of transitions that can be tested by gravitational wave detectors., Comment: 21 pages + 7 pages of Appendix

The broad physics reach of the LUX-ZEPLIN (LZ) experiment covers rare phenomena beyond the direct detection of dark matter. We report precise measurements of the extremely rare decay of $^{124}$Xe through the process of two-neutrino double electron capture (2$\nu$2EC), utilizing a $1.39\,\mathrm{kg} \times \mathrm{yr}$ isotopic exposure from the first LZ science run. A half-life of $T_{1/2}^{2\nu2\mathrm{EC}} = (1.09 \pm 0.14_{\text{stat}} \pm 0.05_{\text{sys}}) \times 10^{22}\,\mathrm{yr}$ is observed with a statistical significance of $8.3\,\sigma$, in agreement with literature. First empirical measurements of the KK capture fraction relative to other K-shell modes were conducted, and demonstrate consistency with respect to recent signal models at the $1.4\,\sigma$ level., Comment: 15 pages, 3 figures

Quantum computing has tremendous potential to overcome some of the fundamental limitations present in classical information processing. Yet, today's technological limitations in the quality and scaling prevent exploiting its full potential. Quantum computing based on superconducting quantum processing units (QPUs) is among the most promising approaches towards practical quantum advantage. In this article the basic technological approach of IQM Quantum Computers is described covering both the QPU and the rest of the full-stack quantum computer. In particular, the focus is on a 20-qubit quantum computer featuring the Garnet QPU and its architecture, which we will scale up to 150 qubits. We also present QPU and system-level benchmarks, including a median 2-qubit gate fidelity of 99.5% and genuinely entangling all 20 qubits in a Greenberger-Horne-Zeilinger (GHZ) state.

This paper analyses Conversational AI multi-agent interoperability frameworks and describes the novel architecture proposed by the Open Voice Interoperability initiative (Linux Foundation AI and DATA), also known briefly as OVON (Open Voice Network). The new approach is illustrated, along with the main components, delineating the key benefits and use cases for deploying standard multi-modal AI agency (or agentic AI) communications. Beginning with Universal APIs based on Natural Language, the framework establishes and enables interoperable interactions among diverse Conversational AI agents, including chatbots, voicebots, videobots, and human agents. Furthermore, a new Discovery specification framework is introduced, designed to efficiently look up agents providing specific services and to obtain accurate information about these services through a standard Manifest publication, accessible via an extended set of Natural Language-based APIs. The main purpose of this contribution is to significantly enhance the capabilities and scalability of AI interactions across various platforms. The novel architecture for interoperable Conversational AI assistants is designed to generalize, being replicable and accessible via open repositories., Comment: 22 pages, 8 figures

We propose and demonstrate an alternate, effective approach to simple slice sampling. Using the probability integral transform, we first generalize Neal's shrinkage algorithm, standardizing the procedure to an automatic and universal starting point: the unit interval. This enables the introduction of approximate (pseudo-) targets through importance reweighting, a technique that has popularized elliptical slice sampling. Reasonably accurate pseudo-targets can boost sampler efficiency by requiring fewer rejections and by reducing target skewness. This strategy is effective when a natural, possibly crude, approximation to the target exists. Alternatively, obtaining a marginal pseudo-target from initial samples provides an intuitive and automatic tuning procedure. We consider two metrics for evaluating the quality of approximation; each can be used as a criterion to find an optimal pseudo-target or as an interpretable diagnostic. We examine performance of the proposed sampler relative to other popular, easily implemented MCMC samplers on standard targets in isolation, and as steps within a Gibbs sampler in a Bayesian modeling context. We extend the transformation method to multivariate slice samplers and demonstrate with a constrained state-space model for which a readily available forward-backward algorithm provides the target approximation.

The development of a colloidal synthesis procedure to produce nanomaterials of a specific size with high shape and size purity is often a time consuming, iterative process. This is often due to the time, resource and expertise intensive characterization methods required for quantitative determination of nanomaterial size and shape. Absorption spectroscopy is often the easiest method of colloidal nanomaterial characterization, however, due to the lack of a reliable method to extract nanoparticle shapes from absorption spectroscopy, it is generally treated as a more qualitative measure for metal nanoparticles. This work demonstrates a gold nanorod (AuNR) spectral morphology analysis (SMA) tool, AuNR-SMA, which is a fast and accurate method to extract quantitative information about an AuNR sample's structural parameters from its absorption spectra. We apply AuNR-SMA in three distinct applications. First, we demonstrate its utility as an automated analysis tool in a high throughput AuNR synthesis procedure by generating quantitative size information from optical spectra. Second, we use the predictions generated by this model to train a machine learning model capable of predicting the resulting AuNR size distributions from the reaction conditions used to synthesize them. Third, we turn this model to spectra extracted from the literature where no size distributions are reported to impute unreported quantitative information of AuNR synthesis. This approach can potentially be extended to any other nanocrystal system where the absorption spectra are size dependent and accurate numerical simulation of the absorption spectra is possible. In addition, this pipeline could be integrated into automated synthesis apparatuses to provide interpretable data from simple measurements and help explore the synthesis science of nanoparticles in a rational manner or facilitate closed-loop workflows.

Gravitational waves (GWs) generated by a first-order phase transition at the electroweak scale are detectable by future space-based detectors like LISA. The lifetime of the resulting shock waves plays an important role in determining the intensity of the generated GWs. We have simulated decaying primordial acoustic turbulence in three dimensions and make a prediction for the universal shape of the energy spectrum by using its self-similar decay properties and the shape of individual shock waves. The shape for the spectrum is used to determine the time dependence of the fluid kinetic energy and the energy containing length scale at late times. The inertial range power law is found to be close to the classically predicted $k^{-2}$ and approaches it with increasing Reynolds number. The resulting model for the velocity spectrum and its decay in time is combined with the sound shell model assumptions about the correlations of the velocity field to compute the GW power spectrum for flows that decay in less than the Hubble time. The decay is found to bring about a convergence in the spectral amplitude and the peak power law that leads to a power law shallower than the $k^9$ of the stationary case., Comment: 32 pages, 18 figures, 9 tables

Weakly interacting massive particles (WIMPs) may interact with a virtual pion that is exchanged between nucleons. This interaction channel is important to consider in models where the spin-independent isoscalar channel is suppressed. Using data from the first science run of the LUX-ZEPLIN dark matter experiment, containing 60 live days of data in a 5.5~tonne fiducial mass of liquid xenon, we report the results on a search for WIMP-pion interactions. We observe no significant excess and set an upper limit of $1.5\times10^{-46}$~cm$^2$ at a 90\% confidence level for a WIMP mass of 33~GeV/c$^2$ for this interaction.

Two-dimensional van der Waals magnets hosting topological magnetic textures, such as skyrmions, show promise for applications in spintronics and quantum computing. Electrical control of these topological spin textures would enable novel devices with enhanced performance and functionality. Here, using electron microscopy combined with in situ electric and magnetic biasing, we show that the skyrmion chirality, whether left-handed or right-handed, in insulating Cr2Ge2Te6, is controlled by external electric field direction applied during magnetic field cooling process. The electric-field-tuned chirality remains stable, even amid variations in magnetic and electric fields. Our theoretical investigation reveals that nonzero Dzyaloshinskii-Moriya interactions between the nearest neighbors, induced by the external electric field, change their sign upon reversing the electric field direction, thereby facilitating chirality selection. The electrical control of magnetic chirality demonstrated in this study can be extended to other non-metallic centrosymmetric skyrmion-hosting magnets, opening avenues for future device designs in topological spintronics and quantum computing.

Legal practice has witnessed a sharp rise in products incorporating artificial intelligence (AI). Such tools are designed to assist with a wide range of core legal tasks, from search and summarization of caselaw to document drafting. But the large language models used in these tools are prone to "hallucinate," or make up false information, making their use risky in high-stakes domains. Recently, certain legal research providers have touted methods such as retrieval-augmented generation (RAG) as "eliminating" (Casetext, 2023) or "avoid[ing]" hallucinations (Thomson Reuters, 2023), or guaranteeing "hallucination-free" legal citations (LexisNexis, 2023). Because of the closed nature of these systems, systematically assessing these claims is challenging. In this article, we design and report on the first preregistered empirical evaluation of AI-driven legal research tools. We demonstrate that the providers' claims are overstated. While hallucinations are reduced relative to general-purpose chatbots (GPT-4), we find that the AI research tools made by LexisNexis (Lexis+ AI) and Thomson Reuters (Westlaw AI-Assisted Research and Ask Practical Law AI) each hallucinate between 17% and 33% of the time. We also document substantial differences between systems in responsiveness and accuracy. Our article makes four key contributions. It is the first to assess and report the performance of RAG-based proprietary legal AI tools. Second, it introduces a comprehensive, preregistered dataset for identifying and understanding vulnerabilities in these systems. Third, it proposes a clear typology for differentiating between hallucinations and accurate legal responses. Last, it provides evidence to inform the responsibilities of legal professionals in supervising and verifying AI outputs, which remains a central open question for the responsible integration of AI into law., Comment: Our dataset, tool outputs, and labels will be made available upon publication. This version of the manuscript (May 30, 2024) is updated to reflect an evaluation of Westlaw's AI-Assisted Research

The Scintillating Bubble Chamber (SBC) collaboration purchased 32 Hamamatsu VUV4 silicon photomultipliers (SiPMs) for use in SBC-LAr10, a bubble chamber containing 10~kg of liquid argon. A dark-count characterization technique, which avoids the use of a single-photon source, was used at two temperatures to measure the VUV4 SiPMs breakdown voltage ($V_{\text{BD}}$), the SiPM gain ($g_{\text{SiPM}}$), the rate of change of $g_{\text{SiPM}}$ with respect to voltage ($m$), the dark count rate (DCR), and the probability of a correlated avalanche (P$_{\text{CA}}$) as well as the temperature coefficients of these parameters. A Peltier-based chilled vacuum chamber was developed at Queen's University to cool down the Quads to $233.15\pm0.2$~K and $255.15\pm0.2$~K with average stability of $\pm20$~mK. An analysis framework was developed to estimate $V_{\text{BD}}$ to tens of mV precision and DCR close to Poissonian error. The temperature dependence of $V_{\text{BD}}$ was found to be $56\pm2$~mV~K$^{-1}$, and $m$ on average across all Quads was found to be $(459\pm3(\rm{stat.})\pm23(\rm{sys.}))\times 10^{3}~e^-$~PE$^{-1}$~V$^{-1}$. The average DCR temperature coefficient was estimated to be $0.099\pm0.008$~K$^{-1}$ corresponding to a reduction factor of 7 for every 20~K drop in temperature. The average temperature dependence of P$_{\text{CA}}$ was estimated to be $4000\pm1000$~ppm~K$^{-1}$. P$_{\text{CA}}$ estimated from the average across all SiPMs is a better estimator than the P$_{\text{CA}}$ calculated from individual SiPMs, for all of the other parameters, the opposite is true. All the estimated parameters were measured to the precision required for SBC-LAr10, and the Quads will be used in conditions to optimize the signal-to-noise ratio., Comment: 25 pages, 19 figures

We present a hardware-reconfigurable ansatz on $N_q$-qubits for the variational preparation of many-body states of the Anderson impurity model (AIM) with $N_{\text{imp}}+N_{\text{bath}}=N_q/2$ sites, which conserves total charge and spin z-component within each variational search subspace. The many-body ground state of the AIM is determined as the minimum over all minima of $O(N_q^2)$ distinct charge-spin sectors. Hamiltonian expectation values are shown to require $\omega(N_q) < N_{\text{meas.}} \leq O(N_{\text{imp}}N_{\text{bath}})$ symmetry-preserving, parallelizable measurement circuits, each amenable to post-selection. To obtain the one-particle impurity Green's function we show how initial Krylov vectors can be computed via mid-circuit measurement and how Lanczos iterations can be computed using the symmetry-preserving ansatz. For a single-impurity Anderson model with a number of bath sites increasing from one to six, we show using numerical emulation that the ease of variational ground-state preparation is suggestive of linear scaling in circuit depth and sub-quartic scaling in optimizer complexity. We therefore expect that, combined with time-dependent methods for Green's function computation, our ansatz provides a useful tool to account for electronic correlations on early fault-tolerant processors. Finally, with a view towards computing real materials properties of interest like magnetic susceptibilities and electron-hole propagators, we provide a straightforward method to compute many-body, time-dependent correlation functions using a combination of time evolution, mid-circuit measurement-conditioned operations, and the Hadamard test.

The Data Acquisition System (DAQ) for the LUX-ZEPLIN (LZ) dark matter detector is described. The signals from 745 PMTs, distributed across three subsystems, are sampled with 100-MHz 32-channel digitizers (DDC-32s). A basic waveform analysis is carried out on the on-board Field Programmable Gate Arrays (FPGAs) to extract information about the observed scintillation and electroluminescence signals. This information is used to determine if the digitized waveforms should be preserved for offline analysis. The system is designed around the Kintex-7 FPGA. In addition to digitizing the PMT signals and providing basic event selection in real time, the flexibility provided by the use of FPGAs allows us to monitor the performance of the detector and the DAQ in parallel to normal data acquisition. The hardware and software/firmware of this FPGA-based Architecture for Data acquisition and Realtime monitoring (FADR) are discussed and performance measurements are described., Comment: 18 pages, 24 figures

LUX-ZEPLIN (LZ) is a tonne-scale experiment searching for direct dark matter interactions and other rare events. It is located at the Sanford Underground Research Facility (SURF) in Lead, South Dakota, USA. The core of the LZ detector is a dual-phase xenon time projection chamber (TPC), designed with the primary goal of detecting Weakly Interacting Massive Particles (WIMPs) via their induced low energy nuclear recoils. Surrounding the TPC, two veto detectors immersed in an ultra-pure water tank enable reducing background events to enhance the discovery potential. Intricate calibration systems are purposely designed to precisely understand the responses of these three detector volumes to various types of particle interactions and to demonstrate LZ's ability to discriminate between signals and backgrounds. In this paper, we present a comprehensive discussion of the key features, requirements, and performance of the LZ calibration systems, which play a crucial role in enabling LZ's WIMP-search and its broad science program. The thorough description of these calibration systems, with an emphasis on their novel aspects, is valuable for future calibration efforts in direct dark matter and other rare-event search experiments.

The first science run of the LUX-ZEPLIN (LZ) experiment, a dual-phase xenon time project chamber operating in the Sanford Underground Research Facility in South Dakota, USA, has reported leading limits on spin-independent WIMP-nucleon interactions and interactions described from a non-relativistic effective field theory (NREFT). Using the same 5.5~t fiducial mass and 60 live days of exposure we report on the results of a relativistic extension to the NREFT. We present constraints on couplings from covariant interactions arising from the coupling of vector, axial currents, and electric dipole moments of the nucleon to the magnetic and electric dipole moments of the WIMP which cannot be described by recasting previous results described by an NREFT. Using a profile-likelihood ratio analysis, in an energy region between 0~keV$_\text{nr}$ to 270~keV$_\text{nr}$, we report 90% confidence level exclusion limits on the coupling strength of five interactions in both the isoscalar and isovector bases., Comment: 7 pages, 4 figures

In this paper, we introduce an inexact regularized proximal Newton method (IRPNM) that does not require any line search. The method is designed to minimize the sum of a twice continuously differentiable function $f$ and a convex (possibly non-smooth and extended-valued) function $\varphi$. Instead of controlling a step size by a line search procedure, we update the regularization parameter in a suitable way, based on the success of the previous iteration. The global convergence of the sequence of iterations and its superlinear convergence rate under a local H\"olderian error bound assumption are shown. Notably, these convergence results are obtained without requiring a global Lipschitz property for $ \nabla f $, which, to the best of the authors' knowledge, is a novel contribution for proximal Newton methods. To highlight the efficiency of our approach, we provide numerical comparisons with an IRPNM using a line search globalization and a modern FISTA-type method., Comment: 32 pages

Diffusion processes govern fundamental phenomena such as phase transformations, doping, and intercalation in van der Waals (vdW) bonded materials. Here, we quantify the diffusion dynamics of W atoms by visualizing the motion of individual atoms at three different vdW interfaces: BN/vacuum, BN/BN, and BN/WSe2, by recording scanning transmission electron microscopy movies. Supported by density functional theory calculations, we infer that in all cases diffusion is governed by intermittent trapping at electron beam-generated defect sites. This leads to diffusion properties that depend strongly on the number of defects. These results suggest that diffusion and intercalation processes in vdW materials are highly tunable and sensitive to crystal quality. The demonstration of imaging, with high spatial and temporal resolution, of layers and individual atoms inside vdW heterostructures offers possibilities for direct visualization of diffusion and atomic interactions, as well as for experiments exploring atomic structures, their in-situ modification, and electrical property measurements of active devices combined with atomic resolution imaging., Comment: 12 pages, 6 figures

The submillimeter and millimeter ((sub-)mm) sky contains a vast wealth of information that is both complementary and inaccessible to other wavelengths. Over half the light we receive is observable at (sub-)mm wavelengths, yet we have mapped only a small portion of the sky at sufficient spatial resolution and sensitivity to detect and resolve distant galaxies or star forming cores within their their large-scale environment. For decades the astronomical community has highlighted the need for a large, high-throughput (sub-)mm ($\lambda\sim0.35-10$ mm) single dish; The Atacama Large Aperture Submillimeter Telescope (AtLAST), with its 50-m aperture and $2^\circ$ maximal field of view, aims to be such a facility. We present here the full design concept for AtLAST, developed through an EU-funded project. Our design approach begins with a long lineage of (sub-)mm telescopes, relies on calculations and simulations to realize the optics, and uses finite element analysis to optimize the mechanical structure and subsystems. The demanding design requirements for AtLAST, set by transformative science goals, combine novel concepts with lessons learned from past experience. The result is an innovative rocking chair design with six instrument bays, two of which are mounted on Nasmyth platforms. AtLAST will be capable of $3^\circ\,\rm s^{-1}$ scanning and $1^\circ\,\rm s^{-2}$ acceleration, and aims to feature a surface accuracy of $\leq 20~\mu$m half wavefront error under static deformations, allowing observations up to $\approx 950$~GHz. Crucially, AtLAST will be a sustainable, visionary facility that will allow upgrades for decades to come. While some aspects require further testing, prototyping, and field demonstrations, we estimate that the design will be construction-ready this decade., Comment: This version addresses the first round A&A referee reports

This paper introduces a new tool, OccCANINE, to automatically transform occupational descriptions into the HISCO classification system. The manual work involved in processing and classifying occupational descriptions is error-prone, tedious, and time-consuming. We finetune a preexisting language model (CANINE) to do this automatically, thereby performing in seconds and minutes what previously took days and weeks. The model is trained on 14 million pairs of occupational descriptions and HISCO codes in 13 different languages contributed by 22 different sources. Our approach is shown to have accuracy, recall, and precision above 90 percent. Our tool breaks the metaphorical HISCO barrier and makes this data readily available for analysis of occupational structures with broad applicability in economics, economic history, and various related disciplines., Comment: All code and guides on how to use OccCANINE is available on GitHub https://github.com/christianvedels/OccCANINE

This paper examines QAOA in the context of parity network synthesis. We propose a pair of algorithms for parity network synthesis and linear circuit inversion. Together, these algorithms can build the diagonal component of the QAOA circuit, generally the most expensive in terms of two qubit gates. We compare the CNOT count of our strategy to off-the-shelf compiler tools for random, full, and graph-based optimization problems and find that ours outperforms the alternatives., Comment: 12 pages, 5 figures

Searches for dark matter with liquid xenon time projection chamber experiments have traditionally focused on the region of the parameter space that is characteristic of weakly interacting massive particles, ranging from a few GeV/$c^2$ to a few TeV/$c^2$. Models of dark matter with a mass much heavier than this are well motivated by early production mechanisms different from the standard thermal freeze-out, but they have generally been less explored experimentally. In this work, we present a re-analysis of the first science run (SR1) of the LZ experiment, with an exposure of $0.9$ tonne$\times$year, to search for ultraheavy particle dark matter. The signal topology consists of multiple energy deposits in the active region of the detector forming a straight line, from which the velocity of the incoming particle can be reconstructed on an event-by-event basis. Zero events with this topology were observed after applying the data selection calibrated on a simulated sample of signal-like events. New experimental constraints are derived, which rule out previously unexplored regions of the dark matter parameter space of spin-independent interactions beyond a mass of 10$^{17}$ GeV/$c^2$., Comment: 9 pages, 7 figures

Do large language models (LLMs) know the law? These models are increasingly being used to augment legal practice, education, and research, yet their revolutionary potential is threatened by the presence of hallucinations -- textual output that is not consistent with legal facts. We present the first systematic evidence of these hallucinations, documenting LLMs' varying performance across jurisdictions, courts, time periods, and cases. Our work makes four key contributions. First, we develop a typology of legal hallucinations, providing a conceptual framework for future research in this area. Second, we find that legal hallucinations are alarmingly prevalent, occurring between 58% of the time with ChatGPT 4 and 88% with Llama 2, when these models are asked specific, verifiable questions about random federal court cases. Third, we illustrate that LLMs often fail to correct a user's incorrect legal assumptions in a contra-factual question setup. Fourth, we provide evidence that LLMs cannot always predict, or do not always know, when they are producing legal hallucinations. Taken together, our findings caution against the rapid and unsupervised integration of popular LLMs into legal tasks. Even experienced lawyers must remain wary of legal hallucinations, and the risks are highest for those who stand to benefit from LLMs the most -- pro se litigants or those without access to traditional legal resources.