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[Display omitted] • A stretchable electret achieves high surface charge and long charge stability. • A stretchable electret-based TENG achieves high charge density (0.2 mC m−2). • A power management module enhances power storage efficiency of the TENG. • The self-charging system provides a stable power supply for wearable electronics. Stretchable power sources capable of accommodating large deformations are urgently demanded for various stretchable and wearable electronics. In this work, we report a stretchable electret-based triboelectric nanogenerator (SEB-TENG) consisting of elastomeric electret as electrification materials and organo-hydrogels as electrodes. The electret elastomer, prepared by uniformly dispersing SiO 2 nanoparticles in the elastomer matrix and thermally injecting static charges, obtains a high surface potential, high tensile strain (796%), and long stability. Then, the SEB-TENG device also achieves high stretchability (423%) and high charge density (0.2 mC m−2). Furthermore, a power management module (PMM) is designed to maximize the energy utilization of the SEB-TENG. The integrated self-charging system can be sufficiently used to constantly power a watch, or charge a Li-ion coin cell which subsequently provides sustainable power supplies to a digital thermometer. This work provides a viable approach to simultaneously achieve high output performances and high stretchability of integrated power sources. [ABSTRACT FROM AUTHOR]

The tribovoltaic effect can convert semiconductor interfacial frictional mechanical energy into direct current (DC) electricity, but the flexibility and durability of semiconductor materials limit its application in wearable electronic. Herein, a robust flexible textile tribovoltaic nanogenerator is presented based on a 2D dynamic heterojunction of 2H‐MoS2/Ta4C3 (MTNG). During the friction process, a built‐in electric field (Eb) and an additional interfacial electric field (ECE) are generated in a continuous dynamic contact of 2H‐MoS2/Ta4C3, and through the 2H‐MoS2/Ta4C3 dynamic heterojunction, a significant number of electron‐hole pairs are excited and move directionally to generate a DC. The influences of mechanical pressure and sliding speed on output performance of MTNGs are systematically investigated. The MTNGs deliver excellent output power density (39.15 mW m2) and outstanding robustness (43 000 cycles). Ten MTNGs can be connected in series to obtain a DC voltage of 3.3 V and in parallel to obtain a DC current of 75 µA. Furthermore, the MTNGs can effectively power a variety of commercial electronic watches and calculators by harvesting human kinetic energy. A 2D dynamic heterojunction 2H‐MoS2/Ta4C3 DC nanogenerator is described and offers a workable option for the creation of flexible DC power sources and self‐powered wearable electronics. [ABSTRACT FROM AUTHOR]

[Display omitted] • H-SiO 2 and PF as fillers to improve the dielectric properties of PFS films. • The performance of TENGs delivered an enhancement by 13 times. • Multiple nanoscales is more favorable to achieve high performance of TENGs. Triboelectric nanogenerators (TENGs), capable of harvesting distributed energy from the environment, have provided a viable solution for self-powered wearable electronics. However, their low power density and susceptibility to contamination still severely limit their practical application. Herein, we reported a "two-step" strategy to implement a waterproof self-powered wearable electronic device based on TENG. Firstly, Perfluoropolyether (PF) and hollow hierarchical silica (H-SiO 2) as fillers significantly improve the dielectric properties of polydimethylsiloxane (PDMS) composite films (PFS films) through polarization effect. Then the nano bumps of 10–30 nm are created on the surface of the films by surface etching, the bumps can increase the contact area of TENG. The voltage of TENG is improved from ∼ 67 V to ∼ 910 V and the current is improved from ∼ 1 μA to ∼ 25 μA. What's more, the investigation of the surface structure of the PFS composite films by Atomic Force Microscope (AFM) revealed that the synergistic combination of multiple nanoscales (10–30 nm, 60–80 nm, 300–500 nm) is more favorable to achieve high performance of TENG. The surface structure composed of multiple nanoscales endows PFS with excellent superhydrophobicity. The PFS films remained fine performance after 40,000 drops of water and 90 days. This work achieves high performance and water resistance of TENG, demonstrating great potential in the field of self-powered wearable electronic devices. [ABSTRACT FROM AUTHOR]

The wearable tactile sensors have attracted great attention in the fields of intelligent robots, healthcare monitors and human-machine interactions. To create active tactile sensors that can directly generate electrical signals in response to stimuli from the surrounding environment is of great significance. Triboelectric nanogenerators (TENGs) have the advantages of high sensitivity, fast response speed and low cost that can convert any type of mechanical motion in the surrounding environment into electrical signals, which provides an effective strategy to design the self-powered active tactile sensors. Here, an overview of the development in TENGs as tactile stimulators for multifunctional sensing and artificial synapses is systematically introduced. Firstly, the applications of TENGs as tactile stimulators in pressure, temperature, proximity sensing, and object recognition are introduced in detail. Then, the research progress of TENGs as tactile stimulators for artificial synapses is emphatically introduced, which is mainly reflected in the electrolyte-gate synaptic transistors, optoelectronic synaptic transistors, floating-gate synaptic transistors, reduced graphene oxides-based artificial synapse, and integrated circuit-based artificial synapse and nervous systems. Finally, the challenges of TENGs as tactile stimulators for multifunctional sensing and artificial synapses in practical applications are summarized, and the future development prospects are expected. [ABSTRACT FROM AUTHOR]