1. Tunable exciton valley-pseudospin orders in moiré superlattices.
- Author
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Xiong, Richen, Brantly, Samuel L., Su, Kaixiang, Nie, Jacob H., Zhang, Zihan, Banerjee, Rounak, Ruddick, Hayley, Watanabe, Kenji, Taniguchi, Takashi, Tongay, Seth Ariel, Xu, Cenke, and Jin, Chenhao
- Subjects
PHASES of matter ,OPTOELECTRONIC devices ,PHASE diagrams ,MAGNETIC fields ,SUPERLATTICES ,PHYSICS ,HELICITY of nuclear particles - Abstract
Excitons in two-dimensional (2D) semiconductors have offered an attractive platform for optoelectronic and valleytronic devices. Further realizations of correlated phases of excitons promise device concepts not possible in the single particle picture. Here we report tunable exciton "spin" orders in WSe
2 /WS2 moiré superlattices. We find evidence of an in-plane (xy) order of exciton "spin"—here, valley pseudospin—around exciton filling vex = 1, which strongly suppresses the out-of-plane "spin" polarization. Upon increasing vex or applying a small magnetic field of ~10 mT, it transitions into an out-of-plane ferromagnetic (FM-z) spin order that spontaneously enhances the "spin" polarization, i.e., the circular helicity of emission light is higher than the excitation. The phase diagram is qualitatively captured by a spin-1/2 Bose–Hubbard model and is distinct from the fermion case. Our study paves the way for engineering exotic phases of matter from correlated spinor bosons, opening the door to a host of unconventional quantum devices. Control of correlated excitonic states is a key goal of modern optoelectronic physics. Here, the authors demonstrate filling- and field-tunable exciton valley-pseudospin orders in a moiré heterostructure. [ABSTRACT FROM AUTHOR]- Published
- 2024
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