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Australia experienced record‐breaking wildfires during 2019–2020, which emitted large amounts of carbonaceous aerosols (CAs) to the atmosphere. In this study, we explored the atmospheric dynamics and thermodynamic mechanism of the long‐range transport of CAs during November 2019–February 2020. The results indicate that the emitted CAs had a ternary advective spreading pattern across the Pacific Ocean in the Southern Hemisphere (SH), influenced mainly by the westerlies and anticyclonic systems. Upward vertical motion over the convergence zone and heat released from smoke pyro‐cumulonimbus clouds and strong light absorption of CAs provided strong vertical lift as the predominant injection pathway of the CAs into the stratosphere in the central Pacific Ocean in the SH. The abundant tropospheric CAs induced atmospheric heating (and potentially surface cooling), with increasing air temperature and decreasing of surface temperature. The anomalous thermal structure led to changes in atmospheric circulation, which weakened the upward vertical motion. Plain Language Summary: During the summer of 2019–2020, Australia suffered unprecedented wildfires. These wildfires emitted large amounts of pollutants into the free atmosphere. The pollutants are mainly composed of carbonaceous aerosols (CAs). Under the effects of meteorological conditions, the CAs experienced a long‐range spread expanding from the western Pacific Ocean to the eastern Pacific Ocean even arriving at the Atlantic Ocean. During the transportation, the CAs were accumulated over the central Pacific Ocean under the trapping effect of the anticyclone and then exhibited significant lift owing to upward motion over the convergence zone between westerlies and anticyclone and heat buoyancy released from smoke pyro‐cumulonimbus clouds and strong light absorption of CAs. As a response, the strong absorption of CAs resulted in the warming of the atmosphere and cooling of the surface, which enhanced atmospheric stratification and constrained the development of atmospheric instability. Thus, the upward vertical motion was weakened. Key Points: The westerlies and anticyclonic system dominated the advective spread of carbonaceous aerosols (CAs)The upward vertical motion, heat released from smoke pyro‐cumulonimbus clouds, and strong CAs light absorption contributed to CAs liftThe CAs caused warming of air temperature and cooling of surface temperature, which weakened the upward vertical motion [ABSTRACT FROM AUTHOR]