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Theory suggests that the response time of alluvial channel long-profiles to perturbations in climate is related to the magnitude of the forcing and the length of the system. Shorter systems may record a higher frequency of forcing compared to longer systems. Empirical field evidence that system length plays a role in the climate periodicity preserved within the sedimentary record is, however, sparse. The Toro Basin in the Eastern Cordillera of NW Argentina provides an opportunity to test these theoretical relationships as this single source-to-sink system contains a range of sediment deposits, located at varying distances from the source. A suite of eight alluvial fan deposits is preserved along the western flanks of the Sierra de Pascha. Farther downstream, a flight of cut-and-fill terraces have been linked to eccentricity-driven (100-kyr) climate cycles since ca. 500 ka. We applied cosmogenic radionuclide (10Be) exposure dating to the fan surfaces to explore (1) how channel responses to external perturbations may or may not propagate downstream, and (2) the differences in landscape response to forcing frequency as a function of channel length. We identified two generations of fan surfaces: the first (G1) records surface activity and abandonment between ca. 800 and 500 ka and the second (G2) within the last 100 kyr. G1 fans record a prolonged phase of net incision, which has been recognised throughout the Central Andes, and was likely triggered by enhanced 100-kyr global glacial cycles following the Mid-Pleistocene Transition. Relative fan surface stability followed, while 100-kyr cut-and-fill cycles occurred downstream, suggesting a disconnect in behaviour between the two channel reaches. G2 fans record higher frequency climate forcing, possibly the result of precessional forcing of climate (ca. 21/40-kyr timescales). The lack of a high-frequency signal farther downstream provides field support for theoretical predictions of a filtering of high-frequency climate forcing with increasing channel length. We show that multiple climate periodicities can be preserved within the sedimentary record of a single basin. Differences in the timing of alluvial fan and fluvial terrace development in the Toro Basin appears to be associated with how channel length affects fluvial response times to climate forcing as well as local controls on net incision, such as tectonic deformation. [ABSTRACT FROM AUTHOR]

The hydrogen isotope composition of leaf wax biomarkers (δ2 H wax) is a valuable tool for reconstructing continental paleohydrology, since it serves as a proxy for the hydrogen isotope composition of precipitation (δ2 H pre). To yield robust palaeohydrological reconstructions using δ2 H wax in marine archives, it is necessary to examine the impacts of regional climate on δ2 H wax and assess the similarity between marine sedimentary δ2 H wax and the source of continental δ2 H wax. Here, we examined an aridity gradient from hyperarid to humid along the Chilean coast. We sampled sediments at the outlets of rivers draining into the Pacific as well as soils within catchments and marine surface sediments adjacent to the outlets of the studied rivers and analyzed the relationship between climatic variables and δ2 H wax values. We found that apparent fractionation between leaf waxes and source water is relatively constant in humid and semiarid regions (average: - 121 ‰). However, it becomes less negative in hyperarid regions (average: - 86 ‰) as a result of evapotranspirative processes affecting soil and leaf water 2 H enrichment. We also observed that along strong aridity gradients, the 2 H enrichment of δ2 H wax follows a non-linear relationship with water content and water flux variables, driven by strong soil evaporation and plant transpiration. Furthermore, our results indicate that δ2 H wax values in marine surface sediments largely reflect δ2 H wax values from the continent, confirming the robustness of marine δ2 H wax records for paleohydrological reconstructions along the Chilean margin. These findings also highlight the importance of considering the effects of hyperaridity in the interpretation of δ2 H wax values and pave the way for more quantitative paleohydrological reconstructions using δ2 H wax. [ABSTRACT FROM AUTHOR]

The hydrogen isotope composition of leaf wax biomarkers (δ2Hwax) is a valuable tool for reconstructing continental paleohydrology, as it serves as a proxy for the hydrogen isotope composition of precipitation (δ2Hpre). To yield robust palaeohydrological reconstructions using δ2Hwax in marine archives, it is necessary to examine the impacts of regional climate on δ2Hwax and assess the similarity between marine sedimentary δ2Hwax and the source of continental δ2Hwax. Here, we examined an aridity gradient from hyperarid to humid along the Chilean coast. We sampled sediments at the outlets of rivers draining into the Pacific, soils within catchments and marine surface sediments adjacent to the outlets of the studied rivers and analyzed the relationship between climatic variables and δ2Hwax values. We find that apparent fractionation between leaf waxes and source water is relatively constant in humid/semiarid regions (average: −121 ‰). However, it becomes less negative in hyperarid regions (average: −86 ‰) as a result of evapotranspirative processes affecting soil and leaf water 2H enrichment. We also observed that along strong aridity gradients, the 2H enrichment of δ2Hwax follows a non-linear relationship with water content and water flux variables, driven by strong soil evaporation and plant transpiration. Furthermore, our results indicated that δ2Hwax values in marine surface sediments largely reflect δ2Hwax values from the continent, confirming the robustness of marine δ2Hwax records for paleohydrological reconstructions along the Chilean margin. These findings also highlight the importance of considering the effects of hyperaridity in the interpretation of δ2Hwax values and pave the way for more quantitative paleohydrological reconstructions using δ2Hwax. [ABSTRACT FROM AUTHOR]

While landscapes are broadly sculpted by tectonics and climate, on a catchment scale, sediment size can regulate hillslope denudation rates and thereby influence the location of topographic highs and valleys. In this work, we used in situ 10Be cosmogenic radionuclide analysis to measure the denudation rates of bedrock, boulders, and soil in three granitic landscapes with different climates in Chile. We hypothesize that bedrock and boulders affect differential denudation by denuding more slowly than the surrounding soil; the null hypothesis is that no difference exists between soil and boulder or bedrock denudation rates. To evaluate denudation rates, we present a simple model that assesses differential denudation of boulders and the surrounding soil by evaluating boulder protrusion height against a two-stage erosion model and measured 10Be concentrations of boulder tops. We found that hillslope bedrock and boulders consistently denude more slowly than soil in two out of three of our field sites, which have a humid and a semi-arid climate: denudation rates range from ∼5 to 15 m Myr -1 for bedrock and boulders and from ∼8 to 20 m Myr -1 for soil. Furthermore, across a bedrock ridge at the humid site, denudation rates increase with increasing fracture density. At our lower-sloping field sites, boulders and bedrock appear to be similarly immobile based on similar 10Be concentrations. However, in the site with a Mediterranean climate, steeper slopes allow for higher denudation rates for both soil and boulders (∼40 –140 m Myr -1), while the bedrock denudation rate remains low (∼22 m Myr -1). Our findings suggest that unfractured bedrock patches and large hillslope boulders affect landscape morphology by inducing differential denudation in lower-sloping landscapes. When occurring long enough, such differential denudation should lead to topographic highs and lows controlled by bedrock exposure and hillslope sediment size, which are both a function of fracture density. We further examined our field sites for fracture control on landscape morphology by comparing fracture, fault, and stream orientations, with the hypothesis that bedrock fracturing leaves bedrock more susceptible to denudation. Similar orientations of fractures, faults, and streams further support the idea that tectonically induced bedrock fracturing guides fluvial incision and accelerates denudation by reducing hillslope sediment size. [ABSTRACT FROM AUTHOR]

While landscapes are broadly sculpted by tectonics and climate, on a catchment scale, the density of bedrock fractures can influence hillslope denudation rates and dictate the location of topographic highs and valleys. In this work, we used 10Be cosmogenic radionuclide analysis to measure the denudation rates of bedrock, boulders, and soil, in three granitic landscapes with different climates in Chile, with the hypothesis that high fracture density reduces grain size and increases denudation rates. Denudation rates range from 10 to 15 m Myr-1 for bedrock and boulders and from 15 to 20 m Myr-1 for soil in the humid and semi-arid climates, and are higher in the mediterranean climate (~40–140 m Myr-1), likely due to steeper slopes. We found that hillslope bedrock and boulders erode more slowly than the surrounding soil in the diffusively-eroding study sites. Furthermore, across a bedrock ridge in the humid site, bedrock denudation rates increase with fracture density. These findings are consistent with the observation that streams in our field sites follow the orientation of at least one major fault orientation. Our results suggest that tectonically-induced fractures and faults dictate landscape evolution through reducing grain size and thus enhancing differential denudation rates. [ABSTRACT FROM AUTHOR]

The denudation of rocks in mountain belts exposes a range of fresh minerals to the surface of the Earth that are chemically weathered by acidic and oxygenated fluids. The impact of the resulting coupling between denudation and weathering rates fundamentally depends on the types of minerals that are weathering. Whereas silicate weathering sequesters CO2 , the combination of sulfide oxidation and carbonate dissolution emits CO2 to the atmosphere. Here, we combine the concentrations of dissolved major elements in stream waters with 10Be basin-wide denudation rates from 35 small catchments in eastern Tibet to elucidate the importance of lithology in modulating the relationships between denudation rate, chemical weathering pathways, and CO2 consumption or release. Our catchments span 3 orders of magnitude in denudation rate in low-grade flysch, high-grade metapelites, and granitoid rocks. For each stream, we estimate the concentrations of solutes sourced from silicate weathering, carbonate dissolution, and sulfide oxidation using a mixing model. We find that for all lithologies, cation concentrations from silicate weathering are largely independent of denudation rate, but solute concentrations from carbonates and, where present, sulfides increase with increasing denudation rate. With increasing denudation rates, weathering may therefore shift from consuming to releasing CO2 in both (meta)sedimentary and granitoid lithologies. For a given denudation rate, we report dissolved solid concentrations and inferred weathering fluxes in catchments underlain by (meta)sedimentary rock that are 2–10 times higher compared to catchments containing granitoid lithologies, even though climatic and topographic parameters do not vary systematically between these catchments. Thus, varying proportions of exposed (meta)sedimentary and igneous rocks during orogenesis could lead to changes in the sequestration and release of CO2 that are independent of denudation rate. [ABSTRACT FROM AUTHOR]