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3 results on '"Universitad polytecnica de Cataluna"'

1. Structural heterogeneities and mechanical behavior of amorphous alloys

Author

Riccardo Casalini, Eloi Pineda, Yao Yao, Q. Wang, J.C. Qiao, Hidemi Kato, Jean-Marc Pelletier, Yong Yang, Daniel Crespo, Matériaux, ingénierie et science [Villeurbanne] (MATEIS), Centre National de la Recherche Scientifique (CNRS)-Université Claude Bernard Lyon 1 (UCBL), Université de Lyon-Université de Lyon-Institut National des Sciences Appliquées de Lyon (INSA Lyon), Institut National des Sciences Appliquées (INSA)-Université de Lyon-Institut National des Sciences Appliquées (INSA), Optimisation des régulations physiologiques (ORPHY (EA 4324)), Institut Brestois Santé Agro Matière (IBSAM), Université de Brest (UBO)-Université de Brest (UBO)-Université de Brest (UBO)-Centre Hospitalier Régional Universitaire de Brest (CHRU Brest), Institute for Materials Research, Tohoku University, Tohoku University [Sendai], ESAB, Universitad polytecnica de Cataluna, Chinese Academy of Sciences [Beijing] (CAS), Universitat Politècnica de Catalunya. Departament de Física, and Universitat Politècnica de Catalunya. GCM - Grup de Caracterització de Materials

Subjects
Materials science, Amorphous alloys, Local heterogeneity, Mechanical properties, 02 engineering and technology, Mechanical relaxation, Plasticity, Structural heterogeneity, Enginyeria dels materials [Àrees temàtiques de la UPC], 010402 general chemistry, 01 natural sciences, Viscoelasticity, [SPI.MAT]Engineering Sciences [physics]/Materials, Materials -- Mechanical properties, Materials -- Propietats mecàniques, Condensed Matter::Materials Science, General Materials Science, Anelastic relaxation, Mechanical behavior, Supercooling, Translational symmetry, Amorphous metal, 021001 nanoscience & nanotechnology, 0104 chemical sciences, Nonequilibrium state, Dynamics, Mechanical spectroscopy, Metallic glass, Macroscopic scale, Chemical physics, Relaxation (physics), Glass, Deformation (engineering), 0210 nano-technology, Glass transition, Relaxation dynamics, Mechanical deformation
Abstract

cited By 22; Although the atomic structure of amorphous alloys, which lacks long-range translational symmetry, may appear homogeneous at the macroscopic scale, their local dynamic and/or static properties however vary significantly according to the recent experimental and simulation results. In the literature of amorphous alloys, the nature of such local heterogeneities is currently an issue under debate. More importantly, since amorphous alloys are in a thermodynamically nonequilibrium state, their local structures constantly evolve during structural relaxation, physical aging and mechanical deformation. As such, local structural heterogeneities, which vary with the thermal and mechanical history of amorphous alloys, could provide a key to understand the structural origin of their mechanical behavior, such as anelasticity, viscoelasticity, plasticity and fracture. In this review article, we first review mechanical spectroscopy or dynamic mechanical analyses as an important tool to study the relaxation dynamics in amorphous alloys, with a focus on the possible correlation between the secondary (also called β)relaxation and the local structural heterogeneities of amorphous alloys. After that, we discuss the recent advances on the understanding of structural heterogeneities in metallic supercooled liquids and the influence of the structural heterogeneities on the overall mechanical properties of the corresponding amorphous alloys. Finally, we briefly discuss the further development of research on this subject. © 2019 Elsevier Ltd

Published
2019

2. Seeds of Life in Space (SOLIS). II. Formamide in protostellar shocks: Evidence for gas-phase formation

Author

Izaskun Jiménez-Serra, Ana Chacón-Tanarro, Claudine Kahane, Andy Pon, R. Neri, Yoko Oya, Patrice Theulé, Leonardo Testi, Audrey Coutens, Paola Caselli, Charlotte Vastel, Serena Viti, François Dulieu, Jaime E. Pineda, R. Choudhury, P. Hily-Blant, J. Ospina, Fanny Vazart, Vincenzo Barone, Ana López-Sepulcre, Ian R. Sims, Laurent Wiesenfeld, Claudio Codella, Anna Punanova, Sandrine Bottinelli, Vianney Taquet, Francesco Fontani, Jacob C. Laas, A. Jaber Al-Edhari, Linda Podio, Cecilia Ceccarelli, Satoshi Yamamoto, Nami Sakai, Felipe O. Alves, Rafael Bachiller, Emmanuel Caux, S. Spezzano, D. Quénard, Nadia Balucani, Siyi Feng, Cécile Favre, Luca Bizzocchi, Cristina Puzzarini, Bertrand Lefloch, Piero Ugliengo, Anton Vasyunin, Jonathan Holdship, Dimitrios Skouteris, Albert Rimola, E. Bianchi, Laboratoire d'Astrophysique de Grenoble (LAOG), Université Joseph Fourier - Grenoble 1 (UJF)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS), INAF - Osservatorio Astrofisico di Arcetri (OAA), Istituto Nazionale di Astrofisica (INAF), Università degli Studi di Perugia (UNIPG), INAF - Osservatorio Astronomico di Brera (OAB), Southern University of Science and Technology [Shenzhen] (SUSTech), Laboratoire d'Etude du Rayonnement et de la Matière en Astrophysique (LERMA), École normale supérieure - Paris (ENS Paris)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire de Paris, PSL Research University (PSL)-PSL Research University (PSL)-Université de Cergy Pontoise (UCP), Université Paris-Seine-Université Paris-Seine-Centre National de la Recherche Scientifique (CNRS), Queen Mary University of London (QMUL), University College of London [London] (UCL), ESAB, Universitad polytecnica de Cataluna, University of Western Ontario (UWO), Max Planck Institute for Extraterrestrial Physics (MPE), Max-Planck-Gesellschaft, Institut de recherche en astrophysique et planétologie (IRAP), Université Toulouse III - Paul Sabatier (UT3), Université Fédérale Toulouse Midi-Pyrénées-Université Fédérale Toulouse Midi-Pyrénées-Observatoire Midi-Pyrénées (OMP), Université Fédérale Toulouse Midi-Pyrénées-Centre National de la Recherche Scientifique (CNRS), Institut de Planétologie et d'Astrophysique de Grenoble (IPAG), Centre National d'Études Spatiales [Toulouse] (CNES)-Université Grenoble Alpes (UGA)-Centre National de la Recherche Scientifique (CNRS)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire des Sciences de l'Univers de Grenoble (OSUG), Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Joseph Fourier - Grenoble 1 (UJF)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes (UGA)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Joseph Fourier - Grenoble 1 (UJF)-Centre National de la Recherche Scientifique (CNRS), departament de Quimica, Universitat Autònoma de Barcelona [Barcelona] (UAB), RIKEN - Institute of Physical and Chemical Research [Japon] (RIKEN), Scuola Normale Superiore di Pisa (SNS), European Southern Observatory (ESO), Physique des interactions ioniques et moléculaires (PIIM), Aix Marseille Université (AMU)-Centre National de la Recherche Scientifique (CNRS), Università degli studi di Torino (UNITO), Codella, C., Ceccarelli, C., Caselli, P., Balucani, N., Barone, V., Fontani, F., Lefloch, B., Podio, L., Viti, S., Feng, S., Bachiller, R., Bianchi, E., Dulieu, F., Jiménez-Serra, I., Holdship, J., Neri, R., Pineda, J.E., Pon, A., Sims, I., Spezzano, S., Vasyunin, A.I., Alves, F., Bizzocchi, L., Bottinelli, S., Caux, E., Chacón-Tanarro, A., Choudhury, R., Coutens, A., Favre, C., Hily-Blant, P., Kahane, C., Jaber Al-Edhari, A., Laas, J., López-Sepulcre, A., Ospina, J., Oya, Y., Punanova, A., Puzzarini, C., Quenard, D., Rimola, A., Sakai, N., Skouteris, D., Taquet, V., Testi, L., Theulé, P., Ugliengo, P., Vastel, C., Vazart, F., Wiesenfeld, L., Yamamoto, S., Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Observatoire des Sciences de l'Univers de Grenoble (OSUG ), Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Institut national des sciences de l'Univers (INSU - CNRS)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes [2016-2019] (UGA [2016-2019])-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes [2016-2019] (UGA [2016-2019]), Università degli Studi di Perugia = University of Perugia (UNIPG), Southern University of Science and Technology (SUSTech), LERMA Cergy (LERMA), Laboratoire d'Etude du Rayonnement et de la Matière en Astrophysique (LERMA (UMR_8112)), Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire de Paris, Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Université de Cergy Pontoise (UCP), Université Paris-Seine-Université Paris-Seine-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire de Paris, Université Paris-Seine-Université Paris-Seine-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire Midi-Pyrénées (OMP), Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Centre National de la Recherche Scientifique (CNRS), Universitat Autònoma de Barcelona (UAB), Università degli studi di Torino = University of Turin (UNITO), Pineda, J. E., Vasyunin, A. I., Sorbonne Université (SU)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Cergy Pontoise (UCP), Université Paris-Seine-Université Paris-Seine-Observatoire de Paris, Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Sorbonne Université (SU)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Cergy Pontoise (UCP), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL), Institut national des sciences de l'Univers (INSU - CNRS)-Université Toulouse III - Paul Sabatier (UT3), Météo France-Centre National d'Études Spatiales [Toulouse] (CNES)-Université Fédérale Toulouse Midi-Pyrénées-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Météo France-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Centre National de la Recherche Scientifique (CNRS), and Centre National de la Recherche Scientifique (CNRS)-Aix Marseille Université (AMU)

Subjects
Formamide, Abundance (chemistry), Direct evidence, Stars: formation, FOS: Physical sciences, Context (language use), Astrophysics, ISM: molecule, 01 natural sciences, chemistry.chemical_compound, 0103 physical sciences, Protostar, molecule [ISM], 010303 astronomy & astrophysics, ISM: jets and outflow, formation [Stars], ComputingMilieux_MISCELLANEOUS, Line (formation), Earth and Planetary Astrophysics (astro-ph.EP), ISM: individual objects: L1157-B1, ISM: jets and outflows, ISM: molecules, Astronomy and Astrophysics, Space and Planetary Science, Physics, [PHYS]Physics [physics], 010308 nuclear & particles physics, jets and outflow [ISM], individual objects: L1157-B1 [ISM], Astronomy and Astrophysic, Stars, chemistry, Millimeter, [PHYS.ASTR]Physics [physics]/Astrophysics [astro-ph], Astrophysics - Earth and Planetary Astrophysics
Abstract

Context: Modern versions of the Miller-Urey experiment claim that formamide (NH$_2$CHO) could be the starting point for the formation of metabolic and genetic macromolecules. Intriguingly, formamide is indeed observed in regions forming Solar-type stars as well as in external galaxies. Aims: How NH$_2$CHO is formed has been a puzzle for decades: our goal is to contribute to the hotly debated question of whether formamide is mostly formed via gas-phase or grain surface chemistry. Methods: We used the NOEMA interferometer to image NH$_2$CHO towards the L1157-B1 blue-shifted shock, a well known interstellar laboratory, to study how the components of dust mantles and cores released into the gas phase triggers the formation of formamide. Results: We report the first spatially resolved image (size $\sim$ 9", $\sim$ 2300 AU) of formamide emission in a shocked region around a Sun-like protostar: the line profiles are blueshifted and have a FWHM $\simeq$ 5 km s$^{-1}$. A column density of $N_{\rm NH_2CHO}$ = 8 $\times$ 10$^{12}$ cm$^{-1}$, and an abundance (with respect to H-nuclei) of 4 $\times$ 10$^{-9}$ are derived. We show a spatial segregation of formamide with respect to other organic species. Our observations, coupled with a chemical modelling analysis, indicate that the formamide observed in L1157-B1 is formed by gas-phase chemical process, and not on grain surfaces as previously suggested. Conclusions: The SOLIS interferometric observations of formamide provide direct evidence that this potentially crucial brick of life is efficiently formed in the gas-phase around Sun-like protostars., 7 pages, 1 table, 5 figures, A&A Letters, in press

Published
2017

3. Physical aging effects on the dynamic relaxation behavior and mechanical properties of Cu46Zr46Al8 metallic glass

Author

Shidong Feng, Eloi Pineda, Jean-Marc Pelletier, Jichao Qiao, Yuan Yao, Daniel Crespo, Matériaux, ingénierie et science [Villeurbanne] (MATEIS), Université Claude Bernard Lyon 1 (UCBL), Université de Lyon-Université de Lyon-Institut National des Sciences Appliquées de Lyon (INSA Lyon), Institut National des Sciences Appliquées (INSA)-Université de Lyon-Institut National des Sciences Appliquées (INSA)-Centre National de la Recherche Scientifique (CNRS), ESAB, Universitad polytecnica de Cataluna, 11572249, National Natural Science Foundation of China, 2016JM5009, Natural Science Foundation of Shaanxi Province, 2015ZF53072, Aeronautical Science Foundation of China, Generalitat de Catalunya, 51611130120, Programme de Recherche Conjoint CNRS/National Natural Science Foundation of China, FIS2014-54734-P, Mineco, SKLSP201608, State Key Laboratory of Solidification Processing in NWPU, Universitat Politècnica de Catalunya. Departament de Física, and Universitat Politècnica de Catalunya. GCM - Grup de Caracterització de Materials

Subjects
Ternary alloys, Materials science, Dynamic relaxation, Mechanical properties, 02 engineering and technology, Molecular dynamics, Condensed Matter::Disordered Systems and Neural Networks, 01 natural sciences, [SPI.MAT]Engineering Sciences [physics]/Materials, Copper alloys, Glass transition temperature Tg, 0103 physical sciences, Metal crystals, Materials Chemistry, Point defects, Composite material, 010306 general physics, Spectroscopy, Dynamic mechanical relaxation, Metallic glasses, Mechanical and physical properties, Zirconium alloys, Amorphous metal, Física [Àrees temàtiques de la UPC], Molecular dynamics simulations, Mechanical Engineering, Physical aging, Metals and Alloys, Dynamic mechanical analysis, 021001 nanoscience & nanotechnology, Aluminum alloys, Dynamics, Shear (sheet metal), Metallic glass, Mechanical spectroscopy, Mechanics of Materials, Metals, Relaxation (physics), Dynamic mechanical test, Defects, Glass, 0210 nano-technology, Glass transition, Cristalls metàl·lics
Abstract

cited By 2; International audience; Mechanical relaxation of glassy materials is strongly influenced by their mechanical and physical properties. In the current study, dynamic mechanical relaxation of Cu46Zr46Al8 metallic glass has been investigated by mechanical spectroscopy and molecular dynamics simulations. Our results show that mechanical properties of metallic glasses are highly dependent on their thermal history. α relaxation in the frequency region of the Cu46Zr46Al8 metallic glass was described by Havriliak-Negami (HN) model. In the framework of the quasi-point defects theory, the correlated factor χ could be used to characterize the concentration of “defects” of glassy materials. By molecular dynamics simulations of dynamic mechanical tests at different temperatures and frequencies, it is noted that adjusting of defects is inversely correlated to storage modulus at the atomic level. On the other hand, physical aging below the glass transition temperature Tg reduces the concentration of defects and narrows down the width of shear bands, which corresponds to decreasing of the atomic mobility. © 2017 Elsevier B.V.

Published
2017
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