Search

We developed a CANDLES-III system to study the neutrino-less double beta (0$\nu\beta\beta$) decay of $^{48}$Ca. The proposed system employs 96 CaF$_{2}$ scintillation crystals (305 kg) with natural Ca ($^{\rm nat.}$Ca) isotope which corresponds 350\,g of $^{48}$Ca. External backgrounds were rejected using a 4$\pi$ active shield of a liquid scintillator surrounding the CaF$_2$ crystals. The internal backgrounds caused by the radioactive impurities within the CaF$_2$ crystals can be reduced effectively through analysis of the signal pulse shape. We analyzed the data obtained in the Kamioka underground for a live-time of 130.4\,days to evaluate the feasibility of the low background measurement with the CANDLES-III detector. Using Monte Carlo simulations, we estimated the background rate from the radioactive impurities in the CaF$_{2}$ crystals and the rate of high energy $\gamma$-rays caused by the (n, $\gamma$) reactions induced by environmental neutrons. The expected background rate was in a good agreement with the measured rate, i.e., approximately 10$^{-3}$ events/keV/yr/(kg of $^{\rm nat.}$Ca), in the 0$\nu\beta\beta$ window. In conclusion, the background candidates were estimated properly by comparing the measured energy spectrum with the background simulations. With this measurement method, we performed the first search for 0$\nu\beta\beta$ decay in a low background condition using a detector with a Ca isotope, in which the Ca present was not enriched, in a scale of hundreds of kg. The $^{48}$Ca isotope has a high potential for use in 0$\nu\beta\beta$ decay search, and is expected to be useful for the development of a next-generation detector for highly sensitive measurements.

A search has been performed for neutrinos from two sources, the $hep$ reaction in the solar $pp$ fusion chain and the $��_e$ component of the diffuse supernova neutrino background (DSNB), using the full dataset of the Sudbury Neutrino Observatory with a total exposure of 2.47 kton-years after fiducialization. The $hep$ search is performed using both a single-bin counting analysis and a likelihood fit. We find a best-fit flux that is compatible with solar model predictions while remaining consistent with zero flux, and set a one-sided upper limit of $��_{hep} < 30\times10^{3}~\mathrm{cm}^{-2}~\mathrm{s}^{-1}$ [90% credible interval (CI)]. No events are observed in the DSNB search region, and we set an improved upper bound on the $��_e$ component of the DSNB flux of $��^\mathrm{DSNB}_{��_e} < 19~\textrm{cm}^{-2}~\textrm{s}^{-1}$ (90% CI) in the energy range $22.9 < E_��< 36.9$~MeV., 11 pages, 6 figures

In the CANDLES experiment aiming to search for the very rare neutrino-less double beta decays (0νββ) using 48Ca, we introduced a new shielding system for high energy γ-rays from neutron captures in massive materials near the detector, in addition to the background reduction for 232Th decays in the 0νββ target of CaF2 crystals. The method of background reduction and the performance of newly installed shielding system are described.

High energy γ rays with several MeV produced by (n,γ) reactions can be a trouble for low background measurements in the underground laboratories such as double beta decay experiments. In the CANDLES project, which aimed to observe the neutrino-less double beta decay from 48Ca, γ rays caused by (n,γ) reactions were found to be the most significant background. The profile of the background was studied by measurements with a neutron source and a simulation with a validity check of neutron processes in Geant4. The observed spectrum of γ rays from (n,γ) reactions was well reproduced by the simulated spectra, which were originated from the surrounding rock and a detector tank made of stainless steel. The environmental neutron flux was derived by the observed event rate of γ rays from (n,γ) reactions using the simulation. The thermal and non-thermal neutron flux were found to be ( 1.3 ± 0.6 ) × 10 − 6 cm − 2 s − 1 and ( 1.1 ± 0.5 ) × 10 − 5 cm − 2 s − 1 , respectively. It is necessary to install an additional shield to reduce the background from (n,γ) reaction to the required level.

We study a strategy to reduce veto-time in the search for neutrino-less double-beta decay (0υββ) with CANDLES-III system. We develop a new likelihood analysis and apply it to our new Run010 data. We show that we can increase the un-vetoed live-time by 11.8%. Thanks to this improvements, We expect to increase a limit on the life-time of 0υββ by a factor of three by analyzing both Run009 and Run010 data.

CAlcium fluoride for the study of Neutrinos and Dark matters by Low-energy Spectrometer (CANDLES) searches for neutrino-less double beta decay of $^{48}$Ca using a CaF$_2$ scintillator array. A high Q-value of $^{48}$Ca at 4,272 keV enabled us to achieve very low background condition, however, at the same it causes difficulties in calibrating the detector's Q-value region because of the absence of a standard high-energy $\gamma$-ray source. Therefore, we have developed a novel calibration system based on $\gamma$-ray emission by neutron capture on $^{28}$Si, $^{56}$Fe and $^{58}$Ni nuclei. In the paper, we report the development of the new calibration system as well as the results of energy calibration in CANDLES up to 9 MeV., Comment: 6 pages, 7 figures

In a neutrinoless double-beta decay ($0\nu\beta\beta$) experiment, energy resolution is important to distinguish between $0\nu\beta\beta$ and background events. CAlcium fluoride for studies of Neutrino and Dark matters by Low Energy Spectrometer (CANDLES) discerns the $0\nu\beta\beta$ of $^{48}$Ca using a CaF$_2$ scintillator as the detector and source. Photomultiplier tubes (PMTs) collect scintillation photons. At the Q-value of $^{48}$Ca, the current energy resolution (2.6%) exceeds the ideal statistical fluctuation of the number of photoelectrons (1.6%). Because of CaF$_2$'s long decay constant of 1000 ns, a signal integration within 4000 ns is used to calculate the energy. The baseline fluctuation ($\sigma_{baseline}$) is accumulated in the signal integration, thus degrading the energy resolution. This paper studies $\sigma_{baseline}$ in the CANDLES detector, which severely degrades the resolution by 1% at the Q-value of $^{48}$Ca. To avoid $\sigma_{\rm baseline}$, photon counting can be used to obtain the number of photoelectrons in each PMT; however, a significant photoelectron signal overlapping probability in each PMT causes missing photoelectrons in counting and reduces the energy resolution. "Partial photon counting" reduces $\sigma_{baseline}$ and minimizes photoelectron loss. We obtain improved energy resolutions of 4.5-4.0% at 1460.8 keV ($\gamma$-ray of $^{40}$K), and 3.3-2.9% at 2614.5 keV ($\gamma$-ray of $^{208}$Tl). The energy resolution at the Q-value is estimated to be improved from 2.6% to 2.2%, and the detector sensitivity for the $0\nu\beta\beta$ half-life of $^{48}$Ca can be improved by 1.09 times., Comment: This manuscript is prepared for submission to IEEE Transaction on Nuclear Science. It contains 11 pages, 19 figures, and 1 table

The neutrino-less double beta decay (0νββ) is a powerful tool to probe the neutrino mass. The 0νββ is forbidden in Standard Model (SM) due to the violation of lepton number conservation. In experiments searching for 0νββ, the two-neutrino double beta decay (2νββ), which is an allowed process in SM, behaves as an irreducible background within the energy of interest. To discriminate the 0νββ from 2νββ, the energy resolution must be improved. The CANDLES experiment is searching for the 0νββ of 48Ca using CaF 2 (pure) scintillator as the detector and the source. Scintillation photons are collected by Photo Multiplier Tubes (PMTs) surrounding the crystals. A Flash Analog-to-Digital Converter records the waveform of each PMT. Because of the long decay time of CaF 2 (1 µsec), we make a signal integral of 4 µsec to calculate the obtained energy. Thus, the other fluctuation in the baseline is accumulated in the signal integration, and it makes the energy resolution worse. To reduce this fluctuation, we can count the number of photoelectrons in every PMT. Still, we have a significant overlapping probability of single photoelectron signals. This overlapping probability implies the photoelectrons lost, which causes terrible energy resolution. To improve the energy resolution, we introduce an alternative method named "partial photon counting" by dividing the waveform into two parts, then, perform signal integral in the prompt part and photon counting the second part. As a result, the energy resolution is reduced 4.0-3.5 % at 1460 keV (γ-ray of 40K) and 3-2.7 % at 2615 keV (γ-ray of 208Tl).

The highly radiopure NaI(Tl) was developed to search for particle candidates of dark matter. The optimized methods were combined to reduce various radioactive impurities. The $^{40}$K was effectively reduced by the re-crystallization method. The progenies of the decay chains of uranium and thorium were reduced by appropriate resins. The concentration of natural potassium in NaI(Tl) crystal was reduced down to 20 ppb. Concentrations of alpha-ray emitters were successfully reduced by appropriate selection of resin. The present concentration of thorium series and 226Ra were $1.2 \pm1.4$ $\mu$Bq/kg and $13\pm4$ $\mu$Bq/kg, respectively. No significant excess in the concentration of $^{210}$Pb was obtained, and the upper limit was 5.7 $\mu$Bq/kg at 90% C. L. The achieved level of radiopurity of NaI(Tl) crystals makes construction of a dark matter detector possible., Comment: 11 pages, 6 figures, accepted to Progress of Theoretical and Experimental Physics

The current status of laboratory for Dark Matter search at the Kamioka mine and specialized facility for production of NaI(Tl) detectors is described. Techniques developed for purification and growth of ultra-low background NaI(Tl) crystals are reported. Achieved activity levels of the 210Pb, 40K, 238U, 232 Th isotopes in the latest NaI(Tl) Dark Matter detector prototypes and the DAMA/LIBRA detectors are compared.

A new data acquisition (DAQ) system for the CANDLES experiment was developed using the SpaceWire protocol and the DAQ-Middleware framework. The CANDLES experiment uses a trigger board and Flash Analog-to-Digital Converters (FADCs). The SpaceWire helps us construct the DAQ system with a flexible and multi-path access to FADCs and the trigger board. FADCs have a ring buffer with three buffers to detect sequential decays from backgrounds. We developed the DAQ system with parallel read-out to reduce the dead time at high trigger rates using three read-out personal computers (PCs) that are connected to the three buffers in FADCs one by one. Each PC connects all FADCs and the trigger board and gathers a complete data set of one event without any event builder. The maximum DAQ speed of parallel read-out by three PCs was 2.4 times higher than that of single read-out. In order to collect event data sets from PCs, we built the network distributed DAQ system through Ethernet, which is naturally introduced with the DAQ-Middleware. To realize remote monitoring and histogram modification while the DAQ running, we also developed a dynamic online monitor system independent with the DAQ-Middleware.

CANDLES studies the double beta decay of 48Ca through CaF2 scintillation crystals. The CANDLES III detector, located in Kamioka underground laboratory, is currently running. Here we describe recent status of data analysis which includes detector performance, detector stability, and background estimation. Current sensitivity for 0 ν β β half-life is also discussed in this paper.

CANDLES aims to measure the very rare neutrino-less double beta decays using 48Ca which has the highest value among all isotope candidates. Low background techniques are the key to observe such rare phenomena. The largest background was found to be the high energy gamma rays from neutron captures on abundant material near the detector. The shielding system consisted of lead and B-contained rubber sheet was constructed to reduce the background. Performance of the constructed shielding system were described in this paper.

The neutrino-less double beta decay is acquiring great interest after the confirmation of neutrino oscillation which demonstrated nonzero neutrino mass. In order to search for neutrino-less double beta decay of $^{48}$Ca, we proposed the CANDLES project by using CaF$_{2}$(pure) scintillators. Now we installed the CANDLES III system at the Kamioka underground laboratory. The CANDLES III system realizes the low background condition by a characteristic structure and data analyses for background rejection. Furthermore we installed new shielding system in order to reduce $\gamma$-ray backgrounds from neutron capture reaction. Here we report performances of the CANDLES III system.

Direct search for dark matter is one of the most important problems in astrophysics. Significant signal for dark matter will be a hint to clarify the origin of the universe. Only DAMA/LIBRA experiment with NaI(Tl) detector has ever suggested the presence of dark matter signal. Verifying the DAMA/LIBRA result by a NaI(Tl) detector is urgent and important task. We have tried to purify NaI(Tl) crystal to search for dark matter. In this presentation, the present status of purification will be discussed. The concentration of potassium is successfully reduced to desired sensitivity. The 210Pb, which is difficult to reduce, has been reduced effectively. Present status of low background measurement in Kamioka observatory will be shown.

The PICOLON project is developing a high purity NaI(Tl) crystal by optimizing the purification methods. The reduction method for 40K was established and we got sufficiently pure NaI(Tl) crystal for 40K. On the other hand, the concentration of 210Pb is still higher than our goal. The investigation is now in progress to fix the origin of the contamination. The construction of the second phase detector system of PICOLON detector will be started in 2020 spring. The total mass of the second phase is about 54 kg. The background level by the test measurement using a single module is reported.

We have studied the neutrino-less double beta decay(0νββ) of 48Ca by using CaF2(pure) scintillators. Analysis for rejection of backgrounds(212Bi→ 212Po events and 208Tl events) was effective to reduce backgrounds in Qββ-value region. No events are observed in the Qββ-value region for the data of 131 days × 86 kg. It gives a lower limit (90% confidence level) of (math) > 6.2 × 1022 year (preliminary) for the half-life of 0νββ of 48Ca.

Recent data from the DAMA/LIBRA phase-2 confirmed detection of a signal with independent Dark Matter (DM) annual modulation signature at a 12.9 σ CL. Our attempts to verify the DAMA/LIBRA DM observation claim led to construction of underground clean rooms at the KamLAND site and specialized laboratory for production of NaI(Tl) detectors. Current status of these facilities, methods used to grow ultra-low background NaI(Tl) crystals, and radio-purity of the latest NaI(Tl) DM detector prototype are discussed.

The concentration of 7Be in surface air and rainwater at Daito, Osaka (34.71 N, 135.64 E) has been measured during the period from January 8 to October 29, 2018 and April 1 to October 31, 2018, respectively. The weekly concentration of 7Be in surface air in the range of 8.92 ± 0.08 to 1.03 ± 0.02 mBq/m3 showing seasonal trend with maxima in spring and autumn and minima in summer, which can be ascribed to the transport of air masses from low latitudes carrying low 7Be concentration into the middle latitude region. The factors influences on the concentration of 7Be were examined. It was shown that the positive and negative correlation was found in PM2.5 (cc = 0.62) and relative humidity (cc = –0.57), respectively. The weak positive correlation was found in cosmic ray intensity (cc = 0.23), the weak negative correlation was found in precipitation (cc = –0.14) and sunspot number (cc = –0.05). The deposition rate was analyzed by using the rainwater samples. It shown negative correlation between deposition rate and precipitation (cc = –0.53). High volumes of precipitation can reduce the 7Be concentration of air by wash-out.

A high purity and large volume NaI(Tl) scintillator was developed to search for cosmic dark matter. The required densities of radioactive impurities (RIs) such as U-chain, Th-chain are less than a few ppt to establish high sensitivity to dark matter. The impurity of RIs were effectively reduced by selecting raw materials of crucible and by performing chemical reduction of lead ion in NaI raw powder. The impurity of $^{226}$Ra was reduced less than 100 $\mu$Bq/kg in NaI(Tl) crystal. It should be remarked that the impurity of $^{210}$Pb, which is difficult to reduce, is effectively reduced by chemical processing of NaI raw powder down to less than 30 $\mu$Bq/kg. The expected sensitivity to cosmic dark matter by using 250 kg of the high purity and large volume NaI(Tl) scintillator (PICO-LON; Pure Inorganic Crystal Observatory for LOw-background Neutr(al)ino) is 7$\times$10$^{-45}$ cm$^{2}$ for 50 GeV$/c^{2}$ WIMPs., Comment: 6 pages, 2 Figures, Proceedings of International Symposium on Radiation Detectors and Their Uses (ISRD2016). Talk given on 19th Jan. 2016 by K.Fushimi. To be published in Proceedings will be published as JPS conference proceedings (2016)

A low background HPGe detector system was developed at CANDLES Experimental Hall for multipurpose use. Various low background techniques were employed, including hermatic shield design, radon gas suppression, and background reduction analysis. A new pulse shape discrimination (PSD) method was specially created for coaxial Ge detector. Using this PSD method, microphonics noise and background event at low energy region less than 200 keV can be rejected effectively. Monte Carlo simulation by GEANT4 was performed to acquire the detection efficiency and study the interaction of gamma-rays with detector system. For rare decay measurement, the detector was utilized to detect the nature’s most stable isomer tantalum-180m (180Tam) decay. Two phases of tantalum physics run were completed with total livetime of 358.2 days, which Phase II has upgraded shield configuration. The world most stringent half-life limit of 180Tam has been successfully achieved.

The PICO-LON project aims at search for cold dark matter by means of highly radio-pure and large volume NaI(Tl) scintillator. The NaI powder was purifed by chemical processing to remove lead isotopes and selecting a high purity graphite crucible. The concentrations of radioactive impurities of $^{226}$Ra and $^{228}$Th were effectively reduced to 58$\pm$4 $\mu$Bq/kg and 1.5$\pm$1.9 $\mu$Bq/kg, respectively. It should be remarked that the concentration of $^{210}$Pb, which is crucial for the sensitivity to dark matter, was reduced to 24$\pm$2 $\mu$Bq/kg. The total background rate at 10 keVee was as low as 8 keV$^{-1}$kg$^{-1}$day$^{-1}$, which was sufficiently low to search for dark matter. Further purification of NaI(Tl) ingot and future prospect of PICO-LON project is discussed., Comment: Submitted to Proceedings of TAUP 2015

The observation of neutrino-less double beta decay (0νββ) would be the most practical way to prove the Majorana nature of the neutrino and lepton number violation. CANDLES studies 48Ca double beta decay using CaF2 scintillator. The main advantage of 48Ca is that it has the highest Q-value (4.27 MeV) among all the isotope candidates for 0νββ. The CANDLES III detector is currently operating with 300kg CaF2 crystals in the Kamioka underground observatory, Japan. In 2014, a detector cooling system and a magnetic cancellation coil was installed with the aim to increase light emission of CaF2 scintillator and photo-electron collection efficiency of the photo-multipliers. After this upgrade, light yield was increased to 1000 p.e./MeV which is 1.6 times larger than before. According to data analysis and simulation, main background source in CANDLES is turned out to be high energy external gamma-ray originating neutron capture on the surrounding materials, so called (n,γ). Upgrading the detector by installing neutron and gamma-ray shield can reduce the remaining main backgrounds by two order magnitude. In this report, we discuss the detail of (n,γ) and background reduction by additional shielding.