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The discovery of the new proton emitter $^{116}_{~57}$La$_{59}$, 23 neutrons away from the only stable La isotope, $^{139}_{~57}$La$_{82}$, is reported. The $^{116}$La nuclei were synthesised in the fusion-evaporation reaction $^{58}$Ni($^{64}$Zn, p4n)$^{116}$La and identified via their proton radioactivity using the MARA mass spectrometer and the silicon detectors placed at its focal plane. Comparisons of the measured proton energy ($E_{p} = 718 \pm 9 $ keV) and half-life ($T_{1/2} = 50 \pm 22$ ms) with values calculated using %microscopic nuclear barrier penetration theory the Universal Decay Law approach indicate that the proton is emitted with an orbital angular momentum $l=2$ and that its emission probability is enhanced relative to its closest, less exotic, odd-even lanthanum isotope ($^{117}_{~57}$La$_{60}$) while the proton-emission $Q$-value is lower. We propose this to be a signature for the presence of strong neutron-proton pair correlations in this exotic, neutron deficient system. The observations of $\gamma$ decays from isomeric states in $^{116}$La and $^{117}$La are also reported.

5 pags., 4 figs., Excited states in Zn were populated following one-neutron removal from a Zn beam impinging on a Be target at intermediate energies in an experiment conducted at the Radioactive Isotope Beam Factory at RIKEN. Three γ rays were observed and tentatively assigned to the 6→4→2→0 yrast sequence. This turns Zn into the heaviest T=−2 nucleus in which excited states are known. The excitation-energy differences between these levels and the isobaric analogue states in the T=+2 mirror partner, Fe, are compared with large-scale shell-model calculations considering the full pf valence space and various isospin-breaking contributions. This comparison, together with an analysis of the mirror energy differences in the A=58, T=±1 pair Zn and Ni, provides valuable information with respect to the size of the monopole radial and the isovector multipole isospin-breaking terms in the region above doubly-magic Ni., We thank the RIKEN Nishina Center accelerator staff and the BigRIPS team for providing excellent beams to the experiment. This work was supported by the Spanish Ministerio de Ciencia e Inno- vación under contracts FPA2017-84756-C4-2-P, PGC-2018-94583, and SEV-2016-0597, the Swedish Research Council (Vetenskap- srådet, VR 2016-3969), and the UK Science and Technology Facil- ities Council (STFC) under grants ST/L005727/1 and ST/P003885/1. FB is supported by the RIKEN Special Postdoctoral Researcher Pro- gram

Decay spectroscopy of the odd-proton nuclei $^{249}$Md and $^{251}$Md has been performed. High-K isomeric states were identified for the first time in these two nuclei through the measurement of their electromagnetic decay. An isomeric state with a half-life of 2.8(5) ms and an excitation energy $\ge 910$ keV was found in $^{249}$Md. In $^{251}$Md, an isomeric state with a half-life of 1.4(3) s and an excitation energy $\ge 844$ keV was found. Similarly to the neighbouring $^{255}$Lr, these two isomeric states are interpreted as 3 quasi-particle high-K states and compared to new theoretical calculations. Excited nuclear configurations were calculated within two scenarios: via blocking nuclear states located in proximity to the Fermi surface or/and using the quasiparticle Bardeen–Cooper–Schrieffer method. Relevant states were selected on the basis of the microscopic-macroscopic model with a deformed Woods–Saxon potential. The most probable candidates for the configurations of K-isomeric states in Md nuclei are proposed. Decay spectroscopy of the odd-proton nuclei $^{249}$Md and $^{251}$Md has been performed. High-$K$ isomeric states were identified for the first time in these two nuclei through the measurement of their electromagnetic decay. An isomeric state with a half-life of $2.8(5)$ ms and an excitation energy $\geq 910$ keV was found in $^{249}$Md. In $^{251}$Md, an isomeric state with a half-life of $1.4(3)$ s and an excitation energy $\geq 844$ keV was found. Similarly to the neighbouring $^{255}$Lr, these two isomeric states are interpreted as 3 quasi-particle high-$K$ states and compared to new theoretical calculations. Excited nuclear configurations were calculated within two scenarios: via blocking nuclear states located in proximity to the Fermi surface or/and using the quasiparticle Bardeen-Cooper-Schrieffer method. Relevant states were selected on the basis of the microscopic-macroscopic model with a deformed Woods-Saxon potential. The most probable candidates for the configurations of $K$-isomeric states in Md nuclei are proposed.

International audience; Prolate-oblate shape coexistence close to the ground state in the strongly-deformed proton-rich A≈120 nuclei is reported for the first time. One of the four reported bands in 119Cs, built on a 11/2− state at 670 keV, consists of nearly degenerate signature partners, and has properties which unequivocally indicate the strongly-coupled πh11/2[505]11/2− configuration associated with oblate shape. Together with the decoupled πh11/2[541]3/2− band built on the 11/2− prolate state at 110 keV, for which a half-life of T1/2=55(5)μs has been measured, the new bands bring evidence of shape coexistence at low spin in the proton-rich strongly deformed A≈120 nuclei, a phenomenon predicted since long time, but not yet observed. Calculations using the particle-number conserving cranked shell model and two dimensional tilted axis cranking covariant density functional theory support and well reproduce the observed oblate and prolate coexisting low-energy states in 119Cs.

Gamma-Ray Infrastructure For Fundamental Investigations of Nuclei, GRIFFIN, is a new high-efficiency γ -ray spectrometer designed for use in decay spectroscopy experiments with low-energy radioactive ion beams provided by TRIUMF’s Isotope Separator and Accelerator (ISAC-I) facility. GRIFFIN is composed of sixteen Compton-suppressed large-volume clover-type high-purity germanium (HPGe) γ -ray detectors combined with a suite of ancillary detection systems and coupled to a custom digital data acquisition system. The infrastructure and detectors of the spectrometer as well as the performance characteristics and the analysis techniques applied to the experimental data are described.

Two new excited bands built on the πh11/2 configuration have been identified in Nd135 in addition to the known πh11/2 band. The energy spectra of the excited bands and the available electromagnetic transition probabilities are in good agreement with theoretical results obtained using quasiparticle-plus-triaxial-rotor model calculations. The properties of the bands identify them as tilted precession bands instead of wobbling bands. Our results give a new insight into the interpretation of the low-lying bands in odd-A mass nuclei, and can stimulate future studies to address the nuclear triaxiality.

Lifetime measurements in $$^{178}$$ 178 Pt with excited states de-exciting through $$\gamma $$ γ -ray transitions and internal electron conversions have been performed. Ionic charges were selected by the in-flight mass separator MARA and measured at the focal plane in coincidence with the $$4_1^+\rightarrow 2_1^+$$ 4 1 + → 2 1 + $$257\,$$ 257 keV $$\gamma $$ γ -ray transition detected using the JUROGAM 3 spectrometer. The resulting charge-state distributions were analysed using the differential decay curve method (DDCM) framework to obtain a lifetime value of 430(20) ps for the $$2_1^+$$ 2 1 + state. This work builds on a method that combines the charge plunger technique with the DDCM analysis. As an alternative analysis, ions were selected in coincidence with the $$^{178}$$ 178 Pt alpha decay ($$E_{\mathrm {alpha}} = 5.458(5)$$ E alpha = 5.458 ( 5 ) MeV) at the focal plane. Lifetime information was obtained by fitting a two-state Bateman equation to the decay curve with the lifetime of individual states defined by a single quadrupole moment. This yielded a lifetime value of 430(50) ps for the $$2_1^+$$ 2 1 + state, and 54(6) ps for the $$4_1^+$$ 4 1 + state. An analysis method based around the Bateman equation will become especially important when using the charge plunger method for the cases where utilising coincidences between prompt $$\gamma $$ γ rays and recoils is not feasible.

Fine structure in the α decay of Th90221, populating excited states in Ra88217, was studied using αγ-coincidence spectroscopy. Two α-decay branches from Th221 have been newly observed, with Eα(keV)[bα(%)]=7951(8)[0.14(3)] and 8247(3)[1.51(12)], together with three previously known branches. Also, two new states in Ra217 were identified at E = 177 and 227 keV. The ground-state configurations of the odd-A, N = 131 transitional isotones above Pb208 are interpreted from their α-decay fine structure systematics and considered in terms of predictions using spherical shell and reflection-asymmetric models.

A high-precision branching ratio measurement for the superallowed Fermi $\beta^{+}$ emitter $^{62}$Ga was performed with the Gamma-Ray Infrastructure for Fundamental Investigations of Nuclei (GRIFFIN) spectrometer at the Isotope Separator and Accelerator (ISAC) radioactive ion beam facility at TRIUMF. The high efficiency of the GRIFFIN spectrometer allowed 63 $\gamma$-ray transitions, with intensities down to $\approx$1 part per million (ppm) per $^{62}$Ga $\beta^{+}$ decay, to be placed in the level scheme of the daughter nucleus $^{62}$Zn, establishing the superallowed $\beta$ branching ratio for $^{62}$Ga decay to be 99.8577$^{+0.0023}_{-0.0029}\%$, a factor of 4 more precise than the previous world average. For several cascades, $\gamma-\gamma$ angular correlation measurements were performed to assign spins and/or determine the mixing ratios of transitions. In particular, the spin of the 2.342 MeV excited state in the daughter nucleus $^{62}$Zn was definitively assigned as $J = 0$. This assignment resolves a discrepancy between previous measurements and has important implications for the isospin symmetry breaking correction, $\delta_{C1}$, in $^{62}$Ga superallowed Fermi $\beta$ decay.

High-spin states of the odd–odd $${}^{194}$$ Bi nucleus have been studied by means of nuclear spectroscopy for the first time. Two low-lying rotational bands were observed. The positive-parity band built on a short-lived isomeric state 633 keV above the $$\alpha $$ and $$\beta $$ decaying long-lived (10 $$^-$$ ) state is assigned a $${\pi i_{13/2} \otimes \nu i_{13/2 }^{-1}}$$ configuration, while the other band is attributed to the $${\pi h_{9/2} \otimes \nu i_{13/2 }^{-1}}$$ configuration. Both of these bands are assumed to have oblate shape. Three band-like structures composed predominantly of $$\Delta I = 1$$ transitions were also found. One of the shears band candidates is firmly linked to the lower lying level structures whereas for the other two links to lower-lying structures remain missing.

The jurogam 3 spectrometer has been constructed for in-beam $$\gamma $$γ-ray spectroscopy experiments in the Accelerator Laboratory of the University of Jyväskylä, Finland. jurogam 3 consists of germanium-detector modules in a compact geometry surrounding a target to measure $$\gamma $$γ rays emitted from radioactive nuclei. jurogam 3 can be employed in conjunction with one of two recoil separators, the mara vacuum-mode separator or the ritu gas-filled separator, and other ancillary devices.

Decay spectroscopy of No250 has been performed using digital electronics and pulse-shape analysis of the fast nuclear decays for the first time. Previous studies of No250 reported two distinct fission decay lifetimes, related to the direct fission of the ground state and to the decay of an isomeric state but without the possibility to determine if the isomeric state decayed directly via fission or via internal electromagnetic transitions to the ground state. The data obtained in the current experiment allowed the puzzle to finally be resolved, attributing the shorter half-life of t1/2=3.8±0.3μs to the ground state and the longer half-life t1/2=34.9−3.2+3.9μs to the decay of an isomeric state. No250 becomes, thus, one of a very few examples of very heavy nuclei with an isomeric state living considerably longer than its ground state. This phenomenon has important consequences for the nuclear-structure models aiming to determine the borders of the island of stability of superheavy elements.

High-spin states in the N = 128 nucleus 218Th have been investigated following fusion–evaporation reactions, using the recoil-decay tagging technique. Due to the short-lived nature of the ground state of 218Th prompt γ rays have been correlated with the α decay of the daughter nucleus 214Ra. The level scheme representing the decay of excited states has been extended to (16+) with the observation of six previously unreported transitions. The observations are compared with the results of shell model calculations and within the context of the systematics of neighbouring nuclei.

Two new bands have been identified in $^{137}$Nd from a high-statistics JUROGAM II gamma-ray spectroscopy experiment. Constrained density functional theory and particle rotor model calculations are used to assign configurations and investigate the band properties, which are well described and understood. It is demonstrated that these two new bands can be interpreted as chiral partners of previously known three-quasiparticle positive- and negative-parity bands. The newly observed chiral doublet bands in $^{137}$Nd represent an important support to the existence of multiple chiral bands in nuclei. The present results constitute the missing stone in the series of Nd nuclei showing multiple chiral bands, which becomes the most extended sequence of odd–even and even-even nuclei presenting multiple chiral bands in the Segré chart. Two new bands have been identified in $^{137}$Nd from a high-statistics JUROGAM II gamma-ray spectroscopy experiment. Constrained density functional theory and particle rotor model calculations are used to assign configurations and investigate the band properties, which are well described and understood. It is demonstrated that these two new bands can be interpreted as chiral partners of previously known three-quasiparticle positive- and negative-parity bands. The newly observed chiral doublet bands in $^{137}$Nd represent an important support to the existence of multiple chiral bands in nuclei. The present results constitute the missing stone in the series of Nd nuclei showing multiple chiral bands, which becomes the most extended sequence of nuclei presenting multiple chiral bands in the Segr\'e chart.

The extremely neutron-deficient isotopes 177,179Au were studied by means of in-beam ?-ray spectroscopy. Specific tagging techniques, ?-decay tagging in 177Au and isomer tagging in 179Au, were used for these studies. Feeding of positive-parity, nearly spherical states, which are associated with 2d3/2 and 3s1/2 proton-hole configurations, from the 1i13/2 proton-intruder configuration was observed in 177Au. Such a decay path has no precedent in odd-Au isotopes and it is explained by the effect of mixing of wave functions of the initial state. © 2020, 262010 2/0129/17 Science and Technology Facilities Council, STFC European Research Council, ERC: 203481 Academy of Finland: 131665 Agentúra na Podporu V?skumu a V?voja, APVV: APVV-15-0225, The authors express their gratitude to the staff of the Accelerator Laboratory at the University of Jyväskylä for their excellent technical support. This work has been supported by the EU-FP7-IA project ENSAR (No. 262010 ), the Academy of Finland (CoE in Nuclear and Accelerator Based Physics, grant to T.G., Contract No. 131665 ), the European Research Council through the project SHESTRUCT (Grant Agreement No. 203481 ), the UK Science and Technology Facilities Council , the Slovak Research and Development Agency under Contract No. APVV-15-0225 , and the Slovak Grant Agency VEGA (Contract No. 2/0129/17 ).

Excited states in the extremely neutron-deficient nucleus $$^{172}{\mathrm {Pt}}$$172Pt were populated via $$^{96}\mathrm {Ru}(^{78}\mathrm {Kr},2p)$$96Ru(78Kr,2p) and $$^{92}\mathrm {Mo}(^{83}\mathrm {Kr},3n)$$92Mo(83Kr,3n) reactions. The level scheme has been extended up to an excitation energy of $$\approx 5~\hbox {MeV}$$≈5MeV and tentative spin-parity assignments up to $$I^\pi = 18^+$$Iπ=18+. Linear polarization and angular distribution measurements were used to determine the electromagnetic E1 character of the dipole transitions connecting the positive-parity ground-state band with an excited side-band, firmly establishing it as a negative-parity band. The lowest member of this negative-parity structure was firmly assigned spin-parity $$3^-$$3-. In addition, we observed an E3 transition from this $$3^-$$3- state to the ground state, providing direct evidence for octupole collectivity in $$^{172}{\mathrm {Pt}}$$172Pt. Large-scale shell model (LSSM) and total Routhian surface (TRS) calculations have been performed, supporting the interpretation of the $$3^-$$3- state as a collective octupole-vibrational state.

The TIGRESS Integrated Plunger device (TIP) has been developed for recoil distance method (RDM) lifetime measurements using the TIGRESS array of HPGe γ -ray detectors at TRIUMF’s ISAC-II facility. A commissioning experiment was conducted utilizing a 250 MeV 84Kr beam at ≈ 2 × 1 0 8 particles per second. The 84Kr beam was Coulomb excited to the 2 1 + state on a movable 27Al target. A thin Cu foil fixed downstream from the target was used as a degrader. Excited nuclei emerged from the target and decayed by γ -ray emission at a distance determined by their velocity and the lifetime of the 2 1 + state. The ratio of decays which occur between the target and degrader to those occurring after traversing the degrader changes as a function of the target–degrader separation distance. Gamma-ray spectra at 13 target–degrader separation distances were measured and compared to simulated lineshapes to extract the lifetime. The result of τ = 5 . 541 ± 0 . 013 (stat.) ± 0 . 063 (sys.) ps is shorter than the literature value of 5 . 84 ± 0 . 18 ps with a reduction in uncertainty by a factor of approximately two. The TIP plunger device, experimental technique, analysis tools, and result are discussed.

The mean lifetimes of the lowest energy 2(+), 8(+) and 9(-) states in Os-166 have been measured using the recoil distance Doppler-shift method in conjunction with a selective recoil-decay tagging t ...

© 2019 American Physical Society. An analysis technique has been developed in order to mitigate energy summing due to sequential short-lived α decays from nuclei implanted into a silicon detector. Using this technique, α-decay spectroscopy of the N=130 isotones Ra218 (Z=88) and Th220 (Z=90) has been performed. The energies of the α particles emitted in the Ra218→Rn214 and Th220→Ra216 ground-state-to-ground-state decays have been measured to be 8381(4) keV and 8818(13) keV, respectively. The half-lives of the ground states of Ra218 and Th220 have been measured to be 25.99(10) μs and 10.4(4) μs, respectively. The half-lives of the ground states of the α-decay daughters, Rn214 and Ra216, have been measured to be 259(3) ns and 161(11) ns, respectively. Fine structure in the α decay of Ra218 has been observed for the first time, populating the 695-keV 21+ state in Rn214. The fine-structure α decay has an α-particle energy of 7715(40) keV and branching ratio bα=0.123(11)%.

The Tz=−32 nucleus 21Mg has been studied by Coulomb excitation on 196Pt and 110Pd targets. A 205.6(1)-keV γ-ray transition resulting from the Coulomb excitation of the 52+ ground state to the first excited 12+ state in 21Mg was observed for the first time. Coulomb excitation cross-section measurements with both targets and a measurement of the half-life of the 12+ state yield an adopted value of B(E2;52+→12+)=13.3(4) W.u. A new excited state at 1672(1) keV with tentative 92+ assignment was also identified in 21Mg. This work demonstrates a large difference in the B(E2;52+→12+) value between T=32, A=21 mirror nuclei. The difference is investigated in the shell-model framework employing both isospin conserving and breaking USD interactions and using modern ab initio nuclear structure calculations, which have recently become applicable in the sd shell. (Less)

A Triple-foil differential Plunger for Exotic Nuclei (TPEN) has been developed to measure the lifetimes of excited states in nuclei with small production cross-sections. TPEN utilises one target foil and two degrader foils to make differential lifetime measurements: directly determining the decay function and its derivative at a single plunger distance setting. The direct measurement of the decay function and its derivative removes the requirement to measure γ -ray intensities at several target-to-degrader distances, thereby reducing the beam-time required relative to a conventional plunger with a single-degrader foil. This paper describes the commissioning of TPEN in the lifetime measurement of the first excited 4 + state in 156Dy using this differential lifetime technique. The 46(2) ps measured lifetime was found to be in good agreement with the 45.6(5) ps deduced from a previous high-statistics experiment using a conventional two-foil plunger. A comparison between the differential mode with TPEN, and that using TPEN as a conventional two-foil plunger reveals that it achieves the same statistical accuracy with a ∼ 4 -fold reduction in beam-time in the differential mode, for the reaction and experimental setup used in this work. TPEN opens up new opportunities to study exotic nuclei with lower production cross-sections that were previously not accessible.

In the study of the odd-$Z$, even-$N$ nuclei $^{243}$Es and $^{249}$Md, performed at the University of Jyv\"askyl\"a, the fusion-evaporation reactions $^{197}$Au($^{48}$Ca,2$n$)$^{243}$Es and $^{203}$Tl($^{48}$Ca,2$n$)$^{249}$Md have been used for the first time. Fusion-evaporation residues were selected and detected using the RITU gas-filled separator coupled with the focal-plane spectrometer GREAT. For $^{243}$Es, the recoil decay correlation analysis yielded a half-life of $24 \pm 3$s, and a maximum production cross section of $37 \pm 10$ nb. In the same way, a half-life of $26 \pm 1$ s, an $\alpha$ branching ratio of 75 $\pm$ 5%, and a maximum production cross section of 300 $\pm$ 80 nb were determined for $^{249}$Md. The decay properties of $^{245}$Es, the daughter of $^{249}$Md, were also measured: an $\alpha$ branching ratio of 54 $\pm$ 7% and a half-life of 65 $\pm$ 6 s. Experimental cross sections were compared to the results of calculations performed using the KEWPIE2 statistical fusion-evaporation code.

International audience; Three new highly-deformed (HD) bands are identified in Nd136 and the highly deformed band of Nd137 is extended at higher spin by four transitions, revealing a band crossing associated with the occupation of the second νi13/2 intruder orbital. Extended cranked Nilsson-Strutinsky calculations are performed for all HD bands observed in Nd134, Nd136, and Nd137, achieving for the first time a consistent interpretation of all HD bands in the Nd nuclei. The new interpretation has significant consequences, like the change of parity of the yrast HD bands of Nd134 and Nd136, and the involvement of two negative-parity neutron intruder orbitals in the configurations of most HD bands. The present experimental results and their theoretical interpretation represent an important step forward in the understanding of the second-minimum excitations in the Nd nuclei.

International audience; Multipolarity measurements are presented for transitions in the deformed odd-mass nucleus$^{167}$ Yb in support of tentative spin assignments and level interpretations based upon the cranked-Nilsson model. Internal-conversion coefficients were measured with the SAGE (Silicon And GErmanium) spectrometer confirming several E2 transition assignments. The array of high-purity germanium detectors enabled the recording of high-multiplicity events from which $\gamma\gamma\gamma$ and $\gamma\gamma e^{-}$ data sets were extracted and the technique of high-fold $\gamma$ -ray gating was demonstrated to cleanly isolate transitions of interest.

A charge plunger device has been commissioned based on the DPUNS plunger (Taylor et al., 2013) using the in-flight mass separator MARA at the University of Jyvaskyla. The 152 Sm (32 S ,4 n )180 Pt reaction was used to populate excited states in 180 Pt . A lifetime measurement of the 2 1 + state was performed by applying the charge plunger technique, which relies on the detection of the charge state-distribution of recoils rather than the detection of the emitted γ rays. This state was a good candidate to test the charge plunger technique as it has a known lifetime and depopulates through a converted transition that competes strongly with γ -ray emission. The lifetime of the 2 1 + state was measured to be 480 ( 10 ) ps , which is consistent with previously reported lifetimes that relied on the standard γ -ray techniques. The charge plunger technique is a complementary approach to lifetime measurements of excited states that depopulate through both γ -ray emission and internal conversion. In cases where it is not possible to detect Doppler-shifted γ rays, for example, in heavy nuclei where internal conversion dominates, it may well be the only feasible lifetime analysis approach.

The SPectrometer for Internal Conversion Electrons (SPICE) has been commissioned for use in conjunction with the TIGRESS $\gamma$-ray spectrometer at TRIUMF's ISAC-II facility. SPICE features a permanent rare-earth magnetic lens to collect and direct internal conversion electrons emitted from nuclear reactions to a thick, highly segmented, lithium-drifted silicon detector. This arrangement, combined with TIGRESS, enables in-beam $\gamma$-ray and internal conversion electron spectroscopy to be performed with stable and radioactive ion beams. Technical aspects of the device, capabilities, and initial performance are presented.

Internal conversion coefficients have been measured for transitions in 110Pd to allow the determination of electric monopole (E0) transition strengths. Excited states were populated through inelastic alpha scattering and the SPICE+TIGRESS detectors at TRIUMF-ISAC-II were used to detect the emitted gamma rays and internal conversion electrons. The E0 transition strengths are found to be small and are consistent with the expectation for transitions from a K = 2 band to the K = 0 ground-state band in the axial rotor model.

Fine structure in the a decay of high-spin isomers in Lu-155( 25/2(-)) and Hf-156(8(+))has been studied for the first time using alpha gamma- coincidence analysis. Three new a decays from Lu-155(25 ...

A multiparticle spin-trap isomeric state having a half-life of 179(4) ns and lying 2601 keV above the yrast 10(+) state in Lu-156 has been discovered. The Lu-156 nuclei were produced by bombarding ...

Many-body nuclear theory utilizing microscopic or chiral potentials has developed to the point that collectivity might be dealt with in an {\it ab initio} framework without the use of effective charges; for example with the proper evolution of operators, or alternatively, through the use of an appropriate and manageable subset of particle-hole excitations. We present a precise determination of $E2$ strength in $^{22}$Mg and its mirror $^{22}$Ne by Coulomb excitation, allowing for rigorous comparisons with theory. No-core symplectic shell-model calculations were performed and agree with the new $B(E2)$ values while in-medium similarity-renormalization-group calculations consistently underpredict the absolute strength, with the missing strength found to have both isoscalar and isovector components., 7 pages, 5 figures. To be submitted to Physics Letters B

Lifetimes of the first excited 2(+) and 4(+) states in the extremely neutron -deficient nuclide Pt-172 have been measured for the first time using the recoil-distance Doppler shift and recoil-decay tagging techniques. An unusually low value of the ratio B(E2: 4(1)(+) -> 2(1)(+)/B(E2: 2(1)(+) -> 0(gs)(+)) = 0.55(19) was found, similar to a handful of other such anomalous cases observed in the entire Segre chart. The observation adds to a cluster of a few extremely neutron -deficient nuclides of the heavy transition metals with neutron numbers N approximate to 90-94 featuring the effect. No theoretical model calculations reported to date have been able to explain the anomalously low B(E2: 4(1)(+) -> 2(1)(+)/B(E2: 2(1)(+) -> 0(gs)(+)) ratios observed in these cases. Such low values cannot, e.g., be explained within the framework of the geometrical collective model or by algebraic approaches within the interacting boson model framework. It is proposed that the group of B(E2: 4(1)(+) -> 2(1)(+)/B(E2: 2(1)(+) -> 0(gs)(+)) ratios in the extremely neutron-deficient even-even W, Os, and Pt nuclei around neutron numbers N approximate to 90-94 reveal a quantum phase transition from a seniority-conserving structure to a collective regime as a function of neutron number. Although a system governed by seniority symmetry is the only theoretical framework for which such an effect may naturally occur, the phenomenon is highly unexpected for these nuclei that are not situated near closed shells.

Background: The evolution of nuclear magic numbers at extremes of isospin is a topic at the forefront of contemporary nuclear physics. $N=50$ is a prime example, with increasing experimental data coming to light on potentially doubly magic $^{100}\mathrm{Sn}$ and $^{78}\mathrm{Ni}$ at the proton-rich and proton-deficient extremes, respectively; however, experimental discrepancies exist in the data for less exotic systems.Purpose: In $^{86}\mathrm{Kr}$ the $B(E2;{2}_{1}^{+}\ensuremath{\rightarrow}{0}_{1}^{+})$ value---a key indicator of shell evolution---has been experimentally determined by two different methodologies, with the results deviating by $3\ensuremath{\sigma}$. Here, we report on a new high-precision measurement of this value, as well as the first measured lifetimes and hence transition strengths for the ${2}_{2}^{+}$ and ${3}_{(2)}^{\ensuremath{-}}$ states in the nucleus.Methods: The Doppler-shift attenuation method was implemented using the TRIUMF-ISAC $\ensuremath{\gamma}$-ray escape-suppressed spectrometer (TIGRESS) $\ensuremath{\gamma}$-ray spectrometer and the TIGRESS integrated plunger device. High-statistics Monte Carlo simulations were utilized to extract lifetimes in accordance with state-of-the-art methodologies.Results: Lifetimes of $\ensuremath{\tau}({2}_{1}^{+})=336\ifmmode\pm\else\textpm\fi{}4\text{(stat.)}\ifmmode\pm\else\textpm\fi{}20\text{(sys.)}$ fs, $\ensuremath{\tau}({2}_{2}^{+})=263\ifmmode\pm\else\textpm\fi{}9\text{(stat.)}\ifmmode\pm\else\textpm\fi{}19\text{(sys.)}$ fs, and $\ensuremath{\tau}({3}_{(2)}^{\ensuremath{-}})=73\ifmmode\pm\else\textpm\fi{}6\text{(stat.)}\ifmmode\pm\else\textpm\fi{}32\text{(sys.)}$ fs were extracted. This yields a transition strength for the first-excited state of $B(E2;{2}_{1}^{+}\ensuremath{\rightarrow}{0}_{1}^{+})=259\ifmmode\pm\else\textpm\fi{}3\text{(stat.)}\ifmmode\pm\else\textpm\fi{}16\text{(sys.)}$ ${e}^{2}$ ${\mathrm{fm}}^{4}$.Conclusions: The measured lifetime disagrees with the previous Doppler-shift attenuation method measurement by more than $3\ensuremath{\sigma}$, while agreeing well with a previous value extracted from Coulomb excitation. The newly extracted $B(E2;{2}_{1}^{+}\ensuremath{\rightarrow}{0}_{1}^{+})$ value indicates a more significant reduction in the $N=50$ isotones approaching $Z=40$.

WOS: 000406755100001, Lifetimes of excited states in the yrast band of the neutron-deficient nuclide W-166 have been measured utilizing the DPUNS plunger device at the target position of the JUROGAM II gamma-ray spectrometer in conjunction with the RITU gas-filled separator and the GREAT focal-plane spectrometer. Excited states in W-166 were populated in the Mo-92(Kr-78, 4p) reaction at a bombarding energy of 380 MeV. The measurements reveal a low value for the ratio of reduced transitions probabilities for the lowest-lying transitions B(E2; 4(+)-> 2(+)) / B(E2; 2(+)-> 0(+)) = 0.33(5), compared with the expected ratio for an axially deformed rotor (B-4/2 = 1.43)., EURONS (European Commission)European Commission Joint Research Centre [RII3-CT-2004-506065]; Academy of Finland under the Finnish Centre of Excellence Programme (Nuclear and Accelerator Based Physics) [213503]; UK Science and Technology Facilities CouncilScience & Technology Facilities Council (STFC); Academy of FinlandAcademy of Finland [131665], This work has been supported through EURONS (European Commission Contract No. RII3-CT-2004-506065), the Academy of Finland under the Finnish Centre of Excellence Programme 2006-2011 (Nuclear and Accelerator Based Physics Contract No. 213503), and the UK Science and Technology Facilities Council. The UK/France (STFC/IN2P3) Loan Pool and GAMMAPOOL network are acknowledged for the EUROGAMdetectors of JUROGAMII. T.G. acknowledge the support of the Academy of Finland (Contract No. 131665).

Excited states in the proton-unbound nuclide $^{177}$Au were populated in the $^92}$Mo($^{88}$Sr, p2n) reaction and identified using the Jurogam-II and GREAT spectrometers in conjunction with the RITU gas-filled separator at the University of Jyvaskyla Accelerator Laboratory. A strongly coupled band and its decay path to the 11/2−α-decaying isomer have been identified using recoil-decay tagging. Comparisons with cranked Hartree-Fock-Bogoliubov (HFB) calculations based on Skyrme energy functionals suggest that the band has a prolate deformation and is based upon coupling the odd 1h11/2 proton hole to the excited 02+ configuration in the $^{178}$Hg core. Although these configurations might be expected to follow the parabolic trend of core Hg(02+) states as a function of neutron number, the electromagnetic decay paths from the strongly coupled band in $^{177}$Au are markedly different from those observed in the heavier isotopes above the midshell. This indicates that a significant change in the structure of the underlying A+1Hg core occurs below the neutron midshell.

Lifetimes of the first excited 2(+) states in the extremely neutron- deficient W-162 and W-164 nuclei have been measured using the recoil distance Doppler shift technique. Experimental B(E2) data f ...

Relatively neutron-rich thorium isotopes lie at the heart of a nuclear region of nuclei exhibiting octupole correlation effects. The detailed level structure of Th223 has been investigated in measurements of γ radiation following the fusion-evaporation channel of the Pb208(O18,3n)Th223 reaction at 85 MeV beam energy. The level structure has been extended up to spin 49/2, and 33 new γ rays have been added using triple-γ coincidence data. The spins and parities of the newly observed states have been confirmed by angular distribution ratios. In addition to the two known yrast bands based on a K=5/2 configuration, a non-yrast band has been established up to spin 35/2. We interpret this new structure as based on the same configuration as the yrast band in Th221 having dominant K=1/2 contribution. At the highest spin a backbending occurs around a rotational frequency of ℏω=0.23 MeV, very close to the one predicted in Th222, where a sharp transition to a reflection-symmetric shape is expected.

The new neutron-deficient nuclei 240 Es and 236 Bk were synthesised at the gas-filled recoil separator RITU. They were identified by their radioactive decay chains starting from 240 Es produced in the fusion–evaporation reaction 209 Bi( 34 S,3n) 240 Es. Half-lives of 6 ( 2 ) s and 22 − 6 + 13 s were obtained for 240 Es and 236 Bk, respectively. Two groups of α particles with energies E α = 8.19 ( 3 ) MeV and 8.09 ( 3 ) MeV were unambiguously assigned to 240 Es. Electron-capture delayed fission branches with probabilities of 0.16 ( 6 ) and 0.04 ( 2 ) were measured for 240 Es and 236 Bk, respectively. These new data show a continuation of the exponential increase of ECDF probabilities in more neutron-deficient isotopes.

The recoil-β tagging technique has been used in conjunction with the 40 Ca(32 S ,2n) reaction at a beam energy of 88 MeV to identify transitions associated with the decay of the 2 + and, tentatively, 4 + states in the nucleus 70 Kr. These data are used, along with previously published data, to examine the triplet energy differences (TED) for the mass 70 isobars. The experimental TED values are compared with shell model calculations, performed with the JUN45 interaction in the fpg model space, that include a J = 0 isospin nonconserving (INC) interaction with an isotensor strength of 100 keV. The agreement is found to be very good up to spin 4 and supports the expectation for analog states that all three nuclei have the same oblate shape at low-spin. The A = 70 results are compared with the experimental and shell model predicted TED and mirror energy differences (MED) for the mass 66 and 74 systems. The comparisons clearly demonstrate the importance of the isotensor INC interaction in replicating the TED data in this region. Issues related to the observed MED values and their interpretation within the shell model are discussed.

The lifetime of the $(11/{2}^{+})$ state in the band above the proton-emitting $(3/{2}^{+})$ state in $^{113}\mathrm{Cs}$ has been measured to be $\ensuremath{\tau}=24(6)$ ps from a recoil-decay-tagged differential-plunger experiment. The measured lifetime was used to deduce the deformation of the states using wave functions from a nonadiabatic quasiparticle model to independently calculate both proton-emission and electromagnetic $\ensuremath{\gamma}$-ray transition rates as a function of deformation. The only quadrupole deformation, which was able to reproduce the experimental excitation energies of the states, the electromagnetic decay rate of the $(11/{2}^{+})$ state and the proton-emission rate of the $(3/{2}^{+})$ state, was found to be ${\ensuremath{\beta}}_{2}=0.22(6)$. This deformation is in agreement with the earlier proton emission studies which concluded that $^{113}\mathrm{Cs}$ was best described as a deformed proton emitter, however, it is now more firmly supported by the present measurement of the electromagnetic transition rate.

The triple $\ensuremath{\alpha}$-decay chain $^{114}\mathrm{Ba}\ensuremath{\rightarrow}^{110}\mathrm{Xe}\ensuremath{\rightarrow}^{106}\mathrm{Te}\ensuremath{\rightarrow}^{102}\mathrm{Sn}$ has been directly observed for the first time, following the $^{58}\mathrm{Ni}(^{58}\mathrm{Ni},2n)$ reaction. Implantation of $^{114}\mathrm{Ba}$ nuclei into a double-sided silicon-strip detector has allowed their $\ensuremath{\alpha}$ decays to be correlated in position and time with the $\ensuremath{\alpha}$ decays of the daughter $(^{110}\mathrm{Xe})$ and granddaughter $(^{106}\mathrm{Te})$ nuclei. In total, 17 events have been assigned to the $^{114}\mathrm{Ba}\ensuremath{\rightarrow}^{110}\mathrm{Xe}\ensuremath{\rightarrow}^{106}\mathrm{Te}\ensuremath{\rightarrow}^{102}\mathrm{Sn}$ triple $\ensuremath{\alpha}$-decay chain. The energy of the $^{114}\mathrm{Ba} \ensuremath{\alpha}$ decay has been measured to be ${E}_{\ensuremath{\alpha}}=3480$(20) keV, which is 70 keV higher than the previously measured value, and the half-life of $^{114}\mathrm{Ba}$ has been measured with improved accuracy, to be ${380}_{\ensuremath{-}110}^{+190}$ ms. A revised ${Q}_{^{12}\mathrm{C}}$ value of 19 035(45) keV for $^{114}\mathrm{Ba}$ is presented.

Excited states in the neutron-deficient odd-odd proton-unbound nuclide $^{158}\mathrm{Ta}$ have been investigated in two separate experiments. In the first experiment, $^{166}\mathrm{Ir}$ nuclei were produced in the reactions of 380 MeV $^{78}\mathrm{Kr}$ ions with an isotopically enriched $^{92}\mathrm{Mo}$ target. The $\ensuremath{\alpha}$-decay chain of the ${9}^{+}$ state in $^{166}\mathrm{Ir}$ was analyzed. Fine structure in the $\ensuremath{\alpha}$ decay of the ${9}^{+}$ state in $^{162}\mathrm{Re}$ established a 66 keV difference in excitation energy between the lowest-lying ${9}^{+}$ and ${10}^{+}$ states in $^{158}\mathrm{Ta}$. Higher-lying states in $^{158}\mathrm{Ta}$ were populated in the reactions of 255 MeV $^{58}\mathrm{Ni}$ ions with an isotopically enriched $^{102}\mathrm{Pd}$ target. Gamma-ray decay paths that populate, depopulate, and bypass a ${19}^{\ensuremath{-}}$ isomeric state have been identified. The general features of the deduced level scheme are discussed and the prospects for observing proton emission branches from excited states are considered.

Excited states in the neutron-deficient nuclides(74)(162)W(88) and W-164(74)90 were investigated by using the gamma-ray spectrometer Jurogam. A change in structure is apparent from the first rotational alignments in W-162 and W-164, whose rotationally aligned bands are interpreted as nu(h(9/2))(2) and nu(i(13/2))(2) configurations, respectively. The level schemes have been extended using recoil (-decay) correlations with the observation of excited collective structures. Configuration assignments have been made on the basis of comparisons of the deduced aligned angular momentum, as a function of rotational frequency, with the predictions of the cranked shell model.

WOS: 000371740600004, Lifetimes of excited states in the neutron-deficient odd-odd nucleus Re-166 have been measured for the first time using the recoil distance Doppler-shift method. The measured lifetime for the (8(-)) state; tau = 480 (80) ps, enabled an assessment of the multipolarities of the gamma rays depopulating this state. Information on electromagnetic transition strengths were deduced for the gamma-ray transitions from the (9(-)), (10(-)), and (11(-)) states, and in the case of the (10(-)) and (11(-)) states limits on the B (M1) and B(E2) strengths were estimated. The results are compared with total Routhian surface predictions and semiclassical calculations. Tilted-axis cranking calculations based on a relativistic mean-field approach (TAC-RMF) have also been performed in order to test the possibility of magnetic rotation in the 166Re nucleus. While the TAC-RMF calculations predict a quadrupole-deformed nuclear shape with similar beta(2) deformation as obtained by using the TRS model, it was found that the experimental electromagnetic transition rates are in better agreement with a collective -rotational description., Swedish Research CouncilSwedish Research Council [621-2010-3694]; Academy of Finland under the Finnish Centre of Excellence ProgrammeAcademy of Finland; UK Science and Technology Facilities CouncilScience & Technology Facilities Council (STFC); European UnionEuropean Union (EU) [262010]; China Scholarship CouncilChina Scholarship Council [201306210205]; Academy of FinlandAcademy of Finland [131665]; Science and Technology Facilities CouncilScience & Technology Facilities Council (STFC) [ST/L005670/1, EP/E004385/1, ST/L005689/1, ST/G008671/1, ST/J000094/1, EP/C015266/1], The authors would like to thank the staff at the Accelerator Laboratory of the University of Jyvaskyla for their excellent technical support. This work was supported by the Swedish Research Council (Project No. 621-2010-3694), the Academy of Finland under the Finnish Centre of Excellence Programme 2012 - 2017, the UK Science and Technology Facilities Council, and the European Union Seventh Framework Programme Integrating Activities-Transnational Access, Project No. 262010 (ENSAR). Li is supported in part by the China Scholarship Council under Grant No. 201306210205. Additionally, we thank the GAMMAPOOL European Spectroscopy Resource for the loan of the detectors for JUROGAM II array. T.G. acknowledges the support from the Academy of Finland (Contract No. 131665).

The β-decay half lives of nuclei near the r-process path are critical information required for abundance calculations, especially those near neutron number N = 82. Specifically, the nuclei below doubly-magic 132Sn are key, and play an important role in the formation and shape of the second r-process abundance peak. The half lives in this region are challenging to measure due to the significant β-delayed neutron decay branches and the population of isomeric states with half lives comparable to the ground states. However, by measuring the time distribution of γ rays, these complications can be eliminated. This requires, however, a very effcient γ-ray spectrometer since the production of isotopes in this region is very limited. The new GRIFFIN array at TRIUMF-ISAC provides the high effciency required for these measurements. Recent improvements in the quality of the beams produced at TRIUMF, employing the IG-LIS device, are outlined, as well as the current status of the ARIEL facility. The GRIFFIN spectrometer and its use are briefly described. The experiment to measure the half lives of 128-130Cd is outlined and the results given, and some examples of the power of GRIFFIN to expand decay schemes, specifically for the decay of 128Cd to 128In, are given.