Search

The calcium isotopes are an ideal system to investigate the evolution of shell structure and magic numbers. Although the properties of surface nucleons in calcium have been well studied, probing the structure of deeply bound nucleons remains a challenge. Here, we report on the first measurement of unbound states in $^{53}$Ca and $^{55}$Ca, populated from \ts{54,56}Ca($p,pn$) reactions at a beam energy of around 216 MeV/nucleon at the RIKEN Radioactive Isotopes Beam Factory. The resonance properties, partial cross sections, and momentum distributions of these unbound states were analyzed. Orbital angular momentum $l$ assignments were extracted from momentum distributions based on calculations using the distorted wave impulse approximation (DWIA) reaction model. The resonances at excitation energies of 5516(41)\,keV in $^{53}$Ca and 6000(250)\,keV in $^{55}$Ca indicate a significant $l$\, =\,3 component, providing the first experimental evidence for the $\nu 0f_{7/2}$ single-particle strength of unbound hole states in the neutron-rich Ca isotopes. The observed excitation energies and cross-sections point towards extremely localized and well separated strength distributions, with some fragmentation for the $\nu 0f_{7/2}$ orbital in $^{55}$Ca. These results are in good agreement with predictions from shell-model calculations using the effective GXPF1Bs interaction and \textit{ab initio} calculations and diverge markedly from the experimental distributions in the nickel isotones at $Z=28$., Comment: 13 pages, 7 figures

The cluster structure of the neutron-rich isotope $^{10}$Be has been probed via the $(p,p\alpha)$ reaction at 150 MeV/nucleon in inverse kinematics and in quasifree conditions. The populated states of $^{6}$He residues were investigated through missing mass spectroscopy. The triple differential cross-section for the ground-state transition was extracted for quasifree angle pairs ($\theta_{p}$, $\theta_{\alpha}$) and compared to distorted-wave impulse approximation reaction calculations performed in a microscopic framework using successively the Tohsaki-Horiuchi-Schuck-R\"opke product wave-function and the wave-function deduced from Antisymmetrized Molecular Dynamics calculations. The remarkable agreement between calculated and measured cross-sections in both shape and magnitude validates the molecular structure description of the $^{10}$Be ground-state, configured as an $\alpha$-$\alpha$ core with two valence neutrons occupying $\pi$-type molecular orbitals., Comment: 7 pages, 3 figures, 1 tables

Gamma decays were observed in $^{56}$Ca and $^{58}$Ca following quasi-free one-proton knockout reactions from $^{57,59}$Sc beams at $\approx 200$ MeV/nucleon. For $^{56}$Ca, a $\gamma$ ray transition was measured to be 1456(12) keV, while for $^{58}$Ca an indication for a transition was observed at 1115(34) keV. Both transitions were tentatively assigned as the $2^+_1 \rightarrow 0^+_{gs}$ decays, and were compared to results from ab initio and conventional shell-model approaches. A shell-model calculation in a wide model space with a marginally modified effective nucleon-nucleon interaction depicts excellent agreement with experiment for $2^+_1$ level energies, two-neutron separation energies, and reaction cross sections, corroborating the formation of a new nuclear shell above the $N$ = 34 shell. Its constituents, the $0f_{5/2}$ and $0g_{9/2}$ orbitals, are almost degenerate. This degeneracy precludes the possibility for a doubly magic $^{60}$Ca and potentially drives the dripline of Ca isotopes to $^{70}$Ca or even beyond., Comment: 8 pages, 3 figures

Detailed $\gamma$-ray spectroscopy of the exotic neon isotope $^{28}$Ne has been performed for the first time using the one-neutron removal reaction from $^{29}$Ne on a liquid hydrogen target at 240~MeV/nucleon. Based on an analysis of parallel momentum distributions, a level scheme with spin-parity assignments has been constructed for $^{28}$Ne and the negative-parity states are identified for the first time. The measured partial cross sections and momentum distributions reveal a significant intruder $p$-wave strength providing evidence of the breakdown of the $N=20$ and $N=28$ shell gaps. Only a weak, possible $f$-wave strength was observed to bound final states. Large-scale shell-model calculations with different effective interactions do not reproduce the large $p$-wave and small $f$-wave strength observed experimentally, indicating an ongoing challenge for a complete theoretical description of the transition into the island of inversion along the Ne isotopic chain.

We report on the first proton-induced single proton- and neutron-removal reactions from the neutron-deficient $^{14}$O nucleus with large Fermi-surface asymmetry $S_n-S_p$ = 18.6 MeV at $\sim$100 MeV/nucleon, a widely used energy regime for rare-isotope studies. The measured inclusive cross sections and parallel momentum distributions of the $^{13}$N and $^{13}$O residues are compared to the state-of-the-art reaction models, with nuclear structure inputs from many-body shell-model calculations. Our results provide the first quantitative contributions of multiple reaction mechanisms including the quasifree knockout, inelastic scattering and nucleon transfer processes. It is shown that the inelastic scattering and nucleon transfer, usually neglected at such energy regime, contribute about 50% and 30% to the loosely bound proton and deeply bound neutron removal, respectively. These multiple reaction mechanisms should be considered in analyses of inclusive one-nucleon removal cross sections measured at intermediate energies for quantitative investigation of single-particle strengths and correlations in atomic nuclei.

We demonstrate the modulation of spin Seebeck effect (SSE) by hydrogenation in Pd/YIG bilayers. In the presence of 3% hydrogen gas, SSE voltage decreases by more than 50% from the magnitude observed in pure Ar gas. The modulation of the SSE voltage is reversible, but the recovery of the SSE voltage to the prehydrogenation value takes a few days because of a long time constant of hydrogen desorption. We also demonstrate that the spin Hall magnetoresistance of the identical sample reduces significantly with hydrogen exposure, supporting that the observed modulation of spin current signals originates from hydrogenation of Pd/YIG.

States in the $N=35$ and 37 isotopes $^{55,57}$Ca have been populated by direct proton-induced nucleon removal reactions from $^{56,58}$Sc and $^{56}$Ca beams at the RIBF. In addition, the $(p,2p)$ quasi-free single-proton removal reaction from $^{56}$Ca was studied. Excited states in $^{55}$K, $^{55}$Ca, and $^{57}$Ca were established for the first time via in-beam $\gamma$-ray spectroscopy. Results for the proton and neutron removal reactions from $^{56}$Ca to states in $^{55}$K and $^{55}$Ca for the level energies, excited state lifetimes, and exclusive cross sections agree well with state-of-the-art theoretical calculations using different approaches. The observation of a short-lived state in $^{57}$Ca suggests a transition in the calcium isotopic chain from single-particle dominated states at $N=35$ to collective excitations at $N=37$., Comment: accepted Phys. Lett. B

Atomic nuclei are composite systems, and they may be dynamically excited during nuclear reactions. Such excitations are not only relevant to inelastic scattering but they also affect other reaction processes such as elastic scattering and fusion. The coupled-channels approach is a framework which can describe these reaction processes in a unified manner. It expands the total wave function of the system in terms of the ground and excited states of the colliding nuclei, and solves the coupled Shr\"odinger equations to obtain the $S$-matrix, from which several cross sections can be constructed. This approach has been a standard tool to analyze experimental data for nuclear reactions. In this paper, we review the present status and the recent developments of the coupled-channels approach. This includes the microscopic coupled-channels method and its application to cluster physics, the continuum discretized coupled-channels (CDCC) method for breakup reactions, the semi-microscopic approach to heavy-ion subbarrier fusion reactions, the channel coupling effects on nuclear astrophysics and syntheses of superheavy elements, and inclusive breakup and incomplete fusion reactions of weakly-bound nuclei., Comment: 90 pages, 37 figures. Accepted for publication in Progress in Particle and Nuclear Physics

A first gamma-ray study of 47,49Cl spectroscopy was performed at the Radioactive Isotope Beam Factory with 50Ar projectiles at 217 MeV/nucleon, impinging on the liquid hydrogen target of the MINOS device. Prompt de-excitation gamma-rays were measured with the NaI(Tl) array DALI2+. Through the one-proton knockout reaction 50Ar(p,2p), a spin assignment could be determined for the low-lying states of 49Cl from the momentum distribution obtained with the SAMURAI spectrometer. A spin-parity J = 3/2+ is deduced for the ground state of 49Cl, similar to the recently studied N = 32 isotope 51K.

Both ($e$,$e'p$) and ($p$,$2p$) reactions have been performed to study the proton single-particle character of nuclear states with its related spectroscopic factor. Recently, the dispersive optical model (DOM) was applied to the ($e$,$e'p$) analysis revealing that the traditional treatment of the single-particle overlap function, distorted waves, and nonlocality must be further improved to achieve quantitative nuclear spectroscopy. We apply the DOM wave functions to the traditional ($p$,$2p$) analysis and investigate the consistency of the DOM spectroscopic factor that describes the ($e$,$e'p$) cross section with the result of the ($p$,$2p$) analysis. Additionally, we make a comparison with a phenomenological single-particle wave function and optical potential. Uncertainty arising from a choice of $p$-$p$ interaction is also investigated. We implement the DOM wave functions to the distorted wave impulse approximation (DWIA) framework for ($p$,$2p$) reactions. DOM + DWIA analysis on $^{40}$Ca($p$,$2p$)$^{39}$K data generates a proton $0d_{3/2}$ spectroscopic factor of 0.560, which is meaningfully smaller than the DOM value of 0.71 shown to be consistent with the ($e$,$e'p$) analysis. Uncertainties arising from choices of single-particle wave function, optical potential, and $p$-$p$ interaction do not explain this inconsistency. The inconsistency in the spectroscopic factor suggests there is urgent need for improving the description of $p$-$p$ scattering in a nucleus and the resulting in-medium interaction with corresponding implications for the analysis of this reaction in inverse kinematics.

The momentum correlation functions of S = -2 baryon pairs (p Xi^- and Lambda Lambda) produced in high-energy pp and pA collisions are investigated on the basis of the coupled-channel formalism. The strong interaction is described by the coupled-channel HAL QCD potential obtained by the lattice QCD simulations near physical quark masses, while the hadronic source function is taken to be a static Gaussian form. The coupled-channel effect, the threshold difference, the realistic strong interaction, and the Coulomb interaction are fully taken into account for the first time in the femtoscopic analysis of baryon-baryon correlations. The characteristic features of the experimental data for the p Xi^- and Lambda Lambda pairs at LHC are reproduced quantitatively with a suitable choice of non-femtoscopic parameters and the source size. The agreement between theory and experiment indicates that the N Xi (Lambda Lambda) interaction is moderately (weakly) attractive without having a quasi-bound (bound) state., Comment: 13 pages, 10 figures

A kinematically complete quasi-free $(p,pn)$ experiment in inverse kinematics was performed to study the structure of the Borromean nucleus $^{17}$B, which had long been considered to have neutron halo. By analyzing the momentum distributions and exclusive cross sections, we obtained the spectroscopic factors for $1s_{1/2}$ and $0d_{5/2}$ orbitals, and a surprisingly small percentage of 9(2)$\%$ was determined for $1s_{1/2}$. Our finding of such a small $1s_{1/2}$ component and the halo features reported in prior experiments can be explained by the deformed relativistic Hartree-Bogoliubov theory in continuum, revealing a definite but not dominant neutron halo in $^{17}$B. The present work gives the smallest $s$- or $p$-orbital component among known nuclei exhibiting halo features, and implies that the dominant occupation of $s$ or $p$ orbitals is not a prerequisite for the occurrence of neutron halo., Comment: Accepted for publication in Physical Review Letters,8 pages, 4 figures

In this review article we discuss the present status of direct nuclear reactions and the nuclear structure aspects one can study with them. We discuss the spectroscopic information we can assess in experiments involving transfer reactions, heavy-ion-induced knockout reactions and quasifree scattering with (p,2p), (p,pn), and (e,e'p) reactions. In particular, we focus on the proton-to-neutron asymmetry of the quenching of the spectroscopic strength., Comment: 138 pages, 63 figures

Low-lying excited states in the $N=32$ isotope $^{50}$Ar were investigated by in-beam $\gamma$-ray spectroscopy following proton- and neutron-knockout, multi-nucleon removal, and proton inelastic scattering at the RIKEN Radioactive Isotope Beam Factory. The energies of the two previously reported transitions have been confirmed, and five additional states are presented for the first time, including a candidate for a 3$^-$ state. The level scheme built using $\gamma\gamma$ coincidences was compared to shell-model calculations in the $sd-pf$ model space, and to ab initio predictions based on chiral two- and three-nucleon interactions. Theoretical proton- and neutron-knockout cross sections suggest that two of the new transitions correspond to $2^+$ states, while the previously proposed $4^+$ state could also correspond to a $2^+$ state., Comment: Accepted for Phys. Rev. C

The formation of a dineutron in the nucleus $^{11}$Li is found to be localized to the surface region. The experiment measured the intrinsic momentum of the struck neutron in $^{11}$Li via the $(p,pn)$ knockout reaction at 246 MeV/nucleon. The correlation angle between the two neutrons is, for the first time, measured as a function of the intrinsic neutron momentum. A comparison with reaction calculations reveals the localization of the dineutron at $r\sim3.6$ fm. The results also support the density dependence of dineutron formation as deduced from Hartree-Fock-Bogoliubov calculations for nuclear matter., Comment: 19 pages, 4 figures. Accepted for Physical Review Letters

Excited states in the $N=40$ isotone $^{62}$Ti were populated via the $^{63}$V$(p,2p)$$^{62}$Ti reaction at $\sim$200~MeV/u at the Radioactive Isotope Beam Factory and studied using $\gamma$-ray spectroscopy. The energies of the $2^+_1 \rightarrow 0^{+}_{\mathrm{gs}}$ and $4^+_1 \rightarrow 2^+_1$ transitions, observed here for the first time, indicate a deformed $^{62}$Ti ground state. These energies are increased compared to the neighboring $^{64}$Cr and $^{66}$Fe isotones, suggesting a small decrease of quadrupole collectivity. The present measurement is well reproduced by large-scale shell-model calculations based on effective interactions, while ab initio and beyond mean-field calculations do not yet reproduce our findings. The shell-model calculations for $^{62}$Ti show a dominant configuration with four neutrons excited across the $N=40$ gap. Likewise, they indicate that the $N=40$ island of inversion extends down to $Z=20$, disfavoring a possible doubly magic character of the elusive $^{60}$Ca.

Nuclear magic numbers, which emerge from the strong nuclear force based on quantum chromodynamics, correspond to fully occupied energy shells of protons, or neutrons inside atomic nuclei. Doubly magic nuclei, with magic numbers for both protons and neutrons, are spherical and extremely rare across the nuclear landscape. While the sequence of magic numbers is well established for stable nuclei, evidence reveals modifications for nuclei with a large proton-to-neutron asymmetry. Here, we provide the first spectroscopic study of the doubly magic nucleus $^{78}$Ni, fourteen neutrons beyond the last stable nickel isotope. We provide direct evidence for its doubly magic nature, which is also predicted by ab initio calculations based on chiral effective field theory interactions and the quasi-particle random-phase approximation. However, our results also provide the first indication of the breakdown of the neutron magic number 50 and proton magic number 28 beyond this stronghold, caused by a competing deformed structure. State-of-the-art phenomenological shell-model calculations reproduce this shape coexistence, predicting further a rapid transition from spherical to deformed ground states with $^{78}$Ni as turning point.

The neutron-shell structure of $^{25}$F was studied using quasi-free (p,2p) knockout reaction at 270A MeV in inverse kinematics. The sum of spectroscopic factors of $\pi$0d$_{5/2}$ orbital is found to be $1.0 \pm 0.3$. However, the spectroscopic factor for the ground-state to ground-state transition ($^{25}$F, $^{24}$O$_{g.s.}$) is only $0.36\pm 0.13$, and $^{24}$O excited states are produced from the 0d$_{5/2}$ proton knockout. The result shows that the $^{24}$O core of $^{25}$F nucleus significantly differs from a free $^{24}$O nucleus, and the core consists of 35% $^{24}$O$_{g.s}$. and 65% excited $^{24}$O., Comment: 5 pages, 5 figures

Despite recent significant developments of Si composites, use of silicon with significance in the anodes for Li-ion batteries is still limited. In fact, nominal energy density is to be saturated around ~750 Wh/L regardless of cell-types under the current material strategies. Use of Si-rich anode can push the limit; however, the prolonged irreversible Li consumption becomes more prominent. We previously showed that repeating c-Li3.75(+{\delta})Si formation/decomposition, typically recognized to degrade the anodes, can improve the irreversibility and accumulatively minimize the gross consumption. Utilizing the insights combined with prelithiation techniques, here we provide prototypic cell designs that can nonlinearly deplete the consumption., Comment: 10 pages, 3 figures

Controlled formation of porous silicon has been of primary importance for numerous landmark applications such as light emitting sources, sensors, actuators, drug delivery systems, and energy storage applications. Frequently explored methods to form the structures have long relied on selective etching of silicon, which still stands as the most controllable and reliable methods to highlight essence of the applications. Here, we demonstrate an unprecedented approach to form silicon framework, which is spontaneously formed with atomistic arrangement of silicon without gravimetric loss via single electrochemical (de)alloying with lithium. Carefully controlling bare crystallinity of Si and composite/electrode designs, we reveal that the key prerequisite to forming the structure lies in using unique dealloying dynamics of crystalline-amorphous phase transformations at room temperature. Using the feature, we clearly highlight that commercially available nano-structured silicon particles can abruptly yet uniformly transform into continuous sub-2 nm spherical silicon frameworks with size-tunable pores., Comment: Main body 24 pages (4 figures), Supplementary Information 14 pages (10 supplementary figures)

[Background] Proton-induced knockout reactions of the form $(p,pN)$ have experienced a renewed interest in recent years due to the possibility of performing these measurements with rare isotopes, using inverse kinematics. Several theoretical models are being used for the interpretation of these new data, such as the distorted-wave impulse approximation (DWIA), the transition amplitude formulation of the Faddeev equations due to Alt, Grassberger and Sandhas (FAGS) and, more recently, a coupled-channels method here referred to as transfer-to-the-continuum (TC). [Purpose] Our goal is to compare the momentum distributions calculated with the DWIA and TC models for the same reactions, using whenever possible the same inputs (e.g. distorting potential). A comparison with already published results for the FAGS formalism is performed as well. [Method] We choose the $^{15}$C($p$,$pn$)$^{14}$C reaction at an incident energy of 420 MeV/u, which has been previously studied with the FAGS formalism. The knocked-out neutron is assumed to be in a $2s$ single-particle orbital. Longitudinal and transverse momentum distributions are calculated for different assumed separation energies. [Results] For all cases considered, we find a very good agreement between DWIA and TC results. The energy dependence of the distorting optical potentials is found to affect in a modest way the shape and magnitude of the momentum distributions. Moreover, when relativistic kinematics corrections are omitted, our calculations reproduce remarkably well the FAGS result. [Conclusions] The results found in this work provide confidence on the consistency and accuracy of the DWIA and TC models for analyzing momentum distributions for $(p,pn)$ reactions at intermediate energies., Comment: 6 pages, 4 figures

Background: Deuteron-induced one-neutron transfer reactions have been used to extract single-particle properties of nuclei, and the adiabatic (AD) approximation is often used to simply treat the deuteron breakup states. Purpose: The primary goal is to examine the validity of the AD approximation for the ($d,p$) reaction systematically. We clarify also the role of the closed-channels often ignored in the description of breakup reactions. Methods: We calculate the ($d,p$) cross sections with the continuum-discretized coupled-channels method (CDCC) for 128 reactions systems and compare the results with those obtained by the CDCC calculation with the AD approximation. Effect of the closed channels are investigated by ignoring the closed channels in CDCC. Results: The AD approximation affects in general the ($d,p$) cross section by less than 20 %, but some exceptional nonadiabatic cases for which the AD approximation breaks down are found. The closed channels turn out to give significant effects on the cross section at deuteron energies less than about 10 MeV. Conclusions: The use of the AD approximation in the description of the ($d,p$) reaction can be justified in many cases, with the uncertainty of less than about 20 %. The existence of some nonadiabatic cases nevertheless should be realized. The neglect of the closed channels without confirming the convergence of the CDCC result is not recommended., Comment: 9 pages, 9 figures, 3 tables

The study of exotic nuclear structures, such as halo nuclei, is usually performed through nuclear reactions. An accurate reaction model coupled to a realistic description of the projectile is needed to correctly interpret experimental data. In this contribution, we briefly summarise the assumptions made within the modelling of reactions involving halo nuclei. We describe briefly the Continuum-Discretised Coupled Channel method (CDCC) and the Dynamical Eikonal Approximation (DEA) in particular and present a comparison between them for the breakup of 15C on Pb at 68AMeV. We show the problem faced by the models based on the eikonal approximation at low energy and detail a correction that enables their extension down to lower beam energies. A new reaction observable is also presented. It consists of the ratio between angular distributions for two different processes, such as elastic scattering and breakup. This ratio is completely independent of the reaction mechanism and hence is more sensitive to the projectile structure than usual reaction observables, which makes it a very powerful tool to study exotic structures far from stability., Comment: Contribution to the proceedings of the XXI International School on Nuclear Physics and Applications & the International Symposium on Exotic Nuclei, dedicated to the 60th Anniversary of the JINR (Dubna) (Varna, Bulgaria, 6-12 September 2015), 7 pages, 4 figures