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The manipulation and transformation of quantum resources are key parts of quantum mechanics. Among them, asymmetry is one of the most useful operational resources, which is widely used in quantum clocks, quantum metrology, and other tasks. Recent studies have shown that the asymmetry of quantum states can be significantly amplified with the assistance of correlating catalysts which are finite-dimensional auxiliaries. In the experiment, we perform translationally invariant operations, ensuring that the asymmetric resources of the entire system remain non-increasing, on a composite system composed of a catalytic system and a quantum system. The experimental results demonstrate an asymmetry amplification of 0.0172\pm0.0022 in the system following the catalytic process. Our work showcases the potential of quantum catalytic processes and is expected to inspire further research in the field of quantum resource theories., Comment: 17pages,7figures

Device-independent randomness certification based on Bell nonlocality does not require any assumptions about the devices and therefore provides adequate security. Great effort has been made to demonstrate that nonlocality is necessary for generating quantum randomness, but the minimal resource required for random number generation has not been clarified. Here we first prove and experimentally demonstrate that violating any two-input Bell inequality is both necessary and sufficient for certifying randomness, however, for the multi-input cases, this sufficiency ceases to apply, leading to certain states exhibiting Bell nonlocality without the capability to certify randomness. We examine two typical classes of Bell inequalities with multi-input and multi-output, the facet inequalities and Salavrakos-Augusiak-Tura-Wittek-Ac\'in-Pironio Bell inequalities, in the high-dimensional photonic system, and observe the violation of the latter one can always certify randomness which is not true for the former. The private randomness with a generation rate of 1.867\pm0.018 bits per photon pair is obtained in the scenario of Salavrakos-Augusiak-Tura-Wittek-Ac\'in-Pironio Bell inequalities with 3-input and 4-output. Our work unravels the internal connection between randomness and nonlocality, and effectively enhances the performance of tasks such as device-independent random number generation., Comment: 25 pages, 6 figures

The release of causal structure of physical events from a well-defined order to an indefinite one stimulates remarkable enhancements in various quantum information tasks. Some of these advantages, however, are questioned for the ambiguous role of the control system in the quantum switch that is an experimentally realized process with indefinite causal structure. In communications, for example, not only the superposition of alternative causal orders, but also the superposition of alternative trajectories can accelerate information transmissions. Here, we follow the proposal of Liu et al. [Phys. Rev. Lett. 129, 230604 (2022)], and examine the information enhancement effect of indefinite causal orders with the toolkit of thermodynamics in a photonic platform. Specifically, we simulate the thermal interaction between a system qubit and two heat baths embedded in a quantum switch by implementing the corresponding switched thermal channels. Although its action on the system qubit only is thermally free, our results suggest that the quantum switch should be seen as a resource when the control qubit is also considered. Moreover, we characterize the non-Markovian property in this scenario by measuring the information backflows from the heat baths to the system qubit.

In the past decade, the toolkit of quantum information has been expanded to include processes in which the basic operations do not have definite causal relations. Originally considered in the context of the unification of quantum mechanics and general relativity, these causally indefinite processes have been shown to offer advantages in a wide variety of quantum information processing tasks, ranging from quantum computation to quantum metrology. Here we overview these advantages and the experimental efforts to realise them. We survey both the different experimental techniques employed, as well as theoretical methods developed in support of the experiments, before discussing the interpretations of current experimental results and giving an outlook on the future of the field., Comment: 22 page review article. Comments welcome!

In the last decade, it was understood that quantum networks involving several independent sources of entanglement which are distributed and measured by several parties allowed for completely novel forms of nonclassical quantum correlations, when entangled measurements are performed. Here, we experimentally obtain quantum correlations in a triangle network structure, and provide solid evidence of its nonlocality. Specifically, we first obtain the elegant distribution proposed in (Entropy 21, 325) by performing a six-photon experiment. Then, we justify its nonlocality based on machine learning tools to estimate the distance of the experimentally obtained correlation to the local set, and through the violation of a family of conjectured inequalities tailored for the triangle network.

Quantum steering ellipsoid visualizes the set of all qubit states that can be steered by measuring on another correlated qubit in the Bloch picture. Together with local reduced states, it provides a faithful geometric characterization of the underlying two-qubit state so that almost all nonclassical state features can be reflected in its geometric properties. Consequently, the various types of quantum ellipsoids with different geometric properties form an ellipsoid zoo, which, in this work, is experimentally verified via measurements on many polarization-path photonic states. By generating two-qubit states with high fidelity, the corresponding ellipsoids are constructed to certify the presence of entanglement, one-way Einstein-Podolsky-Rosen steering, discord, and steering incompleteness. It is also experimentally verified that the steering ellipsoid can be reconstructed from using the twelve vertices of the icosahedron as measurement directions. Our results aid progress in applying the quantum steering ellipsoid to reveal nonclassical features of the multi-qubit system., Comment: Several references are added and the presentation is close to the publication version

Symmetric informationally complete measurements are both important building blocks in many quantum information protocols and the seminal example of a generalised, non-orthogonal, quantum measurement. In higher-dimensional systems, these measurements become both increasingly interesting and increasingly complex to implement. Here, we demonstrate an integrated quantum photonic platform to realize such a measurement on three-level quantum systems. The device operates at the high fidelities necessary for verifying a genuine many-outcome quantum measurement, performing near-optimal quantum state discrimination, and beating the projective limit in quantum random number generation. Moreover, it is programmable and can readily implement other quantum measurements at similarly high quality. Our work paves the way for the implementation of sophisticated higher-dimensional quantum measurements that go beyond the traditional orthogonal projections., Comment: 21 pages,13 figures

Distributed quantum computing provides a viable approach towards scalable quantum computation, which relies on nonlocal quantum gates to connect distant quantum nodes, to overcome the limitation of a single device. However, such an approach has only been realized within single nodes or between nodes separated by a few tens of meters, preventing the target of harnessing computing resources in large-scale quantum networks. Here, we demonstrate distributed quantum computing between two nodes spatially separated by 7.0 km, using stationary qubits based on multiplexed quantum memories, flying qubits at telecom wavelengths, and active feedforward control based on field-deployed fiber. Specifically, we illustrate quantum parallelism by implementing Deutsch-Jozsa algorithm and quantum phase estimation algorithm between the two remote nodes. These results represent the first demonstration of distributed quantum computing over metropolitan-scale distances and lay the foundation for the construction of large-scale quantum computing networks relying on existing fiber channels., Comment: 6 pages, 3 figures

In recent years, analysis methods for quantum states based on randomized measurements have been investigated extensively. Still, in the experimental implementations these methods were typically used for characterizing strongly entangled states and not to analyze the different families of multiparticle or weakly entangled states. In this work, we experimentally prepare various entangled states with path-polarization hyper-entangled photon pairs, and study their entanglement properties using the full toolbox of randomized measurements. First, we successfully characterize the correlations of a series of GHZ-W mixed states using the second moments of the random outcomes, and demonstrate the advantages of this method by comparing it with the well-known three-tangle and squared concurrence. Second, we generate bound entangled chessboard states of two three-dimensional systems and verify their weak entanglement with a criterion derived from moments of randomized measurements., Comment: 10 pages, 6 figures, Comments are welcome

Shared entanglement can significantly amplify classical correlations between systems interacting over a limited quantum channel. A natural avenue is to use entanglement of the same dimension as the channel because this allows for unitary encodings, which preserve global coherence until a measurement is performed. Contrasting this, we here demonstrate a distributed task based on a qubit channel, for which irreversible encoding operations can outperform any possible coherence-preserving protocol. This corresponds to using high-dimensional entanglement and encoding information by compressing one of the subsystems into a qubit. Demonstrating this phenomenon requires the preparation of a four-dimensional maximally entangled state, the compression of two qubits into one and joint qubit-ququart entangled measurements, with all modules executed at near-optimal fidelity. We report on a proof-of-principle experiment that achieves the advantage by realizing separate systems in distinct and independently controlled paths of a single photon. Our result demonstrates the relevance of high-dimensional entanglement and non-unitary operations for enhancing the communication capabilities of standard qubit transmissions., Comment: 7 pages, 5 figures + appendix. Comments are welcome. V2: expanded and reformatted theory section, added experimental details

Multipartite high-dimensional entanglement presents different physics from multipartite two-dimensional entanglement. However, how to prepare multipartite high-dimensional entanglement is still a challenge with linear optics. In this paper, a multiphoton GHZ state with arbitrary dimensions preparation protocol is proposed in optical systems. In this protocol, we use auxiliary entanglements to realize a high-dimensional entanglement gate, so that high-dimensional entangled pairs can be connected into a multipartite high-dimensional GHZ state. Specifically, we give an example of using photons' path degree of freedom to prepare a 4-particle 3-dimensional GHZ state. Our method can be extended to other degrees of freedom and can generate arbitrary GHZ entanglement in any dimension., Comment: 10 pages, 3 figures

The precision of quantum metrology is widely believed to be restricted by the Heisenberg limit, corresponding to a root mean square error that is inversely proportional to the number of independent processes probed in an experiment, N. In the past, some proposals have challenged this belief, for example using non-linear interactions among the probes. However, these proposals turned out to still obey the Heisenberg limit with respect to other relevant resources, such as the total energy of the probes. Here, we present a photonic implementation of a quantum metrology protocol surpassing the Heisenberg limit by probing two groups of independent processes in a superposition of two alternative causal orders. Each process creates a phase space displacement, and our setup is able to estimate a geometric phase associated to two sets of N displacements with an error that falls quadratically with N. Our results only require a single-photon probe with an initial energy that is independent of N. Using a superposition of causal orders outperforms every setup where the displacements are probed in a definite order. Our experiment features the demonstration of indefinite causal order in a continuous-variable system, and opens up the experimental investigation of quantum metrology setups boosted by indefinite causal order.

Traditional refrigeration is driven either by external force or an information-feedback mechanism. Surprisingly, the quantum measurement and collapse, which are generally detrimental, can also be used to power a cooling engine even without requiring any feedback mechanism. In this work, we experimentally demonstrate quantum measurement cooling (QMC) powered by entangled measurement by using a novel linear optical simulator. In the simulator, different thermodynamic processes can be simulated by adjusting the energy-level spacing of working substance and the temperature of thermal bath. We show experimentally that, without prior knowledge about the measurement to be made, QMC remains likely to occur. We also demonstrate that QMC is robust against measurement noise. Those experimental results show that quantum measurement is not always detrimental but can be a valuable thermodynamic resource., Comment: 11 pages, 8 figures, 1 table

Networks composed of independent sources of entangled particles that connect distant users are a rapidly developing quantum technology and an increasingly promising test-bed for fundamental physics. Here we address the certification of their post-classical properties through demonstrations of full network nonlocality. Full network nonlocality goes beyond standard nonlocality in networks by falsifying any model in which at least one source is classical, even if all the other sources are limited only by the no-signaling principle. We report on the observation of full network nonlocality in a star-shaped network featuring three independent sources of photonic qubits and joint three-qubit entanglement-swapping measurements. Our results constitute the first experimental demonstration of full network nonlocality beyond the bilocal network., Comment: 15+10+6 pages (main + materials + supplementary), 3+4+1 figures. The computational appendix is available at https://www.github.com/apozas/three-star-fnn

Quantum theory allows information to flow through a single device in a coherent superposition of two opposite directions, resulting into situations where the input-output direction is indefinite. Here we introduce a theoretical method to witness input-output indefiniteness in a single quantum device, and we experimentally demonstrate it by constructing a photonic setup that exhibits input-output indefiniteness with a statistical significance exceeding 69 standard deviations. Our results provide a way to characterize input-output indefiniteness as a resource for quantum information and photonic quantum technologies and enable table-top simulations of hypothetical scenarios exhibiting quantum indefiniteness in the direction of time., Comment: 5 + 18 pages, 11 figures

Entanglement enhanced quantum metrology has been well investigated for beating the standard quantum limit (SQL). However, the metrological advantage of entangled states becomes much more elusive in the presence of noise. Under strictly Markovian dephasing noise, the uncorrelated and maximally entangled states achieve exactly the same measurement precision. However, it was predicted that in a non-Markovian dephasing channel, the entangled probes can recover their metrological advantage. Here, by using a highly controlled photonic system, we simulate a non-Markovian dephasing channel fulfill the quadratic decay behaviour. Under such a channel, we demonstrate the GHZ states can surpass the SQL in a scaling manner, up to six photons. Since the quadratic decay behavior is quite general for short time expansion in open quantum systems (also known as the quantum Zeno effect), our results suggest a universal and scalable method to beat the SQL in the real-word metrology tasks., Comment: 11 Pages, 6 Figures

We present the general Hardy-like quantum pigeonhole paradoxes for \textit{n}-particle states, and find that each of such paradoxes can be simply associated to an un-colorable solution of a specific vertex-coloring problem induced from the projected-coloring graph (a kind of unconventional graph). Besides, as a special kind of Hardy's paradox, several kinds of Hardy-like quantum pigeonhole paradoxes can even give rise to higher success probability in demonstrating the conflict between quantum mechanics and local or noncontextual realism than the previous Hardy's paradoxes. Moreover, not only multi-qubit states, but high-dimensional states can exhibit the paradoxes. In contrast to only one type of contradiction presented in the original quantum pigeonhole paradox, two kinds of three-qubit projected-coloring graph states as the minimal illustration are discussed in our work, and an optical experiment to verify such stronger paradox is performed. This quantum paradox provides innovative thoughts and methods in exploring new types of stronger multi-party quantum nonlocality and may have potential applications in multi-party untrusted communications and device-independent random number generation., Comment: 11 pages, 5 figures

Quantum contextuality is one of the most perplexing and peculiar features of quantum mechanics. Concisely, it refers to the observation that the result of a single measurement in quantum mechanics depends on the set of joint measurements actually performed. The study of contextuality has a long history at University of Science and Technology of China (USTC). Here we review the theoretical and experimental advances in this direction achieved at USTC over the last 20 years. We start by introducing the renowned simplest proof of state-independent contextuality. We then present several experimental tests of quantum versus noncontextual theories with photons. Finally, we discuss the investigation on the role of contextuality in general quantum information science and its application in quantum computation., Comment: 24 pages, 11 figures. Comments are welcome! v2: minor updates

We use hyper-entanglement to experimentally realize deterministic entanglement swapping based on quantum Elegant Joint Measurements. These are joint projections of two qubits onto highly symmetric, iso-entangled, bases. We report measurement fidelities no smaller than $97.4\%$. We showcase the applications of these measurements by using the entanglement swapping procedure to demonstrate quantum correlations in the form of proof-of-principle violations of both bilocal Bell inequalities and more stringent correlation criteria corresponding to full network nonlocality. Our results are a foray into entangled measurements and nonlocality beyond the paradigmatic Bell state measurement and they show the relevance of more general measurements in entanglement swapping scenarios.

Certifying individual quantum devices with minimal assumptions is crucial for the development of quantum technologies. Here, we investigate how to leverage single-system contextuality to realize self-testing. We develop a robust self-testing protocol based on the simplest contextuality witness for the simplest contextual quantum system, the Klyachko-Can-Binicio\u{g}lu-Shumovsky (KCBS) inequality for the qutrit. We establish a lower bound on the fidelity of the state and the measurements (to an ideal configuration) as a function of the value of the witness under a pragmatic assumption on the measurements we call the KCBS orthogonality condition. We apply the method in an experiment with randomly chosen measurements on a single trapped $^{40}{\rm Ca}^+$ and near-perfect detection efficiency. The observed statistics allow us to self-test the system and provide the first experimental demonstration of quantum self-testing of a single system. Further, we quantify and report that deviations from our assumptions are minimal, an aspect previously overlooked by contextuality experiments., Comment: 19+6 pages, 2+1 figures

We report an experimental certification of indefinite causal order that relies only on the characterization of the operations of a single party. We do so in the semi-device-independent scenario with the fewest possible assumptions of characterization of the parties' local operations in which indefinite causal order can be demonstrated with the quantum switch. To achieve this result, we introduce the concept of semi-device-independent causal inequalities and show that the correlations generated in a photonic quantum switch, in which all parties are able to collect local outcome statistics, achieve a violation of this inequality of 224 standard deviations. This result consists of the experimental demonstration of indefinite causal order with the fewest device-characterization assumptions to date., Comment: 9 + 4 pages, 5 + 1 figures. Close to the published version

Quantum theory predicts the existence of genuinely tripartite-entangled states, which cannot be obtained from local operations over any bipartite entangled states and unlimited shared randomness. Some of us recently proved that this feature is a fundamental signature of quantum theory. The state $\left|{GHZ}_3\right\rangle=(\left|000\right\rangle+\left|111\right\rangle)/\sqrt{2}$ gives rise to tripartite quantum correlations which cannot be explained by any causal theory limited to bipartite nonclassical common causes of any kind (generalising entanglement) assisted with unlimited shared randomness. Hence, any conceivable physical theory which would reproduce quantum predictions will necessarily include genuinely tripartite resources. In this work, we verify that such tripartite correlations are experimentally achievable. We derive a new device-independent witness capable of falsifying causal theories wherein nonclassical resources are merely bipartite. Using a high-performance photonic $\left|{GHZ}_3\right\rangle$ states with fidelities of $ 0.9741\pm0.002$, we provide a clear experimental violation of that witness by more than $26.3$ standard deviation, under the locality and fair sampling assumption. We generalise our work to the $\left|{GHZ}_4\right\rangle$ state, obtaining correlations which cannot be explained by any causal theory limited to tripartite nonclassical common causes assisted with unlimited shared randomness., Comment: See related work by Ya-Li Mao et al. (arXiv:2201.12753). 12 pages (7 of appendices), 5 figures (2 in appendices). H.C., M-O.R. and C.Z contributed equally to this work

Entanglement purification is to distill high-quality entangled states from low-quality entangled states. It is a key step in quantum repeaters, determines the efficiency and communication rates of quantum communication protocols, and is hence of central importance in long-distance communications and quantum networks. In this work, we report the first experimental demonstration of deterministic entanglement purification using polarization and spatial mode hyperentanglement. After purification, the fidelity of polarization entanglement arises from $0.268\pm0.002$ to $0.989\pm0.001$. Assisted with robust spatial mode entanglement, the total purification efficiency can be estimated as $10^{9}$ times that of the entanglement purification protocols using two copies of entangled states when one uses the spontaneous parametric down-conversion sources. Our work may have the potential to be implemented as a part of full repeater protocols.

The monogamy relations of entanglement are highly significant. However, they involve only amounts of entanglement shared by different subsystems. Results on monogamy relations between entanglement and other kinds of correlations, and particularly classical correlations, are very scarce. Here we experimentally observe a tradeoff relation between internal quantum nonseparability and external total correlations in a photonic system and found that even purely classical external correlations have a detrimental effect on internal nonseparability. The nonseparability we consider, measured by the concurrence, is between different degrees of freedom within the same photon, and the external classical correlations, measured by the standard quantum mutual information, are generated between the photons of a photon pair using the time-bin method. Our observations show that to preserve the internal entanglement in a system, it is necessary to maintain low external correlations, including classical ones, between the system and its environment., Comment: 8 pages, 4 figures

In the classical world, physical events always happen in a fixed causal order. However, it was recently revealed that quantum mechanics allows events to occur with indefinite causal order (ICO). In this study, we use an optical quantum switch to experimentally investigate the application of ICO in thermodynamic tasks. Specifically, we simulate the working system interacting with two identical thermal reservoirs in an ICO, observing the quantum heat extraction even though they are in thermal equilibrium where heat extraction is unaccessible by traditional thermal contact. Using such a process, we simulate an ICO refrigeration cycle and investigate its properties. We also show that by passing through the ICO channel multiple times, one can extract more heat per cycle and thus obtain a higher refrigeration performance. Our results suggest that the causal nonseparability can be a powerful resource for quantum thermodynamic tasks., Comment: 17 pages, 13 figures, including 5 pages, 4 figures of maintext and 12 pages, 9 figures of supplemental