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Excitation functions for the formation of the radionuclides 51Cr, 52Mn and 54Mn via deuteron-induced activation of natural iron were measured up to deuteron energies of 35 MeV. The available experimental databases of the reaction products 51Cr, 52Mn and 54Mn were extended and compared with the nuclear model calculations using the TALYS code. The model calculations reproduce our measured data after a careful choice of the input model parameters. Some information obtained on competition between the emission of multinucleons and a bound α-particle. [ABSTRACT FROM AUTHOR]