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Nitrogen-vacancy (NV) centers in diamond have shown promise as inherently localized electric-field sensors, capable of detecting individual charges with nanometer resolution. Working with NV ensembles, we demonstrate that a detailed understanding of the internal electric field environment enables enhanced sensitivity in the detection of external electric fields. We follow this logic along two complementary paths. First, using excitation tuned near the NV's zero-phonon line, we perform optically detected magnetic resonance (ODMR) spectroscopy at cryogenic temperatures in order to precisely measure the NV center's excited-state susceptibility to electric fields. In doing so, we demonstrate that the characteristically observed contrast inversion arises from an interplay between spin-selective optical pumping and the NV centers' local charge distribution. Second, motivated by this understanding, we propose and analyze a novel scheme for optically-enhanced electric-field sensing using NV ensembles; we estimate that our approach should enable order of magnitude improvements in the DC electric-field sensitivity., Comment: 6+10 pages, 3+6 figures

Pressure alters the physical, chemical and electronic properties of matter. The development of the diamond anvil cell (DAC) enables tabletop experiments to investigate a diverse landscape of high-pressure phenomena ranging from the properties of planetary interiors to transitions between quantum mechanical phases. In this work, we introduce and utilize a novel nanoscale sensing platform, which integrates nitrogen-vacancy (NV) color centers directly into the culet (tip) of diamond anvils. We demonstrate the versatility of this platform by performing diffraction-limited imaging (~600 nm) of both stress fields and magnetism, up to pressures ~30 GPa and for temperatures ranging from 25-340 K. For the former, we quantify all six (normal and shear) stress components with accuracy $<0.01$ GPa, offering unique new capabilities for characterizing the strength and effective viscosity of solids and fluids under pressure. For the latter, we demonstrate vector magnetic field imaging with dipole accuracy $<10^{-11}$ emu, enabling us to measure the pressure-driven $\alpha\leftrightarrow\epsilon$ phase transition in iron as well as the complex pressure-temperature phase diagram of gadolinium. In addition to DC vector magnetometry, we highlight a complementary NV-sensing modality using T1 noise spectroscopy; crucially, this demonstrates our ability to characterize phase transitions even in the absence of static magnetic signatures. By integrating an atomic-scale sensor directly into DACs, our platform enables the in situ imaging of elastic, electric and magnetic phenomena at high pressures., Comment: 18 + 50 pages, 4 + 19 figures

We experimentally demonstrate room-temperature storage of quantum entanglement using two nuclear spins weakly coupled to the electronic spin carried by a single nitrogen-vacancy center in diamond. We realize universal quantum gate control over the three-qubit spin system and produce entangled states encoded within the decoherence-free subspace of the two nuclear spins. By injecting arbitrary collective noise, we demonstrate that the decoherence-free entangled state has coherence time longer than that of other entangled states by an order of magnitude in our experiment.

We experimentally demonstrate a robust dynamical decoupling protocol with bounded controls using long soft pulses, eliminating a challenging requirement of strong control pulses in conventional implementations. This protocol is accomplished by designing the decoupling propagators to go through a Eulerian cycle of the coupler group [Phys. Rev. Lett. 90, 037901(2003)]. We demonstrate that this Eulerian decoupling scheme increases the coherence time by two orders of magnitude in our experiment under either dephasing or a universal noise environment., Comment: 7 pages, 4 figures

With the recent development of optomechanics, the vibration in solids, involving collective motion of trillions of atoms, gradually enters into the realm of quantum control. Built on the recent remarkable progress in optical control of motional states of diamonds, here we report an experimental demonstration of quantum teleportation from light beams to vibrational states of a macroscopic diamond under ambient conditions. Through quantum process tomography, we demonstrate average teleportation fidelity (90.6+/- 1.0)%, clearly exceeding the classical limit of 2/3. The experiment pushes the target of quantum teleportation to the biggest object so far, with interesting implications for optomechanical quantum control and quantum information science., Comment: 7 pages, 4 figures

The router is a key element for a network. We describe a scheme to realize genuine quantum routing of single-photon pulses based on cascading of conditional quantum gates in a Mach-Zehnder interferometer and report a proof-of-principle experiment for its demonstration using linear optics quantum gates. The polarization of the control photon routes in a coherent way the path of the signal photon while preserving the qubit state of the signal photon represented by its polarization. We demonstrate quantum nature of this router by showing entanglement generated between the initially unentangled control and signal photons, and confirm that the qubit state of the signal photon is well preserved by the router through quantum process tomography.

Experimental realization of a universal set of quantum logic gates is the central requirement for implementation of a quantum computer. An all-geometric approach to quantum computation offered a paradigm for implementation where all the quantum gates are achieved based on the Berry phases and their non-abelian extensions, the holonomies, from geometric transformation of quantum states in the Hilbert space. Apart from its fundamental interest and rich mathematical structure, the geometric approach has some built-in noise-resilient features. On the experimental side, geometric phases and holonomies have been observed using nuclear magnetic resonance with thermal ensembles of liquid molecules, however, such systems are known to be non-scalable for quantum computing. There are proposals to implement geometric quantum computation in scalable experimental platforms such as trapped ions, superconducting qubits, or quantum dots, and a recent experiment has realized geometric single-bit gates with the superconducting system. Here, we report the experimental realization of a universal set of geometric quantum gates with solid-state spins of the diamond defects. The diamond defects provide a scalable experimental platform with the potential for room-temperature quantum computing, which has attracted strong interest in recent years. Based on advance of coherent control in this system, our experiment shows that all-geometric and potentially robust quantum computation can be realized with solid-state spin qubits.

It was shown recently that entanglement of identical particles has a feature called dualism [Phys. Rev. Lett. 110, 140404 (2013)], which is fundamentally connected with quantum indistinguishability. Here we report an experiment that observes the entanglement duality for the first time with two identical photons, which manifest polarization entanglement when labeled by different paths or path entanglement when labeled by polarization states. By adjusting the mismatch in frequency or arrival time of the entangled photons, we tune the photon indistinguishability from quantum to classical limit and observe that the entanglement duality disappears under emergence of classical distinguishability, confirming it as a characteristic feature of quantum indistinguishable particles., Comment: 9 pages, 4 figures

We report the first experimental demonstration of distillation of quantum nonlocality, confirming the recent theoretical protocol [\textit{Phys. Rev. Lett. 102, 120401 (2009)}]. Quantum nonlocality is described by a correlation box with binary inputs and outputs, and the nonlocal boxes are realized through appropriate measurements on polarization entangled photon pairs. We demonstrate that nonlocality is amplified by connecting two nonlocal boxes into a composite one through local operations and four-photon coincidence measurements.

This is a reply to the comment from E. Amselem et al. on our paper (Phys. Rev. Lett. 109, 150401 (2012), arXiv:1207.0059)., Comment: 1 page, 1 figure, to appear in Phys. Rev. Lett. 2013

Random numbers represent an indispensable resource for many applications. A recent remarkable result is the realization that non-locality in quantum mechanics can be used to certify genuine randomness through Bell's theorem, producing reliable random numbers in a device independent way. Here, we explore the contextuality aspect of quantum mechanics and show that true random numbers can be generated using only single qutrit (three-state systems) without entanglement and non-locality. In particular, we show that any observed violation of the Klyachko-Can-Binicioglu-Shumovsky (KCBS) inequality [Phys. Rev. Lett. 101, 20403 (2008)] provides a positive lower bound on genuine randomness. As a proof-of-concept experiment, we demonstrate with photonic qutrits that at least 5246 net true random numbers are generated with a confidence level of 99.9%., Comment: Paper : 4.5 pages, 4 figures; Supplementary material : 5 pages, 2 figures

We report an experiment that uses the environmental selection, a key concept in the recent theory of quantum Darwinism, as a mechanism to realize the entanglement filter, a useful quantum information device that filters out certain entangled states. In the experiment, the environment of two qubits is controlled to favor an entangled state and kill other competing components in the input state. The initial state has vanishing entanglement, but the state surviving after interaction with the environment is close to a maximally entangled state, with an entanglement fidelity of $(94.7\pm 1.9)%$ measured through the quantum state tomography. We experimentally demonstrate that the generated entanglement is robust under change of the initial state configurations and the environmental parameters.

We report an experiment that demonstrates full function of a quantum router using entangled photons, where the paths of a single-photon pulse are controlled in a coherent fashion by polarization of another single photon. Through a projective measurement, we prepare the polarization of the control photon in arbitrary superposition states, leading to coherent routing of the target photon in quantum superposition of different paths. We demonstrate quantum nature of this router through optical measurements based on quantum state tomography and show an average fidelity of $(93.24\pm 0.23)%$ for the quantum routing operation., Comment: "This paper has been withdrawn and it will be replaced by a new experiment that does not require prior entanglement between the control and the data photons."

We report the first state-independent experimental test of quantum contextuality on a single photonic qutrit (three-dimensional system), based on a recent theoretical proposal [Yu and Oh, Phys. Rev. Lett. 108, 030402 (2012)]. Our experiment spotlights quantum contextuality in its most basic form, in a way that is independent of either the state or the tensor product structure of the system.