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Ionising radiation interactions in matter can trigger a cascade of processes that underpin long-lived damage in the medium. To date, however, a lack of suitable methodologies has precluded our ability to understand the role that material nanostructure plays in this cascade. Here, we use transient photoabsorption to track the lifetime of free electrons (t_c) in bulk and nanostructured SiO2 (aerogel) irradiated by picosecond-scale (10^-12 s) bursts of X-rays and protons from a laser-driven accelerator. Optical streaking reveals a sharp increase in t_c from < 1 ps to > 50 ps over a narrow average density (p_av) range spanning the expected phonon-fracton crossover in aerogels. Numerical modelling suggests that this discontinuity can be understood by a quenching of rapid, phonon-assisted recovery in irradiated nanostructured SiO_2. This is shown to lead to an extended period of enhanced energy density in the excited electron population. Overall, these results open a direct route to tracking how low-level processes in complex systems can underpin macroscopically observed phenomena and, importantly, the conditions that permit them to emerge.

We report on a direct search for elastic photon-photon scattering using x-ray and $\gamma$ photons from a laser-plasma based experiment. A gamma photon beam produced by a laser wakefield accelerator provided a broadband gamma spectrum extending to above $E_\gamma = 200$ MeV. These were collided with a dense x-ray field produced by the emission from a laser heated germanium foil at $E_x \approx 1.4$ keV, corresponding to an invariant mass of $\sqrt{s} = 1.22 \pm 0.22$ MeV. In these asymmetric collisions elastic scattering removes one x-ray and one high-energy $\gamma$ photon and outputs two lower energy $\gamma$ photons. No changes in the $\gamma$ photon spectrum were observed as a result of the collisions allowing us to place a 95% upper bound on the cross section of $1.5 \times 10^{15}\,\mu$b. Although far from the QED prediction, this represents the lowest upper limit obtained so far for $\sqrt{s} \lesssim 1$ MeV., Comment: 6 pages, 10 figures

Radiation reaction describes the effective force experienced by an accelerated charge due to radiation emission. Quantum effects dominate charge dynamics and radiation production[1][2] for charges accelerated by fields with strengths approaching the Schwinger field, $\mathbf{E_{sch}=}$\textbf{\SI[detect-weight]{1.3e18}{\volt\per\metre}[3]. Such fields exist in extreme astrophysical environments such as pulsar magnetospheres[4], may be accessed by high-power laser systems[5-7], dense particle beams interacting with plasma[8], crystals[9], and at the interaction point of next generation particle colliders[10]. Classical radiation reaction theories do not limit the frequency of radiation emitted by accelerating charges and omit stochastic effects inherent in photon emission[11], thus demanding a quantum treatment. Two quantum radiation reaction models, the quantum-continuous[12] and quantum-stochastic[13] models, correct the former issue, while only the quantum-stochastic model incorporates stochasticity[12]. Such models are of fundamental importance, providing insight into the effect of the electron self-force on its dynamics in electromagnetic fields. The difficulty of accessing conditions where quantum effects dominate inhibited previous efforts to observe quantum radiation reaction in charged particle dynamics with high significance. We report the first direct, high significance $(>5{\sigma})$ observation of strong-field radiation reaction on charged particles. Furthermore, we obtain strong evidence favouring the quantum radiation reaction models, which perform equivalently, over the classical model. Robust model comparison was facilitated by a novel Bayesian framework which inferred collision parameters. This framework has widespread utility for experiments where parameters governing lepton-laser collisions cannot be directly measured, including those using conventional accelerators., Comment: 31 pages, 14 figures

Quantum field theory predicts a nonlinear response of the vacuum to strong electromagnetic fields of macroscopic extent. This fundamental tenet has remained experimentally challenging and is yet to be tested in the laboratory. A particularly distinct signature of the resulting optical activity of the quantum vacuum is vacuum birefringence. This offers an excellent opportunity for a precision test of nonlinear quantum electrodynamics in an uncharted parameter regime. Recently, the operation of the high-intensity laser ReLaX provided by the Helmholtz International Beamline for Extreme Fields (HIBEF) has been inaugurated at the High Energy Density (HED) scientific instrument of the European XFEL. We make the case that this worldwide unique combination of an x-ray free-electron laser and an ultra-intense near-infrared laser together with recent advances in high-precision x-ray polarimetry, refinements of prospective discovery scenarios, and progress in their accurate theoretical modelling have set the stage for performing an actual discovery experiment of quantum vacuum nonlinearity., Comment: 34 pages, 21 figures

Near-future experiments intend to detect strong-field Breit-Wheeler pair creation from the collision between bremsstrahlung bursts containing GeV-$\gamma$ quanta and high-intensity laser pulses. In this theoretical study, we investigate the influence of laser focusing, radiation reaction and a broad bremsstrahlung $\gamma$ spectrum on the energy and angular distributions of created pairs. Understanding the role of these inherent reaction attributes provides relevant insights for experimental detection strategies and data interpretation. We show that the inclusion of radiation reaction leads to a narrow energy spectrum of the yielded particles, whose maximum is shifted to substantially lower energies as compared to the case in which radiative energy losses are ignored. The broad bremsstrahlung spectrum also has distinct influence on the particle distributions, whereas the impact of laser focusing turns out to be rather moderate in the considered parameter regime., Comment: 11 pages, 7 figures

Novel schemes for generating ultra-low emittance electron beams have been developed in past years and promise compact particle sources with excellent beam quality suitable for future high-energy physics experiments and free-electron lasers. Recent theoretical work has proposed a laser-based method capable of resolving emittances in the sub 0.1 mm mrad regime, by modulating the electron phase-space ponderomotively. Here we present a first experimental demonstration of this scheme using a laser wakefield accelerator. The observed emittance and source size is consistent with published values. We also show calculations demonstrating that tight bounds on the upper limit for emittance and source size can be derived from the 'laser-grating' method even in the presence of low signal to noise and uncertainty in laser-grating parameters., Comment: 13 pages, 13 figures; journal published version

This Technical Design Report presents a detailed description of all aspects of the LUXE (Laser Und XFEL Experiment), an experiment that will combine the high-quality and high-energy electron beam of the European XFEL with a high-intensity laser, to explore the uncharted terrain of strong-field quantum electrodynamics characterised by both high energy and high intensity, reaching the Schwinger field and beyond. The further implications for the search of physics beyond the Standard Model are also discussed.

We present experimental results, which show a laser polarization dependent contribution to electron beam pointing jitter in laser wakefield accelerators (LWFA). We develop a theoretical model for the polarization dependence in terms of the transverse dynamics of trapped electrons, resonantly driven by bubble centroid oscillations. The latter are generated by the carrier wave phase evolution at the self-steepened laser pulse front. In the model, the polarization dependent jitter originates from shot-to-shot fluctuations of the laser carrier envelope phase. The model is verified by particle in cell simulations and suggests that for non-CEP stabilized systems the polarization dependent jitter may form an ultimate limit to beam pointing stability in LWFAs.

Measuring signatures of strong-field quantum electrodynamics (SF-QED) processes in an intense laser field is an experimental challenge: it requires detectors to be highly sensitive to single electrons and positrons in the presence of the typically very strong x-ray and $\gamma$-photon background levels. In this paper, we describe a particle detector capable of diagnosing single leptons from SF-QED interactions and discuss the background level simulations for the upcoming Experiment-320 at FACET-II (SLAC National Accelerator Laboratory). The single particle detection system described here combines pixelated scintillation LYSO screens and a Cherenkov calorimeter. We detail the performance of the system using simulations and a calibration of the Cherenkov detector at the ELBE accelerator. Single 3 GeV leptons are expected to produce approximately 537 detectable photons in a single calorimeter channel. This signal is compared to Monte-Carlo simulations of the experiment. A signal-to-noise ratio of 18 in a single Cherenkov calorimeter detector is expected and a spectral resolution of 2% is achieved using the pixelated LYSO screens.

We describe a laser-plasma platform for photon-photon collision experiments to measure fundamental quantum electrodynamic processes such as the linear Breit-Wheeler process with real photons. The platform has been developed using the Gemini laser facility at the Rutherford Appleton Laboratory. A laser wakefield accelerator and a bremsstrahlung convertor are used to generate a collimated beam of photons with energies of hundreds of MeV, that collide with keV x-ray photons generated by a laser heated plasma target. To detect the pairs generated by the photon-photon collisions, a magnetic transport system has been developed which directs the pairs onto scintillation-based and hybrid silicon pixel single particle detectors. We present commissioning results from an experimental campaign using this laser-plasma platform for photon-photon physics, demonstrating successful generation of both photon sources, characterisation of the magnetic transport system and calibration of the single particle detectors, and discuss the feasibility of this platform for the observation of the Breit-Wheeler process. The design of the platform will also serve as the basis for the investigation of strong-field quantum electrodynamic processes such as the nonlinear Breit-Wheeler and the Trident process, or eventually, photon-photon scattering., Comment: 28 pages, 14 figures

The extreme intensities obtainable with lasers such as Gemini allow non-linear QED phenomena to be investigated according to our calculations. Electron-positron pair production from a pure vacuum target, which has yet to be observed experimentally, is possibly the most iconic process. Beyond pair-production our campaign will allow the experimental investigation of currently unexplored extreme radiation regimes, like the quantum radiation dominated regime (where quantum and self-field effects become important) and non-linear Compton scattering. This is the first experiment in a multi-part campaign proposed by a major international collaboration to investigate non-linear QED. This proposal is for the first experiment in a series of 3 to achieve our most high-profile experimental goal of pair production in vacuum, but each experiment is designed to have its own tangible high-profile outcome.

A new regime in the interaction of a two-colour ($\omega$,$2\omega$) laser with a nanometre-scale foil is identified, resulting in the emission of extremely intense, isolated attosecond pulses - even in the case of multi-cycle lasers. For foils irradiated by lasers exceeding the blow-out field strength (i.e. capable of fully separating electrons from the ion background), the addition of a second harmonic field results in the stabilization of the foil up to the blow-out intensity. This is then followed by a sharp transition to transparency that essentially occurs in a single optical cycle. During the transition cycle, a dense, nanometre-scale electron bunch is accelerated to relativistic velocities and emits a single, strong attosecond pulse with a peak intensity approaching that of the laser field.

This Letter of Intent describes LUXE (Laser Und XFEL Experiment), an experiment that aims to use the high-quality and high-energy electron beam of the European XFEL and a powerful laser. The scientific objective of the experiment is to study quantum electrodynamics processes in the regime of strong fields. High-energy electrons, accelerated by the European XFEL linear accelerator, and high-energy photons, produced via Bremsstrahlung of those beam electrons, colliding with a laser beam shall experience an electric field up to three times larger than the Schwinger critical field (the field at which the vacuum itself is expected to become unstable and spark with spontaneous creation of electron-positron pairs) and access a new regime of quantum physics. The processes to be investigated, which include nonlinear Compton scattering and nonlinear Breit-Wheeler pair production, are relevant to a variety of phenomena in Nature, e.g. in the areas of astrophysics and collider physics and complement recent results in atomic physics. The setup requires in particular the extraction of a minute fraction of the electron bunches from the European XFEL accelerator, the installation of a powerful laser with sophisticated diagnostics, and an array of precision detectors optimised to measure electrons, positrons and photons. Physics sensitivity projections based on simulations are also provided.

The dispersive behavior of materials with atomic charge numbers varing from $Z = 4$ (beryllium, Be) to $Z = 82$ (lead, Pb) was investigated experimentally and theoretically at $\gamma$-ray energies up to 2 MeV. The experiment was performed at the double-crystal gamma spectrometer GAMS6 of the ILL in Grenoble. The experimental results were compared with theoretical calculations which account for all major elastic processes involved. Overall, we found a good agreement between theory and experiment. We find that for the development of refractive optics at $\gamma$-ray energies beyond those currently in use high-Z materials become increasingly attractive compared to the beryllium lens-stacks used at X-ray energies., Comment: submitted to Phys. Rev. A

We report the experimental generation of highly energetic carbon ions up to 48 MeV per nucleon by shooting double-layer targets composed of well-controlled slightly underdense plasma (SUP) and ultrathin foils with ultra-intense femtosecond laser pulses. Particle-in-cell simulations reveal that carbon ions residing in the ultrathin foils undergo radiation pressure acceleration and long-time sheath field acceleration in sequence due to the existence of the SUP in front of the foils. Such an acceleration scheme is especially suited for heavy ion acceleration with femtosecond laser pulses. The breakthrough of heavy ion energy up to multi-tens of MeV/u at high-repetition-rate would be able to trigger significant advances in nuclear physics, high energy density physics, and medical physics.

We report on the experimental studies of laser driven ion acceleration from double-layer target where a near-critical density target with a few-micron thickness is coated in front of a nanometer thin diamond-like carbon foil. A significant enhancement of proton maximum energies from 12 to ~30 MeV is observed when relativistic laser pulse impinge on the double-layer target under linear polarization. We attributed the enhanced acceleration to superponderomotive electrons that were simultaneously measured in the experiments with energies far beyond the free-electron ponderomotive limit. Our interpretation is supported by two-dimensional simulation results.

The description of the dynamics of an electron in an external electromagnetic field of arbitrary intensity is one of the most fundamental outstanding problems in electrodynamics. Remarkably, to date there is no unanimously accepted theoretical solution for ultra-high intensities and little or no experimental data. The basic challenge is the inclusion of the self-interaction of the electron with the field emitted by the electron itself - the so-called radiation reaction force. We report here on the experimental evidence of strong radiation reaction, in an all-optical experiment, during the propagation of highly relativistic electrons (maximum energy exceeding 2 GeV) through the field of an ultra-intense laser (peak intensity of $4\times10^{20}$ W/cm$^2$). In their own rest frame, the highest energy electrons experience an electric field as high as one quarter of the critical field of quantum electrodynamics and are seen to lose up to 30% of their kinetic energy during the propagation through the laser field. The experimental data show signatures of quantum effects in the electron dynamics in the external laser field, potentially showing departures from the constant cross field approximation.

The dynamics of energetic particles in strong electromagnetic fields can be heavily influenced by the energy loss arising from the emission of radiation during acceleration, known as radiation reaction. When interacting with a high-energy electron beam, today's lasers are sufficiently intense to explore the transition between the classical and quantum radiation reaction regimes. We report on the observation of radiation reaction in the collision of an ultra-relativistic electron beam generated by laser wakefield acceleration ($\varepsilon > 500$ MeV) with an intense laser pulse ($a_0 > 10$). We measure an energy loss in the post-collision electron spectrum that is correlated with the detected signal of hard photons ($\gamma$-rays), consistent with a quantum (stochastic) description of radiation reaction. The generated $\gamma$-rays have the highest energies yet reported from an all-optical inverse Compton scattering scheme, with critical energy $\varepsilon_{\rm crit} > $ 30 MeV., Comment: 11 pages, 9 figures, accepted for publication in PRX

The refractive index of silicon at $\gamma$-ray energies from 181 - 1959 keV was investigated using the GAMS6 double crystal spectrometer and found to follow the predictions of the classical scattering model. This is in contrast to earlier measurements on the GAMS5 spectrometer, which suggested a sign-change in the refractive index for photon energies above 500 keV. We present a re-evaluation of the original data from 2011 as well as data from a 2013 campaign in which we show that systematic errors due to diffraction effects of the prism can explain the earlier data., Comment: submitted to Physical Review C

The birth of attosecond light sources is expected to inspire a breakthrough in ultrafast optics, which may extend human real-time measurement and control techniques into atomic-scale electronic dynamics. For applications, it is essential to obtain a single attosecond pulse of high intensity, large photon energy and short duration. Here we show that single 100-terawatt attosecond X-ray light pulse with intensity ${1\times10^{21}}\textrm{W}/\textrm{cm}^{{ 2}}$ and duration ${7.9} \textrm{as}$ can be produced by intense laser irradiation on a capacitor-nanofoil target composed of two separate nanofoils. In the interaction, a strong electrostatic potential develops between two nanofoils, which drags electrons out of the second foil and piles them up in vacuum, forming an ultradense relativistic electron nanobunch. This nanobunch exists in only half a laser cycle and smears out in others, resulting in coherent synchrotron emission of a single pulse. Such an unprecedentedly giant attosecond X-ray pulse may bring us to view a real attoworld., Comment: 11 pages, 4 figures

Energy coupling during relativistically intense laser-matter interactions is encoded in the attosecond motion of strongly driven electrons at the pre-formed plasma-vacuum boundary. Studying and controlling this motion can reveal details about the microscopic processes that govern a vast array of light-matter interaction physics and applications. These include research areas right at the forefront of extreme laser-plasma science such as laser-driven ion acceleration1, bright attosecond pulse generation2,3 and efficient energy coupling for the generation and study of warm dense matter4. Here we demonstrate attosecond control over the trajectories of relativistic electron bunches formed during such interactions by studying the emission of extreme ultraviolet (XUV) harmonic radiation. We describe how the precise addition of a second laser beam operating at the second harmonic of the driving laser pulse can significantly transform the interaction by modifying the accelerating potential provided by the fundamental frequency to drive strong coherent emission. Numerical particle-in-cell code simulations and experimental observations demonstrate that this modification is extremely sensitive to the relative phase of the two beams and can lead to significant enhancements in the resulting harmonic yield. This work also reveals that the ability to control these extreme interactions with attosecond precision is an essential requirement for generation of ultra-bright, high temporal contrast attosecond radiation for atomic and molecular pump-probe experiments5,6.

The microscopic dynamics of laser-driven coherent synchrotron emission transmitted through thin foils are investigated using particle-in-cell simulations. For normal incidence interactions, we identify the formation of two distinct electron nanobunches from which emission takes place each half-cycle of the driving laser pulse. These emissions are separated temporally by 130 attoseconds and are dominant in different frequency ranges, which is a direct consequence of the distinct characteristics of each electron nanobunch. This may be exploited through spectral filtering to isolate these emissions, generating electromagnetic pulses of duration ~70 as.

We present a comprehensive model for predicting the full performance of a second harmonic generationoptical parametric amplification system that aims at enhancing the temporal contrast of laser pulses. The model simultaneously takes into account all the main parameters at play in the system such as the group velocity mismatch, the beam divergence, the spectral content, the pump depletion, and the length of the nonlinear crystals. We monitor the influence of the initial parameters of the input pulse and the interdependence of the two related non-linear processes on the performance of the system and show its optimum configuration. The influence of the initial beam divergence on the spectral and the temporal characteristics of the generated pulse is discussed. In addition, we show that using a crystal slightly longer than the optimum length and introducing small delay between the seed and the pump ensures maximum efficiency and compensates for the spectral shift in the optical parametric amplification stage in case of chirped input pulse. As an example, calculations for bandwidth transform limited and chirped pulses of sub-picosecond duration in beta barium borate crystal are presented., Comment: 23 pages, 18 figures

Calibration of three scintillators (EJ232Q, BC422Q and EJ410) in a time-of-flight (TOF) arrangement using a laser drive-neutron source is presented. The three plastic scintillator detectors were calibrated with gamma insensitive bubble detector spectrometers, which were absolutely calibrated over a wide range of neutron energies ranging from sub MeV to 20 MeV. A typical set of data obtained simultaneously by the detectors are shown, measuring the neutron spectrum emitted from a petawatt laser irradiated thin foil.

The jets of compact accreting objects are composed of electrons and a mixture of positrons and ions. These outflows impinge on the interstellar or intergalactic medium and both plasmas interact via collisionless processes. Filamentation (beam-Weibel) instabilities give rise to the growth of strong electromagnetic fields. These fields thermalize the interpenetrating plasmas. Hitherto, the effects imposed by a spatial non-uniformity on filamentation instabilities have remained unexplored. We examine the interaction between spatially uniform background electrons and a minuscule cloud of electrons and positrons. A square micro-cloud of equally dense electrons and positrons impinges in our particle-in-cell (PIC) simulation on a spatially uniform plasma at rest. The mean speed of the micro-cloud corresponds to a relativistic factor of 15, which is relevant for laboratory experiments and for relativistic astrophysical outflows. The spatial distributions of the leptons and of the electromagnetic fields are examined at several times. A filamentation instability develops between the magnetic field carried by the micro-cloud and the background electrons. The electromagnetic fields, which grow from noise levels, redistribute the electrons and positrons within the cloud, which boosts the peak magnetic field amplitude. The current density and the moduli of the electromagnetic fields grow aperiodically in time and steadily along the direction that is anti-parallel to the cloud's velocity vector. The micro-cloud remains conjoined during the simulation. The instability induces an electrostatic wakefield in the background plasma., Comment: 10 pages, 13 figures, Astronomy and Astrophysics (in press)

We report on the successful demonstration of selective acceleration of deuterium ions by target-normal sheath acceleration (TNSA) with a high-energy petawatt laser. TNSA typically produces a multi-species ion beam that originates from the intrinsic hydrocarbon and water vapor contaminants on the target surface. Using the method first developed by Morrison, et al.,$^{1}$ an ion beam with $>$99$\%$ deuterium ions and peak energy 14 MeV/nucleon is produced with a 200 J, 700 fs, $>10^{20} W/cm^{2}$ laser pulse by cryogenically freezing heavy water (D$_{2}$O) vapor onto the rear surface of the target prior to the shot. Within the range of our detectors (0-8.5$^{\circ}$), we find laser-to-deuterium-ion energy conversion efficiency of 4.3$\%$ above 0.7 MeV/nucleon while a conservative estimate of the total beam gives a conversion efficiency of 9.4$\%$., Comment: 5 pages, 5 figures

Direct investigation of ion-induced dynamics in matter on picosecond (ps, 10-12 s) timescales has been precluded to date by the relatively long nanosecond (ns, 10-9 s) scale ion pulses typically provided by radiofrequency accelerators1. By contrast, laser-driven ion accelerators provide bursts of ps duration2, but have yet to be applied to the study of ultrafast ion-induced transients in matter. We report on the evolution of an electron-hole plasma excited in borosilicate glass by such bursts. This is observed as an onset of opacity to synchronised optical probe radiation and is characterised by the 3.0 +/- 0.8 ps ion pump rise-time . The observed decay-time of 35 +/- 3 ps i.e. is in excellent agreement with modelling and reveals the rapidly evolving electron temperature (>10 3 K) and carrier number density (>10 17cm-3). This result demonstrates that ps laser accelerated ion bursts are directly applicable to investigating the ultrafast response of matter to ion interactions and, in particular, to ultrafast pulsed ion radiolysis of water3-5, the radiolytic decompositions of which underpin biological cell damage and hadrontherapy for cancer treatment6., Comment: 11 pages

Synchronising ultra-short (~fs) and focussed laser pulses is a particularly difficult task, as this timescale lies orders of magnitude below the typical range of fast electronic devices. Here we present an optical technique that allows for femtosecond-scale synchronisation of the focal planes of two focussed laser pulses. This technique is virtually applicable to any focussing geometry and relative intensity of the two lasers. Experimental implementation of this technique provides excellent quantitative agreement with theoretical expectations. The proposed technique will prove highly beneficial for the next generation of multiple, petawatt class laser systems.

A novel method for characterising the full spectrum of deuteron ions emitted by laser driven multi-species ion sources is discussed. The procedure is based on using differential filtering over the detector of a Thompson parabola ion spectrometer, which enables discrimination of deuterium ions from heavier ion species with the same charge-to-mass ratio (such as C6+, O8+, etc.). Commonly used Fuji Image plates were used as detectors in the spectrometer, whose absolute response to deuterium ions over a wide range of energies was calibrated by using slotted CR-39 nuclear track detectors. A typical deuterium ion spectrum diagnosed in a recent experimental campaign is presented., Comment: 7 pages, 7 figures

Laser-wakefield acceleration is a promising technique for the next generation of ultra-compact, high-energy particle accelerators. However, for a meaningful use of laser-driven particle beams it is necessary that they present a high degree of pointing stability in order to be injected into transport lines and further acceleration stages. Here we show a comprehensive experimental study of the main factors limiting the pointing stability of laser-wakefield accelerated electron beams. It is shown that gas-cells provide a much more stable electron generation axis, if compared to gas-jet targets, virtually regardless of the gas density used. A sub-mrad shot-to-shot fluctuation in pointing is measured and a consistent non-zero offset of the electron axis in respect to the laser propagation axis is found to be solely related to a residual angular dispersion introduced by the laser compression system and can be used as a precise diagnostic tool for compression oprtimisation in chirped pulse amplified lasers.

We report on the generation of a narrow divergence ($\theta\approx 2.5$ mrad), multi-MeV ($E_\text{MAX} = 18$ MeV) and ultra-high brilliance ($\approx 2\times10^{19}$ photons s$^{-1}$ mm$^{-2}$ mrad $^{-2}$ 0.1\% BW) $\gamma$-ray beam from the scattering of an ultra-relativistic laser-wakefield accelerated electron beam in the field of a relativistically intense laser (dimensionless amplitude $a_0\approx2$). The spectrum of the generated $\gamma$-ray beam is measured, with MeV resolution, seamlessly from 6 MeV to 18 MeV, giving clear evidence of the onset of non-linear Thomson scattering. The photon source has the highest brilliance in the multi-MeV regime ever reported in the literature.

We report the enhancement of individual harmonics generated at a relativistic ultra-steep plasma vacuum interface. Simulations show the harmonic emission to be due to the coupled action of two high velocity oscillations -- at the fundamental $\omega_L$ and at the plasma frequency $\omega_P$ of the bulk plasma. The synthesis of the enhanced harmonics can be described by the reflection of the incident laser pulse at a relativistic mirror oscillating at $\omega_L$ and $\omega_P$., Comment: 5 pages, 3 figures. arXiv admin note: substantial text overlap with arXiv:1307.5635

Spectrally-peaked proton beams ($E_{p}\approx 8$ MeV, $\Delta E\approx 4$ MeV) have been observed from the interaction of an intense laser ($> 10^{19 }$ Wcm$^{-2}$) with ultrathin CH foils, as measured by spectrally-resolved full beam profiles. These beams are reproducibly generated for foil thicknesses (5-100 nm), and exhibit narrowing divergence with decreasing target thickness down to $\approx 8^\circ$ for 5 nm. Simulations demonstrate that the narrow energy spread feature is a result of buffered acceleration of protons. Due to their higher charge-to-mass ratio, the protons outrun a carbon plasma driven in the relativistic transparency regime.

We have studied the propagation of fast electrons through laser irradiated Ti foils by monitoring the emission of hard X-rays and K-{\alpha} radiation from bare foils and foils backed by a thick epoxy layer. Key observations include strong refluxing of electrons and divergence of the electron beam in the foil with evidence of magnetic field collimation. Our diagnostics have allowed us to estimate the fast electron temperature and fraction of laser energy converted to fast electrons. We have observed clear differences between the fast electron temperatures observed with bare and epoxy backed targets which may be due to the effects of refluxing.

A novel design for a compact gamma-ray spectrometer is presented. The proposed system allows for spectroscopy of high-flux multi-MeV gamma-ray beams with MeV energy resolution in a compact design. In its basic configuration, the spectrometer exploits conversion of gamma-rays into electrons via Compton scattering in a low-Z material. The scattered electron population is then spectrally resolved using a magnetic spectrometer. The detector is shown to be effective for gamma-ray energies between 3 and 20MeV. The main properties of the spectrometer are confirmed by Monte-Carlo simulations.

Relativistic electrons are prodigious sources of photons. Beyond classical accelerators, ultra-intense laser interactions are of particular interest as they allow the coherent motion of relativistic electrons to be controlled and exploited as sources of radiation. Under extreme laser conditions theory predicts that isolated free relativistic electron sheets (FRES) can be produced and exploited for the production of a new class of radiation - unipolar extreme ultraviolet(XUV) pulses. However, the combination of extremely rapid rise-time and highest peak intensity in these simulations is still beyond current laser technology. We demonstrate a route to isolated FRES with existing lasers by exploiting relativistic transparency to produce an ultra-intense pulse with a steep rise time. When such an FRES interacts with a second, oblique target foil the electron sheet is rapidly accelerated ('kicked'). The radiation signature and simulations demonstrate that a single, nanometer thick FRES was produced. The experimental observations together with our theoretical modeling suggest the production of the first unipolar (half-cycle) pulse in the XUV - an achievement that has so far only been realized in the terahertz spectral domain., Comment: 10 pages, 3 figures

The nonlinear optical properties of a plasma due to the relativistic electron motion in an intense laser field are of fundamental importance for current research and the generation of brilliant laser-driven sources of particles and photons1-15. Yet, one of the most interesting regimes, where the frequency of the laser becomes resonant with the plasma, has remained experimentally hard to access. We overcome this limitation by utilizing ultrathin carbon nanotube foam16 (CNF) targets allowing the strong relativistic nonlinearities at near- critical density (NCD) to be exploited for the first time. We report on the experimental realization of relativistic plasma optics to spatio-temporally compress the laser pulse within a few micrometers of propagation, while maintaining about half its energy. We also apply the enhanced laser pulses to substantially improve the properties of an ion bunch accelerated from a secondary target. Our results provide first insights into the rich physics of NCD plasmas and the opportunities waiting to be harvested for applications., Comment: 11 pages+5 pages (supplementary information), 4 figures+ 2 figures (supplementary information)

We report on the laser-driven generation of purely neutral, relativistic electron-positron pair plasmas. The overall charge neutrality, high average Lorentz factor ($\gamma_{e/p} \approx 15$), small divergence ($\theta_{e/p} \approx 10 - 20$ mrad), and high density ($n_{e/p}\simeq 10^{15}$cm$^{-3}$) of these plasmas open the pathway for the experimental study of the dynamics of this exotic state of matter, in regimes that are of relevance to electron-positron astrophysical plasmas., Comment: The manuscript is withdrawn from ArXiv because of conflicting interests

Waveform shaping and frequency synthesis based on waveform modulation is ubiquitous in electronics, telecommunication technology, and optics. For optical waveforms, the carrier frequency is on the order of several hundred THz, while the modulation frequencies used in conventional devices like electro- or acousto-optical modulators are orders of magnitude lower. As a consequence, any new frequencies are typically very close to the fundamental. The synthesis of new frequencies in the extreme ultraviolet (XUV), e.g. by using relativistic oscillating mirrors, requires modulation frequencies in the optical regime or even in the extreme ultraviolet. The latter has not been proven possible to date. Here we demonstrate that individual strong harmonics can indeed be generated by reflecting light off a plasma surface that oscillates at XUV frequencies. The strong harmonics are explained by nonlinear frequency mixing of near-infrared light and a laser-driven plasma oscillation in the extreme ultra-violet mediated by a relativistic non-linearity., Comment: 17 pages, 4 figures

The generation of ultra-relativistic positron beams with short duration ($\tau_{e^+} \leq 30$ fs), small divergence ($\theta_{e^+} \simeq 3$ mrad), and high density ($n_{e^+} \simeq 10^{14} - 10^{15}$ cm$^{-3}$) from a fully optical setup is reported. The detected positron beam propagates with a high-density electron beam and $\gamma$-rays of similar spectral shape and peak energy, thus closely resembling the structure of an astrophysical leptonic jet. It is envisaged that this experimental evidence, besides the intrinsic relevance to laser-driven particle acceleration, may open the pathway for the small-scale study of astrophysical leptonic jets in the laboratory.

The acceleration of ions from ultra-thin foils has been investigated using 250 TW, sub-ps laser pulses, focused on target at intensities up to $3\times10^{20} \Wcm2$. The ion spectra show the appearance of narrow band features for proton and Carbon peaked at higher energy (in the 5-10 MeV/nucleon range) and with significantly higher flux than previously reported. The spectral features, and their scaling with laser and target parameters, provide evidence of a multispecies scenario of Radiation Pressure Acceleration in the Light Sail mode, as confirmed by analytical estimates and 2D Particle In Cell simulations. The scaling indicates that monoenergetic peaks with more than 100 MeV/nucleon energies are obtainable with moderate improvements of the target and laser characteristics, which are within reach of ongoing technical developments.

A novel regime is proposed where, employing linearly polarized laser pulses at intensities $10^{21}\textrm{Wcm}^{-2}$ as two order of magnitude lower than earlier predicted [T. Esirkepov et al., Phys. Rev. Lett. 92, 175003 (2004)], ions are dominantly accelerated from ultrathin foils by the radiation pressure, and have monoenergetic spectra. In the regime, ions accelerated from the hole-boring process quickly catch up with the ions accelerated by target normal sheath acceleration (TNSA), and they then join in a single bunch, undergoing a hybrid Light-Sail/TNSA acceleration. Under an appropriate coupling condition between foil thickness, laser intensity and pulse duration, laser radiation pressure can be dominant in this hybrid acceleration. Two-dimensional PIC simulations show that $1.26\textrm{GeV}$ quasimonoenergetic $\textrm{C}^{6+}$ beams are obtained by linearly polarized laser pulses at intensities of $10^{21}\textrm{Wcm}^{-2}$., Comment: 6 pages, 4 figures

In this letter we report on an experimental study of high harmonic radiation generated in nanometer-scale foil targets irradiated under normal incidence. The experiments constitute the first unambiguous observation of odd-numbered relativistic harmonics generated by the $\vec{v}\times\vec{B}$ component of the Lorentz force verifying a long predicted property of solid target harmonics. Simultaneously the observed harmonic spectra allow in-situ extraction of the target density in an experimental scenario which is of utmost interest for applications such as ion acceleration by the radiation pressure of an ultraintense laser., Comment: 5 pages, 4 figures

The transport of relativistic electrons generated in the interaction of petawatt class lasers with solid targets has been studied through measurements of the optical emission from their rear surface. The high degree of polarization of the emission indicates that it is predominantly optical transition radiation. A halo that surrounds the main region of emission is also polarized, and is attributed to the effect of electron recirculation. The variation of the amplitude of the transition radiation with respect to observation angle provides evidence for the presence of {$\mu$m-size} filaments., Comment: 12 pages, 7 figures

In laser-plasma interactions it is widely accepted that a non-uniform interaction surface will invariably seed hydrodynamic instabilities and a growth in the amplitude of the initial modulation. Recent experimental results [Dromey, Nat. Phys. 2009] have demonstrated that there must be target smoothing in femtosecond timescale relativistic interactions, contrary to prevailing expectation. In this paper we develop a theoretical description of the physical process that underlies this novel phenomena. We show that the surface dynamics in the few-cycle relativistic regime is dominated by the coherent electron motion resulting in a smoothing of the electron surface. This stabilization of plasma surfaces is unique in laser-plasma interactions and demonstrates that dynamics in the few-cycle regime differ fundamentally from the longer pulse regimes. This has important consequences for applications such as radiation pressure acceleration of protons and ions and harmonic generation from relativistically oscillating surfaces., Comment: 5 pages, 4 figures

The emission characteristics of intense laser driven protons are controlled using ultra-strong (of the order of 10^9 V/m) electrostatic fields varying on a few ps timescale. The field structures are achieved by exploiting the high potential of the target (reaching multi-MV during the laser interaction). Suitably shaped targets result in a reduction in the proton beam divergence, and hence an increase in proton flux while preserving the high beam quality. The peak focusing power and its temporal variation are shown to depend on the target characteristics, allowing for the collimation of the inherently highly divergent beam and the design of achromatic electrostatic lenses., Comment: 9 Pages, 5 figures

A new regime is described for Radiation Pressure Acceleration of a thin foil by an intense laser beam of above 10^20 W/cm^2. Highly monoenergetic proton beams extending to GeV energies can be produced with very high efficiency using circularly polarized light. The proton beams have a very small divergence angle (less than 4 degrees). This new method allows the construction of ultra-compact proton and ion accelerators with ultra-short particle bursts.

Selective enhancement (>10^3) of harmonics extending to the water window (~4nm) generated in an argon gas filled straight bore capillary waveguide is demonstrated. This enhancement is in good agreement with modeling which indicates that multimode quasi-phasematching (MMQPM) is achieved by rapid axial intensity modulations caused by beating between the fundamental and higher order capillary modes. Substantial pulse-energies (>10nJ per pulse per harmonic order) at wavelengths beyond the carbon K-edge (~4.37nm, ~284eV) up to ~360eV are observed from argon ions for the first time., Comment: 13 pages including 4 figures

A new scheme for quasi-phasematching high harmonic generation (HHG) in gases is proposed. In this, the rapid variation of the axial intensity resulting from excitation of more than one mode of a waveguide is used to achieve quasi phasematching. Numerical modeling demonstrates enhancement of the harmonic signal over that achieved for a single coherence length by factors >10^4., Comment: 6 pages including 3 figures