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With their incomparable time-frequency accuracy, frequency combs have significantly advanced precision spectroscopy, ultra-sensitive detection, and atomic clocks. Traditional methods to create photonic, phononic, and magnonic frequency combs hinge on material nonlinearities which are often weak, necessitating high power densities to surpass their initiation thresholds, which subsequently limits their applications. Here, we introduce a novel nonlinear process to efficiently generate magnonic frequency combs (MFCs) by exploiting exceptional points (EPs) in a coupled system comprising a pump-induced magnon mode and a Kittel mode. Even without any cavity, our method greatly improves the efficiency of nonlinear frequency conversion and achieves optimal MFCs at low pump power. Additionally, our novel nonlinear process enables excellent tunability of EPs using the polarization and power of the pump, simplifying MFC generation and manipulation. Our work establishes a synergistic relationship between non-Hermitian physics and MFCs, which is advantages for coherent/quantum information processing and ultra-sensitive detection., Comment: 7 pages, 4 figures

Angle-resolved second harmonic generation (SHG) spectra of ZnO microwires show characteristic Fano resonances in the spectral vicinity of exciton-polariton modes. The output SHG spectra after SHG interacting with exciton polariton shows a resonant enhancement peak accompanied by a suppression dip originating from the constructive and destructive interference respectively. It is demonstrated that the Fano line shape, and thus the Fano asymmetry parameter q, can be tuned by the phase-shift of the two channels. The phase-dependent q was calculated and the model describes our experimental results well. In particular, the phase-to-q relation unveil the crucial information about the dynamics of the system, e.g., defining the line shape of output SHG spectra in a superposition of quantum states.

We demonstrate the selective coupling of a single quantum dot exciton spin state with the cavity mode in a quantum dot-micropillar cavity system. By tuning an external magnetic field, the Zeeman splitted exciton spin states coupled differently with the cavity due to field manipulated energy detuning. We found a 26 times increase in the emission intensity of spin-up exciton state with respect to spin-down exciton state at resonance due to Purcell effect, which gives rise to the selective enhancement of light emission with the circular polarization degree up to 93%. A four-level rate equation model is developed and quantitatively agrees well with our experimental data. Our results pave the way for the realization of future quantum light sources and the quantum information processing applications., Comment: 11 pages, 4 figures

A cavity-polariton, formed due to the strong coupling between exciton and cavity mode, is one of the most promising composite bosons for realizing macroscopic spontaneous coherence at high temperature. Up to date, most of polariton quantum degeneracy experiments were conducted in the complicated two-dimensional (2D) planar microcavities. The role of dimensionality in coherent quantum degeneracy of a composite bosonic system of exciton polaritons remains mysterious. Here we report the first experimental observation of a one-dimensional (1D) polariton condensate in a ZnO microwire at room temperature. The massive occupation of the polariton ground state above a distinct pump power threshold is clearly demonstrated by using the angular resolved spectroscopy under non-resonant excitation. The power threshold is one order of magnitude lower than that of Mott transition. Furthermore, a well-defined far field emission pattern from the polariton condensate mode is observed, manifesting the coherence build-up in the condensed polariton system., Comment: 18 pages, 4 figures

Phonon damping is the main source of pure dephasing in the solid state, limiting many fundamental quantum effects to low temperature observations. Here we show how excitons in semiconductors can be totally decoupled from the phonon bath, even at room temperature, thanks to their strong interaction with photons. To do so, we investigated ZnO microwires, a new semiconductor nanostructure made of large band-gap material where the light can be trapped and guided into whispering gallery modes. In this system, the very large coupling regime between exciton and photon results in unusual exciton-polariton of one-dimensional character and Rabi splitting as large as 300meV. We find that polariton modes of excitonic fraction up to 75% exhibit no thermal broadening up to room temperature. We show that this remarkable behavior is due to the very large Rabi splitting as compared to the LO phonon energy., Comment: 17 pages, 3 figures

We report direct observation of the strong exciton-photon coupling in ZnO tapered whispering gallery (WG) microcavity at room temperature. By scanning excitations along the tapered arm of ZnO tetrapod using micro-photoluminescence spectrometer with different polarizations, we observed a transition from the pure WG optical modes in the weak interaction regime to the excitonic polariton in the strong coupling regime. The experimental observations are well described by using the plane wave model including excitonic polariton dispersion relation. This provides a direct mapping of the polariton dispersion, and thus a comprehensive picture for coupling of different excitons with differently polarized WG modes., Comment: 16 pages, 3 figures, 1 table