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The development of dispersion of nanoparticles in the W-1%Y$_2$O$_3$ and W-1%La$_2$O$_3$ (wt%) alloys processed by hot isostatic pressing has been investigated using small angle neutron scattering. The mode values of these centers are found at 10 and 40 nm in W-1%Y$_2$O$_3$, and 15 and 80 nm in W-1%La$_2$O$_3$. The scanning electron microscopy analyses showed the presence of small second phase particles. The contribution of the pore space to the scattering curves has been analyzed using the results obtained for pure W processed following the same procedure used for the alloys, and the porosity measurements of the samples., Comment: 4 pages, 4 figures, 2 tables, research article

We present the first fully differential next-to-next-to-leading order (NNLO) QCD calculation for the production of a top-antitop quark pair in association with a Higgs boson ($t \bar t H$) at hadron colliders. The computation is exact, except for the finite part of the two-loop virtual contribution, which we estimate using two different methods that yield consistent results within their respective uncertainties. The first method relies on a soft-Higgs factorisation formula that we develop up to the three-loop order. The second is based on a high-energy expansion in the small top-mass limit. Combining the newly computed corrections with the complete set of next-to-leading order (NLO) QCD+EW results provides the most advanced perturbative prediction currently available at the LHC for both inclusive and differential $t \bar t H$ cross sections. The uncertainties due to the missing exact two-loop contribution are conservatively estimated to be below the percent level, both for the total cross section and for most of the differential distributions, and therefore significantly smaller than the residual perturbative uncertainties., Comment: 36 pages, 6 figures, 2 tables

$FeCr_2S_4$ is a ferrimagnet with two oppositely-ordered spin sublattices (Fe and Cr), connected via superexchange interaction, giving a non-zero net magnetic moment. We show how the magnetic dynamics of the sublattices can be selectively manipulated by resonantly perturbing the Fe sublattice using ultrashort laser pulses. The mid-infrared excitation through intra-atomic Fe $d-d$ transitions triggers a markedly slower magneto-optical Kerr effect dynamics compared to an off-resonant pumping affecting both the two sublattices simultaneously. The analysis and conclusions are supported by probing resonantly and off-resonantly to the Fe sublattice., Comment: 29 pages, 19 figures

Materials with linear electronic dispersion often feature high carrier mobilities and unusually strong nonlinear optical interactions. In this work, we investigate the THz nonlinear dynamics of one such material, HgCdTe, with an electronic band dispersion heavily dependent on both temperature and stoichiometry. We show how the band gap, carrier concentration and band shape together determine the nonlinear response of the system. At low temperatures, carrier generation from Zener tunneling dominates the nonlinear response with a reduction in the overall transmission. At room temperature, quasi-ballistic electronic dynamics drive the largest observed nonlinear optical interactions, leading to a transmission increase. Our results demonstrate the sensitivity of these nonlinear optical properties of narrow-gap materials to small changes in the electronic dispersion and carrier concentration., Comment: 48 pages, 21 figures

Liquid crystal based technologies have found considerably diversified uses and areas of application over the last few decades, proving to be excellent materials for tunable optical elements from visible to near-infrared frequencies. Currently, much effort is devoted to demonstrating their applicability in the far-infrared or THz spectral frequency (1 - 10 THz), where tremendous advances have been achieved in terms of broadband and intense sources. Yet a detailed understanding of the dynamics triggered by THz light in liquid crystals is far from complete. In this work, we perform broadband THz Time Domain Spectroscopy on the low-frequency modes of 4-cyano-4'-alkylbiphenyl (nCB) and 5-phenylcyclohexanes (PCH5) across different mesophases. DFT calculations on isolated molecules capture the majority of the measured response above 3 THz. In particular, the pronounced modes around 4.5 and 5.5 THz mainly originate from in-plane and out-of-plane bending of the cyano group. In contrast, the broad response below 3 THz, linked to modes of the alkyl chain, disagrees with the single molecule calculation. Here, we identify a clear intermolecular character of the response, supported by dimer and trimer calculations., Comment: 14 pages, 4 figures

Resonant driving of electronic transitions with coherent laser sources creates quantum coherent superpositions of the involved electronic states. Most time-resolved studies have focused on gases or isolated subsystems embedded in insulating solids, aiming for applications in quantum information. Here, we demonstrate coherent control of orbital wavefunctions in pyrochlore $Tb_{2}Ti_{2}O_{7}$, which forms an interacting spin liquid ground state. We show that resonant excitation with a strong THz pulse creates a coherent superposition of the lowest energy Tb 4f states before the magnetic interactions eventually dephase them. The coherence manifests itself as a macroscopic oscillating magnetic dipole, which is detected by ultrafast resonant x-ray diffraction. The induced quantum coherence demonstrates coherent control of orbital wave functions, a new tool for the ultrafast manipulation and investigation of quantum materials.

We consider the class of inclusive hadron collider processes in which one or more energetic jets are produced, possibly accompanied by colourless particles. We provide a general formulation of a slicing scheme for this class of processes, by identifying the various contributions that need to be computed up to next-to-leading order (NLO) in QCD perturbation theory. We focus on two novel observables, the one-jet resolution variable $\Delta E_t$ and the $n$-jet resolution variable $k_{T}^{\mathrm{ness}}$, and explicitly compute all the ingredients needed to carry out NLO computations using these variables. We contrast the behaviour of these variables when the slicing parameter becomes small. In the case of $k_{T}^{\mathrm{ness}}$ we also present results for the hadroproduction of multiple jets., Comment: 47 pages, 3 figures. Minor modifications. Version published in JHEP

The production of a top-antitop quark pair in association with a $W$ boson ($t\bar tW$) is one of the heaviest signatures currently probed at the Large Hadron Collider (LHC). Since the first observation reported in 2015 the corresponding rates have been found to be consistently higher than the Standard Model predictions, which are based on next-to-leading order~(NLO) calculations in the QCD and electroweak (EW) interactions. We present the first next-to-next-to-leading order (NNLO) QCD computation of $t\bar tW$ production at hadron colliders. The calculation is exact, except for the finite part of the two-loop virtual corrections, which is estimated using two different approaches that lead to consistent results within their uncertainties. We combine the newly computed NNLO QCD corrections with the complete NLO QCD+EW results, thus obtaining the most advanced perturbative prediction available to date for the \ttW inclusive cross section. The tension with the latest ATLAS and CMS results remains at the $1\sigma-2\sigma$ level., Comment: 7 pages, 3 figures, 1 table. Minor changes, version published on PRL

Interactions between the different degrees of freedom form the basis of many manifestations of intriguing physics in condensed matter. In this respect, quantifying the dynamics of normal modes that themselves arise from these interactions and how they interact with other excitations is of central importance. Of the different types of coupling that are often important, spin-lattice coupling is relevant to several sub-fields of condensed matter physics; examples include spintronics, high-TC superconductivity, and topological materials. While theories of materials where spin-lattice coupling is relevant can sometimes be used to infer the magnitude and character of this interaction, experimental approaches that can directly measure it are rare and incomplete. Here we use time-resolved X-ray diffraction to directly access the spin-lattice coupling by measuring both ultrafast atomic motion and the associated spin dynamics following the excitation of a coherent electromagnon by an intense THz pulse in a multiferroic hexaferrite. Comparing the dynamics of the two different components, one striking outcome is the different phase shifts relative to the driving field. This phase shift provides insight into the excitation process of such a coupled mode. This direct observation of combined lattice and magnetization dynamics paves the way to access the mode-selective spin-lattice coupling strength, which remains a missing fundamental parameter for ultrafast control of magnetism and is relevant to a wide variety of correlated electron physics., Comment: 4 figures

We present the first calculation for the hadroproduction of a $W$ boson in association with a massive bottom ($b$) quark-antiquark pair at next-to-next-to-leading order (NNLO) in QCD perturbation theory. We exploit the hierarchy between the $b$ quark mass and the characteristic energy scale of the process to obtain a reliable analytic expression for the two-loop virtual amplitude with three massive legs, starting from the corresponding result available for massless bottom quarks. The use of massive $b$ quarks avoids the ambiguities associated with the correct flavour assignment in massless calculations, paving the way to a more realistic comparison with experimental data. We present phenomenological results considering proton-proton collisions at centre-of-mass energy $\sqrt{s}=13.6$ TeV for inclusive $Wb \bar b$ production and within a fiducial region relevant for the associated production of a $W$ boson and a Higgs boson decaying into a $b \bar b$ pair, for which $Wb \bar b$ production represents one of the most relevant backgrounds. We find that the NNLO corrections are substantial and that their inclusion is mandatory to obtain reliable predictions., Comment: 8 pages, 2 figures, 2 tables. Final version published in PRD

The associated production of a Higgs boson with a top-antitop quark pair is a crucial process at the LHC since it allows for a direct measurement of the top-quark Yukawa coupling. We present the computation of the radiative corrections to this process at the next-to-next-to-leading order (NNLO) in QCD perturbation theory. This is the very first computation for a $2 \to 3$ process with massive coloured particles at this perturbative order. We develop a soft Higgs boson approximation for loop amplitudes, which enables us to reliably quantify the impact of the yet unknown two-loop contribution. At the centre-of-mass energy $\sqrt{s}=13$ TeV the NNLO corrections increase the next-to-leading order result for the total cross section by about 4% and lead to a significant reduction of perturbative uncertainties., Comment: 8 pages, 2 tables, 1 figure. Version published on PRL

Using two-dimensional THz spectroscopy in combination with numerical models, we investigate the dynamics linked to carrier multiplication caused by high-field THz excitation of the low-gap semiconductor InSb. In addition to previously observed dynamics connected with quasi-ballistic carrier dynamics, we observe other spectral and temporal features that we attribute to impact ionization for peak fields above 60 kV/cm, which continue up to the maximum investigated peak field of 430 kV/cm. At the highest fields we estimate a carrier multiplication factor greater than 10 due to impact ionization, which is well-reproduced by a numerical simulation of the impact ionization process which we have developed., Comment: 25 pages, 5 figures

We report the coherent generation and detection of terahertz (THz) pulses covering the bandwidth of 0.1-9 THz in a high repetition rate, low pulse energy laser system. In this work we demonstrate the application and evaluation of solid-state biased coherent detection in combination with a spintronic emitter. This combination was used to generate and detect THz pulses in a time-domain spectroscopy (TDS) setup and tested on bulk nonlinear crystals. These results establish a new promising candidate to extend the possibilities for compact, broadband THz TDS systems driven by high repetition rate lasers.

We consider the class of inclusive hadron collider processes in which several energetic jets are produced, possibly accompanied by colourless particles (such as Higgs boson(s), vector boson(s) with their leptonic decays, and so forth). We propose a new variable that smoothly captures the $N+1$ to $N$-jet transition. This variable, that we dub $k_T^{\rm ness}$, represents an effective transverse momentum controlling the singularities of the $N+1$-jet cross section when the additional jet is unresolved. The $k_T^{\rm ness}$ variable offers novel opportunities to perform higher-order calculations in Quantum Chromodynamics (QCD) by using non-local subtraction schemes. We study the singular behavior of the $N+1$-jet cross section as $k_T^{\rm ness}\to 0$ and, as a phenomenological application, we use the ensuing results to evaluate next-to-leading order corrections to $H$+jet and $Z$+2 jet production at the LHC. We show that $k_T^{\rm ness}$ performs extremely well as a resolution variable and appears to be very stable with respect to hadronization and multiple-parton interactions., Comment: 9 pages, 3 figures. Added appendix with details on jet and soft functions at NLO. Version published in Phys.Rev.D

We use time-resolved hard x-ray diffraction to investigate the structural dynamics of the multiferroic insulator TbMnO$_3$ in the low temperature antiferromagnetic and ferroelectrically ordered phase. The lattice response following photoexcitation at 1.55 eV is detected by measuring the (0 2 4) and (1 3 -5) Bragg reflections. A 0.02% tensile strain, normal to the surface, is seen to arise within 20 - 30 ps. The magnitude of this transient strain is over an order of magnitude lower than that predicted from laser-induced heating, which we attribute to a bottleneck in the energy transfer between the electronic and lattice subsystems. The timescale for the transient expansion is consistent with that of previously reported demagnetization dynamics. We discuss a possible relationship between structural and demagnetization dynamics in TbMnO$_3$, in which photoinduced atomic motion modulates the exchange interaction, leading to a destruction of the magnetic order in the system., Comment: 3 figures, 4 footnotes

Understanding ultrafast magnetization dynamics on the microscopic level is of strong current interest due to the potential for applications in information storage. In recent years, the spin-lattice coupling has been recognized to be essential for ultrafast magnetization dynamics. Magnetoelectric multiferroics of type II possess intrinsic correlations among magnetic sublattices and electric polarization (P) through spin-lattice coupling, enabling fundamentally coupled dynamics between spins and lattice. Here we report on ultrafast magnetization dynamics in a room-temperature multiferroic hexaferrite possessing ferrimagnetic and antiferromagnetic sublattices, revealed by time-resolved resonant x-ray diffraction. A femtosecond above-bandgap excitation triggers a coherent magnon in which the two magnetic sublattices entangle and give rise to a transient modulation of P. A novel microscopic mechanism for triggering the coherent magnon in this ferrimagnetic insulator based on the spin-lattice coupling is proposed. Our finding opens up a novel but general pathway for ultrafast control of magnetism., Comment: 18 pages, 7 figures + 21 pages supplementary information

Nonlinear electron kinetic structures are regularly observed in space and experimental magnetized plasmas, called electron phase-space holes (EHs). The existence of EHs is conditioned and varies according to the ambient magnetic field and the parameters of the electron beam(s) that may generate them. The objective of this paper is to extend the 3D Bernstein-Greene-Kruskal (BGK) model with cylindrical geometry developed by Chen et al. (2004,2004) to include simultaneously finite effects due to (i) the strength of the ambient magnetic field $\vec{B}_0$, by modifying the Poisson equation with a term derived from the electron polarization current, and (ii) the drift velocity $\vec{u}_e$ of the background plasma electrons with respect to the EH, by considering velocity-shifted Maxwellian distributions for the boundary conditions. This allows us to more realistically determine the distributions of trapped and passing particles forming the EHs, as well as the width-amplitude relationships for their existence., Comment: Submitted to Physics of Plasma Journal on October, 15th 2023

We consider the hadroproduction of a massive charged lepton plus the corresponding neutrino through the Drell-Yan mechanism. We present a new computation of the mixed QCD-EW corrections to this process. The cancellation of soft and collinear singularities is achieved by using a formulation of the $q_T$ subtraction formalism derived from the next-to-next-to-leading order QCD calculation for heavy-quark production. For the first time, all the real and virtual contributions due to initial- and final-state radiation are consistently included without any approximation, except for the finite part of the two-loop virtual correction, which is computed in the pole approximation and suitably improved through a reweighting procedure. We demonstrate that our calculation is reliable in both on-shell and off-shell regions, thereby providing the first prediction of the mixed QCD-EW corrections in the entire region of the lepton transverse momentum. The computed corrections are in qualitative agreement with what we obtain in a factorised approach of QCD and EW corrections. At large values of the lepton $p_T$, the mixed QCD-EW corrections are negative and increase in size, to about $-20\%$ with respect to the next-to-leading order QCD result at $p_T=500\,$GeV., Comment: 18 pages, 4 figures, 1 table, v2: extended version of the manuscript that has been accepted for publication by PRD (one extra figure on systematic uncertainties, updated table of cross sections)

The interaction of many-body systems with intense light pulses may lead to novel emergent phenomena far from equilibrium. Recent discoveries, such as the optical enhancement of the critical temperature in certain superconductors and the photo-stabilization of hidden phases, have turned this field into an important research frontier. Here, we demonstrate nonthermal charge-density-wave (CDW) order at electronic temperatures far greater than the thermodynamic transition temperature. Using time- and angle-resolved photoemission spectroscopy and time-resolved X-ray diffraction, we investigate the electronic and structural order parameters of an ultrafast photoinduced CDW-to-metal transition. Tracking the dynamical CDW recovery as a function of electronic temperature reveals a behaviour markedly different from equilibrium, which we attribute to the suppression of lattice fluctuations in the transient nonthermal phonon distribution. A complete description of the system's coherent and incoherent order-parameter dynamics is given by a time-dependent Ginzburg-Landau framework, providing access to the transient potential energy surfaces., Comment: 23 pages, 14 figures

In ionic Raman scattering, infrared-active phonons mediate a scattering process that results in the creation or destruction of a Raman-active phonon. This mechanism relies on nonlinear interactions between phonons and has in recent years been associated with a variety of emergent lattice-driven phenomena in complex transition-metal oxides, but the underlying mechanism is often obscured by the presence of multiple coupled order parameters in play. Here, we use time-resolved spectroscopy to compare coherent phonons generated by ionic Raman scattering with those created by more conventional electronic Raman scattering on the nonmagnetic and non-strongly-correlated wide band-gap insulator LaAlO$_3$. We find that the oscillatory amplitude of the low-frequency Raman-active $E_g$ mode exhibits a sharp peak when we tune our pump frequency into resonance with the high-frequency infrared-active $E_u$ mode, consistent with first-principles calculations. Our results suggest that ionic Raman scattering can strongly dominate electronic Raman scattering in wide band-gap insulating materials. We also see evidence of competing scattering channels at fluences above 28~mJ/cm$^2$ that alter the measured amplitude of the coherent phonon response., Comment: 10 pages, 6 figures

The general idea of using ultrashort light pulses to control ferroic order parameters has recently attracted attention as a means to achieve control over material properties on unprecedented time scales. Much of the challenge in such work is in understanding the mechanisms by which this control can be achieved, and in particular how observables can be connected to structural and electronic properties. Here we report on a combination of experimental and computational methods to study the electronic structure of the semiconducting ferroelectric GeTe when driven out of equilibrium by absorption of a femtosecond pulse of light. We observe coherent modulations of second harmonic generations on the order of 50%, which we attribute to a combination of atomic and electronic structure changes due to a coherently excited soft mode. Comparison of the observed experimental data with model calculations indicates that this effect is predominantly due to an ultrafast modulation of the covalency of the bonding between Ge and Te ions. This stands in contrast to previously held assumptions in other systems, indicating that care should be exercised in using indirect measurements of electronic structure to make strong conclusions about the magnitude of nuclear motions.

Femtosecond time-resolved x-ray diffraction is employed to study the dynamics of the periodic lattice distortion (PLD) associated with the charge-density-wave (CDW) in K0.3MoO3. Using a multi-pulse scheme we show the ability to extend the lifetime of coherent oscillations of the PLD about the undistorted structure through re-excitation of the electronic states. This suggests that it is possible to enter a regime where the symmetry of the potential energy landscape corresponds to the high symmetry phase but the scattering pathways that lead to the damping of coherent dynamics are still controllable by altering the electronic state population. The demonstrated control over the coherence time offers new routes for manipulation of coherent lattice states., Comment: 18 pages, 5 figures, including supplementary information

Using reflective cross-polarized 2D THz time-domain spectroscopy in the range of 1-12 THz, we follow the trajectory of the out-of-equilibrium electron population in the low-bandgap semiconductor InSb. The 2D THz spectra show a set of distinct features at combinations of the plasma-edge and vibration frequencies. Using finite difference time domain simulations combined with a tight binding model of the band structure, we assign these features to electronic nonlinearities and show that the nonlinear response in the first picoseconds is dominated by coherent ballistic motion of the electrons. We demonstrate that this technique can be used to investigate the landscape of the band curvature near the Gamma-point as illustrated by the observation of anisotropy in the (100)-plane.

Sub-picosecond magnetisation manipulation via femtosecond optical pumping has attracted wide attention ever since its original discovery in 1996. However, the spatial evolution of the magnetisation is not yet well understood, in part due to the difficulty in experimentally probing such rapid dynamics. Here, we find evidence of rapid magnetic order recovery in materials with perpendicular magnetic anisotropy via nonlinear magnon processes. We identify both localisation and coalescence regimes, whereby localised magnetic textures nucleate and subsequently evolve in accordance with a power law formalism. Coalescence is observed for optical excitations both above and below the switching threshold. Simulations indicate that the ultrafast generation of noncollinear magnetisation via optical pumping establishes exchange-mediated spin currents with an equivalent 100% spin polarised charge current density of $10^8$ A/cm$^2$. Such large spin currents precipitate rapid recovery of magnetic order after optical pumping. These processes suggest an ultrafast optical route for the stabilization of desired meta-stable states, e.g., isolated skyrmions.

The ultrafast dynamics of the octahedral rotation in Ca:SrTiO3 is studied by time resolved x-ray diffraction after photo excitation over the band gap. By monitoring the diffraction intensity of a superlattice reflection that is directly related to the structural order parameter of the soft-mode driven antiferrodistortive phase in Ca:SrTiO3, we observe a ultrafast relaxation on a 0.2 ps timescale of the rotation of the oxygen octahedron, which is found to be independent of the initial temperaure despite large changes in the corresponding soft-mode frequency. A further, much smaller reduction on a slower picosecond timescale is attributed to thermal effects. Time-dependent density-functional-theory calculations show that the fast response can be ascribed to an ultrafast displacive modification of the soft-mode potential towards the normal state, induced by holes created in the oxygen 2p states.

The original observation of the Einstein-de Haas effect was a landmark experiment in the early history of modern physics that illustrates the relationship between magnetism and angular momentum. Today the effect is still discussed in elementary physics courses to demonstrate that the angular momentum associated with the aligned electron spins in a ferromagnet can be converted to mechanical angular momentum by reversing the direction of magnetisation using an external magnetic field. In recent times, a related problem in magnetism concerns the time-scale over which this angular momentum transfer can occur. It is known experimentally for several metallic ferromagnets that intense photoexcitation leads to a drop in the magnetisation on a time scale shorter than 100 fs, a phenomenon called ultrafast demagnetisation. The microscopic mechanism for this process has been hotly debated, with one key question still unanswered: where does the angular momentum go on these sub-picosecond time scales? Here we show using femtosecond time-resolved x-ray diffraction that a large fraction of the angular momentum lost from the spin system on the laserinduced demagnetisation of ferromagnetic iron is transferred to the lattice on sub-picosecond timescales, manifesting as a transverse strain wave that propagates from the surface into the bulk. By fitting a simple model of the x-ray data to simulations and optical data, we roughly estimate that the angular momentum occurs on a time scale of 200 fs and corresponds to 80% of the angular momentum lost from the spin system. Our results show that interaction with the lattice plays an essential role in the process of ultrafast demagnetisation in this system., Comment: 39 pages, 2 tables, 7 figures

We use femtosecond x-ray diffraction to study the structural response of charge and orbitally ordered Pr$_{1-x}$Ca$_x$MnO$_3$ thin films across a phase transition induced by 800 nm laser pulses. By investigating the dynamics of both superlattice reflections and regular Bragg peaks, we disentangle the different structural contributions and analyze their relevant time-scales. The dynamics of the structural and charge order response are qualitatively different when excited above and below a critical fluence $f_c$. For excitations below $f_c$ the charge order and the superlattice is only partially suppressed and the ground state recovers within a few tens of nanosecond via diffusive cooling. When exciting above the critical fluence the superlattice vanishes within approximately half a picosecond followed by a change of the unit cell parameters on a 10 picoseconds time-scale. At this point all memory from the symmetry breaking is lost and the recovery time increases by many order of magnitudes due to the first order character of the structural phase transition.

Recent experiments have shown that the high temperature incommensurate (I) charge density wave (CDW) phase of 1T-TaS2 can be photoinduced from the lower temperature, nearly commensurate (NC) CDW state. Here we report a time-resolved x-ray diffraction study of the growth process of the photoinduced I-CDW domains. The layered nature of the material results in a marked anisotropy in the size of the photoinduced domains of the I-phase. These are found to grow self-similarly, their shape remaining unchanged throughout the growth process. The photoinduced dynamics of the newly formed I-CDW phase was probed at various stages of the growth process using a double pump scheme, where a first pump creates I-CDW domains and a second pump excites the newly formed I-CDW state. We observe larger magnitudes of the coherently excited I-CDW amplitude mode in smaller domains, which suggests that the incommensurate lattice distortion is less stable for smaller domain sizes., Comment: 8 pages, 8 figures

The Prototypical magnetic memory shape alloy Ni$_2$MnGa undergoes various phase transitions as a function of temperature, pressure, and doping. In the low-temperature phases below 260 K, an incommensurate structural modulation occurs along the [110] direction which is thought to arise from softening of a phonon mode. It is not at present clear how this phenomenon is related, if at all, to the magnetic memory effect. Here we report time-resolved measurements which track both the structural and magnetic components of the phase transition from the modulated cubic phase as it is brought into the high-symmetry phase. The results suggest that the photoinduced demagnetization modifies the Fermi surface in regions that couple strongly to the periodicity of the structural modulation through the nesting vector. The amplitude of the periodic lattice distortion, however, appears to be less affected by the demagnetizaton., Comment: 7 pages, 4 figures

Femtosecond time-resolved X-ray diffraction is used to study a photo-induced phase transition between two charge density wave (CDW) states in 1T-TaS$_2$, namely the nearly commensurate (NC) and the incommensurate (I) CDW states. Structural modulations associated with the NC-CDW order are found to disappear within 400 fs. The photo-induced I-CDW phase then develops through a nucleation/growth process which ends 100 ps after laser excitation. We demonstrate that the newly formed I-CDW phase is fragmented into several nanometric domains that are growing through a coarsening process. The coarsening dynamics is found to follow the universal Lifshitz-Allen-Cahn growth law, which describes the ordering kinetics in systems exhibiting a non-conservative order parameter., Comment: 6 pages, 5 figures

Light-matter interaction at the nanoscale in magnetic materials is a topic of intense research in view of potential applications in next-generation high-density magnetic recording. Laser-assisted switching provides a pathway for overcoming the material constraints of high-anisotropy and high-packing density media, though much about the dynamics of the switching process remains unexplored. We use ultrafast small-angle x-ray scattering at an x-ray free-electron laser to probe the magnetic switching dynamics of FePt nanoparticles embedded in a carbon matrix following excitation by an optical femtosecond laser pulse. We observe that the combination of laser excitation and applied static magnetic field, one order of magnitude smaller than the coercive field, can overcome the magnetic anisotropy barrier between "up" and "down" magnetization, enabling magnetization switching. This magnetic switching is found to be inhomogeneous throughout the material, with some individual FePt nanoparticles neither switching nor demagnetizing. The origin of this behavior is identified as the near-field modification of the incident laser radiation around FePt nanoparticles. The fraction of not-switching nanoparticles is influenced by the heat flow between FePt and a heat-sink layer.

Using photo-emission electron microscopy with X-ray magnetic circular dichroism as a contrast mechanism, new insights into the all-optical magnetization switching (AOS) phenomenon in GdFe based rare-earth transition metal ferrimagnetic alloys are provided. From a sequence of static images taken after single linearly polarized laser pulse excitation, the repeatability of AOS can be measured with a correlation coefficient. It is found that low coercivity enables thermally activated domain wall motion, limiting in turn the repeatability of the switching. Time-resolved measurement of the magnetization dynamics reveal that while AOS occurs below and above the magnetization compensation temperature $T_\text{M}$, it is not observed in GdFe samples where $T_\text{M}$ is absent. Finally, AOS is experimentally demonstrated against an applied magnetic field of up to 180 mT., Comment: 18 pages, 4 figures

All-optical switching (AOS) of magnetic domains by femtosecond laser pulses was first observed in the transition metal-rare earth (TM-RE) alloy GdFeCo1-5; this phenomenon demonstrated the potential for optical control of magnetism for the development of ever faster future magnetic recording technologies. The technological potential of AOS has recently increased due to the discovery of the same effect in other materials, including RE-free magnetic multilayers6,7. However, to be technologically meaningful, AOS must compete with the bit densities of conventional storage devices, restricting optically-switched magnetic areas to sizes well below the diffraction limit. Here, we demonstrate reproducible and robust all-optical switching of magnetic domains of 53 nm size in a ferrimagnetic TbFeCo alloy using gold plasmonic antenna structures. The confined nanoscale magnetic reversal is imaged around and beneath plasmonic antennas using x-ray resonant holographic imaging. Our results demonstrate the potential of future AOS-based magnetic recording technologies., Comment: 15 pages (including Supplementary Materials)

The recently discovered magnetization reversal driven solely by a femtosecond laser pulse has been shown to be a promising way to record information at record breaking speeds. Seeking to improve the recording density has raised intriguing fundamental question about the feasibility to combine the ultrafast temporal with sub-wavelength spatial resolution of magnetic recording. Here we report about the first experimental demonstration of sub-diffraction and sub-100 ps all-optical magnetic switching. Using computational methods we reveal the feasibility of sub-diffraction magnetic switching even for an unfocused incoming laser pulse. This effect is achieved via structuring the sample such that the laser pulse experiences a passive wavefront shaping as it couples and propagates inside the magnetic structure. Time-resolved studies with the help of photo-emission electron microscopy clearly reveal that the sub-wavelength switching with the help of the passive wave-front shaping can be pushed into sub-100 ps regime.

We report the creation and real-space observation of magnetic structures with well-defined topological properties and a lateral size as low as about 150 nm. They are generated in a thin ferrimagnetic film by ultrashort single optical laser pulses. Thanks to their topological properties, such structures can be classified as Skyrmions of a particular type that does not require an externally applied magnetic field for stabilization. Besides Skyrmions, we are able to generate magnetic features with topological characteristics that can be tuned by changing the laser fluence. The stability of such features is accounted for by an analytical model based on the interplay between the exchange and the magnetic dipole-dipole interactions, Comment: 8 pages, 3 figures

Employing plasmonic antennas for subdiffraction focusing of light on recording media requires to take into account the complete structure of the medium, including dielectric cover layers. We find, with finite difference time domain simulations, that optical energy transfer to the magnetic recording layer is most efficient for an off-resonant antenna. Furthermore, we show that the focal spot in the magnetic film is well below the diffraction limit, making nanoscale all-optical magnetic data recording achievable., Comment: 11 pages, 4 figures

By exploiting photo-induced reorientation in azo-polymer thin films, we demonstrate all-optical polarization-encoded information storage with a scanning near-field optical microscope. In the writing routine, 5-level bits are created by associating different bit values to different birefringence directions, induced in the polymer after illumination with linearly polarized light. The reading routine is then performed by implementing polarization-modulation techniques on the same near-field microscope, in order to measure the encoded birefringence direction., Comment: 13 pages, 5 figures