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Spin transport through magnetic insulators has been demonstrated in a variety of materials and is an emerging pathway for next-generation spin-based computing. To modulate spin transport in these systems, one typically applies a sufficiently strong magnetic field to allow for deterministic control of magnetic order. Here, we make use of the well-known multiferroic magnetoelectric, BiFeO3, to demonstrate non-volatile, hysteretic, electric-field control of thermally excited magnon current in the absence of an applied magnetic field. These findings are an important step toward magnon-based devices, where electric-field-only control is highly desirable., Comment: 34 pages, 4 figures, 9 supplemental figures

In condensed-matter systems, competition between ground states at phase boundaries can lead to significant changes in material properties under external stimuli, particularly when these ground states have different crystal symmetries. A key scientific and technological challenge is to stabilize and control coexistence of symmetry-distinct phases with external stimuli. Using BiFeO3 (BFO) layers confined between layers of the dielectric TbScO3 as a model system, we stabilize the mixed-phase coexistence of centrosymmetric and non-centrosymmetric BFO phases with antipolar, insulating and polar, semiconducting behavior, respectively at room temperature. Application of in-plane electric (polar) fields can both remove and introduce centrosymmetry from the system resulting in reversible, nonvolatile interconversion between the two phases. This interconversion between the centrosymmetric insulating and non-centrosymmetric semiconducting phases coincides with simultaneous changes in the non-linear optical response of over three orders of magnitude, a change in resistivity of over five orders of magnitude, and a change in the polar order. Our work establishes a materials platform allowing for novel cross-functional devices which take advantage of changes in optical, electrical, and ferroic responses., Comment: L Caretta and Y-T Shao contributed equally. 64 pages, 4 figures, 25 supplemental figures, 1 supplemental table

A qubit sensor with an electric dipole moment acquires an additional contribution to its depolarization rate when it is placed in the vicinity of a polar or dielectric material as a consequence of electrical noise arising from polarization fluctuations in the material. Here, we characterize this relaxation rate as a function of experimentally tunable parameters such as sample-probe distance, probe-frequency, and temperature, and demonstrate that it offers a window into dielectric properties of insulating materials over a wide range of frequencies and length scales. We discuss the experimental feasibility of our proposal and illustrate its ability to probe a variety of phenomena, ranging from collective polar excitations to phase transitions and disorder-dominated physics in relaxor ferroelectrics. Our proposal paves the way for a novel table-top probe of polar and dielectric materials in a parameter regime complementary to existing tools and techniques., Comment: 5 + 2 + 15 pages; 2 figures