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A seamless chip-to-world photonic interface enables wide-ranging advancements in optical ranging, display, communication, computation, imaging, and light-matter interaction. An optimal solution allows for 2D scanning of a diffraction-limited beam from anywhere on a photonic chip over a large number of beam-spots in free-space. Currently, devices with direct PIC integration rely on tiled apertures with poor mode qualities, large footprints, and complex control systems. Micro-mechanical beam scanners have good beam quality but lack direct PIC integration and are inertially-limited due to the use of bulk optical components or structures in which the optical aperture and actuator sizes are inextricably linked, resulting in trade-offs among resolution, speed, and footprint. Here, we overcome these limitations with the photonic "ski-jump": a nanoscale optical waveguide monolithically integrated atop a piezoelectrically actuated cantilever which passively curls ~90$^{\circ}$ out-of-plane in a footprint of <0.1 mm$^{2}$, emits sub-micron diffraction-limited optical modes, and exhibits kHz-rate mechanical resonances with quality factors exceeding 10,000. This enables two-dimensional beam-scanning with footprint-adjusted spot-rates of 68.6 mega-spots/(s$\cdot$mm$^{2}$) at CMOS-level voltages, which is equivalent to a 1 megapixel display at 100 Hz from a 1.5 mm$^{2}$ footprint, and exceeds the performance of state-of-the-art MEMS mirrors by >50$\times$. Using this device, we demonstrate image projection, video projection, and the initialization and readout of single photons from silicon vacancy centers in diamond waveguides. Based on current performance, we identify pathways for achieving >1 giga-spots at kHz-rates in a ~1 cm$^{2}$ area to provide a seamless, scalable optical pipeline between integrated photonic processors and the free-space world., Comment: 12 pages main text, 1 page methods, 10 pages supplementary information

Programmable photonic integrated circuits (PICs) are emerging as powerful tools for the precise manipulation of light, with applications in quantum information processing, optical range finding, and artificial intelligence. The leading architecture for programmable PICs is the mesh of Mach-Zehnder interferometers (MZIs) embedded with reconfigurable optical phase shifters. Low-power implementations of these PICs involve micromechanical structures driven capacitively or piezoelectrically but are limited in modulation bandwidth by mechanical resonances and high operating voltages. However, circuits designed to operate exclusively at these mechanical resonances would reduce the necessary driving voltage from resonantly enhanced modulation as well as maintaining high actuation speeds. Here we introduce a synchronous, micromechanically resonant design architecture for programmable PICs, which exploits micromechanical eigenmodes for modulation enhancement. This approach combines high-frequency mechanical resonances and optically broadband phase shifters to increase the modulation response on the order of the mechanical quality factor $Q_m$, thereby reducing the PIC's power consumption, voltage-loss product, and footprint. The architecture is useful for broadly applicable circuits such as optical phased arrays, $1$ x $N$, and $N$ x $N$ photonic switches. We report a proof-of-principle programmable 1 x 8 switch with piezoelectric phase shifters at specifically targeted mechanical eigenfrequencies, showing a full switching cycle of all eight channels spaced by approximately 11 ns and operating at >3x average modulation enhancement across all on-chip modulators. By further leveraging micromechanical devices with high $Q_m$, which can exceed 1 million, our design architecture should enable a new class of low-voltage and high-speed programmable PICs., Comment: 18 pages, 5 figures, 5 supplementary figures

A central goal in creating long-distance quantum networks and distributed quantum computing is the development of interconnected and individually controlled qubit nodes. Atom-like emitters in diamond have emerged as a leading system for optically networked quantum memories, motivating the development of visible-spectrum, multi-channel photonic integrated circuit (PIC) systems for scalable atom control. However, it has remained an open challenge to realize optical programmability with a qubit layer that can achieve high optical detection probability over many optical channels. Here, we address this problem by introducing a modular architecture of piezoelectrically-actuated atom-control PICs (APICs) and artificial atoms embedded in diamond nanostructures designed for high-efficiency free-space collection. The high-speed 4-channel APIC is based on a splitting tree mesh with triple-phase shifter Mach-Zehnder interferometers. This design simultaneously achieves optically broadband operation at visible wavelengths, high-fidelity switching ($> 40$ dB) at low voltages, sub-$\mu$s modulation timescales ($> 30$ MHz), and minimal channel-to-channel crosstalk for repeatable optical pulse carving. Via a reconfigurable free-space interconnect, we use the APIC to address single silicon vacancy color centers in individual diamond waveguides with inverse tapered couplers, achieving efficient single photon detection probabilities (15$\%$) and second-order autocorrelation measurements $g^{(2)}(0) < 0.14$ for all channels. The modularity of this distributed APIC - quantum memory system simplifies the quantum control problem, potentially enabling further scaling to 1000s of channels.

Large-scale generation of quantum entanglement between individually controllable qubits is at the core of quantum computing, communications, and sensing. Modular architectures of remotely-connected quantum technologies have been proposed for a variety of physical qubits, with demonstrations reported in atomic and all-photonic systems. However, an open challenge in these architectures lies in constructing high-speed and high-fidelity reconfigurable photonic networks for optically-heralded entanglement among target qubits. Here we introduce a programmable photonic integrated circuit (PIC), realized in a piezo-actuated silicon nitride (SiN)-in-oxide CMOS-compatible process, that implements an N x N Mach-Zehnder mesh (MZM) capable of high-speed execution of linear optical transformations. The visible-spectrum photonic integrated mesh is programmed to generate optical connectivity on up to N = 8 inputs for a range of optically-heralded entanglement protocols. In particular, we experimentally demonstrated optical connections between 16 independent pairwise mode couplings through the MZM, with optical transformation fidelities averaging 0.991 +/- 0.0063. The PIC's reconfigurable optical connectivity suffices for the production of 8-qubit resource states as building blocks of larger topological cluster states for quantum computing. Our programmable PIC platform enables the fast and scalable optical switching technology necessary for network-based quantum information processors., Comment: 21 pages, 4 figures, 6 supplementary figures

The plasmon resonance of a structure is primarily dictated by its optical properties and geometry, which can be modified to enable hot-carrier photodetectors with superior performance. Recently, metal-alloys have played a prominent role in tuning the resonance of plasmonic structures through chemical composition engineering. However, it has been unclear how alloying modifies the time dynamics of generated hot-carriers. In this work, we elucidate the role of chemical composition on the relaxation time of hot-carriers for the archetypal Aux Ag1-x thin-film system. Through time-resolved optical spectroscopy measurements in the visible wavelength range, we measure composition-dependent relaxation times that vary up to 8x for constant pump fluency. Surprisingly, we find that the addition of 2% of Ag into Au films can increase the hot carrier lifetime by approximately 35% under fixed fluence, as a result of a decrease in optical loss. Further, the relaxation time is found to be inversely proportional to the imaginary part of the permittivity. Our results indicate that alloying is a promising approach to effectively control hot-carrier relaxation time in metals.

Metal hydrides often display dramatic changes in optical properties upon hydrogenation. These shifts make them prime candidates for many tunable optical devices, such as optical hydrogen sensors and switchable mirrors. While some of these metals, such as palladium, have been well studied, many other promising materials have only been characterized over a limited optical range and lack direct in situ measurements of hydrogen loading, limiting their potential applications. Further, there have been no systematic studies that allow for a clear comparison between these metals. In this work, we present such a systematic study of the dynamically tunable optical properties of Pd, Mg, Zr, Ti, and V throughout hydrogenation with a wavelength range of 250 - 1690 nm. These measurements were performed in an environmental chamber, which combines mass measurements via a quartz crystal microbalance with ellipsometric measurements in up to 7 bar of hydrogen gas, allowing us to determine the optical properties during hydrogen loading. In addition, we demonstrate a further tunability of the optical properties of titanium and its hydride by altering annealing conditions, and we investigate the optical and gravimetric hysteresis that occurs during hydrogenation cycling of palladium. Finally, we demonstrate several nanoscale optical and plasmonic structures based on these dynamic properties. We show structures that, upon hydrogenation, demonstrate five orders of magnitude change in reflectivity, resonance shifts of >200 nm, and relative transmission switching of >3000%, suggesting a wide range of applications.

In atomic force microscopy (AFM), the angle relative to the vertical ($\theta_{i}$) that the tip apex of a cantilever moves is determined by the tilt of the probe holder and the geometries of the cantilever and actuated eigenmode $i$. Even though the effects of $\theta_{i}$ on static and single-frequency AFM are known (increased effective spring constant, sensitivity to sample anisotropy, etc), the higher eigenmodes used in multifrequency force microscopy lead to additional effects that have not been fully explored. Here we use Kelvin probe force microscopy (KPFM) to investigate how $\theta_{i}$ affects not only the signal amplitude and phase, but can also lead to behaviors such as destabilization of the KPFM voltage feedback loop. We find that longer cantilevers and modified sample orientations improve voltage feedback loop stability, even though variations to scanning parameters such as cantilever shake amplitude and lift height do not., Comment: 5 pages of text, 5 figures. Revision replaces discussion of bimodal AFM with more discussion of experimental results