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Coherent dispersive wave emission, as an important phenomenon of soliton dynamics, manifests itself in multiple platforms of nonlinear optics from fibre waveguides to integrated photonics. Limited by its resonance nature, efficient generation of coherent dispersive wave with ultra-broad bandwidth has, however, proved difficult to realize. Here, we unveil a new regime of soliton dynamics in which the dispersive wave emission process strongly couples with the splitting dynamics of the driving pulse. High-order dispersion and self-steepening effects, accumulated over soliton self-compression, break the system symmetry, giving rise to high-efficiency generation of coherent dispersive wave in the ultraviolet region. Simultaneously, asymmetric soliton splitting results in the appearance of a temporally-delayed ultrashort pulse with high intensity, overlapping and copropagating with the dispersive wave pulse. Intense cross-phase modulations lead to octave-wide broadening of the dispersive wave spectrum, covering 200 to 400 nm wavelengths. The highly-coherent, octave-wide ultraviolet spectrum, generated from the simple capillary fibre set-up, is in great demand for time-resolved spectroscopy, ultrafast electron microscopy and frequency metrology applications, and the critical role of the secondary pulse in this process reveals some new opportunities for all-optical control of versatile soliton dynamics.

We studied the underlying mechanism of broadband dispersive-wave emission within a resonance band of gas-filled anti-resonant hollow-core fiber. Both theoretical and experimental results unveiled that the high-order soliton, launched into the hollow-core fiber, experienced two stages of pulse compression, resulting in a multi-peak structure of the dispersive-wave spectrum. Over the first-stage pulse compression, a sharp increase of the pulse peak power triggered the first time of dispersion-wave emission, and simultaneously caused ionization of the noble gas filled in the fiber core. Strong soliton-plasma interactions led to blue shifting of the pump pulse, and the blue-shifted pulse experienced a decreasing dispersion value in the fiber waveguide, resulting in an increase of its soliton order. Then, the second-stage pulse compression due to the high-order soliton effect triggered the second time of dispersive-wave emission at a phase-matched frequency slightly lower than that in the first stage. Multi-peak spectra of the output dispersive-waves and their formation dynamics were clearly observed in our experiments, which can be understood using a delicate coupling mechanism among three nonlinear effects including high-order-soliton compression, soliton-plasma interaction and phase-matched dispersive-wave emission. The output broadband dispersive-wave could be potentially compressed to sub-30 fs duration using precise chirp-compensation technique.

Femtosecond light pulses carrying optical angular momentums (OAMs), possessing intriguing properties of helical phase fronts and ultrafast temporal profiles, enable many applications in nonlinear optics, strong-field physics and laser micro-machining. While generation of OAM-carrying ultrafast pulses and their interactions with matters have been intensively studied in experiments, three-dimensional characterization of ultrafast OAM-carrying light beams in spatio-temporal domain has, however, proved difficult to achieve. Conventional measurement schemes rely on the use of a reference pulsed light beam which needs to be well-characterized in its phase front and to have sufficient overlap and coherence with the beam under test, largely limiting practical applications of these schemes. Here we demonstrate a self-referencing set-up based on a tilted interferometer that can be used to measure complete spatio-temporal information of OAM-carrying femtosecond pulses with different topological charges. Through scanning one interferometer arm, the spectral phase over the pulse spatial profile can be obtained using the tilted interference signal, and the temporal envelope of the light field at one particular position around its phase singularity can be retrieved simultaneously, enabling three-dimensional beam reconstruction. This self-referencing technique, capable of measuring spatio-temporal ultrafast optical-vortex beams, may find many applications in fields of nonlinear optics and light-matter interactions.

High-energy ultraviolet pulse generation in gas-filled hollow capillary fibers (HCFs) through dispersive-wave-emission process, has attracted considerable attentions in recent several years due to its great application potentials in ultraviolet spectroscopy and photochemistry. While the ability of this technique to deliver high-energy, ultrafast ultraviolet pulses is widely recognized, few-fs duration of {\mu}J-level dispersive-wave (DW) pulses has, however, escaped direct measurements. In this letter, we demonstrate that using several chirped mirrors, few-fs ultraviolet DW pulses can be obtained in atmosphere environment without the use of vacuum chambers. The pulse temporal profiles, measured using a self-diffraction frequency-resolved optical gating set-up, exhibit full-width-half-maximum pulse widths of 9.6 fs at 384 nm and 9.4 fs at 430 nm, close to the Fourier-transform limits. Moreover, theoretical and experimental studies reveal the strong influences of driving pulse energy and HCF length on temporal width and shape of the measured DW pulses. The ultraviolet pulses obtained in atmosphere environment with {\mu}J-level pulse energy, few-fs pulse width and broadband wavelength tunability are ready to be used in many applications.