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Ultimate limits for sensing of fields and forces are set by the quantum noise of a sensor. Entanglement allows for suppression of such noise and for achieving sensitivity beyond standard quantum limits. Applicability of quantum optical sensing is often restricted by fixed wavelengths of available photonic quantum sources. Another ubiquitous limitation is associated with challenges of achieving quantum-noise-limited sensitivity in the acoustic noise frequency range relevant for a number of applications. Here we demonstrate a novel tool for broadband quantum sensing by quantum state processing that can be applied to a wide range of the optical spectrum, and by suppressing quantum noise over an octave in the acoustic frequency range. An atomic spin ensemble in the quantum regime is strongly coupled to one of the tunable frequency modes of an Einstein-Podolsky-Rosen (EPR) source of light. The other EPR mode of light, entangled with the first one, is tuned to a disparate wavelength. Engineering the spin ensemble to act as a negative- or positive-mass oscillator we demonstrate frequency-dependent, entanglement-enabled quantum noise reduction for measurements at the disparate wavelength. The tunability of the spin ensemble allows to target quantum noise in a variety of systems with dynamics ranging from kHz to MHz. As an example of the broadband quantum noise reduction in the acoustic frequency range, we analyse the applicability of our approach to state-of-the-art gravitational wave detectors. Other possible applications include continuous-variable quantum repeaters and distributed quantum sensing., Comment: Main text (6 pages with 3 figures), methods (11 pages with 3 extended data figures) + supplementary information. Comments are welcome

We report on the observation and correction of an imaging artifact attributed to the Talbot effect in the context of acousto-optic imaging using structured acoustic waves. When ultrasound waves are emitted with a periodic structure, the Talbot effect produces $\pi$ -phase shifts of that periodic structure at every half of the Talbot distance in propagation. This unwanted artifact is detrimental to the image reconstruction, which assumes near-field diffraction is negligible. Here, we demonstrate both theoretically and experimentally how imposing an additional phase modulation on the acoustic periodic structure induces a symmetry constraint leading to the annihilation of the Talbot effect. This will significantly improve the acousto-optic image reconstruction quality and allows for an improvement of the reachable spatial resolution of the image.

Discriminating between ballistic and diffuse components of light propagating through highly scattering media is not only important for imaging purposes but also for investigating the fundamental diffusion properties of the medium itself. Massively developed to this end over the past 20 years, nonlinear temporal gating remains limited to about 10e-10 transmission factors. Here, we report nonlinear time gated measurements of highly scattered femtosecond pulses with transmission factors as low as 10e-12. Our approach is based on third-order nonlinear cross-correlation of femtosecond pulses, a standard diagnostic used in high-power laser science, applied for the first time to the study of fundamental light scattering properties.

We report evidence for the first generation of XUV spectra from relativistic surface high-harmonic generation (SHHG) on plasma mirrors at a kilohertz repetition rate, emitted simultaneously with energetic electrons. SHHG spectra and electron angular distributions are measured as a function of the experimentally controlled plasma density gradient scale length $L_\mathrm{g}$ for three increasingly short and intense driving pulses: 24~fs and $a_0=1.1$, 8~fs and $a_0=1.6$, and finally 4~fs and $a_0\approx2.1$, where $a_0$ is the peak vector potential normalized by $m_\mathrm{e} c/e$ with the elementary charge $e$, the electron rest mass $m_\mathrm{e}$, and the vacuum light velocity $c$. For all driver pulses, we observe correlated relativistic SHHG and electron emission in the range $L_\mathrm{g}\in[\lambda/25,\lambda/5]$, with an optimum gradient scale length of $L_\mathrm{g}\approx\lambda/10$.

function of the CEP, we observe a transition from a modulated to a continuous SHHG spectrum, indicating the transition from double to high-contrast isolated attosecond pulse emission. Single shot-acquisitions of XUV spectral continua support isolated attosecond pulses with isolation degrees between 10 and 50 for the majority of the driving pulse CEPs, which represents a significant improvement in terms of isolation degree as well as repetition rate over previous results obtained with 2-cycle drivers at 10-Hz. 2D Particle-in-cell simulations corroborate this interpretation and predict percent-level efficiencies for the generation of an isolated attosecond pulse even without any spectral filtering.

We present a laser source delivering waveform-controlled 1.5-cycle pulses that can be focused to relativistic intensity at 1 kHz repetition rate. These pulses are generated by nonlinear compression of high-temporal-contrast sub-25\,fs pulses from a kHz Ti:Sapphire double-chirped pulse amplifier in a stretched flexible hollow fiber compressor scaled for high peak power. The unique capabilities of this source are demonstrated by observing carrier-envelope phase effects in laser-wakefield acceleration of relativistic electrons for the first time.

Ultrasound modulated optical tomography (UOT) is a powerful imaging technique to discriminate healthy from unhealthy biological tissues based on their optical signature. Among the numerous detection techniques developed for acousto-optic imaging, only those based on spectral filtering are intrinsically immune to speckle decorrelation. This paper reports on UOT imaging based on spectral hole burning in Tm:YAG crystal under a moderate magnetic field (200G) with a well-defined orientation. The deep and long-lasting holes translate into a more efficient UOT imaging with a higher contrast and faster imaging frame rate. We demonstrate the potential of this method by imaging calibrated phantom scattering gels., Comment: 4 pages, 5 figures

We measure the emission of energetic electrons from the interaction between ultrashort laser pulses and a solid density plasma in the relativistic regime. We detect an electron beam that only appears with few-cycle pulses (< 10 fs) and large plasma scale lengths ($L > \lambda_0$). Numerical simulations, in agreement with the experiments, reveal that these electrons are accelerated by a laser wakefield. Plasma waves are indeed resonantly excited by the few-cycle laser pulses in the near-critical-density region of the plasma. Electrons are then injected by ionization into the plasma waves and accelerated to relativistic energies. This study provides an unprecedented insight into the physics happening in the few-cycle regime.

Diffuse Optical Tomography (DOT) is a reliable and widespread technique for monitoring qualitative changes in absorption inside highly scattering media. It has been shown, however, that Acousto-Optic (AO) imaging can provide significantly more qualitative information, without the need for inversion algorithms, due to the spatial resolution afforded by ultrasound probing. In this article, we show how, by using multiple-wavelength AO imaging, it is also possible to perform quantitative measurements of absorber concentration inside scattering media.

We report for the first time on the anticorrelated emission of high-order harmonics and energetic electron beams from a solid-density plasma with a sharp vacuum interface$-$plasma mirror$-$driven by an intense ultrashort laser pulse. We highlight the key role played by the nanoscale structure of the plasma surface during the interaction by measuring the spatial and spectral properties of harmonics and electron beams emitted by a plasma mirror. We show that the nanoscale behavior of the plasma mirror can be controlled by tuning the scale length of the electronic density gradient, which is measured in-situ using spatial-domain interferometry.

Laser-plasma acceleration is an emerging technique for accelerating electrons to high energies over very short distances. The accelerated electron bunches have femtosecond duration, making them particularly relevant for applications such as ultrafast imaging or femtosecond X-ray generation. Current laser-plasma accelerators are typically driven by Joule-class laser systems that have two main drawbacks: their relatively large scale and their low repetition-rate, with a few shots per second at best. The accelerated electron beams have energies ranging from 100 MeV to multi-GeV, however a MeV electron source would be more suited to many societal and scientific applications. Here, we demonstrate a compact and reliable laser-plasma accelerator producing high-quality few-MeV electron beams at kilohertz repetition rate. This breakthrough was made possible by using near-single-cycle light pulses, which lowered the required laser energy for driving the accelerator by three orders of magnitude, thus enabling high repetition-rate operation and dramatic downsizing of the laser system. The measured electron bunches are collimated, with an energy distribution that peaks at 5 MeV and contains up to 1 pC of charge. Numerical simulations reproduce all experimental features and indicate that the electron bunches are only $\sim 1$ fs long. We anticipate that the advent of these kHz femtosecond relativistic electron sources will pave the way to wide-impact applications, such as ultrafast electron diffraction in materials with an unprecedented sub-10 fs resolution.

A high repetition rate electron source was generated by tightly focusing kHz, few-mJ laser pulses into an underdense plasma. This high intensity laser-plasma interaction led to stable electron beams over several hours but with strikingly complex transverse distributions even for good quality laser focal spots. Analysis of the experimental data, along with results of PIC simulations demonstrate the role of the laser wavefront on the acceleration of electrons. Distortions of the laser wavefront cause spatial inhomogeneities in the out-of-focus laser distribution and consequently, the laser pulse drives an inhomogenous transverse wakefield whose focusing/defocusing properties affect the electron distribution. These findings explain the experimental results and suggest the possibility of controlling the electron spatial distribution in laser-plasma accelerators by tailoring the laser wavefront.

We investigated the carrier-envelope phase (CEP) stability of a hollow-fiber setup used for high-energy, few-cycle pulse generation. Saturation of the output pulse energy is observed at 0.6 mJ for a 260 um inner-diameter, 1 m long fiber, statically filled with neon, with the pressure adjusted to achieve an output spectrum capable of supporting sub-4fs pulses. The maximum output pulse energy can be increased to 0.8mJ by using either differential pumping, or circularly polarized input pulses. We observe the onset of an ionization-induced CEP instability, which does not increase beyond an input pulse energy of 1.25 mJ due to losses in the fiber caused by ionization. There is no significant difference in the CEP stability with differential pumping compared to static-fill, demonstrating that gas flow in differentially pumped fibers does not degrade the CEP stabilization., Comment: 4 pages, 4 figures