Search

The design of fast reactors burning MOX fuels requires accurate capture and fission cross sections. For the particular case of neutron capture on 242Pu, the NEA recommends that an accuracy of 8-12% should be achieved in the fast energy region (2 keV-500 keV) compared to their estimation of 35% for the current uncertainty. Integral irradiation experiments suggest that the evaluated cross section of the JEFF-3.1 library overestimates the 242Pu(n,{\gamma}) cross section by 14% in the range between 1 keV and 1 MeV. In addition, the last measurement at LANSCE reported a systematic reduction of 20-30% in the 1-40 keV range relative to the evaluated libraries and previous data sets. In the present work this cross section has been determined up to 600 keV in order to solve the mentioned discrepancies. A 242Pu target of 95(4) mg enriched to 99.959% was irradiated at the n TOF-EAR1 facility at CERN. The capture cross section of 242Pu has been obtained between 1 and 600 keV with a systematic uncertainty (dominated by background subtraction) between 8 and 12%, reducing the current uncertainties of 35% and achieving the accuracy requested by the NEA in a large energy range. The shape of the cross section has been analyzed in terms of average resonance parameters using the FITACS code as implemented in SAMMY, yielding results compatible with our recent analysis of the resolved resonance region.The results are in good agreement with the data of Wisshak and K\"appeler and on average 10-14% below JEFF-3.2 from 1 to 250 keV, which helps to achieve consistency between integral experiments and cross section data. At higher energies our results show a reasonable agreement within uncertainties with both ENDF/B-VII.1 and JEFF-3.2. Our results indicate that the last experiment from DANCE underestimates the capture cross section of 242Pu by as much as 40% above a few keV., Comment: 20 pages, 19 figures, submitted to Phys. Rev. C

The probabilities for gamma-ray and particle emission as a function of the excitation energy of a decaying nucleus are valuable observables for constraining the ingredients of the models that describe the de-excitation of nuclei near the particle emission threshold. These models are essential in nuclear astrophysics and applications. In this work, we have for the first time simultaneously measured the gamma-ray and neutron emission probabilities of 208Pb. The measurement was performed in inverse kinematics at the Experimental Storage Ring (ESR) of the GSI/FAIR facility, where a 208Pb beam interacted through the 208Pb(p,p') reaction with a hydrogen gas jet target. Instead of detecting the gamma-rays and neutrons emitted by 208Pb, we detected the heavy beam-like residues produced after gamma and neutron emission. These heavy residues were fully separated by a dipole magnet of the ESR and were detected with outstanding efficiencies. The comparison of the measured probabilities with model calculations has allowed us to test and select different descriptions of the gamma-ray strength function and the nuclear level density available in the literature., Comment: 23 pages, 14 figures

The $^{246}$Cm(n,$\gamma$) and $^{248}$Cm(n,$\gamma$) cross-sections have been measured at the Experimental Area 2 (EAR2) of the n_TOF facility at CERN with three C$_6$D$_6$ detectors. This measurement is part of a collective effort to improve the capture cross-section data for Minor Actinides (MAs), which are required to estimate the production and transmutation rates of these isotopes in light water reactors and innovative reactor systems. In particular, the neutron capture in $^{246}$Cm and $^{248}$Cm open the path for the formation of other Cm isotopes and heavier elements such as Bk and Cf and the knowledge of (n,$\gamma$) cross-sections of these Cm isotopes plays an important role in the transport, transmutation and storage of the spent nuclear fuel. The reactions $^{246}$Cm(n,$\gamma$) and $^{248}$Cm(n,$\gamma$) have been the two first capture measurements analyzed at n_TOF EAR2. Until this experiment and two recent measurements performed at J-PARC, there was only one set of data of the capture cross-sections of $^{246}$Cm and $^{248}$Cm, that was obtained in 1969 in an underground nuclear explosion experiment. In the measurement at n_TOF a total of 13 resonances of $^{246}$Cm between 4 and 400 eV and 5 of $^{248}$Cm between 7 and 100 eV have been identified and fitted. The radiative kernels obtained for $^{246}$Cm are compatible with JENDL-5, but some of them are not with JENDL-4, which has been adopted by JEFF-3.3 and ENDF/B-VIII.0. The radiative kernels obtained for the first three $^{248}$Cm resonances are compatible with JENDL-5, however, the other two are not compatible with any other evaluation and are 20% and 60% larger than JENDL-5.

Neutron-induced reaction cross sections of short-lived nuclei are imperative to understand the origin of heavy elements in stellar nucleosynthesis and for societal applications, but their measurement is extremely complicated due to the radioactivity of the targets involved. One way of overcoming this issue is to combine surrogate reactions with the unique possibilities offered by heavy-ion storage rings. In this work, we describe the first surrogate-reaction experiment in inverse kinematics, which we successfully conducted at the Experimental Storage Ring (ESR) of the GSI/FAIR facility, using the 208Pb(p,p') reaction as a surrogate for neutron capture on 207Pb. Thanks to the outstanding detection efficiencies possible at the ESR, we were able to measure for the first time the neutron-emission probability as a function of the excitation energy of 208Pb. We have used this probability to select different descriptions of the gamma-ray strength function and nuclear level density, and provide reliable results for the neutron-induced radiative capture cross section of 207Pb at energies for which no experimental data exist., Comment: 10 pages and 5 figures

Nuclear fission is still one of the most complex physical processes we can observe in nature due to the interplay of macroscopic and microscopic nuclear properties that decide the result. An example of this coupling is the presence of nuclear dissipation as an important ingredient that contributes to drive the dynamics and has a clear impact on the time of the process. However, different theoretical interpretations, and scarce experimental data make it poorly understood. In this letter, we present the first experimental determination of the dissipation energy in fission as a function of the fragment split, for three different fissioning systems. The amount of dissipation was obtained through the measurement of the relative production of fragments with even and odd atomic numbers with respect to different initial fission energies. The results reveal a clear effect of particular nuclear shells on the dissipation and fission dynamics. In addition, the relative production of fragments with even and odd atomic numbers appears as a potential contributor to the long-standing problem of the time scale in fission.

Background: The $^{14}$N(n,p)$^{14}$C reaction is of interest in neutron capture therapy, where nitrogen-related dose is the main component due to low-energy neutrons, and in astrophysics, where 14N acts as a neutron poison in the s-process. Several discrepancies remain between the existing data obtained in partial energy ranges: thermal energy, keV region and resonance region. Purpose: Measuring the 14N(n,p)14C cross section from thermal to the resonance region in a single measurement for the first time, including characterization of the first resonances, and providing calculations of Maxwellian averaged cross sections (MACS). Method: Time-of-flight technique. Experimental Area 2 (EAR-2) of the neutron time-of-flight (n_TOF) facility at CERN. $^{10}$B(n,${\alpha}$)$^7$Li and $^{235}$U(n,f) reactions as references. Two detection systems running simultaneously, one on-beam and another off-beam. Description of the resonances with the R-matrix code sammy. Results: The cross section has been measured from sub-thermal energy to 800 keV resolving the two first resonances (at 492.7 and 644 keV). A thermal cross-section (1.809$\pm$0.045 b) lower than the two most recent measurements by slightly more than one standard deviation, but in line with the ENDF/B-VIII.0 and JEFF-3.3 evaluations has been obtained. A 1/v energy dependence of the cross section has been confirmed up to tens of keV neutron energy. The low energy tail of the first resonance at 492.7 keV is lower than suggested by evaluated values, while the overall resonance strength agrees with evaluations. Conclusions: Our measurement has allowed to determine the $^{14}$N(n,p) cross-section over a wide energy range for the first time. We have obtained cross-sections with high accuracy (2.5 %) from sub-thermal energy to 800 keV and used these data to calculate the MACS for kT = 5 to kT = 100 keV., Comment: 18 pages, 15 figures, 4 tables

Despite the recent experimental and theoretical progress in the investigation of the nuclear fission process, a complete description still represents a challenge in nuclear physics because it is a very complex dynamical process, whose description involves the coupling between intrinsic and collective degrees of freedom, as well as different quantum-mechanical phenomena. To improve on the existing data on nuclear fission, we produce fission reactions of heavy nuclei in inverse kinematics by using quasi-free (p,2p) scattering, which induce fission through particle-hole excitations that can range from few to ten's of MeV. The measurement of the four-momenta of the two outgoing protons allows to reconstruct the excitation energy of the fissioning compound nucleus and therefore to study the evolution of the fission yields with temperature. The realization of this kind of experiment requires a complex experimental setup, providing full isotopic identification of both fission fragments and an accurate measurement of the momenta of the two outgoing protons. This was realized recently at the GSI/FAIR facility and here some preliminary results are presented., Comment: 6 pages, 2 figures, FAIRNESS 2022. arXiv admin note: text overlap with arXiv:2210.04741

In the last decades, measurements of spallation, fragmentation and Coulex induced fission reactions in inverse kinematics have provided valuable data to accurately investigate the fission dynamics and nuclear structure at large deformations of a large variety of stable and non-stable heavy nuclei. To go a step further, we propose now to induce fission by the use of quasi-free (p,2p) scattering reactions in inverse kinematics, which allows us to reconstruct the excitation energy of the compound fissioning system by using the four-momenta of the two outgoing protons. Therefore, this new approach might permit to correlate the excitation energy with the charge and mass distributions of the fission fragments and with the fission probabilities, given for the first time direct access to the simultaneous measurement of the fission yield dependence on temperature and fission barrier heights of exotic heavy nuclei, respectively. The first experiment based on this methodology was realized recently at the GSI/FAIR facility and a detailed description of the experimental setup is given here., Comment: 4 pages, 15th International Conference on Nuclear Data for Science and Technology (ND2022)

The 235U(n,f) cross section was measured in a wide energy range (25 meV - 170 keV) at the n_TOF facility at CERN, relative to 6Li(n,t) and 10B(n,alpha) standard reactions, with high resolution and accuracy, with a setup based on a stack of six samples and six silicon detectors placed in the neutron beam. In this paper we report on the results in the region between thermal and 10 keV neutron energy. A resonance analysis has been performed up to 200 eV, with the code SAMMY. The resulting fission kernels are compared with the ones extracted on the basis of the resonance parameters of the most recent major evaluated data libraries. A comparison of the n_TOF data with the evaluated cross sections is also performed from thermal to 10 keV neutron energy for the energy-averaged cross section in energy groups of suitably chosen width. A good agreement is found in average between the new results and the latest evaluated data files ENDF-B/VIII and JEFF-3.3, as well as with respect to the IAEA reference files. However, some discrepancies are still present in some specific energy regions. The new dataset here presented, characterized by unprecedented resolution and accuracy, can help improving the evaluations in the Resolved Resonance Region and up to 10 keV, and reduce the uncertainties that affect this region.

i-TED is an innovative detection system which exploits Compton imaging techniques to achieve a superior signal-to-background ratio in ($n,\gamma$) cross-section measurements using time-of-flight technique. This work presents the first experimental validation of the i-TED apparatus for high-resolution time-of-flight experiments and demonstrates for the first time the concept proposed for background rejection. To this aim both $^{197}$Au($n,\gamma$) and $^{56}$Fe($n, \gamma$) reactions were measured at CERN n\_TOF using an i-TED demonstrator based on only three position-sensitive detectors. Two \cds detectors were also used to benchmark the performance of i-TED. The i-TED prototype built for this study shows a factor of $\sim$3 higher detection sensitivity than state-of-the-art \cds detectors in the $\sim$10~keV neutron energy range of astrophysical interest. This paper explores also the perspectives of further enhancement in performance attainable with the final i-TED array consisting of twenty position-sensitive detectors and new analysis methodologies based on Machine-Learning techniques., Comment: 16 pages, 16 figures

It has been suggested that hydrogen ingestion into the helium shell of massive stars could lead to high $^{13}$C and $^{15}$N excesses when the shock of a core-collapse supernova passes through its helium shell. This prediction questions the origin of extremely high $^{13}$C and $^{15}$N abundances observed in rare presolar SiC grains which is usually attributed to classical novae. In this context $^{13}$N($\alpha$,p)$^{16}$O the reaction plays an important role since it is in competition with $^{13}$N $\beta^+$-decay to $^{13}$C. The $^{13}$N($\alpha$,p)$^{16}$O reaction rate used in stellar evolution calculations comes from the CF88 compilation with very scarce information on the origin of this rate. The goal of this work is to provide a recommended $^{13}$N($\alpha$,p)$^{16}$O reaction rate, based on available experimental data. Unbound nuclear states in the $^{17}$F compound nucleus were studied using the spectroscopic information of the analog states in $^{17}$O nucleus that were measured at the Alto facility using the $^{13}$C($^7$Li,t)$^{17}$O alpha-transfer reaction, and spectroscopic factors were derived using a DWBA analysis. This spectroscopic information was used to calculate a recommended $^{13}$N($\alpha$,p)$^{16}$O reaction rate with meaningful uncertainty using a Monte Carlo approach. The present $^{13}$N($\alpha$,p)$^{16}$O reaction rate is found to be within a factor of two of the previous evaluation, with a typical uncertainty of a factor 2-3. The source of this uncertainty comes from the three resonances at $E_r^{c.m.} = 221$, 741 and 959 keV. This new error estimation translates to an overall uncertainty in the $^{13}$C production of a factor of 50. The main source of uncertainty on the re-evaluated $^{13}$N($\alpha$,p)$^{16}$O reaction rate currently comes from the uncertain alpha-width of relevant $^{17}$F states.

The simultaneous measurement of the isotopic fission-fragment yields and fission-fragment velocities of $^{239}$U has been performed for the first time. The $^{239}$U fissioning system was produced in one-neutron transfer reactions between a $^{238}$U beam at 5.88 MeV/nucleon and a $^{9}$Be target. The combination of inverse kinematics at low energy and the use of the VAMOS++ spectrometer at the GANIL facility allows the isotopic identification of the full fission-fragment distribution and their velocity in the reference frame of the fissioning system. The proton and neutron content of the fragments at scission, their total kinetic and total excitation energy, as well as the neutron multiplicity were determined. Information from the scission point configuration is obtained from these observables and the correlation between them. The role of the octupole-deformed proton and neutron shells in the fission-fragment production is discussed., Comment: 8 pages, 7 figures

Reliable neutron-induced reaction cross sections of unstable nuclei are essential for nuclear astrophysics and applications but their direct measurement is often impossible. The surrogate-reaction method is one of the most promising alternatives to access these cross sections. In this work, we successfully applied the surrogate-reaction method to infer for the first time both the neutron-induced fission and radiative-capture cross sections of 239Pu in a consistent manner from a single measurement. This was achieved by combining simultaneously-measured fission and gamma-emission probabilities for the 240Pu(4He,4He') surrogate reaction with a calculation of the angular-momentum and parity distributions populated in this reaction. While other experiments measure the probabilities for some selected gamma-ray transitions, we measure the gamma-emission probability. This enlarges the applicability of the surrogate-reaction method., Comment: 8 pages, 3 figures

The idea of slow-neutron capture nucleosynthesis formulated in 1957 triggered a tremendous experimental effort in different laboratories worldwide to measure the relevant nuclear physics input quantities, namely ($n,\gamma$) cross sections over the stellar temperature range (from few eV up to several hundred keV) for most of the isotopes involved from Fe up to Bi. A brief historical review focused on total energy detectors will be presented to illustrate how, advances in instrumentation have led, over the years, to the assessment and discovery of many new aspects of $s$-process nucleosynthesis and to the progressive refinement of theoretical models of stellar evolution. A summary will be presented on current efforts to develop new detection concepts, such as the Total-Energy Detector with $\gamma$-ray imaging capability (i-TED). The latter is based on the simultaneous combination of Compton imaging with neutron time-of-flight (TOF) techniques, in order to achieve a superior level of sensitivity and selectivity in the measurement of stellar neutron capture rates., Comment: Nuclear Physics in Astrophysics IX - Conference Proceedings

A direct and complete measurement of isotopic fission-fragment yields of $^{239}$U has been performed for the first time. The $^{239}$U fissioning system was produced with an average excitation energy of 8.3 MeV in one-neutron transfer reactions between a $^{238}$U beam and a $^{9}$Be target at Coulomb barrier energies. The fission fragments were detected and isotopically identified using the VAMOS++ spectrometer at the GANIL facility. This measurement allows to directly evaluate the fission models at excitation energies of fast neutrons, relevant for next-generation nuclear reactors. The present data, in agreement with model calculations, do not support the recently reported anomaly in the fission-fragment yields of $^{239}$U and confirm the persistence of spherical shell effects in the Sn region at excitation energies exceeding the fission barrier by few MeV.

The 235U(n,f) cross section was measured in a wide energy range at n_TOF relative to 6Li(n,t) and 10B(n,alpha), with high resolution and in a wide energy range, with a setup based on a stack of six samples and six silicon detectors placed in the neutron beam. This allowed us to make a direct comparison of the reaction yields under the same experimental conditions, and taking into account the forward/backward emission asymmetry. A hint of an anomaly in the 10{\div}30 keV neutron energy range had been previously observed in other experiments, indicating a cross section systematically lower by several percent relative to major evaluations. The present results indicate that the evaluated cross section in the 9{\div}18 keV neutron energy range is indeed overestimated, both in the recent updates of ENDF/B-VIII.0 and of the IAEA reference data. Furthermore, these new high-resolution data confirm the existence of resonance-like structures in the keV neutron energy region. The new, high accuracy results here reported may lead to a reduction of the uncertainty in the 1{\div}100 keV neutron energy region. Finally, the present data provide additional confidence on the recently re-evaluated cross section integral between 7.8 and 11 eV., Comment: 22 pages, 20 figures, submitted to PRC

We report on the measurement of the $^{7}$Be($n, p$)$^{7}$Li cross section from thermal to approximately 325 keV neutron energy, performed in the high-flux experimental area (EAR2) of the n\_TOF facility at CERN. This reaction plays a key role in the lithium yield of the Big Bang Nucleosynthesis (BBN) for standard cosmology. The only two previous time-of-flight measurements performed on this reaction did not cover the energy window of interest for BBN, and showed a large discrepancy between each other. The measurement was performed with a Si-telescope, and a high-purity sample produced by implantation of a $^{7}$Be ion beam at the ISOLDE facility at CERN. While a significantly higher cross section is found at low-energy, relative to current evaluations, in the region of BBN interest the present results are consistent with the values inferred from the time-reversal $^{7}$Li($p, n$)$^{7}$Be reaction, thus yielding only a relatively minor improvement on the so-called Cosmological Lithium Problem (CLiP). The relevance of these results on the near-threshold neutron production in the p+$^{7}$Li reaction is also discussed.

Neutron capture measurements on $^{155}$Gd and $^{157}$Gd were performed using the time-of-flight technique at the n\_TOF facility at CERN. Four samples in form of self-sustaining metallic discs isotopically enriched in $^{155}$Gd and $^{157}$Gd were used. The measurements were carried out at the experimental area (EAR1) at 185 m from the neutron source, with an array of 4 C$_6$D$_6$ liquid scintillation detectors. The capture cross sections of $^{155}$Gd and $^{157}$Gd at neutron kinetic energy of 0.0253 eV have been estimated to be 62.2(2.2) kb and 239.8(9.3) kb, respectively, thus up to 6\% different relative to the ones reported in the nuclear data libraries. A resonance shape analysis has been performed in the resolved resonance region up to 180 eV and 300 eV, respectively, in average resonance parameters have been found in good agreement with evaluations. Above these energies the observed resonance-like structures in the cross section have been tentatively characterised in terms of resonance energy and area up to 1 keV.

We report on the measurement of the $^{7}$Be($n, p$)$^{7}$Li cross section from thermal to approximately 325 keV neutron energy, performed in the high-flux experimental area (EAR2) of the n_TOF facility at CERN. This reaction plays a key role in the lithium yield of the Big Bang Nucleosynthesis (BBN) for standard cosmology. The only two previous time-of-flight measurements performed on this reaction did not cover the energy window of interest for BBN, and showed a large discrepancy between each other. The measurement was performed with a Si-telescope, and a high-purity sample produced by implantation of a $^{7}$Be ion beam at the ISOLDE facility at CERN. While a significantly higher cross section is found at low-energy, relative to current evaluations, in the region of BBN interest the present results are consistent with the values inferred from the time-reversal $^{7}$Li($p, n$)$^{7}$Be reaction, thus yielding only a relatively minor improvement on the so-called Cosmological Lithium Problem (CLiP). The relevance of these results on the near-threshold neutron production in the p+$^{7}$Li reaction is also discussed., Comment: arXiv admin note: This submission has been withdrawn by arXiv administrators as it is a duplicate of arXiv:1806.03050. Please refer to that document for any more recent versions

Following the completion of the second neutron beam line and the related experimental area (EAR2) at the n_TOF spallation neutron source at CERN, several experiments were planned and performed. The high instantaneous neutron flux available in EAR2 allows to investigate neutron indiced reactions with charged particles in the exit channel even employing targets made out of small amounts of short-lived radioactive isotopes. After the successful measurement of the 7Be(n,{\alpha}){\alpha} cross section, the 7Be(n,p)7Li reaction was studied in order to provide still missing cross section data of relevance for Big Bang Nucleosynthesis (BBN), in an attempt to find a solution to the cosmological Lithium abundance problem. This paper describes the experimental setup employed in such a measurement and its characterization.

The aim of this work is to provide a precise and accurate measurement of the 238U(n,g) reaction cross section in the energy region from 1 eV to 700 keV. This reaction is of fundamental importance for the design calculations of nuclear reactors, governing the behaviour of the reactor core. In particular, fast reactors, which are experiencing a growing interest for their ability to burn radioactive waste, operate in the high energy region of the neutron spectrum. In this energy region most recent evaluations disagree due to inconsistencies in the existing measurements of up to 15%. In addition, the assessment of nuclear data uncertainty performed for innovative reactor systems shows that the uncertainty in the radiative capture cross-section of 238U should be further reduced to 1-3% in the energy region from 20 eV to 25 keV. To this purpose, addressed by the Nuclear Energy Agency as a priority nuclear data need, complementary experiments, one at the GELINA and two at the n_TOF facility, were proposed and carried out within the 7th Framework Project ANDES of the European Commission. The results of one of these 238U(n,g) measurements performed at the n_TOF CERN facility are presented in this work. The gamma-ray cascade following the radiative neutron capture has been detected exploiting a setup of two C6D6 liquid scintillators. Resonance parameters obtained from this work are on average in excellent agreement with the ones reported in evaluated libraries. In the unresolved resonance region, this work yields a cross section in agreement with evaluated libraries up to 80 keV, while for higher energies our results are significantly higher., Comment: 15 pages, 10 captioned figures

The integral measurement of the $^{12}$C(n,p)$^{12}$B reaction was performed at the neutron time of flight facility n_TOF at CERN. The total number of $^{12}$B nuclei produced per neutron pulse of the n_TOF beam was determined using the activation technique in combination with a time of flight technique. The cross section is integrated over the n_TOF neutron energy spectrum from reaction threshold at 13.6 MeV to 10 GeV. Having been measured up to 1 GeV on basis of the $^{235}$U(n,f) reaction, the neutron energy spectrum above 200 MeV has been reevaluated due to the recent extension of the cross section reference for this particular reaction, which is otherwise considered a standard up to 200 MeV. The results from the dedicated GEANT4 simulations have been used to evaluate the neutron flux from 1 GeV up to 10 GeV. The experimental results related to the $^{12}$C(n,p)$^{12}$B reaction are compared with the evaluated cross sections from major libraries and with the predictions of different GEANT4 models, which mostly underestimate the $^{12}$B production. On the contrary, a good reproduction of the integral cross section derived from measurements is obtained with TALYS-1.6 calculations, with optimized parameters., Comment: 14 pages, 11 figures, 3 tables

The newly built second experimental area EAR2 of the n_TOF spallation neutron source at CERN allows to perform (n, charged particles) experiments on short-lived highly radioactive targets. This paper describes a detection apparatus and the experimental procedure for the determination of the cross-section of the 7Be(n,{\alpha}) reaction, which represents one of the focal points toward the solution of the cosmological Lithium abundance problem, and whose only measurement, at thermal energy, dates back to 1963. The apparently unsurmountable experimental difficulties stemming from the huge 7Be {\gamma}-activity, along with the lack of a suitable neutron beam facility, had so far prevented further measurements. The detection system is subject to considerable radiation damage, but is capable of disentangling the rare reaction signals from the very high background. This newly developed setup could likely be useful also to study other challenging reactions requiring the detectors to be installed directly in the neutron beam., Comment: submitted to Nuclear Instruments and Methods in Physics Research A

The isotopic-yield distributions and kinematic properties of fragments produced in transfer-induced fission of 240Pu and fusion-induced fission of 250Cf, with 9 MeV and 45 MeV of excitation energy respectively, were measured in inverse kinematics with the spectrometer VAMOS. The kinematic properties of identified fission fragments allow to derive properties of the scission configuration such as the distance between fragments, the total kinetic energy, the neutron multiplicity, the total excitation energy, and, for the first time, the proton- and neutron-number sharing during the emergence of the fragments. These properties of the scission point are studied as functions of the fragment atomic number. The correlation between these observables, gathered in one single experiment and for two different fissioning systems at different excitation energies, give valuable information for the understanding and modeling of the fission process., Comment: 12 pages, 8 figures

Background:The design of new nuclear reactors and transmutation devices requires to reduce the present neutron cross section uncertainties of minor actinides. Purpose: Reduce the $^{243}$Am(n,$\gamma$) cross section uncertainty. Method: The $^{243}$Am(n,$\gamma$) cross section has been measured at the n_TOF facility at CERN with a BaF$_{2}$ Total Absorption Calorimeter, in the energy range between 0.7 eV and 2.5 keV. Results: The $^{243}$Am(n,$\gamma$) cross section has been successfully measured in the mentioned energy range. The resolved resonance region has been extended from 250 eV up to 400 eV. In the unresolved resonance region our results are compatible with one of the two incompatible capture data sets available below 2.5 keV. The data available in EXFOR and in the literature has been used to perform a simple analysis above 2.5 keV. Conclusions: The results of this measurement contribute to reduce the $^{243}$Am(n,$\gamma$) cross section uncertainty and suggest that this cross section is underestimated up to 25% in the neutron energy range between 50 eV and a few keV in the present evaluated data libraries.

The $^{238}$U to $^{235}$U fission cross section ratio has been determined at n_TOF up to $\sim$1 GeV, with two different detection systems, in different geometrical configurations. A total of four datasets have been collected and compared. They are all consistent to each other within the relative systematic uncertainty of 3-4%. The data collected at n_TOF have been suitably combined to yield a unique fission cross section ratio as a function of the neutron energy. The result confirms current evaluations up to 200 MeV. A good agreement is also observed with theoretical calculations based on the INCL++/Gemini++ combination up to the highest measured energy. The n_TOF results may help solving a long-standing discrepancy between the two most important experimental dataset available so far above 20 MeV, while extending the neutron energy range for the first time up to $\sim$1 GeV.

The integral cross section of the $^{12}$C($n,p$)$^{12}$B reaction has been determined for the first time in the neutron energy range from threshold to several GeV at the n_TOF facility at CERN. The measurement relies on the activation technique, with the $\beta$-decay of $^{12}$B measured over a period of four half-lives within the same neutron bunch in which the reaction occurs. The results indicate that model predictions, used in a variety of applications, are mostly inadequate. The value of the integral cross section reported here can be used as a benchmark for verifying or tuning model calculations., Comment: 6 pages, 4 figures

The neutron sensitivity of the C$_6$D$_6$ detector setup used at n_TOF for capture measurements has been studied by means of detailed GEANT4 simulations. A realistic software replica of the entire n_TOF experimental hall, including the neutron beam line, sample, detector supports and the walls of the experimental area has been implemented in the simulations. The simulations have been analyzed in the same manner as experimental data, in particular by applying the Pulse Height Weighting Technique. The simulations have been validated against a measurement of the neutron background performed with a $^\mathrm{nat}$C sample, showing an excellent agreement above 1 keV. At lower energies, an additional component in the measured $^\mathrm{nat}$C yield has been discovered, which prevents the use of $^\mathrm{nat}$C data for neutron background estimates at neutron energies below a few hundred eV. The origin and time structure of the neutron background have been derived from the simulations. Examples of the neutron background for two different samples are demonstrating the important role of accurate simulations of the neutron background in capture cross section measurements.

The cross section of the $^{62}$Ni($n,\gamma$) reaction was measured with the time-of-flight technique at the neutron time-of-flight facility n_TOF at CERN. Capture kernels of 42 resonances were analyzed up to 200~keV neutron energy and Maxwellian averaged cross sections (MACS) from $kT=5-100$ keV were calculated. With a total uncertainty of 4.5%, the stellar cross section is in excellent agreement with the the KADoNiS compilation at $kT=30$ keV, while being systematically lower up to a factor of 1.6 at higher stellar temperatures. The cross section of the $^{63}$Ni($n,\gamma$) reaction was measured for the first time at n_TOF. We determined unresolved cross sections from 10 to 270 keV with a systematic uncertainty of 17%. These results provide fundamental constraints on $s$-process production of heavier species, especially the production of Cu in massive stars, which serve as the dominant source of Cu in the solar system.

The $^{58}$Ni $(n,\gamma)$ cross section has been measured at the neutron time of flight facility n_TOF at CERN, in the energy range from 27 meV up to 400 keV. In total, 51 resonances have been analyzed up to 122 keV. Maxwellian averaged cross sections (MACS) have been calculated for stellar temperatures of kT$=$5-100 keV with uncertainties of less than 6%, showing fair agreement with recent experimental and evaluated data up to kT = 50 keV. The MACS extracted in the present work at 30 keV is 34.2$\pm$0.6$_\mathrm{stat}\pm$1.8$_\mathrm{sys}$ mb, in agreement with latest results and evaluations, but 12% lower relative to the recent KADoNIS compilation of astrophysical cross sections. When included in models of the s-process nucleosynthesis in massive stars, this change results in a 60% increase of the abundance of $^{58}$Ni, with a negligible propagation on heavier isotopes. The reason is that, using both the old or the new MACS, 58Ni is efficiently depleted by neutron captures., Comment: 10 pages, 8 figures, 5 tables

Inelastic and multi-nucleon transfer reactions between a $^{238}$U beam, accelerated at 6.14 MeV/u, and a $^{12}$C target were used for the production of neutron-rich, fissioning systems from U to Cm. A Si telescope, devoted to the detection of the target-like nuclei, provided a characterization of the fissioning systems in atomic and mass numbers, as well as in excitation energy. Cross-sections, angular and excitation-energy distributions were measured for the inelastic and transfer channels. Possible excitations of the target-like nuclei were experimentally investigated for the first time, by means of g -ray measurements. The decays from the first excited states of $^{12}$C, $^{11}$B and $^{10}$Be were observed with probabilities of 0.12 - 0.14, while no evidence for the population of higher-lying states was found. Moreover, the fission probabilities of $^{238}$U, $^{239}$Np and $^{240,241,242}$Pu and $^{244}$Cm were determined as a function of the excitation energy., Comment: 16 pages, 12 figures

The observed primordial 7Li abundance in metal-poor halo stars is found to be lower than its Big-Bang nucleosynthesis (BBN) calculated value by a factor of approximately three. Some recent works suggested the possibility that this discrepancy originates from missing resonant reactions which would destroy the 7Be, parent of 7Li. The most promising candidate resonances which were found include a possibly missed 1- or 2- narrow state around 15 MeV in the compound nucleus 10C formed by 7Be+3He and a state close to 7.8 MeV in the compound nucleus 11C formed by 7Be+4He. In this work, we studied the high excitation energy region of 10C and the low excitation energy region in 11C via the reactions 10B(3He,t)10C and 11B(3He,t)11C, respectively, at the incident energy of 35 MeV. Our results for 10C do not support 7Be+3He as a possible solution for the 7Li problem. Concerning 11C results, the data show no new resonances in the excitation energy region of interest and this excludes 7Be+4He reaction channel as an explanation for the 7Li deficit., Comment: Accepted for publication in Phys. Rev. C (Rapid Communication)

The $^{63}$Ni($n, \gamma$) cross section has been measured for the first time at the neutron time-of-flight facility n\_TOF at CERN from thermal neutron energies up to 200 keV. In total, capture kernels of 12 (new) resonances were determined. Maxwellian Averaged Cross Sections were calculated for thermal energies from kT = 5 keV to 100 keV with uncertainties around 20%. Stellar model calculations for a 25 M$_\odot$ star show that the new data have a significant effect on the $s$-process production of $^{63}$Cu, $^{64}$Ni, and $^{64}$Zn in massive stars, allowing stronger constraints on the Cu yields from explosive nucleosynthesis in the subsequent supernova.

A novel method to access the complete identification in atomic number Z and mass A of fragments produced in low-energy fission of actinides is presented. This method, based on the use of multi- nucleon transfer and fusion reactions in inverse kinematics, is applied in this work to reactions between a 238U beam and a 12C target to produce and induce fission of moderately excited actinides. The fission fragments are detected and fully identified with the VAMOS spectrometer of GANIL, allowing the measurement of fragment yields of several hundreds of isotopes in a range between A ~ 80 and ~ 160, and from Z ~ 30 to ~ 64. For the first time, complete isotopic yield distributions of fragments from well-defined fissioning systems are available. Together with the precise measurement of the fragment emission angles and velocities, this technique gives further insight into the nuclear-fission process., Comment: 22 pages, 21 figures

During the fission process, the nucleus deforms and elongates up to the two fragments inception and their final separation at scission deformation. The evolution of the nucleus energy with deformation is determined by the macroscopic properties of the nucleus, and is also strongly influenced by the single-particle structure of the nucleus. The fission fragment distribution is a direct consequence of the deformation path the nucleus has encountered, and therefore is the most genuine experimental observation of the potential energy landscape of the deforming nucleus. Very asymmetric fusion-fission reactions at energy close to the Coulomb barrier, produce well-defined conditions of the compound nucleus formation, where processes such as quasi-fission, pre-equilibrium emission and incomplete fusion are negligible. In the same time, the excitation energy is sufficient to reduce significantly structural effects, and mostly the macroscopic part of the potential is responsible for the formation of the fission fragments. We use inverse kinematics combined with spectrometers to select and identify the fission fragments produced in $^{238}$U+$^{12}$C at a bombarding energy close to and well-above the Coulomb barrier. For the first time, the isotopic yields are measured over the complete atomic-number distribution, between Z=30 and Z=63. The experimental set-up also allows to identify transfer-induced reactions, which lead to low-energy fission where the nuclear shell structure shows a strong influence on the fission-fragment distributions. The resulting set of data gives the possibility to observe the fission fragment properties over a wide range of excitation energy, and they reveal the vanishing of the shell effects in the potential energy of the fissioning nucleus, as well as the influence of fission dynamics., Comment: Invited Plenary Talk given at the 11th International Conference on Nucleus-Nucleus Collisions (NN2012), San Antonio, Texas, USA, May 27-June 1, 2012. To appear in the NN2012 Proceedings in Journal of Physics: Conference Series (JPCS)

The production of heavy neutron-rich nuclei has been investigated using cold fragmentation reactions of $^{238}$U projectiles at relativistic energies. The experiment performed at the high-resolving-power magnetic spectrometer FRS at GSI allowed to identify 45 new heavy neutron-rich nuclei: $^{205}$Pt, $^{207-210}$Au, $^{211-216}$Hg, $^{213-217}$Tl, $^{215-220}$Pb, $^{219-224}$Bi, $^{221-227}$Po, $^{224-229}$At, $^{229-231}$Rn and $^{233}$Fr. The production cross sections of these nuclei were also determined and used to benchmark reaction codes that predict the production of nuclei far from stability., Comment: 5 pages, 2 figures

The existence of nuclei with exotic combinations of protons and neutrons provides fundamental information on the forces acting between nucleons. The maximum number of neutrons a given number of protons can bind, neutron drip line1, is only known for the lightest chemical elements, up to oxygen. For heavier elements, the larger its atomic number, the farther from this limit is the most neutron-rich known isotope. The properties of heavy neutron-rich nuclei also have a direct impact on understanding the observed abundances of chemical elements heavier than iron in our Universe. Above half of the abundances of these elements are thought to be produced in rapid-neutron capture reactions, r-process, taking place in violent stellar scenarios2 where heavy neutron-rich nuclei, far beyond the ones known up today, are produced. Here we present a major step forward in the production of heavy neutron-rich nuclei: the discovery of 73 new neutron-rich isotopes of chemical elements between tantalum (Z=72) and actinium (Z=89). This result proves that cold-fragmentation reactions3 at relativistic energies are governed by large fluctuations in isospin and energy dissipation making possible the massive production of heavy neutron-rich nuclei, paving then the way for the full understanding of the origin of the heavier elements in our Universe. It is expected that further studies providing ground and structural properties of the nuclei presented here will reveal further details on the nuclear shell evolution along Z=82 and N=126, but also on the understanding of the stellar nucleosyntheis r-process around the waiting point at A~190 defining the speed of the matter flow towards heavier fissioning nuclei.

Production cross sections of medium-mass neutron-rich nuclei obtained in the fragmentation of 136Xe projectiles at 1 A GeV have been measured with the FRagment Separator (FRS) at GSI. 125Pd was identified for the first time. The measured cross sections are compared to 238U fission yields and model calculations in order to determine the optimum reaction mechanism to extend the limits of the chart of the nuclides around the r-process waiting point at N=82., Comment: 9 pages, 6 figures

This paper presents the nuclide cross sections and the longitudinal velocity distributions of residues produced in the reactions of 136Xe and 124Xe at 1 A GeV in a lead target, measured at the high-resolution magnetic spectrometer, the Fragment Separator (FRS) of GSI. The data cover a broad range of isotopes of the elements between Z = 3 and Z = 56 for 136Xe and between Z = 5 and Z = 55 for 124Xe, reaching down to cross sections of a few microbarns. The velocity distributions exhibit a Gaussian shape for masses above A = 20, while more complex behaviour is observed for lighter masses. The isotopic distributions for both reactions preserve a memory on the projectile N/Z ratio over the whole residue mass range., Comment: 31 pages, 9 figures, 1 table, background information on http://www.gsi.de/charms

Heavy neutron-rich nuclei close to N=126 were produced by fragmentation of a 1 A GeV 208Pb beam at the FRS at GSI. The beta-decay half-lives of 8 nuclides have been determined. The comparison of the data with model calculations including an approach based on the self-consistent ground-state description and continuum QRPA considering the Gamow-Teller and first-forbidden decays provide a first indication on the importance of first-forbidden transitions around A=195. The measured data indicate that the matter flow in the r-process to heavier fissioning nuclei is faster than previously expected., Comment: 4 pages, 4 figures

We present an extensive overview of production cross sections and kinetic energies for the complete set of nuclides formed in the spallation of 136Xe by protons at the incident energy of 1 GeV per nucleon. The measurement was performed in inverse kinematics at the FRagment Separator (GSI, Darmstadt). Slightly below the Businaro-Gallone point, 136Xe is the stable nuclide with the largest neutron excess. The kinematic data and cross sections collected in this work for the full nuclide production are a general benchmark for modelling the spallation process in a neutron-rich nuclear system, where fission is characterised by predominantly mass-asymmetric splits., Comment: 18 pages, 14 figures

The spallation residues produced in the bombardment of 56}Fe at 1.5, 1.0, 0.75, 0.5 and 0.3 A GeV on a liquid-hydrogen target have been measured using the reverse kinematics technique and the Fragment Separator at GSI (Darmstadt). This technique has permitted the full identification in charge and mass of all isotopes produced with cross-sections larger than 10^{-2} mb down to Z=8. Their individual production cross-sections and recoil velocities at the five energies are presented. Production cross-sections are compared to previously existing data and to empirical parametric formulas, often used in cosmic-ray astrophysics. The experimental data are also extensively compared to different combinations of intra-nuclear cascade and de-excitation models. It is shown that the yields of the lightest isotopes cannot be accounted for by standard evaporation models. The GEMINI model, which includes an asymmetric fission decay mode, gives an overall good agreement with the data. These experimental data can be directly used for the estimation of composition modifications and damages in materials containing iron in spallation sources. They are also useful for improving high precision cosmic-ray measurements., Comment: Submited to Phys. Rev. C (10/2006)

The production cross sections of fragmentation-evaporation residues in the reaction Pb+p at 500A MeV have been measured using the inverse-kinematics method and the FRS spectrometer (GSI). Fragments were identified in nuclear charge using ionisation chambers. The mass identification was performed event-by-event using the B-rho - TOF - Delta-E technique. Although partially-unresolved ionic charge states induced an ambiguity on the mass of some heavy fragments, production rates could be obtained with a high accuracy by systematically accounting for the polluting ionic charge states. The contribution of multiple reactions in the target was subtracted using a new, partly self-consistent code. The isobaric distributions are found to have a shape very close to the one observed in experiments at higher energy. Kinematic properties of the fragments were also measured. The total and the isotopic cross sections, including charge-pickup cross sections, are in good agreement with previous measurements. The data are discussed in the light of previous spallation measurements, especially on lead at 1 GeV.

The feasibility of low-energy fragmentation experiments using a magnetic spectrometer is discussed. The main challenge is the multiplicity of the ionic charge states, which can hamper the identification in both Z and A of the fragments. Three topics are covered. First, a specific set-up for ionization chambers, based on a very large gas thickness, is presented. Its satisfactory performances are discussed in light of the observations during a 500A MeV Pb+p experiment performed at the FRS (GSI). As a second topic, the possibility to use a thick layer of matter (a degrader) as a passive measurement device to identify the nuclear charge and the ionic charge state of fragments is discussed. This method, successfully used for Z identification in experiments such as Pb+p at 1A GeV, fails to measure the charge states at 500A MeV for the same system. It is shown that surface defects of the degrader are probably responsible for this failure. The third topic is the description of new analysis techniques developed in order to account for and subtract the contribution of polluting charge states in the spectrometer, thus making possible a clean estimation of the production cross sections of all fragments. The combination of those new experimental and analysis techniques made the 500A MeV spallation experiment a success.