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Quantum controls realize the unitary or nonunitary operations employed in quantum computers, quantum simulators, quantum communications, and other quantum information devices. They implement the desired quantum dynamics with the help of electric, magnetic, or electromagnetic control fields. Quantum optimal control (QOC) deals with designing an optimal control field modulation that most precisely implements a desired quantum operation with minimum energy consumption and maximum robustness against hardware imperfections as well as external noise. Over the last 2 decades, numerous QOC methods have been proposed. They include asymptotic methods, direct search, gradient methods, variational methods, machine learning methods, etc. In this review, we shall introduce the basic ideas of QOC, discuss practical challenges, and then take an overview of the diverse QOC methods.

The standard procedure for quantum process tomography (QPT) requires a series of experiments. Each experiment involves initialization of the system to a particular basis state, applying the quantum process e on the system, and finally characterizing the output state by quantum state tomography (QST). The output states collected for a complete set of basis states enable us to calculate the / matrix characterizing the process e. The standard procedure for QST itself requires independent experiments, each involving measurement of a set of commuting observables. Thus QPT procedure demands a number of independent measurements and, moreover, this number increases rapidly with the size of the system. However, in ensemble systems, the total number of independent measurements can be greatly reduced with the availability of ancilla qubits. Ancilla-assisted process tomography (AAPT) has earlier been shown to require a single QST of system-ancilla space. Ancilla-assisted quantum state tomography (AAQST) has also been shown to perform QST in a single-scan measurement of an ensemble system. Here we combine AAPT with AAQST to realize a single-scan QPT (SSPT), a procedure to characterize a general quantum process in a single ensemble measurement. We demonstrate experimental SSPT by characterizing several single-qubit processes using a three-qubit NMR quantum register. Furthermore, using the SSPT procedure, we experimentally characterize the twirling process and compare the results with theory. [ABSTRACT FROM AUTHOR]

Precise experimental implementation of unitary operators is one of the most important tasks for quantum information processing. Numerical optimization techniques are widely used to find optimized control fields to realize a desired unitary operator. However, finding high-fidelity control pulses to realize an arbitrary unitary operator in larger spin systems is still a difficult task. In this work, we demonstrate that a combination of the GRAPE algorithm, which is a numerical pulse optimization technique, and a unitary operator decomposition algorithm [Ajoy et al, Phys. Rev. A 85, 030303 (2012)] can realize unitary operators with high experimental fidelity. This is illustrated by simulating the mirror-inversion propagator of an XY spin chain in a five-spin dipolar coupled nuclear spin system. Further, this simulation has been used to demonstrate the transfer of entangled states from one end of the spin chain to the other end. [ABSTRACT FROM AUTHOR]

Due to omnipresent environmental interferences, quantum coherences inevitably undergo irreversible transformations over certain time scales, thus leading to the loss of encoded information. This process, known as decoherence, has been a major obstacle in realizing efficient quantum information processors. Understanding the mechanism of decoherence is crucial in developing tools to inhibit it. Here we utilize a method proposed by Teklemariam et al. [Phys. Rev. A 67, 062316 (2003)] to engineer artificial decoherence in the system qubits by randomly perturbing their surrounding ancilla qubits. Using a two-qubit nuclear magnetic resonance quantum register, we characterize the artificial decoherence by noise spectroscopy and quantum process tomography. Further, we study the efficacy of dynamical decoupling sequences in suppressing the artificial decoherence. Here we describe the experimental results and their comparisons with theoretical simulations. [ABSTRACT FROM AUTHOR]

Stroboscopic spin flips have already been shown to prolong the coherence times of quantum systems under noisy environments. Uhrig's dynamical decoupling scheme provides an optimal sequence for a quantum system interacting with a dephasing bath. Several experimental demonstrations have already verified the efficiency of such dynamical decoupling schemes in preserving single-qubit coherences. In this work we describe the experimental study of Uhrig's dynamical decoupling in preserving two-qubit entangled states using an ensemble of spin-1/2 nuclear pairs in solution state. We find that the performance of odd-order Uhrig sequences in preserving entanglement is superior to both even-order Uhrig sequences and periodic spin-flip sequences. We also find that there exists an optimal order of the Uhrig sequence in which a singlet state can be stored at high correlation for about 30 seconds. [ABSTRACT FROM AUTHOR]

Use of dipolar and quadrupolar couplings for quantum information processing (QIP) by nuclear magnetic resonance (NMR) is described. In these cases, instead of the individual spins being qubits, the 2nenergy levels of the spin-system can be treated as an n-qubit system. It is demonstrated that QIP in such systems can be carried out using transition-selective pulses, in CH3CN, 13CH3CN, 7Li (I=3/2) and 133Cs (I=7/2), oriented in liquid crystals yielding 2 and 3 qubit systems. Creation of pseudopure states, implementation of logic gates and arithmetic operations (half-adder and subtractor) have been carried out in these systems using transition-selective pulses.

We report a nuclear magnetic resonance experiment, which simulates the quantum transverse Ising spin system in a triangular configuration, and further demonstrate that multipartite quantum correlations can be used to distinguish between the frustrated and the nonfrustrated regimes in the ground state of this system. Adiabatic state preparation methods are used to prepare the ground states of the spin system. We employ two different multipartite quantum correlation measures to analyze the experimental ground state of the system in both the frustrated and the nonfrustrated regimes. As expected from theoretical predictions, the experimental data confirm that the nonfrustrated regime shows higher multipartite quantum correlations compared to the frustrated one. [ABSTRACT FROM AUTHOR]

The standard method of quantum state tomography (QST) relies on the measurement of a set of noncommuting observables, realized in a series of independent experiments. Ancilla-assisted QST (AAQST) proposed by Nieuwenhuizen arid co-workers [Phys. Rev. Lett. 92, 120402 (2004)] greatly reduces the number of independent measurements by exploiting an ancilla register in a known initial state. In suitable conditions AAQST allows mapping out density matrix of an input register in a single experiment. Here we describe methods for explicit construction of AAQST experiments in multiqubit registers. We also report nuclear magnetic resonance studies on AAQST of (i) a two-qubit input register using a one-qubit ancilla in an isotropic liquid-state system and (ii) a three-qubit input register using a two-qubit ancilla register in a partially oriented system. The experimental results confirm the effectiveness of AAQST in such multiqubit registers [ABSTRACT FROM AUTHOR]

We investigate evolution of quantum correlations in ensembles of two-qubit nuclear spin systems via nuclear magnetic resonance techniques. We use discord as a measure of quantum correlations and the Werner state as an explicit example. We, first, introduce different ways of measuring discord and geometric discord in two-qubit systems and then describe the following experimental studies:(a) We quantitatively measure discord for Werner-like states prepared using an entangling pulse sequence. An initial thermal state with zero discord is gradually and periodically transformed into a mixed state with maximum discord. The experimental and simulated behavior of rise and fall of discord agree fairly well. (b) We examine the efficiency of dynamical decoupling sequences in preserving quantum correlations. In out experimental setup, the dynamical decoupling sequences preserved the traceless parts of the density matrices at high fidelity. But they could not maintain the purity of the quantum states and so were unable to keep the discord from decaying. (c) We observe the evolution of discord for a singlet-triplet mixed state during a radio-frequency. spin-lock. A simple relaxation model describes the evolution of discord, and the accompanying evolution of fidelity of the long-lived singlet state, reasonably well. [ABSTRACT FROM AUTHOR]

We report an experimental demonstration of a quantum delayed-choice experiment via nuclear magnetic resonance techniques. Two spin-1 /2 nuclei from each molecule of a liquid ensemble are used as target and ancilla qubits. The circuit corresponding to the recently proposed quantum delayed-choice setup has been implemented with different states of an ancilla qubit. As expected theoretically, our experiments clearly demonstrate continuous morphing of the target qubit between particle-like and wave-like behaviors. The experimental visibility of the interference patterns shows good agreement with theory. [ABSTRACT FROM AUTHOR]

Characterizing and understanding noise affecting quantum states has immense benefits in spectroscopy as well as in realizing quantum devices. Transverse relaxation times under a set of dynamical decoupling (DD) sequences with varying interpulse delays were earlier used for obtaining the noise spectral densities of single-qubit coherences. In this work, using a pair of homonuclear spins and NMR techniques, we experimentally characterize noise in certain decoherence-free subspaces. We also explore the noise of similar states in a heteronuclear spin pair. Further, using a 10-qubit system, we investigate noise profiles of various multiqubit coherences and study the scaling of noise with respect to the coherence order. Finally, using the experimentally obtained noise spectrum of the 10-qubit NOON state, we predict the performance of a Uhrig DD sequence and verify it experimentally. [ABSTRACT FROM AUTHOR]

A robust control over quantum dynamics is of paramount importance for quantum technologies. Many of the existing control techniques are based on smooth Hamiltonian modulations involving repeated calculations of basic unitaries resulting in time complexities scaling rapidly with the length of the control sequence. Here we show that bang-bang controls need one-time calculation of basic unitaries and hence scale much more efficiently. By employing a global optimization routine such as the genetic algorithm, it is possible to synthesize not only highly intricate unitaries, but also certain nonunitary operations. We demonstrate the unitary control through the implementation of the optimal fixed-point quantum search algorithm in a three-qubit nuclear magnetic resonance (NMR) system. Moreover, by combining the bang-bang pulses with the crusher gradients, we also demonstrate nonunitary transformations of thermal equilibrium states into effective pure states in three- as well as five-qubit NMR systems. [ABSTRACT FROM AUTHOR]

The interaction of molecules with light may lead to electronic transitions and simultaneous vibrational excitations. Franck-Condon factors (FCFs) play an important role in quantifying the intensities of such vibronic transitions occurring during molecular photoexcitations. In this article, we describe a general method for estimating FCFs using a quantum information processor. The method involves the application of a translation operator followed by the measurement of certain projections. We also illustrate the method by experimentally estimating FCFs with the help of a three-qubit nuclear magnetic resonance quantum information processor. We describe two methods for the measurement of projections: (i) using the Moussa protocol and (ii) using diagonal tomography. The experimental results agree fairly well with the theory. [ABSTRACT FROM AUTHOR]

A sequence of moments obtained from statistical trials encodes a classical probability distribution. However, it is well known, that an incompatible set of moments arises in the quantum scenario, when correlation outcomes associated with measurements on spatially separated entangled states are considered. This feature, viz., the incompatibility of moments with a joint probability distribution, is reflected in the violation of Bell inequalities. Here, we focus on sequential measurements on a single quantum system and investigate if moments and joint probabilities are compatible with each other. By considering sequential measurement of a dichotomic dynamical observable at three different time intervals, we explicitly demonstrate that the moments and the probabilities are inconsistent with each other. Experimental results using a nuclear magnetic resonance system are reported here to corroborate these theoretical observations, viz., the incompatibility of the three-time joint probabilities with those extracted from the moment sequence when sequential measurements on a single-qubit system are considered. [ABSTRACT FROM AUTHOR]

We report an experimental study of recently formulated entropie Leggett-Garg inequality (ELGI) by Usha Devi etal. [Phys. Rev. A 87, 052103 (2013)]. This inequality places a bound on the statistical measurement outcomes of dynamical observables describing a macrorealistic system. Such a bound is not necessarily obeyed by quantum systems, and therefore provides an important way to distinguish quantumness from classical behavior. Here we study ELGI using a two-qubit nuclear magnetic resonance system. To perform the noninvasive measurements required for the ELGI study, we prepare the system qubit in a maximally mixed state as well as use the "ideal negative result measurement" procedure with the help of an ancilla qubit. The experimental results show a clear violation of ELGI by over four standard deviations. These results agree with the predictions of quantum theory. The violation of ELGI is attributed to the fact that certain joint probabilities are not legitimate in the quantum scenario, in the sense they do not reproduce all the marginal probabilities. Using a three-qubit system, we also demonstrate that three-time joint probabilities do not reproduce certain two-time marginal probabilities. [ABSTRACT FROM AUTHOR]

Cooling the qubit into a pure initial state is crucial for realizing fault-tolerant quantum information processing. Here we envisage a star-topology arrangement of reset and computation qubits for this purpose. The reset qubits cool or purify the computation qubit by transferring its entropy to a heat bath with the help of a heat-bath algorithmic cooling procedure. By combining standard NMR methods with powerful quantum control techniques, we cool central qubits of two large star-topology systems, with 13 and 37 spins, respectively. We obtain polarization enhancements by a factor of over 24, and an associated reduction in the spin temperature from 298 K down to 12 K. Exploiting the enhanced polarization of computation qubit, we prepare combination coherences of orders up to 15. By benchmarking the decay of these coherences we investigate the underlying noise process. Further, we also cool a pair of computation qubits and subsequently prepare them in an effective pure state. [ABSTRACT FROM AUTHOR]