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The Australian Community Climate and Earth System Simulator (ACCESS) has contributed to the World Climate Research Programme’s Coupled Model Intercomparison Project Phase 6 (CMIP6) using two fully coupled model versions (ACCESS-CM2 and ACCESS-ESM1.5) and two ocean–sea-ice model versions (1° and 0.25° resolution versions of ACCESS-OM2). The fully coupled models differ primarily in the configuration and version of their atmosphere components (including the aerosol scheme), with smaller differences in their sea-ice and land model versions. Additionally, ACCESS-ESM1.5 includes biogeochemistry in the land and ocean components and can be run with an interactive carbon cycle. CMIP6 comprises core experiments and associated thematic Model Intercomparison Projects (MIPs). This paper provides an overview of the CMIP6 submission, including the methods used for the preparation of input forcing datasets and the post-processing of model output, along with a comprehensive list of experiments performed, detailing their initialisation, duration, ensemble number and computational cost. A small selection of model output is presented, focusing on idealised experiments and their variants at global scale. Differences in the climate simulation of the two coupled models are highlighted. ACCESS-CM2 produces a larger equilibrium climate sensitivity (4.7°C) than ACCESS-ESM1.5 (3.9°C), likely a result of updated atmospheric parameterisation in recent versions of the atmospheric component of ACCESS-CM2. The idealised experiments run with ACCESS-ESM1.5 show that land and ocean carbon fluxes respond to both changing atmospheric CO2 and to changing temperature. ACCESS data submitted to CMIP6 are available from the Earth System Grid Federation (https://doi.org/10.22033/ESGF/CMIP6.2281 and https://doi.org/10.22033/ESGF/CMIP6.2288). The information provided in this paper should facilitate easier use of these significant datasets by the broader climate community.

The Australian Community Climate and Earth System Simulator (ACCESS) has contributed to the World Climate Research Programme’s Coupled Model Intercomparison Project Phase 6 (CMIP6) using two fully coupled model versions (ACCESS-CM2 and ACCESS-ESM1.5) and two ocean–sea-ice model versions (1° and 0.25° resolution versions of ACCESS-OM2). The fully coupled models differ primarily in the configuration and version of their atmosphere components (including the aerosol scheme), with smaller differences in their sea-ice and land model versions. Additionally, ACCESS-ESM1.5 includes biogeochemistry in the land and ocean components and can be run with an interactive carbon cycle. CMIP6 comprises core experiments and associated thematic Model Intercomparison Projects (MIPs). This paper provides an overview of the CMIP6 submission, including the methods used for the preparation of input forcing datasets and the post-processing of model output, along with a comprehensive list of experiments performed, detailing their initialisation, duration, ensemble number and computational cost. A small selection of model output is presented, focusing on idealised experiments and their variants at global scale. Differences in the climate simulation of the two coupled models are highlighted. ACCESS-CM2 produces a larger equilibrium climate sensitivity (4.7°C) than ACCESS-ESM1.5 (3.9°C), likely a result of updated atmospheric parameterisation in recent versions of the atmospheric component of ACCESS-CM2. The idealised experiments run with ACCESS-ESM1.5 show that land and ocean carbon fluxes respond to both changing atmospheric CO2 and to changing temperature. ACCESS data submitted to CMIP6 are available from the Earth System Grid Federation (https://doi.org/10.22033/ESGF/CMIP6.2281 and https://doi.org/10.22033/ESGF/CMIP6.2288). The information provided in this paper should facilitate easier use of these significant datasets by the broader climate community.

The Australian Community Climate and Earth System Simulator (ACCESS) has contributed to the World Climate Research Programme’s Coupled Model Intercomparison Project Phase 6 (CMIP6) using two fully coupled model versions (ACCESS-CM2 and ACCESS-ESM1.5) and two ocean–sea-ice model versions (1° and 0.25° resolution versions of ACCESS-OM2). The fully coupled models differ primarily in the configuration and version of their atmosphere components (including the aerosol scheme), with smaller differences in their sea-ice and land model versions. Additionally, ACCESS-ESM1.5 includes biogeochemistry in the land and ocean components and can be run with an interactive carbon cycle. CMIP6 comprises core experiments and associated thematic Model Intercomparison Projects (MIPs). This paper provides an overview of the CMIP6 submission, including the methods used for the preparation of input forcing datasets and the post-processing of model output, along with a comprehensive list of experiments performed, detailing their initialisation, duration, ensemble number and computational cost. A small selection of model output is presented, focusing on idealised experiments and their variants at global scale. Differences in the climate simulation of the two coupled models are highlighted. ACCESS-CM2 produces a larger equilibrium climate sensitivity (4.7°C) than ACCESS-ESM1.5 (3.9°C), likely a result of updated atmospheric parameterisation in recent versions of the atmospheric component of ACCESS-CM2. The idealised experiments run with ACCESS-ESM1.5 show that land and ocean carbon fluxes respond to both changing atmospheric CO2 and to changing temperature. ACCESS data submitted to CMIP6 are available from the Earth System Grid Federation (https://doi.org/10.22033/ESGF/CMIP6.2281 and https://doi.org/10.22033/ESGF/CMIP6.2288). The information provided in this paper should facilitate easier use of these significant datasets by the broader climate community.

The Australian Community Climate and Earth System Simulator (ACCESS) has contributed to the World Climate Research Programme’s Coupled Model Intercomparison Project Phase 6 (CMIP6) using two fully coupled model versions (ACCESS-CM2 and ACCESS-ESM1.5) and two ocean–sea-ice model versions (1° and 0.25° resolution versions of ACCESS-OM2). The fully coupled models differ primarily in the configuration and version of their atmosphere components (including the aerosol scheme), with smaller differences in their sea-ice and land model versions. Additionally, ACCESS-ESM1.5 includes biogeochemistry in the land and ocean components and can be run with an interactive carbon cycle. CMIP6 comprises core experiments and associated thematic Model Intercomparison Projects (MIPs). This paper provides an overview of the CMIP6 submission, including the methods used for the preparation of input forcing datasets and the post-processing of model output, along with a comprehensive list of experiments performed, detailing their initialisation, duration, ensemble number and computational cost. A small selection of model output is presented, focusing on idealised experiments and their variants at global scale. Differences in the climate simulation of the two coupled models are highlighted. ACCESS-CM2 produces a larger equilibrium climate sensitivity (4.7°C) than ACCESS-ESM1.5 (3.9°C), likely a result of updated atmospheric parameterisation in recent versions of the atmospheric component of ACCESS-CM2. The idealised experiments run with ACCESS-ESM1.5 show that land and ocean carbon fluxes respond to both changing atmospheric CO2 and to changing temperature. ACCESS data submitted to CMIP6 are available from the Earth System Grid Federation (https://doi.org/10.22033/ESGF/CMIP6.2281 and https://doi.org/10.22033/ESGF/CMIP6.2288). The information provided in this paper should facilitate easier use of these significant datasets by the broader climate community.

A method to construct transport matrices from standard ocean-model output, such as mean volume fluxes and mixed-layer depths, is presented. These transport matrices enable highly efficient calculation of deep-water tracer fields that otherwise require long integrations with forward time-stepping ocean models. Comparisons of matrix solutions for ideal mean water age demonstrate that the transport matrices are reasonably accurate representations of the transport in the parent ocean models. Tracer fields calculated using transport matrices provide simple circulation metrics that can be compared to observations. We compare matrix-computed radiocarbon distributions from two versions of ACCESS ocean models with observations. We find matrices based on both models produce realistic circulations; the radiocarbon distribution based on ACCESS forced with CORE climatology fits observations better in the deep Pacific, whereas the fully coupled ACCESS1.3 model fits observations better in the deep Atlantic. When applied to the circulations of ACCESS1.3 climate-change experiments, the transport-matrix solutions show an increase in radiocarbon depletion, or water age, in the projected ocean circulation for the 2090s under the RCP8.5 scenario. By computing the water-mass fractions last ventilated from specific regions, we diagnose a corresponding progressive shutdown in Antarctic Bottom Water formation. The volumetric decrease in Antarctic waters in the global ocean is compensated by an increase in waters last ventilated in the subantarctic and southern subtropics.

The exploration of alternative molecular hole-transporting materials (HTMs) specifically for high performance perovskite solar cells (PSCs) is a relatively recent research area. Aiming for further increasing the 'efficiency-cost ratio' of PSCs, we developed a spiro[fluorene-9,9'-xanthene] based HTM (X59) via two-step synthesis from commercial precursors for perovskite solar cells (PSCs) that works as effectively as the well-known HTM-Spiro-OMeTAD-based device under the same conditions. The molecular structure was analyzed by X-ray crystallography indicating a similar packing regime as for Spiro-OMeTAD. An impressive PCE of 19.8% was achieved by using X59 as HTM in PSC, which can compete with the record PCE of 20.8% by using the state-of-the-art-HTM Spiro-OMeTAD (Tress et al., 2016) [1]. The optimized devices employing X59 as HTM exhibited minimized hysteresis, excellent reproducibility and reasonable stability under dark and dry conditions. The present finding highlights the potential of spiro-type HTM for high performance PSCs and paves the way to a much deceased fabrication cost for potential commercialization of perovskite solar panels., QC 20160516

The most recent Intergovernmental Panel on Climate Change assessment report concludes that the Atlantic Meridional Overturning Circulation (AMOC) could weaken substantially but is very unlikely to collapse in the 21st century. However, the assessment largely neglected Greenland Ice Sheet (GrIS) mass loss, lacked a comprehensive uncertainty analysis, and was limited to the 21st century. Here in a community effort, improved estimates of GrIS mass loss are included in multicentennial projections using eight state‐of‐the‐science climate models, and an AMOC emulator is used to provide a probabilistic uncertainty assessment. We find that GrIS melting affects AMOC projections, even though it is of secondary importance. By years 2090–2100, the AMOC weakens by 18% [−3%, −34%; 90% probability] in an intermediate greenhouse‐gas mitigation scenario and by 37% [−15%, −65%] under continued high emissions. Afterward, it stabilizes in the former but continues to decline in the latter to −74% [+4%, −100%] by 2290–2300, with a 44% likelihood of an AMOC collapse. This result suggests that an AMOC collapse can be avoided by CO2 mitigation.

The most recent Intergovernmental Panel on Climate Change assessment report concludes that the Atlantic Meridional Overturning Circulation (AMOC) could weaken substantially but is very unlikely to collapse in the 21st century. However, the assessment largely neglected Greenland Ice Sheet (GrIS) mass loss, lacked a comprehensive uncertainty analysis, and was limited to the 21st century. Here in a community effort, improved estimates of GrIS mass loss are included in multicentennial projections using eight state‐of‐the‐science climate models, and an AMOC emulator is used to provide a probabilistic uncertainty assessment. We find that GrIS melting affects AMOC projections, even though it is of secondary importance. By years 2090–2100, the AMOC weakens by 18% [−3%, −34%; 90% probability] in an intermediate greenhouse‐gas mitigation scenario and by 37% [−15%, −65%] under continued high emissions. Afterward, it stabilizes in the former but continues to decline in the latter to −74% [+4%, −100%] by 2290–2300, with a 44% likelihood of an AMOC collapse. This result suggests that an AMOC collapse can be avoided by CO2 mitigation.

The most recent Intergovernmental Panel on Climate Change assessment report concludes that the Atlantic Meridional Overturning Circulation (AMOC) could weaken substantially but is very unlikely to collapse in the 21st century. However, the assessment largely neglected Greenland Ice Sheet (GrIS) mass loss, lacked a comprehensive uncertainty analysis, and was limited to the 21st century. Here in a community effort, improved estimates of GrIS mass loss are included in multicentennial projections using eight state‐of‐the‐science climate models, and an AMOC emulator is used to provide a probabilistic uncertainty assessment. We find that GrIS melting affects AMOC projections, even though it is of secondary importance. By years 2090–2100, the AMOC weakens by 18% [−3%, −34%; 90% probability] in an intermediate greenhouse‐gas mitigation scenario and by 37% [−15%, −65%] under continued high emissions. Afterward, it stabilizes in the former but continues to decline in the latter to −74% [+4%, −100%] by 2290–2300, with a 44% likelihood of an AMOC collapse. This result suggests that an AMOC collapse can be avoided by CO2 mitigation.

In the framework of the second phase of the Coordinated Ocean-ice Reference Experiments (CORE-II), we present an analysis of the representation of the Antarctic Circumpolar Current (ACC) and Southern Ocean meridional overturning circulation (MOC) in a suite of seventeen global ocean–sea ice models. We focus on the mean, variability and trends of both the ACC and MOC over the 1958–2007 period, and discuss their relationship with the surface forcing. We aim to quantify the degree of eddy saturation and eddy compensation in the models participating in CORE-II, and compare our results with available observations, previous fine-resolution numerical studies and theoretical constraints. Most models show weak ACC transport sensitivity to changes in forcing during the past five decades, and they can be considered to be in an eddy saturated regime. Larger contrasts arise when considering MOC trends, with a majority of models exhibiting significant strengthening of the MOC during the late 20th and early 21st century. Only a few models show a relatively small sensitivity to forcing changes, responding with an intensified eddy-induced circulation that provides some degree of eddy compensation, while still showing considerable decadal trends. Both ACC and MOC interannual variabilities are largely controlled by the Southern Annular Mode (SAM). Based on these results, models are clustered into two groups. Models with constant or two-dimensional (horizontal) specification of the eddy-induced advection coefficient κ show larger ocean interior decadal trends, larger ACC transport decadal trends and no eddy compensation in the MOC. Eddy-permitting models or models with a three-dimensional time varying κ show smaller changes in isopycnal slopes and associated ACC trends, and partial eddy compensation. As previously argued, a constant in time or space κ is responsible for a poor representation of mesoscale eddy effects and cannot properly simulate the sensitivity of the ACC and MOC to ch

We characterise the representation of the Southern Ocean water mass structure and sea ice within a suite of 15 global ocean-ice models run with the Coordinated Ocean-ice Reference Experiment Phase II (CORE-II) protocol. The main focus is the representation of the present (1988–2007) mode and intermediate waters, thus framing an analysis of winter and summer mixed layer depths; temperature, salinity, and potential vorticity structure; and temporal variability of sea ice distributions. We also consider the interannual variability over the same 20 year period. Comparisons are made between models as well as to observation-based analyses where available. The CORE-II models exhibit several biases relative to Southern Ocean observations, including an underestimation of the model mean mixed layer depths of mode and intermediate water masses in March (associated with greater ocean surface heat gain), and an overestimation in September (associated with greater high latitude ocean heat loss and a more northward winter sea-ice extent). In addition, the models have cold and fresh/warm and salty water column biases centred near 50°S. Over the 1988–2007 period, the CORE-II models consistently simulate spatially variable trends in sea-ice concentration, surface freshwater fluxes, mixed layer depths, and 200–700 m ocean heat content. In particular, sea-ice coverage around most of the Antarctic continental shelf is reduced, leading to a cooling and freshening of the near surface waters. The shoaling of the mixed layer is associated with increased surface buoyancy gain, except in the Pacific where sea ice is also influential. The models are in disagreement, despite the common CORE-II atmospheric state, in their spatial pattern of the 20-year trends in the mixed layer depth and sea-ice.

We characterise the representation of the Southern Ocean water mass structure and sea ice within a suite of 15 global ocean-ice models run with the Coordinated Ocean-ice Reference Experiment Phase II (CORE-II) protocol. The main focus is the representation of the present (1988–2007) mode and intermediate waters, thus framing an analysis of winter and summer mixed layer depths; temperature, salinity, and potential vorticity structure; and temporal variability of sea ice distributions. We also consider the interannual variability over the same 20 year period. Comparisons are made between models as well as to observation-based analyses where available. The CORE-II models exhibit several biases relative to Southern Ocean observations, including an underestimation of the model mean mixed layer depths of mode and intermediate water masses in March (associated with greater ocean surface heat gain), and an overestimation in September (associated with greater high latitude ocean heat loss and a more northward winter sea-ice extent). In addition, the models have cold and fresh/warm and salty water column biases centred near 50°S. Over the 1988–2007 period, the CORE-II models consistently simulate spatially variable trends in sea-ice concentration, surface freshwater fluxes, mixed layer depths, and 200–700 m ocean heat content. In particular, sea-ice coverage around most of the Antarctic continental shelf is reduced, leading to a cooling and freshening of the near surface waters. The shoaling of the mixed layer is associated with increased surface buoyancy gain, except in the Pacific where sea ice is also influential. The models are in disagreement, despite the common CORE-II atmospheric state, in their spatial pattern of the 20-year trends in the mixed layer depth and sea-ice.

We provide an assessment of sea level simulated in a suite of global ocean-sea ice models using the interannual CORE atmospheric state to determine surface ocean boundary buoyancy and momentum fluxes. These CORE-II simulations are compared amongst themselves as well as to observation-based estimates. We focus on the final 15 years of the simulations (1993–2007), as this is a period where the CORE-II atmospheric state is well sampled, and it allows us to compare sea level related fields to both satellite and in situ analyses. The ensemble mean of the CORE-II simulations broadly agree with various global and regional observation-based analyses during this period, though with the global mean thermosteric sea level rise biased low relative to observation-based analyses. The simulations reveal a positive trend in dynamic sea level in the west Pacific and negative trend in the east, with this trend arising from wind shifts and regional changes in upper 700 m ocean heat content. The models also exhibit a thermosteric sea level rise in the subpolar North Atlantic associated with a transition around 1995/1996 of the North Atlantic Oscillation to its negative phase, and the advection of warm subtropical waters into the subpolar gyre. Sea level trends are predominantly associated with steric trends, with thermosteric effects generally far larger than halosteric effects, except in the Arctic and North Atlantic. There is a general anti-correlation between thermosteric and halosteric effects for much of the World Ocean, associated with density compensated changes.

Simulation characteristics from eighteen global ocean–sea-ice coupled models are presented with a focus on the mean Atlantic meridional overturning circulation (AMOC) and other related fields in the North Atlantic. These experiments use inter-annually varying atmospheric forcing data sets for the 60-year per- iod from 1948 to 2007 and are performed as contributions to the second phase of the Coordinated Ocean- ice Reference Experiments (CORE-II). The protocol for conducting such CORE-II experiments is summa- rized. Despite using the same atmospheric forcing, the solutions show significant differences. As most models also differ from available observations, biases in the Labrador Sea region in upper-ocean potential temperature and salinity distributions, mixed layer depths, and sea-ice cover are identified as contribu- tors to differences in AMOC. These differences in the solutions do not suggest an obvious grouping of the models based on their ocean model lineage, their vertical coordinate representations, or surface salinity restoring strengths. Thus, the solution differences among the models are attributed primarily to use of different subgrid scale parameterizations and parameter choices as well as to differences in vertica and horizontal grid resolutions in the ocean models. Use of a wide variety of sea-ice models with diverse snow and sea-ice albedo treatments also contributes to these differences. Based on the diagnostics con- sidered, the majority of the models appear suitable for use in studies involving the North Atlantic, but some models require dedicated development effort.

We provide an assessment of sea level simulated in a suite of global ocean-sea ice models using the interannual CORE atmospheric state to determine surface ocean boundary buoyancy and momentum fluxes. These CORE-II simulations are compared amongst themselves as well as to observation-based estimates. We focus on the final 15 years of the simulations (1993–2007), as this is a period where the CORE-II atmospheric state is well sampled, and it allows us to compare sea level related fields to both satellite and in situ analyses. The ensemble mean of the CORE-II simulations broadly agree with various global and regional observation-based analyses during this period, though with the global mean thermosteric sea level rise biased low relative to observation-based analyses. The simulations reveal a positive trend in dynamic sea level in the west Pacific and negative trend in the east, with this trend arising from wind shifts and regional changes in upper 700 m ocean heat content. The models also exhibit a thermosteric sea level rise in the subpolar North Atlantic associated with a transition around 1995/1996 of the North Atlantic Oscillation to its negative phase, and the advection of warm subtropical waters into the subpolar gyre. Sea level trends are predominantly associated with steric trends, with thermosteric effects generally far larger than halosteric effects, except in the Arctic and North Atlantic. There is a general anti-correlation between thermosteric and halosteric effects for much of the World Ocean, associated with density compensated changes.

Simulation characteristics from eighteen global ocean–sea-ice coupled models are presented with a focus on the mean Atlantic meridional overturning circulation (AMOC) and other related fields in the North Atlantic. These experiments use inter-annually varying atmospheric forcing data sets for the 60-year per- iod from 1948 to 2007 and are performed as contributions to the second phase of the Coordinated Ocean- ice Reference Experiments (CORE-II). The protocol for conducting such CORE-II experiments is summa- rized. Despite using the same atmospheric forcing, the solutions show significant differences. As most models also differ from available observations, biases in the Labrador Sea region in upper-ocean potential temperature and salinity distributions, mixed layer depths, and sea-ice cover are identified as contribu- tors to differences in AMOC. These differences in the solutions do not suggest an obvious grouping of the models based on their ocean model lineage, their vertical coordinate representations, or surface salinity restoring strengths. Thus, the solution differences among the models are attributed primarily to use of different subgrid scale parameterizations and parameter choices as well as to differences in vertica and horizontal grid resolutions in the ocean models. Use of a wide variety of sea-ice models with diverse snow and sea-ice albedo treatments also contributes to these differences. Based on the diagnostics con- sidered, the majority of the models appear suitable for use in studies involving the North Atlantic, but some models require dedicated development effort.

There is a growing number of observation-based measures of sea level related patterns with the advent of the Argo floats (since the early 2000s) and satellite altimeters (since 1993). These measures provide a valuable means to evaluate aspects of global model simulations, such as the global ocean-sea ice simulations run as part of the interannual Coordinated Ocean- ice Reference Experiments Griffies et al. (2009), Danabasoglu et al. (2013). In addition, these CORE-II simulations provide a means for evaluating the likely mechanisms causing sea level variations, particularly when models with different skill are compared against each other and observations. We have conducted an assessment of CORE-II simulations from 13 model configurations Griffies et al. (2013), with a focus on their ability to capture observed trends in ocean heat content as well as the corresponding dynamic sea level over the period 1993- 2007. Here, we provide a synopsis of the assessment.

There is a growing number of observation-based measures of sea level related patterns with the advent of the Argo floats (since the early 2000s) and satellite altimeters (since 1993). These measures provide a valuable means to evaluate aspects of global model simulations, such as the global ocean-sea ice simulations run as part of the interannual Coordinated Ocean- ice Reference Experiments Griffies et al. (2009), Danabasoglu et al. (2013). In addition, these CORE-II simulations provide a means for evaluating the likely mechanisms causing sea level variations, particularly when models with different skill are compared against each other and observations. We have conducted an assessment of CORE-II simulations from 13 model configurations Griffies et al. (2013), with a focus on their ability to capture observed trends in ocean heat content as well as the corresponding dynamic sea level over the period 1993- 2007. Here, we provide a synopsis of the assessment.