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In this article, the authors report the Chebyshev pseudospectral method for solving twodimensional nonlinear Schrodinger equation with fractional order derivative in time and space both. The modified Riemann-Liouville fractional derivatives are used to define the new fractional derivatives matrix at CGL points. Using the Chebyshev fractional derivatives matrices, the given problem is reduced to a diagonally block system of nonlinear algebraic equations, which will be solved using Newton’s Raphson method. The proposed methods have shown error analysis without any dependency on time and space step restrictions. Some model examples of the equations, defined on a convex and rectangular domain, have tested with various values of fractional order α and β. Moreover, numerical solutions are demonstrated to justify the theoretical results.