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Humans rely increasingly on sensors to address grand challenges and to improve quality of life in the era of digitalization and big data. For ubiquitous sensing, flexible sensors are developed to overcome the limitations of conventional rigid counterparts. Despite rapid advancement in bench-side research over the last decade, the market adoption of flexible sensors remains limited. To ease and to expedite their deployment, here, we identify bottlenecks hindering the maturation of flexible sensors and propose promising solutions. We first analyze challenges in achieving satisfactory sensing performance for real-world applications and then summarize issues in compatible sensor-biology interfaces, followed by brief discussions on powering and connecting sensor networks. Issues en route to commercialization and for sustainable growth of the sector are also analyzed, highlighting environmental concerns and emphasizing nontechnical issues such as business, regulatory, and ethical considerations. Additionally, we look at future intelligent flexible sensors. In proposing a comprehensive roadmap, we hope to steer research efforts towards common goals and to guide coordinated development strategies from disparate communities. Through such collaborative efforts, scientific breakthroughs can be made sooner and capitalized for the betterment of humanity.

Neurotransmitters play essential roles in regulating neural circuit dynamics both in the central nervous system as well as at the peripheral, including the gastrointestinal tract1-3. Their real-time monitoring will offer critical information for understanding neural function and diagnosing disease1-3. However, bioelectronic tools to monitor the dynamics of neurotransmitters in vivo, especially in the enteric nervous systems, are underdeveloped. This is mainly owing to the limited availability of biosensing tools that are capable of examining soft, complex and actively moving organs. Here we introduce a tissue-mimicking, stretchable, neurochemical biological interface termed NeuroString, which is prepared by laser patterning of a metal-complexed polyimide into an interconnected graphene/nanoparticle network embedded in an elastomer. NeuroString sensors allow chronic in vivo real-time, multichannel and multiplexed monoamine sensing in the brain of behaving mouse, as well as measuring serotonin dynamics in the gut without undesired stimulations and perturbing peristaltic movements. The described elastic and conformable biosensing interface has broad potential for studying the impact of neurotransmitters on gut microbes, brain-gut communication and may ultimately be extended to biomolecular sensing in other soft organs across the body.

The piezoelectric characteristics of nanowires, thin films and bulk crystals have been closely studied for potential applications in sensors, transducers, energy conversion and electronics (1-3).With their high crystallinity and ability to withstand enormous strain (4-6), two-dimensional materials are of great interest as high-performance piezoelectric materials. Monolayer Mo[S.sub.2] is predicted to be strongly piezoelectric, an effect that disappears in the bulk owing to the opposite orientations of adjacent atomic layers (7, 8). Here we report the first experimental study of the piezoelectric properties of two-dimensional Mo[S.sub.2] and show that cyclic stretching and releasing of thin Mo[S.sub.2] flakes with an odd number of atomic layers produces oscillating piezoelectric voltage and current outputs, whereas no output is observed for flakes with an even number of layers. A single monolayer flake strained by 0.53% generates a peak output of 15 mV and 20 pA, corresponding to a power density of 2 mW [m.sup.-2] and a 5.08% mechanical-to-electrical energy conversion efficiency. In agreement with theoretical predictions, the output increases with decreasing thickness and reverses sign when the strain direction is rotated by 90°. Transport measurements show a strong piezotronic effect in single-layer Mo[S.sub.2], but not in bilayer and bulk Mo[S.sub.2]. The coupling between piezoelectricity and semi-conducting properties in two-dimensional nanomaterials may enable the development of applications in powering nanodevices, adaptive bioprobes and tunable/stretchable electronics/optoelectronics., Crystal structure and symmetry dictate the physical properties of a material and its interaction with external stimuli. Materials with polarization domains, such as Pb(Ti, Zr)[O.sub.3], or with non-centrosymmetric structure, such [...]

Author(s): Sihong Wang [1]; Jie Xu [1]; Weichen Wang [2]; Ging-Ji Nathan Wang [1]; Reza Rastak [3]; Francisco Molina-Lopez [1]; Jong Won Chung [1, 4]; Simiao Niu [1]; Vivian R. [...]

In this study, the discharge voltage behavior of electric double-layer capacitors (EDLCs) during high- g impact is studied both theoretically and experimentally. A micro-scale dynamic mechanism is proposed to describe the physical basis of the increase in the discharge voltage during a high- g impact. Based on this dynamic mechanism, a multi-field model is established, and the simulation and experimental studies of the discharge voltage increase phenomenon are conducted. From the simulation and experimental data, the relationship between the increased voltage and the high- g acceleration is revealed. An acceleration detection range of up to 10,000 g is verified. The design of the device is optimized by studying the influences of the parameters, such as the electrode thickness and discharge current, on the outputs. This work opens up new avenues for the development of autonomous sensor systems based on energy storage devices and is significant for many practical applications such as in collision testing and automobile safety. [ABSTRACT FROM AUTHOR]

The development of wearable and large-area fabric energy harvester and sensor has received great attention due to their promising applications in next-generation autonomous and wearable healthcare technologies. Here, a new type of 'single' thread-based triboelectric nanogenerator (TENG) and its uses in elastically textile-based energy harvesting and sensing have been demonstrated. The energy-harvesting thread composed by one silicone-rubber-coated stainless-steel thread can extract energy during contact with skin. With sewing the energy-harvesting thread into a serpentine shape on an elastic textile, a highly stretchable and scalable TENG textile is realized to scavenge various kinds of human-motion energy. The collected energy is capable to sustainably power a commercial smart watch. Moreover, the simplified single triboelectric thread can be applied in a wide range of thread-based self-powered and active sensing uses, including gesture sensing, human-interactive interfaces, and human physiological signal monitoring. After integration with microcontrollers, more complicated systems, such as wireless wearable keyboards and smart beds, are demonstrated. These results show that the newly designed single-thread-based TENG, with the advantage of interactive, responsive, sewable, and conformal features, can meet application needs of a vast variety of fields, ranging from wearable and stretchable energy harvesters to smart cloth-based articles. [ABSTRACT FROM AUTHOR]

Water waves are increasingly regarded as a promising source for large-scale energy applications. Triboelectric nanogenerators (TENGs) have been recognized as one of the most promising approaches for harvesting wave energy. This work examines a freestanding, fully enclosed TENG that encloses a rolling ball inside a rocking spherical shell. Through the optimization of materials and structural parameters, a spherical TENG of 6 cm in diameter actuated by water waves can provide a peak current of 1 μA over a wide load range from a short-circuit condition to 10 GΩ, with an instantaneous output power of up to 10 mW. A multielectrode arrangement is also studied to improve the output of the TENG under random wave motions from all directions. Moreover, at a frequency of 1.43 Hz, the wave-driven TENG can directly drive tens of LEDs and charge a series of supercapacitors to rated voltage within several hours. The stored energy can power an electronic thermometer for 20 min. This rolling-structured TENG is extremely lightweight, has a simple structure, and is capable of rocking on or in water to harvest wave energy; it provides an innovative and effective approach toward large-scale blue energy harvesting of oceans and lakes. [ABSTRACT FROM AUTHOR]

Human biomechanical energy is characterized by fluctuating amplitudes and variable low frequency, and an effective utilization of such energy cannot be achieved by classical energyharvesting technologies. Here we report a high-efficient self-charging power system for sustainable operation of mobile electronics exploiting exclusively human biomechanical energy, which consists of a high-output triboelectric nanogenerator, a power management circuit to convert the random a.c. energy to d.c. electricity at 60% efficiency, and an energy storage device. With palm tapping as the only energy source, this power unit provides a continuous d.c. electricity of 1.044mW (7.34Wm ― 3) in a regulated and managed manner. This self-charging unit can be universally applied as a standard ‘infinite-lifetime’ power source for continuously driving numerous conventional electronics, such as thermometers, electrocardiograph system, pedometers, wearable watches, scientific calculators and wireless radio-frequency communication system, which indicates the immediate and broad applications in personal sensor systems and internet of things. [ABSTRACT FROM AUTHOR]

A stretchable-rubber-based (SR-based) triboelectric nanogenerator (TENG) is developed that can not only harvest energy but also serve as self-powered multifunctional sensors. It consists of a layer of elastic rubber and a layer of aluminum film that acts as the electrode. By stretching and releasing the rubber, the changes of triboelectric charge distribution/density on the rubber surface relative to the aluminum surface induce alterations to the electrical potential of the aluminum electrode, leading to an alternating charge flow between the aluminum electrode and the ground. The unique working principle of the SR-based TENG is verified by the coupling of numerical calculations and experimental measurements. A comprehensive study is carried out to investigate the factors that may influence the output performance of the SR-based TENG. By integrating the devices into a sensor system, it is capable of detecting movements in different directions. Moreover, the SR-based TENG can be attached to a human body to detect diaphragm breathing and joint motion. This work largely expands the applications of TENG not only as effective power sources but also as active sensors; and opens up a new prospect in future electronics. [ABSTRACT FROM AUTHOR]

Triboelectric nanogenerator (TENG) technology has emerged as a new mechanical energy harvesting technology with numerous advantages. This paper analyzes its charging behavior together with a load capacitor. Through numerical and analytical modeling, the charging performance of a TENG with a bridge rectifier under periodic external mechanical motion is completely analogous to that of a dc voltage source in series with an internal resistance. An optimum load capacitance that matches the TENGs impedance is observed for the maximum stored energy. This optimum load capacitance is theoretically detected to be linearly proportional to the charging cycle numbers and the inherent TENG capacitance. Experiments were also performed to further validate our theoretical anticipation and show the potential application of this paper in guiding real experimental designs. [ABSTRACT FROM AUTHOR]

Motion tracking is of great importance in a wide range of fields such as automation, robotics, security, sports and entertainment. Here, a self-powered, single-electrode-based triboelectric sensor (TES) is reported to accurately detect the movement of a moving object/body in two dimensions. Based on the coupling of triboelectric effect and electrostatic induction, the movement of an object on the top surface of a polytetrafluoroethylene (PTFE) layer induces changes in the electrical potential of the patterned aluminum electrodes underneath. From the measurements of the output performance (open-circuit voltage and short-circuit current), the motion information about the object, such as trajectory, velocity, and acceleration is derived in conformity with the preset values. Moreover, the TES can detect motions of more than one objects moving at the same time. In addition, applications of the TES are demonstrated by using LED illuminations as real-time indicators to visualize the movement of a sliding object and the walking steps of a person. [ABSTRACT FROM AUTHOR]

The piezoelectric characteristics of nanowires, thin films and bulk crystals have been closely studied for potential applications in sensors, transducers, energy conversion and electronics. With their high crystallinity and ability to withstand enormous strain, two-dimensional materials are of great interest as high-performance piezoelectric materials. Monolayer MoS2 is predicted to be strongly piezoelectric, an effect that disappears in the bulk owing to the opposite orientations of adjacent atomic layers. Here we report the first experimental study of the piezoelectric properties of two-dimensional MoS2 and show that cyclic stretching and releasing of thin MoS2 flakes with an odd number of atomic layers produces oscillating piezoelectric voltage and current outputs, whereas no output is observed for flakes with an even number of layers. A single monolayer flake strained by 0.53% generates a peak output of 15 mV and 20 pA, corresponding to a power density of 2 mW m−2 and a 5.08% mechanical-to-electrical energy conversion efficiency. In agreement with theoretical predictions, the output increases with decreasing thickness and reverses sign when the strain direction is rotated by 90°. Transport measurements show a strong piezotronic effect in single-layer MoS2, but not in bilayer and bulk MoS2. The coupling between piezoelectricity and semiconducting properties in two-dimensional nanomaterials may enable the development of applications in powering nanodevices, adaptive bioprobes and tunable/stretchable electronics/optoelectronics. [ABSTRACT FROM AUTHOR]

Single-electrode triboelectric nanogenerators (SETENGs) significantly expand the application of triboelectric nanogenerators in various circumstances, such as touch-pad technologies. In this work, a theoretical model of SETENGs is presented with in-depth interpretation and analysis of their working principle. Electrostatic shield effect from the primary electrode is the main consideration in the design of such SETENGs. On the basis of this analysis, the impacts of two important structural parameters, that is, the electrode gap distance and the area size, on the output performance are theoretically investigated. An optimized electrode gap distance and an optimized area size are observed to provide a maximum transit output power. Parallel connection of multiple SETENGs with micro-scale size and relatively larger spacing should be utilized as the scaling-up strategy. The discussion of the basic working principle and the influence of structural parameters on the whole performance of the device can serve as an important guidance for rational design of the device structure towards the optimum output in specific applications. [ABSTRACT FROM AUTHOR]