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In this paper, the winter visibility in Jiangsu Province is simulated by WRF-Chem (Weather Research and Forecasting (WRF) model coupled with Chemistry) with high spatiotemporal resolutions. Simulation results show that WRF-Chem has good capability to simulate the visibility and related local meteorological elements and air pollutants in Jiangsu in the winters of 2013–2017. For visibility inversion, this study adopts the neural network algorithm. Meteorological elements, including wind speed, humidity and temperature, are introduced to improve the performance of WRF-Chem relative to the visibility inversion scheme, which is based on the Interagency Monitoring of Protected Visual Environments (IMPROVE) extinction coefficient algorithm. The neural network offers a noticeable improvement relative to the inversion scheme of the IMPROVE visibility extinction coefficient, substantially improving the underestimation of winter visibility in Jiangsu Province. For instance, the correlation coefficient increased from 0.17 to 0.42, and root mean square error decreased from 2.62 to 1.76. The visibility inversion results under different humidity and wind speed levels show that the underestimation of the visibility using the IMPROVE scheme is especially remarkable. However, the underestimation issue is essentially solved using the neural network algorithm. This study serves as a basis for further predicting winter haze events in Jiangsu Province using WRF-Chem and deep-learning methods. [ABSTRACT FROM AUTHOR]