M. I. Hegglin, S. Tegtmeier, J. Anderson, A. E. Bourassa, S. Brohede, D. Degenstein, L. Froidevaux, B. Funke, J. Gille, Y. Kasai, E. T. Kyrölä, J. Lumpe, D. Murtagh, J. L. Neu, K. Pérot, E. E. Remsberg, A. Rozanov, M. Toohey, J. Urban, T. von Clarmann, K. A. Walker, H.-J. Wang, C. Arosio, R. Damadeo, R. A. Fuller, G. Lingenfelser, C. McLinden, D. Pendlebury, C. Roth, N. J. Ryan, C. Sioris, L. Smith, K. Weigel, European Commission, Ministerio de Ciencia, Innovación y Universidades (España), Ministerio de Economía y Competitividad (España), European Space Agency, and German Research Foundation
Full list of authors: Hegglin, Michaela I.; Tegtmeier, Susann; Anderson, John; Bourassa, Adam E.; Brohede, Samuel; Degenstein, Doug; Froidevaux, Lucien; Funke, Bernd; Gille, John; Kasai, Yasuko; Kyrölä, Erkki T.; Lumpe, Jerry; Murtagh, Donal; Neu, Jessica L.; Pérot, Kristell; Remsberg, Ellis E.; Rozanov, Alexei; Toohey, Matthew; Urban, Joachim; von Clarmann, Thomas; Walker, Kaley A.; Wang, Hsiang-Jui; Arosio, Carlo; Damadeo, Robert; Fuller, Ryan A.; Lingenfelser, Gretchen; McLinden, Christopher; Pendlebury, Diane; Roth, Chris; Ryan, Niall J.; Sioris, Christopher; Smith, Lesley; Weigel, Katja.-- This is an Open Access article distributed under the terms of the Creative Commons Attribution License (http://creativecommons.org/licenses/by/4.0/), which permits unrestricted reuse, distribution, and reproduction in any medium, provided the original work is properly cited., The Stratosphere-troposphere Processes and their Role in Climate (SPARC) Data Initiative (SPARC, 2017) performed the first comprehensive assessment of currently available stratospheric composition measurements obtained from an international suite of space-based limb sounders. The initiative's main objectives were (1) to assess the state of data availability, (2) to compile time series of vertically resolved, zonal monthly mean trace gas and aerosol fields, and (3) to perform a detailed intercomparison of these time series, summarizing useful information and highlighting differences among datasets. The datasets extend over the region from the upper troposphere to the lower mesosphere (300-0.1 hPa) and are provided on a common latitude-pressure grid. They cover 26 different atmospheric constituents including the stratospheric trace gases of primary interest, ozone (O3) and water vapor (H2O), major long-lived trace gases (SF6, N2O, HF, CCl3F, CCl2F2, NOy ), trace gases with intermediate lifetimes (HCl, CH4, CO, HNO3), and shorter-lived trace gases important to stratospheric chemistry including nitrogen-containing species (NO, NO2, NOx, N2O5, HNO4), halogens (BrO, ClO, ClONO2, HOCl), and other minor species (OH, HO2, CH2O, CH3CN), and aerosol. This overview of the SPARC Data Initiative introduces the updated versions of the SPARC Data Initiative time series for the extended time period 1979-2018 and provides information on the satellite instruments included in the assessment: LIMS, SAGE I/II/III, HALOE, UARS-MLS, POAM II/III, OSIRIS, SMR, MIPAS, GOMOS, SCIAMACHY, ACE-FTS, ACEMAESTRO, Aura-MLS, HIRDLS, SMILES, and OMPS-LP. It describes the Data Initiative's top-down climatological validation approach to compare stratospheric composition measurements based on zonal monthly mean fields, which provides upper bounds to relative inter-instrument biases and an assessment of how well the instruments are able to capture geophysical features of the stratosphere. An update to previously published evaluations of O3 and H2O monthly mean time series is provided. In addition, example trace gas evaluations of methane (CH4), carbon monoxide (CO), a set of nitrogen species (NO, NO2, and HNO3), the reactive nitrogen family (NOy ), and hydroperoxyl (HO2) are presented. The results highlight the quality, strengths and weaknesses, and representativeness of the different datasets. As a summary, the current state of our knowledge of stratospheric composition and variability is provided based on the overall consistency between the datasets. As such, the SPARC Data Initiative datasets and evaluations can serve as an atlas or reference of stratospheric composition and variability during the "golden age"of atmospheric limb sounding. The updated SPARC Data Initiative zonal monthly mean time series for each instrument are publicly available and accessible via the Zenodo data archive (Hegglin et al., 2020). © 2021 The Author(s)., The research of Michaela I. Hegglin was supported by the CSA SSEP (grant no. 9SCIGRA-29), the ESA STSE-SPIN (contract no. 4000105291/12/I-NB), and the ESA Water Vapour Climate Change Initiative (contract no. 4000123554). The research of Susann Tegtmeier was funded by the WGL project TransBrom and the EU project SHIVA (grant no. FP7-ENV-2007-1-226224). Work at the Jet Propulsion Laboratory, California Institute of Technology, was funded by the National Aeronautics and Space Administration (NASA). The Atmospheric Chemistry Experiment is a Canadian-led mission mainly supported by the CSA. Development of the ACE-FTS gridded datasets was supported by grants from the Canadian Foundation for Climate and Atmospheric Sciences and the CSA. MIPAS data analysis and validation was supported by the German Federal Ministry for Economic Affairs and Energy (grant no. 50EE1547) and by the ESA Ozone Climate Change Initiative. Bernd Funke acknowledges support by the Spanish MCINN (grant no. ESP2017-87143-R and PID2019-110689RB-I00) and EC FEDER funds. Development of the SCIA-MACHY and IUP-OMPS gridded datasets at the University of Bremen was funded in part by the German Research Foundation (DFG) Research Units SHARP (grant no. FOR1095) and VolImpact (grant no. FOR2820), the German Aerospace Agency (DLR) SADOS project, ESA SQWG and Ozone CCI projects, EU/ECMWF C3S project, and the University and State of Bremen. Alexei Rozanov and Carlo Arosio also acknowledge the German HLRN (High-Performance Computer Center North) and the thread-safe FOR-TRAN library GALAHAD. In addition, Carlo Arosio acknowledges the support by the PRIME program of the German Academic Exchange Service (DAAD) and ESA's Living Planet Fellowship SOLVE. Work on HIRDLS was supported in the US by the National Aeronautics and Space Administration (NASA) and in the UK by the National Environmental Research Council (NERC). Development of the Odin/SMR gridded datasets was supported by the Swedish National Space Agency (SNSA)., With funding from the Spanish government through the Severo Ochoa Centre of Excellence accreditation SEV-2017-0709.