1. Toward using collective x-ray Thomson scattering to study C–H demixing and hydrogen metallization in warm dense matter conditions
- Author
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D. Ranjan, K. Ramakrishna, K. Voigt, O. S. Humphries, B. Heuser, M. G. Stevenson, J. Lütgert, Z. He, C. Qu, S. Schumacher, P. T. May, A. Amouretti, K. Appel, E. Brambrink, V. Cerantola, D. Chekrygina, L. B. Fletcher, S. Göde, M. Harmand, N. J. Hartley, S. P. Hau-Riege, M. Makita, A. Pelka, A. K. Schuster, M. Šmíd, T. Toncian, M. Zhang, T. R. Preston, U. Zastrau, J. Vorberger, D. Kraus, Ranjan, D, Ramakrishna, K, Voigt, K, Humphries, O, Heuser, B, Stevenson, M, Lütgert, J, He, Z, Qu, C, Schumacher, S, May, P, Amouretti, A, Appel, K, Brambrink, E, Cerantola, V, Chekrygina, D, Fletcher, L, Göde, S, Harmand, M, Hartley, N, Hau-Riege, S, Makita, M, Pelka, A, Schuster, A, Šmíd, M, Toncian, T, Zhang, M, Preston, T, Zastrau, U, Vorberger, J, and Kraus, D
- Subjects
XFEL, Thomson scattering, carbon, hydrogen, planetary interior ,Condensed Matter Physics - Abstract
The insulator–metal transition in liquid hydrogen is an important phenomenon to understand the interiors of gas giants, such as Jupiter and Saturn, as well as the physical and chemical behavior of materials at high pressures and temperatures. Here, the path toward an experimental approach is detailed based on spectrally resolved x-ray scattering, tailored to observe and characterize hydrogen metallization in dynamically compressed hydrocarbons in the regime of carbon–hydrogen phase separation. With the help of time-dependent density functional theory calculations and scattering spectra from undriven carbon samples collected at the European x-ray Free-Electron Laser Facility (EuXFEL), we demonstrate sufficient data quality for observing C–H demixing and investigating the presence of liquid metallic hydrogen in future experiments using the reprated drive laser systems at EuXFEL.
- Published
- 2023