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We explore the preparation of specific nuclear states on gate-based quantum hardware using variational algorithms. Large scale classical diagonalization of the nuclear shell model have reached sizes of $10^9 - 10^{10}$ basis states, but are still severely limited by computational resources. Quantum computing can, in principle, solve such systems exactly with exponentially fewer resources than classical computing. Exact solutions for large systems require many qubits and large gate depth, but variational approaches can effectively limit the required gate depth. We use the unitary coupled cluster approach to construct approximations of the ground-state vectors, later to be used in dynamics calculations. The testing ground is the phenomenological shell model space, which allows us to mimic the complexity of the inter-nucleon interactions. We find that often one needs to minimize over a large number of parameters, using a large number of entanglements that makes challenging the application on existing hardware. Prospects for rapid improvements with more capable hardware are, however, very encouraging., Comment: 10 pages, 5 figures

Nuclear data is critical for many modern applications from stockpile stewardship to cutting edge scientific research. Central to these pursuits is a robust pipeline for nuclear modeling as well as data assimilation and dissemination. We summarize a small portion of the ongoing nuclear data efforts at Los Alamos for medium mass to heavy nuclei. We begin with an overview of the NEXUS framework and show how one of its modules can be used for model parameter optimization using Bayesian techniques. The mathematical framework affords the combination of different measured data in determining model parameters and their associated correlations. It also has the advantage of being able to quantify outliers in data. We exemplify the power of this procedure by highlighting the recently evaluated 239-Pu cross section. We further showcase the success of our tools and pipeline by covering the insight gained from incorporating the latest nuclear modeling and data in astrophysical simulations as part of the Fission In R-process Elements (FIRE) collaboration., Comment: 6 pages, 5 figures, Nuclear Data (2022) conference proceedings. Comments welcome!

The pre-equilibrium reaction mechanism is considered in the context of the exciton model. A modification to the one-particle one-hole state density is studied which can be interpreted as a collective enhancement. The magnitude of the collective enhancement is set by simulating the Lawrence Livermore National Laboratory (LLNL) pulsed-spheres neutron-leakage spectra. The impact of the collective enhancement is explored in the context of the highly deformed actinide, 239-Pu. A consequence of this enhancement is the removal of fictitious levels in the Distorted-Wave Born Approximation often used in modern nuclear reaction codes., Comment: 7 pages, 7 figures. Comments welcome!

The Hauser-Feshbach fission fragment decay model, HF3D, calculates the statistical decay of fission fragments through both prompt and delayed neutron and γ-ray emissions in a deterministic manner. While previously limited to the calculation of only first-chance fission, the model has recently been extended to include multi-chance fission, up to neutron incident energies of 20 MeV. The deterministic decay takes as input prescission quantities–fission probabilities, pre-fission neutron energies, and the average energy causing fission– and post-scission quantities–yields in mass, charge, total kinetic energy, spin, and parity. From those fission fragment initial conditions, the full decay is followed through both prompt and delayed particle emissions. The evaporation of the prompt neutrons and γ rays is calculated through the Hauser-Feshbach statistical theory, taking into account the competition between neutron and γ-ray emission, conserving energy, spin, and parity. The delayed emission is taken into account using time-independent calculation using decay data. This whole formulation allows for the calculation of prompt neutron and γ-ray properties, such as multiplicities and energy distributions, both independent and cumulative fission yields, and delayed neutron observables, in a consistent framework. Here, we describe the implementation of multi-chance fission into the HF3D model, and show an example of prompt and delayed quantities beyond first-chance fission, using the example of neutron-induced fission on 239Pu. This expansion represents significant progress in consistently modeling the emission of prompt and delayed particles from fissile systems.

In the no‐core shell model (NCSM) framework, we calculate the 3He electric dipole moment (EDM) generated by parity‐ and time‐reversal violation in the nucleon‐nucleon interaction. While the results are somehow sensitive to the interaction model chosen for the strong two‐ and three‐body interactions, we demonstrate the pion‐exchange dominance to the EDM of 3He, if the coupling constants for π, ρ and ω‐exchanges are of comparable magnitude, as expected. Finally, our results suggest that a measurement of 3He EDM would be complementary to the currently planned neutron and deuteron experiments, and would constitute a powerful constraint to the models of the pion P‐ and T‐violating interactions.

The no-core shell model (NCSM), in which all A nucleons are treated as active, is an ab initio approach for calculating the properties of nuclei microscopically. We first present the basic NCSM formalism, which allows us to exactly determine the effective Hamiltonian as well as any general operator in a model space of arbitrary size for performing shell-model calculations. Good results for binding energies and spectra have been obtained for nuclei up to mass A = 14 using the best available two-nucleon (NN) and theoretical three-nucleon forces (3NF's). We next present three new applications and extensions of the NCSM approach: I) the use of the NCSM in the three-nucleon (3N) cluster approximation as a method for testing the reliability of different 3NF's, and the application of the NCSM to 2) other general operators and 3) inclusive electromagnetic responses.