1. Nonlinear terahertz Néel spin-orbit torques in antiferromagnetic Mn$_2$Au
- Author
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Behovits, Yannic, Chekhov, Alexander L., Bodnar, Stanislav Yu., Gueckstock, Oliver, Reimers, Sonka, Seifert, Tom S., Wolf, Martin, Gomonay, Olena, Kläui, Mathias, Jourdan, Martin, and Kampfrath, Tobias
- Subjects
Mesoscale and Nanoscale Physics (cond-mat.mes-hall) ,FOS: Physical sciences - Abstract
Antiferromagnets have large potential for ultrafast coherent switching of magnetic order with minimum heat dissipation. In novel materials such as Mn$_2$Au and CuMnAs, electric rather than magnetic fields may control antiferromagnetic order by Néel spin-orbit torques (NSOTs), which have, however, not been observed on ultrafast time scales yet. Here, we excite Mn$_2$Au thin films with phase-locked single-cycle terahertz electromagnetic pulses and monitor the spin response with femtosecond magneto-optic probes. We observe signals whose symmetry, dynamics, terahertz-field scaling and dependence on sample structure are fully consistent with a uniform in-plane antiferromagnetic magnon driven by field-like terahertz NSOTs with a torkance of (150$\pm$50) cm$^2$/A s. At incident terahertz electric fields above 500 kV/cm, we find pronounced nonlinear dynamics with massive Néel-vector deflections by as much as 30°. Our data are in excellent agreement with a micromagnetic model which indicates that fully coherent Néel-vector switching by 90° within 1 ps is within close reach., 16 pages, 4 figures
- Published
- 2023
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