Search

We describe the design and execution of the BORTAS (Quantifying the impact of BOReal forest fires on Tropospheric oxidants over the Atlantic using Aircraft and Satellites) experiment, which has the overarching objective of understanding the chemical aging of air masses that contain the emission products from seasonal boreal wildfires and how these air masses subsequently impact downwind atmospheric composition. The central focus of the experiment was a two-week deployment of the UK BAe-146-301 Atmospheric Research Aircraft (ARA) over eastern Canada, based out of Halifax, Nova Scotia. Atmospheric ground-based and sonde measurements over Canada and the Azores associated with the planned July 2010 deployment of the ARA, which was postponed by 12 months due to UK-based flights related to the dispersal of material emitted by the Eyjafjallajökull volcano, went ahead and constituted phase A of the experiment. Phase B of BORTAS in July 2011 involved the same atmospheric measurements, but included the ARA, special satellite observations and a more comprehensive ground-based measurement suite. The high-frequency aircraft data provided a comprehensive chemical snapshot of pyrogenic plumes from wildfires, corresponding to photochemical (and physical) ages ranging from < 1 day to ~<45 sr 10 days, largely by virtue of widespread fires over Northwestern Ontario. Airborne measurements reported a large number of emitted gases including semi-volatile species, some of which have not been been previously reported in pyrogenic plumes, with the corresponding emission ratios agreeing with previous work for common gases. Analysis of the NOy data shows evidence of net ozone production in pyrogenic plumes, controlled by aerosol abundance, which increases as a function of photochemical age. The coordinated ground-based and sonde data provided detailed but spatially limited information that put the aircraft data into context of the longer burning season in the boundary layer. Ground-based measurements of particulate matter smaller than 2.5 μm (PM2.5) over Halifax show that forest fires can on an episodic basis represent a substantial contribution to total surface PM2.5.

Aircraft observations of wind and temperature are very important for upper air meteorology. In this article, the quality of the meteorological information of an Automatic Dependent Surveillance-Contract (ADS-C) message is assessed. The ADS-C messages broadcast by the aircraft are received at air traffic control centres for surveillance and airline control centres for general aircraft and dispatch management. A comparison is performed against a global numerical prediction (NWP) model and wind and temperature observations derived from Enhanced Surveillance (EHS) air-traffic control radar which interrogates all aircraft in selective mode (Mode-S EHS). Almost 16 000 ADS-C reports with meteorological information were compiled from the Royal Dutch Airlines (KLM) database. The length of the data set is 76 consecutive days and started on 1 January 2011. The wind and temperature observations are of good quality when compared to the global NWP forecast fields from the European Centre for Medium-Range Weather Forecasts (ECMWF). Comparison of ADS-C wind and temperature observations against Mode-S EHS derived observations in the vicinity of Amsterdam Airport Schiphol shows that the wind observations are of similar quality and the temperature observations of ADS-C are of better quality than those from Mode-S EHS. However, the current ADS-C data set has a lower vertical resolution than Mode-S EHS. High vertical resolution can be achieved by requesting more ADS-C when aircraft are ascending or descending, but could result in increased data communication costs.