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This study aims to present the benefits of unmanned aircraft systems (UAS) in atmospheric aerosol research, specifically to obtain information on the vertical variability of aerosol single-scattering properties in the lower troposphere. The results discussed in this paper were obtained during the Polish Radar and Lidar Mobile Observation System (POLIMOS) field campaign in 2018 at a wetland and rural site located in the Rzecin (Poland). UAS was equipped with miniaturised devices (low-cost aerosol optical counter, aethalometer AE-51, RS41 radiosonde) to measure aerosol properties (scattering and absorption coefficient) and air thermodynamic parameters. Typical UAS vertical profiles were conducted up to approximately 1000 m agl. During nighttime, UAS measurements show a very shallow inversion surface layer up to about 100–200 m agl, with significant enhancement of aerosol scattering and absorption coefficient. In this case, the Pearson correlation coefficient between aerosol single-scattering properties measured by ground-based equipment and UAS devices significantly decreases with altitude. In such conditions, aerosol properties at 200 m agl are independent of the ground-based observation. On the contrary, the ground observations are better correlated with UAS measurements at higher altitudes during daytime and under well-mixed conditions. During long-range transport of biomass burning from fire in North America, the aerosol absorption coefficient increases with altitude, probably due to entrainment of such particles into the PBL.

We present the first estimations of single hygroscopic parameter κ for Polish urban area. The results were obtained using an inexpensive OPC-N3 optical particulate matter counter and the ASC 1000 Acoem Aerosol Conditioning System. Our studies were carried out during the winter and spring seasons, between 2020 and 2022 in Warsaw, Poland. We study the difference of κ between these two seasons, as the aerosol has different origins. The mean value of the hygroscopicity parameter for spring (April–June) was 0.13±0.13 and for winter (December-March) it was 0.04±0.04 (obtained using PM1). The mean value of the growth factor for spring (April–June) was 1.52±0.23 and for winter (December–March) it was 1.16±0.13 (obtained using PM1). The values for winter period suggest that during the cold season the aerosol mixture in the atmosphere is dominated by non-hygroscopic particles. However events of higher κ > 0.5 where occurring (mostly for big aerosol particles 1–10 μm in size), when the air mass was coming from North Atlantic carrying sea salt particles. Furthermore, based on κ we propose a method to remove the dependence of PM values on relative humidity on the OPC-N3 optical particulate counter.

The Poland-AOD aerosol research network was established in 2011 to improve aerosol–climate interaction knowledge and provide a real-time and historical, comprehensive, and quantitative database for the aerosol optical properties distribution over Poland. The network consists of research institutions and private owners operating 10 measurement stations and an organization responsible for aerosol model transport simulations. Poland-AOD collaboration provides observations of spectral aerosol optical depth (AOD), Ångstrom Exponent (AE), incoming shortwave (SW) and longwave (LW) radiation fluxes, vertical profiles of aerosol optical properties and surface aerosol scattering and absorption coefficient, as well as microphysical particle properties. Based on the radiative transfer model (RTM), the aerosol radiative forcing (ARF) and the heating rate are simulated. In addition, results from GEM-AQ and WRF-Chem models (e.g., aerosol mass mixing ratio and optical properties for several particle chemical components), and HYSPLIT back-trajectories are used to interpret the results of observation and to describe the 3D aerosol optical properties distribution. Results of Poland-AOD research indicate progressive improvement of air quality and at mospheric turbidity during the last decade. The AOD was reduced by about 0.02/10 yr (at 550 nm), which corresponds to positive trends in ARF. The estimated clear-sky ARF trend is 0.34 W/m2/10 yr and 0.68 W/m2/10 yr, respectively, at TOA and at Earth’s surface. Therefore, reduction in aerosol load observed in Poland can significantly contribute to climate warming.

Peatlands play an important role in the global carbon cycle due to the high carbon storage in the substrate. Ecosystem production depends, for example, on the solar energy amount that reaches the vegetation, however the diffuse component of this flux can substantially increase ecosystem net productivity. This phenomenon is observed in different ecosystems, but the study of the atmosphere optical properties on peatland production is lacking. In this paper, the presented methodology allowed us to disentangle the diffuse radiation impact on the net ecosystem production (NEP) of Rzecin peatland, Poland. It allowed us to assess the impact of the atmospheric scattering process determined by the aerosol presence in the air mass. An application of atmospheric radiation transfer (ART) and ecosystem production (EP) models showed that the increase of aerosol optical thickness from 0.09 to 0.17 caused NEP to rise by 3.4–5.7%. An increase of the diffusion index (DI) by 0.1 resulted in an NEP increase of 6.1–42.3%, while a DI decrease of 0.1 determined an NEP reduction of −49.0 to −10.5%. These results show that low peatland vegetation responds to changes in light scattering. This phenomenon should be taken into account when calculating the global CO2 uptake estimation of such ecosystems.

The aerosol scattering coefficient and Ångström exponent (AE) are important parameters in the understanding of aerosol optical properties and aerosol direct effect. These parameters are usually measured by a nephelometer network which is under-represented geographically; however, a rapid growth of air-pollution monitoring, using low-cost particle sensors, may extend observation networks. This paper presents the results of co-located measurements of aerosol optical properties, such as the aerosol scattering coefficient and the scattering AE, using low-cost sensors and using a scientific-grade polar Aurora 4000 nephelometer. A high Pearson correlation coefficient (0.94–0.96) between the low-cost particulate matter (PM) mass concentration and the aerosol scattering coefficient was found. For the PM10 mass concentration, the aerosol scattering coefficient relation is linear for the Dfrobot SEN0177 sensor and non-linear for the Alphasense OPC-N2 device. After regression analyses, both low-cost instruments provided the aerosol scattering coefficient with a similar mean square error difference (RMSE) of about 20 Mm−1, which corresponds to about 27% of the mean aerosol scattering coefficient. The relative uncertainty is independent of the pollution level. In addition, the ratio of aerosol number concentration between different bins showed a significant statistical (95% of confidence level) correlation with the scattering AE. For the SEN0177, the ratio of the particle number in bin 1 (radius of 0.15–0.25 µm) to bin 4 (radius of 1.25–2.5 µm) was a linear function of the scattering AE, with a Pearson correlation coefficient of 0.74. In the case of OPC-N2, the best correlation (r = 0.66) was found for the ratio between bin 1 (radius of 0.19–0.27 µm) and bin 2 (radius of 0.27–0.39 µm). Comparisons of an estimated scattering AE from a low-cost sensor with Aurora 4000 are given with the RMSE of 0.23–0.24, which corresponds to 16–19%. In addition, a three-year (2016–2019) observation by SEN0177 indicates that this sensor can be used to determine an annual cycle as well as a short-term variability.

Within the framework of the Satellite-based Monitoring Initiative for Regional Air quality (SAMIRA) project, the near-real-time (NRT) operation has been documented for an in-house developed algorithm used for the retrieval of aerosol optical depth (AOD) maps from the Spinning Enhanced Visible and Infrared Imager (SEVIRI) sensor onboard the Meteosat Second Generation (MSG). With the frequency of 15 min at a spatial resolution of roughly 5.5 × 5.5 km the AOD maps are provided for the country domains of Poland, the Czech Republic, Romania, and Southern Norway. A significant improvement has been reported in terms of modification of the existing prototype algorithm that it suits the operational NRT AOD retrieval for an extended area. This is mainly due to the application of the optimal interpolation method for the AOD estimation on reference days with the use of ground-based measurements of the Aerosol Robotic Network (AERONET) and the Aerosol Research Network (PolandAOD-NET) as well as simulations of the Copernicus Atmosphere Monitoring Service (CAMS). The main issues that have been addressed regarding surface reflectance estimation, cloud screening and uncertainty calculation. Exemplary maps of the NRT retrieval have been presented.

The impact of absorbing aerosols on climate is complex, with their potential positive or negative forcing, depending on many factors, including their height distribution and reflective properties of the underlying background. Measurement data is very limited, due to insufficient remote sensing methods dedicated to the retrieval of their vertical distribution. Columnar values of absorbing aerosol optical depth (AAOD) and single scattering albedo (SSA) are retrieved by the Aerosol Robotic Network (AERONET). However, the number of available results is low due to sky condition and aerosol optical depth (AOD) limitation. Presented research describes results of field campaigns in Strzyżów (South-East Poland, Eastern Europe) dedicated to the comparison of the absorption coefficient and SSA measurements performed with on-ground in-situ devices (aethalomter, nephelometer), small unmanned aerial system (UAS) carrying micro-aethalometer, as well as with lidar/ceilometer. An important aspect is the comparison of measurement results with those delivered by AERONET. Correlation of absorption to scattering coefficients measured on ground (0.79) and correlation of extinction on ground to AOD measured by AERONET (0.77) was visibly higher than correlation between AOD and AAOD retrieved by AERONET (0.56). Columnar SSA was weakly correlated with ground SSA (higher values of columnar SSA), which were mainly explained by hygroscopic effects, increasing scattering coefficient in ambient (wet conditions), and partly high uncertainty of SSA retrieval. AAOD derived with the use of profiles from UAS up to PBL height, was estimated to contribute in average to 37% of the total AAOD. A method of AAOD estimation, in the whole troposphere, with use of measured vertical profiles of absorption coefficient and extinction coefficient profiles from lidars was proposed. AAOD measured with this method has poor correlation with AERONET data, however for some measurements, within PBL, AAOD was higher than reported by AERONET, suggesting potential underestimation in photometric measurement under particular conditions. Correlation of absorption coefficient in profile to on ground measurements decrease with altitude. Measurements of SSA from drones agree well with ground measurements and are lower than results from AERONET, which suggests a larger contribution of absorbing aerosols. As an alternative for AAOD estimation in case of lack of AERONET AAOD data simple models are proposed, which base on AOD scaling with SSA measured with different methods. Proposed solution increase potential of absorption coefficient measurements in vertical profiles and columns of the atmosphere. Presented solutions make measurements of absorption coefficients in vertical profiles more affordable and allow rough estimation of columnar values for the whole atmosphere.

During August 2016, a quasi-stationary high-pressure system spreading over Central and North-Eastern Europe, caused weather conditions that allowed for 24/7 observations of aerosol optical properties by using a complex multi-wavelength PollyXT lidar system with Raman, polarization and water vapour capabilities, based at the European Aerosol Research Lidar Network (EARLINET network) urban site in Warsaw, Poland. During 24–30 August 2016, the lidar-derived products (boundary layer height, aerosol optical depth, Ångström exponent, lidar ratio, depolarization ratio) were analysed in terms of air mass transport (HYSPLIT model), aerosol load (CAMS data) and type (NAAPS model) and confronted with active and passive remote sensing at the ground level (PolandAOD, AERONET, WIOS-AQ networks) and aboard satellites (SEVIRI, MODIS, CATS sensors). Optical properties for less than a day-old fresh biomass burning aerosol, advected into Warsaw’s boundary layer from over Ukraine, were compared with the properties of long-range transported 3–5 day-old aged biomass burning aerosol detected in the free troposphere over Warsaw. Analyses of temporal changes of aerosol properties within the boundary layer, revealed an increase of aerosol optical depth and Ångström exponent accompanied by an increase of surface PM10 and PM2.5. Intrusions of advected biomass burning particles into the urban boundary layer seem to affect not only the optical properties observed but also the top height of the boundary layer, by moderating its increase.