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The nature of the pairing symmetry of the first heavy fermion superconductor CeCu$_2$Si$_2$ has recently become the subject of controversy. While CeCu$_2$Si$_2$ was generally believed to be a $d$-wave superconductor, recent low temperature specific heat measurements showed evidence for fully gapped superconductivity, contrary to the nodal behavior inferred from earlier results. Here we report London penetration depth measurements, which also reveal fully gapped behavior at very low temperatures. To explain these seemingly conflicting results, we propose a fully gapped $d+d$ band-mixing pairing state for CeCu$_2$Si$_2$, which yields very good fits to both the superfluid density and specific heat, as well as accounting for a sign change of the superconducting order parameter, as previously concluded from inelastic neutron scattering results., Comment: 9 pages, 6 figures including Supplemental material. Published version in PNAS available online ahead of print at http://www.pnas.org/content/early/2018/05/07/1720291115

In exotic superconductors including high-$T_c$ copper-oxides, the interactions mediating electron Cooper-pairing are widely considered to have a magnetic rather than the conventional electron-phonon origin. Interest in such exotic pairing was initiated by the 1979 discovery of heavy-fermion superconductivity in CeCu$_2$Si$_2$, which exhibits strong antiferromagnetic fluctuations. A hallmark of unconventional pairing by anisotropic repulsive interactions is that the superconducting energy gap changes sign as a function of the electron momentum, often leading to nodes where the gap goes to zero. Here, we report low-temperature specific heat, thermal conductivity and magnetic penetration depth measurements in CeCu$_2$Si$_2$, demonstrating the absence of gap nodes at any point on the Fermi surface. Moreover, electron-irradiation experiments reveal that the superconductivity survives even when the electron mean free path becomes substantially shorter than the superconducting coherence length. This indicates that superconductivity is robust against impurities, implying that there is no sign change in the gap function. These results show that, contrary to long-standing belief, heavy electrons with extremely strong Coulomb repulsions can condense into a fully-gapped s-wave superconducting state, which has an on-site attractive pairing interaction., Comment: 8 pages, 5 figures + Supplement (3 pages, 5 figures)

Angle-resolved photoemission spectroscopy (ARPES) is used to study the scattering rates of charge carriers from the hole pockets near Gamma in the iron-based high-Tc hole doped superconductors KxBa1-xFe2As2 x=0.4 and KxEu1-xFe2As2 x=0.55$ and the electron doped compound Ba(Fe1-xCox)2As2 x=0.075. The scattering rate for any given band is found to depend linearly on energy, indicating a non-Fermi liquid regime. The scattering rates in the hole-doped compound are considerably larger than those in the electron-doped compounds. In the hole-doped systems the scattering rate of the charge carriers of the inner hole pocket is about three times bigger than the binding energy indicating that the spectral weight is heavily incoherent. The strength of the scattering rates and the difference between electron and hole doped compounds signals the importance of Hund's exchange coupling for correlation effects in these iron-based high-Tc superconductors. The experimental results are in qualitative agreement with theoretical calculations in the framework of combined density functional dynamical mean-field theory., 5 pages; 3 figures

In a comprehensive study, we investigate the electronic scattering effects in EuFe 2 ( As 1 − x P x ) 2 by using Fourier-transform infrared spectroscopy. In spite of the fact that Eu 2 + local moments order at around T Eu ∼ 20 K , the overall optical response is strikingly similar to the one of the well-known Ba-122 pnictides. The main difference lies within the suppression of the lower spin-density-wave gap feature. By analyzing our spectra with a multi-component model, we find that the high-energy feature around 0.7 eV – often associated with Hund's rule coupling – is highly sensitive to the spin-density-wave ordering; this further confirms its direct relationship to the dynamics of itinerant carriers. The same model is also used to investigate the in-plane anisotropy of magnetically detwinned EuFe 2 As 2 in the antiferromagnetically ordered state, yielding a higher Drude weight and lower scattering rate along the crystallographic a-axis. Finally, we analyze the development of the room-temperature spectra with isovalent phosphor substitution and highlight changes in the scattering rate of hole-like carriers induced by a Lifshitz transition.

We present our results of a local probe study on EuFe$_{2}$(As$_{1-x}$P$_{x}$)$_{2}$ single crystals with $x$=0.13, 0.19 and 0.28 by means of muon spin rotation and ${}^{57}$Fe M\"ossbauer spectroscopy. We focus our discussion on the sample with $x$=0.19 viz. at the optimal substitution level, where bulk superconductivity ($T_{\text{SC}}=28$ K) sets in above static europium order ($T^{\text{Eu}}=20$K) but well below the onset of the iron antiferromagnetic (AFM) transition ($\sim$100 K). We find enhanced spin dynamics in the Fe sublattice closely above $T_{\text{SC}}$ and propose that these are related to enhanced Eu fluctuations due to the evident coupling of both sublattices observed in our experiments., Comment: Contribution to the 13th International Conference on Muon Spin Rotation, Relaxation and Resonance (MuSR2014)

The magnetic structure of the Eu2+ moments in the superconducting EuFe2(As1-xPx)2 sample with x = 0.15 has been determined using element specific x-ray resonant magnetic scattering. Combining magnetic, thermodynamic and scattering measurements, we conclude that the long range ferromagnetic order of the Eu2+ moments aligned primarily along the c axis coexists with the bulk superconductivity at zero field. At an applied magnetic field >= 0.6 T, superconductivity still coexists with the ferromagnetic Eu2+ moments which are polarized along the field direction. We propose a spontaneous vortex state for the coexistence of superconductivity and ferromagnetism in EuFe2(As0.85P0.15)2., Accepted, Phys. Rev. B

Based on results from femtosecond time-resolved photoemission, we compare three different methods for determination of the electron-phonon coupling constant {\lambda} in Eu and Ba-based 122 FeAs compounds. We find good agreement between all three methods, which reveal a small {\lambda} < 0.2. This makes simple electron-phonon mediated superconductivity unlikely in these compounds., Comment: 11 pages, 3 figures

We report bulk superconductivity (SC) in Eu$_{0.2}$Sr$_{0.8}$(Fe$_{0.86}$Co$_{0.14}$)$_{2}$As$_{2}$ single crystals by means of electrical resistivity, magnetic susceptibility, and specific heat measurements with $T$$_{\mathrm{c}}$ $\simeq$ 20 K with an antiferromagnetic (AFM) ordering of Eu$^{2+}$ moments at $T$$_{\mathrm{N}}$ $\simeq$ 2.0 K in zero field. $^{75}$As NMR experiments have been performed in the two external field directions (H$\|ab$) and (H$\|c$). $^{75}$As-NMR spectra are analyzed in terms of first order quadrupolar interaction. Spin-lattice relaxation rates (1/$T_{1}$) follow a $T^{3}$ law in the temperature range 4.2-15 K. There is no signature of Hebel-Slichter coherence peak just below the SC transition indicating a non s-wave or s$_{\pm}$ type of superconductivity. The increase of 1/$T_{1}T$ with lowering the temperature in the range 160-18 K following $\frac{C}{T+\theta}$ law reflecting 2D AFM spin fluctuations.

Quantum criticality in single crystalline YbRh 2 (Si 1- x Ge x ) 2 with x ≈0.01 is investigated by electrical resistivity measurements down to 15 mK at various magnetic fields applied parallel and perpendicular to the c -axis. Compared to undoped YbRh 2 Si 2 with T N =75 mK (from the onset of the resistive signature), the slightly Ge-doped sample exhibits a reduced Neel temperature of 53 mK. In contrast to the recent report on nominally YbRh 2 (Si 0.95 Ge 0.05 ) 2 , we do not observe evidence for a non-Fermi liquid regime at T →0 over an extended magnetic field range. The obtained phase diagrams rather resemble the case of undoped YbRh 2 Si 2 .

The electron spin resonance absorption spectrum of Eu^{2+} ions serves as a probe of the normal and superconducting state in Eu_{0.5}K_{0.5}Fe_2As_2. The spin-lattice relaxation rate 1/T_1^{\rm ESR} obtained from the ESR linewidth exhibits a Korringa-like linear increase with temperature above T_C evidencing a normal Fermi-liquid behavior. Below 45 K deviations from the Korringa-law occur which are ascribed to enhanced magnetic fluctuations within the FeAs layers upon approaching the superconducting transition. Below T_C the spin-lattice relaxation rate 1/T_1^{\rm ESR} follows a T^{1.5}-behavior without the appearance of a coherence peak., 5 pages, 5 figures

Using angle resolved photoemission it is shown that the low lying electronic states of the iron pnictide parent compound EuFe$_2$As$_2$ are strongly modified in the magnetically ordered, low temperature, orthorhombic state compared to the tetragonal, paramagnetic case above the spin density wave transition temperature. Back-folded bands, reflected in the orthorhombic/ anti-ferromagnetic Brillouin zone boundary hybridize strongly with the non-folded states, leading to the opening of energy gaps. As a direct consequence, the large Fermi surfaces of the tetragonal phase fragment, the low temperature Fermi surface being comprised of small droplets, built up of electron and hole-like sections. These high resolution ARPES data are therefore in keeping with quantum oscillation and optical data from other undoped pnictide parent compounds., 4 figures, 6 pages

We report measurements of the temperature dependence of the electrical resistivity, ρ(T), and magnetic pen-etration depth, λ(T), for polycrystalline samples of Eu0.5K0.5Fe2As2 with Tc = 31 K. ρ(T) follows a linear temperature dependence above Tc and bends over to a weaker temperature dependence around 150 K. The magnetic penetration depth, determined by radio frequency technique displays an unusual minimum around 4 K which is associated with short-range ordering of localized Eu3+ moments.

We have investigated the pressure dependence of the magnetic field-temperature phase-diagram of the tetragonal compound YbRu2Ge2 by electrical resistivity measurements in the pressure range up to 10 GPa and for magnetic fields up to 14 T. peerReviewed