10 results on '"Edwards, Richard Lawrence"'
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2. Improvements in the determination of attogram-sized 231Pa in dissolved and particulate fractions of seawater via multi-collector inductively coupled plasma mass spectrometry
- Author
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Zhang, Pu, Lu, Yanbin, Zhang, Zhe, Edwards, Richard Lawrence, Anderson, Robert, and Lam, Phoebe
- Published
- 2023
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3. A seasonally resolved stalagmite δ18O record indicates the regional activity of tropical cyclones in Southeast China.
- Author
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Chen, Lvfan, Wang, Tianli, Sinha, Ashish, Lin, Fangyuan, Tang, Huiru, Cheng, Hai, Edwards, Richard Lawrence, and Tan, Liangcheng
- Subjects
STALACTITES & stalagmites ,TROPICAL cyclones ,PALEOCLIMATOLOGY - Abstract
Identifying tropical cyclone (TC) signatures in paleoclimate records enhances our understanding of long-term TC activity trends and the climatic factors influencing TC evolution. Stalagmites are considered promising archives for recording TC activity. However, despite the western North Pacific being the most TC-active ocean basin globally, it lacks stalagmite-based TC reconstructions. Here, we present a seasonally resolved stalagmite δ
18 O record from XRY cave in Southeast China, covering the period from 1951 to 2018 CE, to identify annual signals of strong TC activity. We propose that the minimum seasonal XRY δ18 O value of each year can reconstruct regional TC activity, achieving an identification rate of 86% for strong TC years in study area. This demonstrates the feasibility of using stalagmites for TC reconstruction in Southeast China. Moreover, our research shows that inland stalagmites can still capture TC activity signals, which will promote the use of stalagmites in obtaining long-term records of post-landfall TC activity and inland impacts. [ABSTRACT FROM AUTHOR]- Published
- 2024
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4. Multi-scale Holocene Asian monsoon variability deduced from a twin-stalagmite record in southwestern China
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Huang, Wei, Wang, Yongjin, Cheng, Hai, Edwards, Richard Lawrence, Shen, Chuan-Chou, Liu, Dianbing, Shao, Qingfeng, Deng, Chao, Zhang, Zhenqiu, and Wang, Quan
- Published
- 2016
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5. Improvements in the determination of attogram-sized 231Pa in dissolved and particulate fractions of seawater via multi-collector inductively coupled plasma mass spectrometry.
- Author
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Zhang, Pu, Lu, Yanbin, Zhang, Zhe, Edwards, Richard Lawrence, Anderson, Robert, and Lam, Phoebe
- Subjects
INDUCTIVELY coupled plasma mass spectrometry ,SEAWATER ,PARTICULATE matter - Abstract
A technique is developed to quantify the ultra-trace
231 Pa (35–3904 ag) concentration in seawater using multi-collector inductively coupled plasma mass spectrometry (MC-ICP-MS). The method is a modification of the process developed by Shen et al. (Anal Chem 75(5):1075–1079, 2003. https://doi.org/10.1021/ac026247r) and extends it to the application of very low levels of actinides, and the 35 ag231 Pa can be measured with a precision of 15%. The total process blank for the water column was 0.02 ag/g, while the values of the large and small particles were ~ 30 ag/g. The ionization efficiency (ions generated/atom loaded) varies from 0.7 to 2.4%. The measurement time is 2–5 min. The amount of231 Pa needed to produce231 Pa data with an uncertainty of ± 0.8–15% is 35–3904 ag (~ 0.9 × 105 to 10 × 106 atoms). Replicate measurements of known standards and seawater samples demonstrate that the analytical precision approximates that expected from counting statistics, and that based on detection limits of 52 ag, 55 ag, and 28 ag, protactinium can be detected in a minimum seawater sample size of ~ 2.6 L for small suspended particulate matter (> 0.8 μm and < 51 μm), ~ 3.0 L for large suspended particulate matter (> 51 μm), and ~ 56 mL for filtered (< 0.45 μm) seawater. The concentration of231 Pa (several attograms per liter) can be determined with an uncertainty of ± 2–8% (2σ) for suspended particulate matter filtered from ~ 60 L of seawater. For the dissolved fraction, ~ 1 L of seawater yields231 Pa measurements with a precision of 0.8–10%. The sample size requirements are several orders of magnitude less than traditional decay-counting techniques, and the precision is better than that previously reported for ICP-MS techniques. Our technique can also be applied to other environmental samples, including river, lake, and cave water samples. [ABSTRACT FROM AUTHOR]- Published
- 2023
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6. Gradual South‐North Climate Transition in the Atlantic Realm Within the Younger Dryas.
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Zhang, Haiwei, Cheng, Hai, Spötl, Christoph, Zhang, Xu, Cruz, Francisco W., Sinha, Ashish, Auler, Augusto S., Stríkis, Nicolás M., Wang, Xianfeng, Kathayat, Gayatri, Li, Xianglei, Li, Hanying, Pérez‐Mejías, Carlos, Cai, Yanjun, Ning, Youfeng, and Edwards, Richard Lawrence
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YOUNGER Dryas ,SPELEOTHEMS ,INTERTROPICAL convergence zone ,ATMOSPHERIC carbon dioxide ,MERIDIONAL overturning circulation ,WESTERLIES - Abstract
The abrupt climate event Younger Dryas (YD) has been extensively studied; however, its structure is still poorly understood. Climate in northeastern Brazil is very sensitive to the latitudinal position of the intertropical convergence zone (ITCZ) associated with abrupt climate change in the Atlantic. Here, we report changes in the ITCZ position within the YD by using precise speleothem multiproxy records from northeastern Brazil. We provide evidence for a gradual northward migration of the ITCZ preceding poleward shifts of the westerlies and the polar front in northern high latitudes within the YD. This can be attributed to gradual increase in atmospheric CO2 concentration as a consequence of the weakening Atlantic Meridional Overturning Circulation (AMOC). We suggest that a persistent increase in atmospheric CO2 might have triggered a resumption of the AMOC and reorganization of the atmosphere circulation in the Atlantic during the mid‐YD. Plain Language Summary: The Younger Dryas (YD) is the most recent millennial‐scale abrupt climate event in Earth history. Although its origin has been extensively studied, its structure is still poorly understood. Climate in northeastern Brazil is very sensitive to the latitudinal position of the intertropical convergence zone (ITCZ) responds to abrupt climate change in the Atlantic (e.g., YD). By using stable isotope and trace element proxy records of speleothem from Toca da Boa Vista Cave, northeastern Brazil, together with other paleoclimatic records in the Atlantic realm, we provide evidence for a gradual northward migration of the ITCZ preceding poleward shifts of the westerlies and the polar front in northern high latitudes within the YD. This can be attributed to a gradual increase in atmospheric CO2 concentration under the situation of weakening Atlantic Meridional Overturning Circulation (AMOC). A persistent increase in atmospheric CO2 concentration might have triggered a resumption of the AMOC and reorganization of the atmosphere circulation in the Atlantic during the mid‐YD. Key Points: Speleothem and other paleoclimate records confirm a wet climate in tropical South America within the Younger DryasPrecise speleothem multiproxy records reflect a bipartition of the Younger Dryas precipitation in northeastern BrazilGradual South‐North climate transition in the Atlantic responded to a gradual increase in atmospheric CO2 within the YD [ABSTRACT FROM AUTHOR]
- Published
- 2021
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7. From cave geomorphology to Palaeolithic human behaviour: speleogenesis, palaeoenvironmental changes and archaeological insight in the Atxurra‐Armiña cave (northern Iberian Peninsula).
- Author
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Arriolabengoa, Martin, Intxaurbe, Inaki, Medina‐Alcaide, Mª Ángeles, Rivero, Olivia, Rios‐Garaizar, Joseba, LÍbano, Inaki, Bilbao, Peru, Aranburu, Arantza, Cheng, Hai, Edwards, Richard Lawrence, and Garate, Diego
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CAVES ,GEOMORPHOLOGY ,PENINSULAS ,BEHAVIOR ,INSIGHT ,RIVERS - Abstract
A detailed geomorphological study was performed in the Atxurra‐Armiña cave system (northern Iberian Peninsula) to decode landscape evolution, palaeoenvironmental changes and human use of a cave within an Inner Archaeological Context. The results show an average incision rate of the river of <0.083 mm a–1 for at least the last 419 ka, with interruptions due to sedimentary inputs. Moreover, allostratigraphic units comprising fluviokarstic deposits at the base and flowstone formation at the top have been shown to be climatically controlled, formed either during glacial–interglacial cycles or during interstadial cycles. Finally, when the cave was used by humans in the Late Magdalenian, the lower entrance was closed, and they must therefore have entered the cave through the upper entrance. To reach the sectors selected to decorate the panels, they probably travelled from the upper cave level, as the current crawlway was wider than today, according to our U/Th dating. Once these visitors reached the panels, the floor in the main gallery would have been around 15 cm lower than at present. However, the morphology of the conduit was similar; this has significant implications for understanding and interpreting the human use of the cave during the Palaeolithic. [ABSTRACT FROM AUTHOR]
- Published
- 2020
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8. Hydro-climatic variability in the southwestern Indian Ocean between 6000 and 3000 years ago.
- Author
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Li, Hanying, Cheng, Hai, Sinha, Ashish, Kathayat, Gayatri, Spötl, Christoph, André, Aurèle Anquetil, Meunier, Arnaud, Biswas, Jayant, Duan, Pengzhen, Ning, Youfeng, and Edwards, Richard Lawrence
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CLIMATE change ,STABLE isotopes ,SPELEOTHEMS ,METEOROLOGICAL precipitation ,INTERTROPICAL convergence zone ,HOLOCENE Epoch - Abstract
The "4.2 ka event" is frequently described as a major global climate anomaly between 4.2 and 3.9 ka, which defines the beginning of the current Meghalayan age in the Holocene epoch. The "event" has been disproportionately reported from proxy records from the Northern Hemisphere, but its climatic manifestation remains much less clear in the Southern Hemisphere. Here, we present highly resolved and chronologically well-constrained speleothem oxygen and carbon isotopes records between ∼6 and 3 ka from Rodrigues Island in the southwestern subtropical Indian Ocean, located ∼600 km east of Mauritius. Our records show that the 4.2 ka event did not manifest itself as a period of major climate change at Rodrigues Island in the context of our record's length. Instead, we find evidence for a multi-centennial drought that occurred near-continuously between 3.9 and 3.5 ka and temporally coincided with climate change throughout the Southern Hemisphere. [ABSTRACT FROM AUTHOR]
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- 2018
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9. Three distinct Holocene intervals of stalagmite deposition and nondeposition revealed in NW Madagascar, and their paleoclimate implications.
- Author
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Voarintsoa, Ny Riavo Gilbertinie, Railsback, Loren Bruce, Brook, George Albert, Lixin Wang, Kathayat, Gayatri, Hai Cheng, Xianglei Li, Edwards, Richard Lawrence, Michel Rakotondrazafy, Amos Fety, and Madison Razanatseheno, Marie Olga
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HOLOCENE paleoclimatology ,STALACTITES & stalagmites ,PETROLOGY ,MINERALOGY ,INTERTROPICAL convergence zone - Abstract
Petrographic features, mineralogy and stable isotopes from two stalagmites, ANJB-2 and MAJ-5, respectively from Anjohibe and Anjokipoty caves, allow distinction of three intervals of the Holocene in NW Madagascar. The Malagasy early Holocene (between ca. 9.8 and 7.8 ka) and late Holocene (after ca. 1.6 ka) intervals (MEHI and MLHI, respectively) record evidence of stalagmite deposition. The Malagasy middle Holocene interval (MMHI, between ca. 7.8 and 1.6 ka) is marked by a depositional hiatus of ca. 6500 years. Deposition of these stalagmites indicates that the two caves were sufficiently supplied with water to allow stalagmite formation. This suggests that the MEHI and MLHI intervals may have been comparatively wet in NW Madagascar. In contrast, the long-term depositional hiatus during the MMHI implies it was relatively drier than the MEHI and the MLHI. The alternating wet-dry-wet conditions during the Holocene may have been linked to the long-term migrations of the Intertropical Convergence Zone (ITCZ). When the ITCZ's mean position is farther south, NW Madagascar experiences wetter conditions, such as during the MEHI and MLHI and when it moves north, NW Madagascar climate becomes drier, such as during the MMHI. A similar wet- dry-wet succession during the Holocene has been reported in neighboring locations, such as southeastern Africa. Beyond these three subdivisions, the records also suggest wet conditions around the cold 8.2 ka event, suggesting a causal relationship. However, additional Southern Hemisphere highresolution data will be needed to confirm this. [ABSTRACT FROM AUTHOR]
- Published
- 2017
- Full Text
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10. High Precision Thorium-230 Ages of Corals and the Timing of Sea Level Fluctuations in the Late Quaternary
- Author
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Edwards, Richard Lawrence
- Subjects
Geochemistry ,FOS: Earth and related environmental sciences - Abstract
Mass spectrometric techniques for the measurement of ²³⁰Th and ²³⁴U have been developed. These techniques have made it possible to reduce the analytical errors in ²³⁰Th dating of corals using very small samples. Samples of 8 x 10⁷ atoms of ²³⁰Th can be measured to an accuracy of ±130% (2 sigma), 6 x 10⁸ atoms of ²³⁰Th can be measured to an accuracy of ±29%, and 3 x 10¹⁰ atoms of ²³⁰Th can be measured to an accuracy of ±2%. The time range over which useful data on corals can now be obtained ranges from 15 to 500,000 years. The error in age (based on analytical error) for a sample that is 18 years old ±3 years (2 sigma). The error is ±5 years at 180 years, ±44 years at 8294 years, and ±1 ky at 123.1 ky. For young corals, this approach may be preferable to ¹⁴C dating. Fluctuations in climate result in changes in sea level because the ice stored in continental glaciers is ultimately derived from the ocean. Certain species of coral grow close to the sea surface. Fossils of these species therefore record the former height of the sea surface. The precision with which the age of a coral can now be determined makes it possible to determine, with some precision, the timing of sea level fluctuations in the late Quaternary. This record will allow a critical test of the Milankovitch hypothesis, which predicts the timing of Pleistocene climate fluctuations from changes in the distribution of solar insolation that result from changes in the earth's orbital geometry. Analyses of a number of corals that grew during the last interglacial period yield ages of 122 to 130 ky. The ages coincide with or slightly postdate the summer solar insolation high at 65°N latitude, which occurred 128 ky ago. This supports the idea that changes in Pleistocene climate can be the result of orbital forcing. Apparent fluctuations in sea level recorded on tectonically active shorelines are the result of both sea level change and vertical tectonic movement. If the record of sea level change is known (e.g., from the coral record in a stable area), this record can be subtracted from the record of apparent sea level change, in the tectonically active area, to yield a record of vertical tectonic movement. The precision with which coral ages can now be determined may allow us to resolve the ages of individual coseisimic uplift events and thereby date prehistoric earthquakes. This possibility has been examined at two localities, northwest Santo Island and north Malekula Island, Vanuatu. Previous work (Taylor et al., 1980, 1985a, 1987) showed (using the counting of annual growth bands to determine ages) that the tops of partially emerged coral heads at each locality died at the same time as the last major earthquake at each locality (MS = 7.5, 1973, on northwest Santo; and MS = 7.5, 1965, on north Malekula). It was concluded that the tops of these coral heads were killed by coseismic uplift. At each locality, there were also completely emerged coral heads, which were inferred to have been killed by earlier coseismic uplift events. These could not be dated by growth band counting because the coral heads were completely dead. The accuracy of ²³⁰Th ages of very young corals was tested by dating portions of three corals whose ages were known from the counting of growth bands. Within analytical error, the ²³⁰Th ages were the same as the growth band ages for all three samples (dates of growth by counting growth bands - A.D. 1971 to 1973, A.D. 1935 to 1939, and A.D. 1804 to 1810; dates of growth from ²³⁰Th measurements - A.D. 1969 ± 3, A.D. 1932 ± 5, and A.D. 1806 5 [2 sigma ±1) demonstrating that the ²³⁰Th ages were accurate. The ²³⁰Th growth dates of the surfaces of adjacent emerged coral heads, collected from the same elevation (1.2 m) on northwest Santo Island, were, within analytical error, identical (A.D. 1866 ± 4 and A.D. 1864 ± 4). This indicates that the corals died at the same time and is consistent with the idea that they were killed by coseismic uplift. Similar adjacent coral heads on north Malekula Island yielded ²³⁰Th growth dates of A.D. 1729 ± 3 and A.D. 1718 ± 5. The ages are similar but analytically distinguishable. The difference may be due to erosion of the outer, younger, portion of the latter coral head. Using the date of the large historical earthquake at each locality and the ²³⁰Th growth date of the emerged corals at each locality, recurrence intervals of 108 years for northwest Santo and 236 years for north Malekula are calculated. This experiment has shown that it is possible to date corals that grew in the past several centuries to accuracies of ±3 to ±5 years (2 sigma). The main problems with applying this approach to determine seismic histories will be associated with the preservation of fossil corals that have been killed by coseimic uplift and the ability to identify such features in the field.
- Published
- 1988
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