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• Develop a novel two-layer coordinated multi-agent reinforcement learning algorithm. • Synergize traffic signals through local cooperation and global coordination. • Optimization of vehicle emissions and traffic congestion as simultaneous goals. • Proposed method is performed in synthetic network and Cologne urban network on SUMO. Intersection traffic signal control considering vehicle emissions has become an important topic, however, the decision complexity of traffic signal control increases dramatically in a dynamic traffic environment with multi-intersections. It is a severe challenge to coordinate traffic signals at multi-intersections based on Internet of Things information to improve the traffic condition of the road network. This paper proposes a two-layer coordination algorithm based on multi-agent reinforcement learning—Multi-agent Coordinated Policy Optimization (MACoPO), for solving traffic signal control at multi-intersections. MACoPO consists of local cooperation, which adjusts the weights of individual rewards and neighborhood agents' rewards by using local cooperation factors (LCF), and global coordination, which updates the LCF to maximize global rewards. The state and reward functions are designed in terms of the current state of the signal, waiting queue length, vehicle density and emission concentration in the lane, vehicle delay, and vehicle emissions, thus making full use of the intersection state information. The proposed method is extensively assessed through simulation experiments using artificial and real road networks and the numerical results confirm its effectiveness in complex and dynamic real-time traffic environments with multi-intersections. [ABSTRACT FROM AUTHOR]