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For 0 ≤ α ≤ 1, Nikiforov proposed to study the spectral properties of the family of matrices Aα(G) = αD(G)+(1 - α)A(G) of a graph G, where D(G) is the degree diagonal matrix and A(G) is the adjacency matrix of G. The α-spectral radius of G is the largest eigenvalue of Aα(G). For a graph with two pendant paths at a vertex or at two adjacent vertices, we prove results concerning the behavior of the α-spectral radius under relocation of a pendant edge in a pendant path. We give upper bounds for the α-spectral radius for unicyclic graphs G with maximum degree ∆ ≥ 2, connected irregular graphs with given maximum degree and some other graph parameters, and graphs with given domination number, respectively. We determine the unique tree with the second largest α-spectral radius among trees, and the unique tree with the largest α-spectral radius among trees with given diameter. We also determine the unique graphs so that the difference between the maximum degree and the α-spectral radius is maximum among trees, unicyclic graphs and non-bipartite graphs, respectively. [ABSTRACT FROM AUTHOR]