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Measurements of root‐zone soil moisture across spatial scales of tens to thousands of meters have been a challenge for many decades. The mobile application of Cosmic Ray Neutron Sensing (CRNS) is a promising approach to measure field soil moisture noninvasively by surveying large regions with a ground‐based vehicle. Recently, concerns have been raised about a potentially biasing influence of local structures and roads. We employed neutron transport simulations and dedicated experiments to quantify the influence of different road types on the CRNS measurement. We found that roads introduce a substantial bias in the CRNS estimation of field soil moisture compared to off‐road scenarios. However, this effect becomes insignificant at distances beyond a few meters from the road. Neutron measurements on the road could overestimate the field value by up to 40 % depending on road material, width, and the surrounding field water content. The bias could be largely removed with an analytical correction function that accounts for these parameters. Additionally, an empirical approach is proposed that can be used without prior knowledge of field soil moisture. Tests at different study sites demonstrated good agreement between road‐effect corrected measurements and field soil moisture observations. However, if knowledge about the road characteristics is missing, measurements on the road could substantially reduce the accuracy of this method. Our results constitute a practical advancement of the mobile CRNS methodology, which is important for providing unbiased estimates of field‐scale soil moisture to support applications in hydrology, remote sensing, and agriculture. Plain Language Summary: Measurements of root‐zone soil moisture across spatial scales of tens to thousands of meters have been a challenge for many decades. The mobile application of Cosmic Ray Neutron Sensing (CRNS) is a promising approach to measure field soil moisture noninvasively by surveying large regions with a ground‐based vehicle. Recently, concerns have been raised about a potentially biasing influence of roads. We employed physics simulations and dedicated experiments to quantify the influence of different road types on the CRNS measurement. We found that the presence of roads biased the CRNS estimation of field soil moisture compared to nonroad scenarios. Neutron measurements could overestimate the field value by up to 40 % depending on road material, width, surrounding field water content, and distance from the road. We proposed a correction function that successfully removed this bias and works even without prior knowledge of field soil moisture. Tests at different study sites demonstrated good agreement between corrected measurements and other field soil moisture observations. Our results constitute a practical advancement of the mobile CRNS methodology, which is important for providing unbiased estimates of field‐scale soil moisture to support applications in hydrology, remote sensing, and agriculture. Key Points: Mobile Cosmic‐Ray Neutron Sensing can capture small‐scale patterns of root‐zone soil water at scales from tens to hundreds of metersNeutron simulations and field experiments reveal that CRNS estimation of field soil moisture is substantially biased by the presence of roadsWe propose a practical correction approach that is essential to provide unbiased soil water data for hydrological applications [ABSTRACT FROM AUTHOR]