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The exact solution and heuristic solution have their own strengths and weaknesses on solving the Vehicle Routing Problems with Time Windows (VRPTW). This paper proposes a hybrid Column Generation Algorithm with Metaheuristic Optimization (CGAMO) to overcome their weaknesses. Firstly, a Modified Labelling Algorithm (MLA) in the sub-problem of path searching is analysed. And a search strategy in CGAMO based on the demand of sub-problem is proposed to improve the searching efficiency. While putting the paths found in the sub-problem into the main problems of CGAMO, the iterations may fall into endless loops. To avoid this problem and keep the main problems in a reasonable size, two conditions on saving the old paths in the main problem are used. These conditions enlarge the number of constraints considered in the iterations to strengthen the limits of dual variables. Through analysing the sub-problem, we can find many useless paths that have no effect on the objective function. Secondly, in order to reduce the number of useless paths and improve the efficiency, this paper proposes a heuristic optimization strategy of CGAMO for dual variables. It is supposed to accelerate the solving speed from the view of on the dual problem. Finally, extensive experiments show that CGAMO achieves a better performance than other state-of-the-art methods on solving VRPTW. The comparative experiments also present the parameters sensitivity analysis, including the different effects of MLA in the different path selection strategies, the characteristics and the applicable scopes of the two pathkeeping conditions in the main problem. First published online: 25 Oct 2013