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• The mechanism of enhanced for PCF scattering in AlN/GaN HFETs has been clarified. • A large number of additional polarization charges (Δ ρ G) are generated under the gate. • Δ ρ G will become saturated with the decrease in gate bias. • The decreases of 2DEG density will enhance the PCF scattering intensity. AlN/GaN heterostructure field-effect transistors (HFETs) was fabricated. Based on the polarization Coulomb field (PCF) scattering theory model, the additional polarization charges and mobility are obtained by iterative calculation method. By analyzing the results, it is found that (i) the electric field strength in the AlN barrier layer is large because it is ultrathin, and the piezoelectric tensor coefficient of AlN material is large; thus, the inverse piezoelectric effect is very strong. A large number of additional polarization charges are generated under the gate, which can generate a strong PCF scattering potential and enhance PCF scattering. What's more, the AlN barrier layer cannot be infinitely strained by the gate bias with the converse piezoelectric effect, and the additional polarization charges will become saturated with the decrease in gate bias. (ii) The AlN barrier layer of AlN/GaN HFETs is ultrathin, the two-dimensional electron gas (2DEG) density under the gate is quickly decreased by the gate bias, and, with the decrease in 2DEG density, PCF scattering is enhanced. [ABSTRACT FROM AUTHOR]