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Flexible piezoelectric sensors have received widespread attention in wearable electronics for their ability to convert mechanical energy into electrical energy, while the insufficient output power and complex preparation process have limited their application. In this work, several honeycomb structures based on graphene macro-film (GAMF) were created via laser engraving, which can utilize negative Poisson's ratio (NPR) properties to improve the output electric performance of flexible piezoelectric sensors. The effect of different electrode materials on the piezoelectric output was investigated in the experiments and compared with the theoretical equations, indicating that the output power of the sensor could be enhanced up to 142 % by improving the materials auxetic mechanical properties. The stability tests have proven that the sensors can operate effectively for a long time under different operating conditions. Moreover, the optimized sensor shows powerful potential for monitoring human movements such as finger tapping, joint bending, and foot stepping. This work opens up a new development path for the preparation of convenient and high-performance wearable electronic devices. The negative Poisson's ratio characteristic of the honeycomb graphene macro-film is used to increase the deformation of PVDF film to increase the electrical output performance of the flexible piezoelectric sensor. The optimized sensor can be used to detect human movements. [Display omitted] • Honeycomb graphene macro-films with different mechanical properties were prepared by laser engraving. • Flexible piezoelectric sensors based on honeycomb graphene macro-films are prepared. • The output performance of piezoelectric sensors can be improved by adjusting mechanical properties of electrode materials. • The flexible piezoelectric sensors can be used to detect human movements. [ABSTRACT FROM AUTHOR]