1. Ultrafast dynamical Lifshitz transition
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Maciej Dendzik, Nicolas Tancogne-Dejean, Angel Rubio, Samuel Beaulieu, Michael A. Sentef, Laurenz Rettig, Ralph Ernstorfer, Shuo Dong, Julian Maklar, Tommaso Pincelli, R. Patrick Xian, and Martin Wolf
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Colossal magnetoresistance ,Materials Science ,Physics::Optics ,FOS: Physical sciences ,Non-equilibrium thermodynamics ,Weyl semimetal ,02 engineering and technology ,01 natural sciences ,Condensed Matter - Strongly Correlated Electrons ,0103 physical sciences ,Computer Science::Networking and Internet Architecture ,Physics::Atomic and Molecular Clusters ,Physics::Chemical Physics ,010306 general physics ,Quantum ,Research Articles ,Topology (chemistry) ,Condensed Matter::Quantum Gases ,Superconductivity ,Physics ,Condensed Matter - Materials Science ,Multidisciplinary ,Strongly Correlated Electrons (cond-mat.str-el) ,Condensed matter physics ,SciAdv r-articles ,Materials Science (cond-mat.mtrl-sci) ,Fermi surface ,Time-dependent density functional theory ,021001 nanoscience & nanotechnology ,3. Good health ,Condensed Matter::Strongly Correlated Electrons ,0210 nano-technology ,Research Article - Abstract
We demonstate a non-equilibrium route for ultrafast modification of Fermi surface topology in quantum materials., Fermi surface is at the heart of our understanding of metals and strongly correlated many-body systems. An abrupt change in the Fermi surface topology, also called Lifshitz transition, can lead to the emergence of fascinating phenomena like colossal magnetoresistance and superconductivity. While Lifshitz transitions have been demonstrated for a broad range of materials by equilibrium tuning of macroscopic parameters such as strain, doping, pressure, and temperature, a nonequilibrium dynamical route toward ultrafast modification of the Fermi surface topology has not been experimentally demonstrated. Combining time-resolved multidimensional photoemission spectroscopy with state-of-the-art TDDFT+U simulations, we introduce a scheme for driving an ultrafast Lifshitz transition in the correlated type-II Weyl semimetal Td-MoTe2. We demonstrate that this nonequilibrium topological electronic transition finds its microscopic origin in the dynamical modification of the effective electronic correlations. These results shed light on a previously unexplored ultrafast scheme for controlling the Fermi surface topology in correlated quantum materials.
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