Search

Continuous carbon fiber reinforced polymer composite 3D printing has drawn more attention due to its ability to manufacture composite structures with complex shapes. The surface treatment of CF is necessary to improve the combination between carbon fiber (CF) and matrix. In this work, polyurethane with nano‐SiO2 (PU/SiO2) was used to size CF to enhance the compatibility of CF and nylon 6 (PA6). The chemistry and morphology of the CF were characterized by Fourier transform infrared spectroscopy (FTIR), X‐ray photoelectron spectroscopy (XPS), and scanning electron microscopy (SEM). The interface strength between CF and PA6 was tested by the fiber pull‐out test, and eventually obtained optimized concertation of PU/SiO2 sizing agents (with 25 wt% PU and 0.4 wt% nano‐SiO2). The results show that compared with untreated CF, the interfacial shear strength (IFSS) of CF and PA6 after sizing increased by 316.93%. In addition, several CF/PA6 composite specimens printed by a homemade composite 3D printer were used to do mechanical tests. The results show that the flexural strength increased by 33.87%, the tensile strength increased by 20.75%, and the interlaminar shear strength (ILSS) increased by 66.54%. [ABSTRACT FROM AUTHOR]

The inherent defects of the layer‐by‐layer manufacturing process limit the mechanical performance of 3D‐printed composite parts. This paper explores a process optimization method for continuous fiber composites 3D printing to improve the mechanical performance of 3D‐printed CF/PA6 (Carbon Fiber/Nylon 6) parts. First, the effects of printing temperature, printing speed, layer thickness, and side step on the mechanical performance of 3D‐printed CF/PA6 were studied by conducting variable parameter printing experiments. All optimal printing parameters for CF/PA6 were obtained, and their impact mechanisms were analyzed. Second, the coupling effect of temperature and pressure of post‐processing reduced the internal voids of 3D‐printed CF/PA6 and improved its mechanical properties. The influence mechanism of the coupling effect of temperature and pressure was summarized, and the optimal post‐processing parameters applicable to CF/PA6 were obtained. Based on the above process optimization, the fiber volume content of the printed CF/PA6 reached 41.05%, and the bending strength and elastic modulus reached 651.54 MPa and 79.08 GPa, which were 209.05% and 179.53% higher than those before optimization. Moreover, the tensile strength and elastic modulus reached 730 MPa and 29.23GPa, which were 98.10% and 81.10% higher than those before optimization. The experimental results give a positive validation of the effectiveness and feasibility of the proposed methodology. Highlights: The effects of printing temperature, printing speed, layer thickness, and side step on the mechanical properties of 3D‐printed CF/PA6 were investigated. The optimal printing parameters applicable to CF/PA6 were obtained and their influence mechanisms were analyzed.The effects of the heat press processing method on the internal voids and mechanical properties of 3D‐printed CF/PA6 were investigated, and the optimal post‐processing parameters applicable to CF/PA6 were obtained.The study resulted in optimal printing parameters and post‐processing parameters for 3D printing CF/PA6, which greatly enhanced its tensile and flexural strength and modulus. [ABSTRACT FROM AUTHOR]