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In this study, a segmented layered bistable piezoelectric energy harvester (SBPEH) has been developed and thoroughly investigated for its wind energy harvesting capabilities. The SBPEH's performance was comprehensively evaluated through the creation of a detailed 3D finite element model using Abaqus and XFlow software, and further validated via rigorous wind tunnel experiments. The results of this research demonstrate the SBPEH's remarkable potential for wind energy harvesting. With a wide operational wind speed range, it achieved a maximum measured power output of 5.476 mW, coupled with an outstanding power density of 68.45 mW/cm3, both of which were realized at a wind speed of 13 m/s. It is worth noting that as the wind speed surpasses a specific threshold, the energy harvesting efficiency of the SBPEH experiences a decline, emphasizing the importance of identifying the optimal operational wind speed range for maximizing energy output. These findings offer valuable insights for the enhancement and application of SBPEHs, contributing to the advancement of renewable energy technologies and providing an eco‐friendly solution for power generation. Highlights: The study introduces a new segmented layered bistable piezoelectric energy harvester (SBPEH) design for wind energy harvesting, addressing the limitations of traditional harvesters.Performance is evaluated through 3D finite element modeling, ABAQUS, Xflow simulations, and wind tunnel experiments.The SBPEH operates efficiently across a broad wind speed range (6–14 m/s), showcasing optimal output power of 5.476 mW at 13 m/s. [ABSTRACT FROM AUTHOR]