Search

We show that multiple filamentation patterns in high-power laser beams, can be described by means of two statistical physics concepts, namely self-similarity of the patterns over two nested scales, and nearest-neighbor interactions of classical rotators. The resulting lattice spin model perfectly reproduces the evolution of intense laser pulses as simulated by the Non-Linear Schr\"odinger Equation, shedding a new light on multiple filamentation. As a side benefit, this approach drastically reduces the computing time by two orders of magnitude as compared to the standard simulation methods of laser filamentation., Comment: 8 pages, 4 figures

While filaments are generally interpreted as a dynamic balance between Kerr focusing and plasma defocusing, the role of the higher-order Kerr effect (HOKE) is actively debated as a potentially dominant defocusing contribution to filament stabilization. In a pump-probe experiment supported by numerical simulations, we demonstrate the transition between two distinct filamentation regimes at 800 nm. For long pulses (1.2 ps), the plasma substantially contributes to filamentation, while this contribution vanishes for short pulses (70 fs). These results confirm the occurrence, in adequate conditions, of filamentation driven by the HOKE rather than by plasma.

We present a general mechanism for successful discrimination of spectroscopically indistinguishable biochromophores by shaped light. For this purpose we use nonadiabatic dynamics in excited electronic states in the frame of the field-induced surface hopping method driven by the experimentally shaped laser fields. Our findings show that optimal laser fields drive low-frequency vibrational modes localized in the side chains of two biochromophores, thus selecting the parts of their potential energy surfaces characterized by different transition dipole moments leading to different ionization probabilities. The presented mechanism leads to selective fluorescence depletion which serves as a discrimination signal. Our findings offer a promising perspective for using optimally shaped laser pulses in bioanalytical applications by increasing the selectivity beyond the current capability.

We show that higher-order nonlinear indices ($n_4$, $n_6$, $n_8$, $n_{10}$) provide the main defocusing contribution to self-channeling of ultrashort laser pulses in air and Argon at 800 nm, in contrast with the previously accepted mechanism of filamentation where plasma was considered as the dominant defocusing process. Their consideration allows to reproduce experimentally observed intensities and plasma densities in self-guided filaments., 11 pages, 6 figures (11 panels)

The optical-absorption spectrum of Lib has been observed by depletion spectroscopy in the 400-700-nm range. The experimental results are compared with theoretical spectra calculated for the three Li 6 structures in competition and we have been able to unambiguously determine the most stable Li 6 geometry as being the C 2υ tripyramidal geometry

We report the first observation of white-light emission from femtosecond laser-induced plasma in a water droplet. Such emission is not observed with water in a cell. The microdroplet acts as a lens, focusing the incident light to nanosized regions within itself and directing the emission from these regions primarily back toward the laser source. This focusing increases the intensity so that multiphoton ionization generates plasma and causes it to reach the critical density during the initial part of the pulse, enabling the rest of the pulse to heat the plasma enough to emit in the visible.

We demonstrate theoretically and experimentally that one-, two-, and three-photon excited fluorescence from dye molecules in spherical microcavities has an asymmetrical angular distribution and is enhanced in the backward direction. The enhancement ratios (of intensities at 180 degrees and 90 degrees ) are 9, 5, and 1.8 for three-, two-, and one-photon excitation, respectively. Even larger ratios are expected for microspheres with an index of refraction larger than that used in the experiments. Because of the reciprocity principle and concentration of the incident wave inside particles, the backward enhancement is expected to occur even with nonspherical particles.

A l'aide de l'ionisation biphotonique resonnante, identification de l'etat excite 2 2 E' avec une bande origine a 14583 cm −1 . Analyse des donnees a l'aide du modele Jahn-Teller dynamique: les caracteristiques de distorsion et de localisation sont faibles et l'etat vibronique inferieur est situe au-dessus de l'intersection conique, ce qui implique une geometrie D 3h ; le mode symetrique se situe a 326 cm −1 . Analyse des etats rotationnels; facteurs de Franck-Condon

Inner-shell autoionization spectra obtained with synchrotron radiation are reported for mercury clusters ${\mathrm{Hg}}_{n}$, $n\ensuremath{\le}40$. For the small clusters $n\ensuremath{\le}12$ the spectral behavior as a function of size is interpreted in terms of an excitonic model. For larger cluster sizes a gradual deviation from van der Waals bonding is observed. The asymmetry occuring in the line profiles reflects the progressive construction of the $\mathrm{sp}$ conduction band.