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Isomers with three- and five-nucleon-hole configurations have been established in $^{203}$Tl. These include newly identified levels with a three-nucleon structure: {\it I}$^{\pi }$ = (15/2$^{-}$) with {\it T}$_{1/2}$ = 7.9(5) ns, and {\it I}$^{\pi }$ = (35/2$^{-}$) with {\it T}$_{1/2}$ = 4.0(5) ns. In addition, five-quasiparticle states: {\it I}$^{\pi }$ = (39/2$^{-}$) with {\it T}$_{1/2}$ = 1.9(2) ns, and {\it I}$^{\pi }$ = (49/2$^{+}$) with {\it T}$_{1/2}$ = 3.4(4) ns have also been established. The previously determined long-lived decay [{\it T}$_{1/2}$ = 6.6(3) $\mu $s from this work] is associated with isomerism of the {\it I}$^{\pi }$ = (29/2$^{+}$) state. Levels above this long-lived isomer have been identified through a delayed-prompt coincidence measurement. Five-nucleon-hole states with excitation energies {\it E}$_{x}$ $\approx $ 7 MeV have been established as well as possible octupole excitations of the $^{208}$Pb core built on these levels. The level scheme of $^{203}$Tl is extended up to {\it E}$_{x}$ $\approx $ 11 MeV with the inclusion of 25 new transitions. Empirical and shell-model calculations have been performed to aid in the description of the observed states which are found to be predominantly of intrinsic character., Comment: 14 pages, 10 figures

The astrophysical $^{25}\mathrm{Al}(p,\ensuremath{\gamma})\phantom{\rule{0.16em}{0ex}}^{26}\mathrm{Si}$ reaction represents one of the key remaining uncertainties in accurately modeling the abundance of radiogenic $^{26}\mathrm{Al}$ ejected from classical novae. Specifically, the strengths of key proton-unbound resonances in $^{26}\mathrm{Si}$, that govern the rate of the $^{25}\mathrm{Al}(p,\ensuremath{\gamma})$ reaction under explosive astrophysical conditions, remain unsettled. Here, we present a detailed spectroscopy study of the $^{26}\mathrm{Si}$ mirror nucleus $^{26}\mathrm{Mg}$. We have measured the lifetime of the ${3}^{+}$, 6.125-MeV state in $^{26}\mathrm{Mg}$ to be $19(3)\phantom{\rule{0.28em}{0ex}}\mathrm{fs}$ and provide compelling evidence for the existence of a ${1}^{\ensuremath{-}}$ state in the $T=1,\phantom{\rule{0.28em}{0ex}}A=26$ system, indicating a previously unaccounted for $\ensuremath{\ell}=1$ resonance in the $^{25}\mathrm{Al}(p,\ensuremath{\gamma})$ reaction. Using the presently measured lifetime, together with the assumption that the likely ${1}^{\ensuremath{-}}$ state corresponds to a resonance in the $^{25}\mathrm{Al}+p$ system at 435.7(53) keV, we find considerable differences in the $^{25}\mathrm{Al}(p,\ensuremath{\gamma})$ reaction rate compared to previous works. Based on current nova models, we estimate that classical novae may be responsible for up to $\ensuremath{\approx}15%$ of the observed galactic abundance of $^{26}\mathrm{Al}$.

Excited states in the neutron-rich nucleus Fe 68 were populated using a Be 9 ( Co 68 , 68 Fe + γ ) X charge-exchange reaction at 95 MeV/u. The new γ -ray transitions reported here for the first time complement data from β -decay studies and nucleon knockout reactions. In comparison to shell-model calculations with the LNPS effective interaction, two candidate states for the 6 1 + level emerge. The distinct population pattern of excited states and the magnitude of the cross section, σ inc = 0.51 ( 6 ) mb, make this reaction a promising one for future in-beam γ -ray spectroscopy. Reaction calculations with nuclear structure input from a new, locally optimized Hamiltonian, f 7 j 4 a , together with general considerations for heavy-ion-induced charge-exchange reactions appear consistent with most of the observations, although challenges remain.

The $^{24}\mathrm{Mg}+^{12}\mathrm{C}$ fusion reaction was used to perform a detailed $\ensuremath{\gamma}$-ray spectroscopy study of the astrophysically important nucleus $^{34}\mathrm{Ar}$. In particular, an experimental setup, coupling the advanced $\ensuremath{\gamma}$-ray tracking array GRETINA with the well-established Argonne fragment mass analyzer (FMA), was employed to obtain excitation energies and spin-parity assignments for excited states in $^{34}\mathrm{Ar}$, both above and below the proton separation energy. For the first time, an angular distribution analysis of in-beam $\ensuremath{\gamma}$ rays from fusion-evaporation reactions, using a tracking array, has been performed and Coulomb energy differences of analog states in the $T=1,$ $A=34$ mirror system, explored from 0 to 6 MeV. Furthermore, we present a comprehensive discussion of the astrophysical $^{33}\mathrm{Cl}(p,\ensuremath{\gamma})$ stellar reaction rate, together with implications for the identification of nova presolar grains from sulfur isotopic abundances.

The ground-state properties of neutron-rich $^{106}\mathrm{Nb}$ and its $\ensuremath{\beta}$ decay into $^{106}\mathrm{Mo}$ have been studied using the CARIBU radioactive-ion-beam facility at Argonne National Laboratory. Niobium-106 ions were extracted from a $^{252}\mathrm{Cf}$ fission source and mass separated before being delivered as low-energy beams to the Canadian Penning Trap, as well as the X-Array and SATURN $\ensuremath{\beta}$-decay-spectroscopy station. The measured $^{106}\mathrm{Nb}$ ground-state mass excess of $\ensuremath{-}66202.0(13)$ keV is consistent with a recent measurement but has three times better precision; this work also rules out the existence of a second long-lived, $\ensuremath{\beta}$-decaying state in $^{106}\mathrm{Nb}$ above 5 keV in excitation energy. The decay half-life of $^{106}\mathrm{Nb}$ was measured to be 1.097(21) s, which is $8%$ longer than the adopted value. The level scheme of the decay progeny, $^{106}\mathrm{Mo}$, has been expanded up to $\ensuremath{\approx}4\phantom{\rule{4pt}{0ex}}\mathrm{MeV}$. The distribution of decay strength and considerable population of excited states in $^{106}\mathrm{Mo}$ of $J\ensuremath{\ge}3$ emphasizes the need to revise the adopted ${J}^{\ensuremath{\pi}}={1}_{}^{\ensuremath{-}}$ ground-state spin-parity assignment of $^{106}\mathrm{Nb}$; it is more likely to be $J\ensuremath{\ge}3$.

Isomeric states and associated collective structures have been studied up to high spin in $^{198,200,202}\mathrm{Hg}$ using multinucleon transfer reactions and the Gammasphere array. A coupled rotational band, with possible four-quasiparticle character, is established in $^{198}\mathrm{Hg}$. Sequences built on two-quasiparticle, positive- and negative-parity levels are assigned to $^{202}\mathrm{Hg}$. New isomers in $^{202}\mathrm{Hg}$ with ${I}^{\ensuremath{\pi}}=({7}^{\ensuremath{-}})$ and $({9}^{\ensuremath{-}})$, and ${T}_{1/2}$ = 10.4(4) ns and 1.4(3) ns, respectively, have been identified. A half-life of 1.0(3) ns is established for the ${I}^{\ensuremath{\pi}}={12}^{+}$ state in $^{200}\mathrm{Hg}$. $B(E2)$ values deduced from isomeric transitions in Hg isotopes indicate that, while collectivity near the ground state gradually diminishes from $N$ = 112 to $N$ = 124, it is found to increase for the ${12}^{+}$ and ${9}^{\ensuremath{-}}$ states up to $N$ = 118, followed by a reduction for higher neutron numbers. Calculations using the ultimate cranker code provide insight into the variation of deformation with spin and allow for an understanding of observed band crossings. The evolution of collectivity with spin, and along the isotopic chain, is described.

The region of neutron-rich Cr isotopes has garnered much attention in recent years due to a rapid onset of collectivity near neutron number $N=40$. We report here on the first $\ensuremath{\gamma}$-ray spectroscopy beyond the $({4}_{1}^{+})$ state in $^{62,64}\mathrm{Cr}$, using nucleon removal reactions from several projectiles within a rare-isotope beam cocktail. A candidate for the ${6}^{+}$ state in $^{64}\mathrm{Cr}$ is presented as well as one for, possibly, the second excited ${0}^{+}$ state in $^{62}\mathrm{Cr}$. The results are discussed in comparison to the LNPS shell-model predictions that allow for neutron excitations across the $N=40$ harmonic oscillator gap into the ${g}_{9/2}$ and ${d}_{5/2}$ orbitals. The calculated level schemes for $^{62,64}\mathrm{Cr}$ reveal intriguing collective structures. From the predicted neutron particle-hole character of the low-lying states in these Cr isotopes, $^{62}\mathrm{Cr}$ emerges as a transitional system on the path to the center of the $N=40$ island of inversion.

Author(s): Morse, C; MacChiavelli, AO; Crawford, HL; Zhu, S; Wu, CY; Wang, YY; Meng, J; Back, BB; Bucher, B; Campbell, CM; Carpenter, MP; Chen, J; Clark, RM; Cromaz, M; Fallon, P; Henderson, J; Janssens, RVF; Jones, MD; Khoo, TL; Kondev, FG; Lauritsen, T; Lee, IY; Li, J; Potterveld, D; Santamaria, C; Savard, G; Seweryniak, D; Stolze, S; Weisshaar, D | Abstract: The neutron-rich barium nuclei have been the subject of intense interest due to the enhanced octupole correlations they are predicted to exhibit. The observation of enhanced octupole collectivity in Ba144,146 as measured in sub-barrier Coulomb excitation, consistent with static octupole deformation, has further heightened this interest. In the present work, these studies are extended to the neighboring odd-mass Ba143 to investigate the interplay between single-particle and collective octupole degrees of freedom. A new measurement of the first 92 - state lifetime is also presented. Reflection-Asymmetric Triaxial Particle Rotor Model calculations indicate that the negative-parity bands in Ba143 can be understood as a decoupled structure of νh9/2 parentage, while the positive-parity bands are built on a decoupled octupole phonon. No evidence for E3 excitation is observed in this work, but an upper limit is placed on the E3 matrix element to the lowest octupole band.

The fusion-evaporation reaction 28Si + 40Ca at 122 MeV beam energy was used to populate high-spin states in the odd-odd N = Z nucleus 62Ga. With the combination of the Gammasphere spectrometer and the Microball CsI(Tl) charged-particle detector array the decay scheme of 62Ga was extended beyond 10 MeV excitation energy. The onset of band structures was observed. These high-spin rotational states are interpreted and classified by means of cranked Nilsson-Strutinsky calculations.

Excited states in $^{160}\mathrm{Gd}$ were populated via $\ensuremath{\beta}$ decay from the low- and high-spin isomers in $^{160}\mathrm{Eu}$. The high-spin, ${K}^{\ensuremath{\pi}}={5}^{\ensuremath{-}}$ state feeds several two-quasiparticle levels, as well as a sequence associated with a $\ensuremath{\gamma}$ vibration and a ${K}^{\ensuremath{\pi}}={4}^{+}$, hexadecapole vibrational structure. The decay scheme was significantly improved with the observation of new transitions and states when compared with the two competing level schemes from over four decades ago. Configuration assignments for some of the multiquasiparticle levels have been suggested, based upon decay properties, systematics from neighboring nuclei, and comparisons with theoretical calculations. In addition, 15 new low-spin states and approximately 60 new transitions were observed resulting from the decay of the low-spin $^{160}\mathrm{Eu}$ isomer.

A previous study of symmetric collisions of massive nuclei has shown that current models of multinucleon transfer (MNT) reactions do not adequately describe the transfer product yields. To gain further insight into this problem, we have measured the yields of MNT products in the interaction of 977 ($E/A=4.79$ MeV) and 1143 MeV ($E/A=5.60$ MeV) $^{204}\mathrm{Hg}$ with $^{208}\mathrm{Pb}$. We find that the yield of multinucleon transfer products are similar in these two reactions and are substantially lower than those observed in the reaction of 1257 MeV ($E/A=6.16$ MeV) $^{204}\mathrm{Hg}+^{198}\mathrm{Pt}$. We compare our measurements with the predictions of the GRAZING-F, dinuclear systems (DNS), and improved quantum molecular dynamics (ImQMD) models. For the observed isotopes of the elements Au, Hg, Tl, Pb, and Bi, the measured values of the MNT cross sections are orders of magnitude larger than the predicted values. Furthermore, the various models predict the formation of nuclides near the $N=126$ shell, which are not observed.

Author(s): Elman, B; Gade, A; Janssens, RVF; Ayangeakaa, AD; Bazin, D; Belarge, J; Bender, PC; Brown, BA; Campbell, CM; Carpenter, MP; Crawford, HL; Crider, BP; Fallon, P; Forney, AM; Harker, J; Liddick, SN; Longfellow, B; Lunderberg, E; Prokop, CJ; Sethi, J; Taniuchi, R; Walters, WB; Weisshaar, D; Zhu, S | Abstract: The neutron-rich Ni isotopes have attracted attention in recent years because of the occurrence of shape or configuration coexistence. We report on the difference in population of excited final states in Ni70 following γ-ray tagged one-proton, one-neutron, and two-proton knockout from Cu71, Ni71, and Zn72 rare-isotope beams, respectively. Using variations observed in the relative transition intensities, signaling the changed population of specific final states in the different reactions, the role of neutron and proton configurations in excited states of Ni70 is probed schematically, with the goal of identifying those that carry, as leading configuration, proton excitations across the Z=28 shell closure. Such states are suggested in the literature to form a collective structure associated with prolate deformation. Adding to the body of knowledge for Ni70, 29 new transitions are reported, of which 15 are placed in its level scheme.

The decay of $K$ isomers in Cm ($Z$ = 96) isotopes has been studied using inelastic and transfer reactions. The half-life of a previously identified 2-quasiparticle (qp) ${K}^{\ensuremath{\pi}}={8}^{\ensuremath{-}}$ isomer in $^{246}\mathrm{Cm}$ has been measured. A new 2-qp isomer is observed in $^{248}\mathrm{Cm}$, its half-life measured and its decay scheme established. The reduced $K$ hindrances extracted for the decay transitions from the isomers in $^{246,248}\mathrm{Cm}$ indicate $K$ to be a robust quantum number and validate axial symmetry in these nuclei. The excitation energies of the 2-qp isomers in $^{246}\mathrm{Cm}$ ($N$ = 150) and $^{248}\mathrm{Cm}$ ($N$ = 152) support the persistence of a deformed subshell gap at $N$ = 152 in the $Z\ensuremath{\approx}100$ region down to $Z$ = 96 nuclei.

The structure of decoupled positive-parity and semidecoupled negative-parity bands up to high spin in $^{197,199}\mathrm{Hg}$ has been studied using multinucleon transfer reactions with the Gammasphere array. A positive-parity band in $^{199}\mathrm{Hg}$ with the ${(\ensuremath{\nu}{i}_{13/2})}^{3}$ decoupled configuration that deexcites to levels in the negative-parity sequences is newly established. The semidecoupled sequences in both isotopes are extended to higher spin. Rotation-aligned angular momenta and crossing frequencies determined from experiment are in fair agreement with those from cranking calculations. A transition from oblate collective rotation at low spin to triaxial noncollective shapes at high spin is indicated.

The structure of the odd-$A$ isotopes $^{193,195,197}\mathrm{Pt}$, which lie along the line of stability, has been studied up to high spin through multinucleon transfer reactions. Positive- and negative-parity sequences in $^{193,195}\mathrm{Pt}$ have been considerably extended and multiple band crossings established. An isomer with ${T}_{1/2}=5.0(5)$ ns and ${I}^{\ensuremath{\pi}}=25/{2}^{\ensuremath{-}}$ is present in $^{195}\mathrm{Pt}$. The isotopes $^{193,195}\mathrm{Pt}$ are characterized by moderate oblate deformation, and angular momentum generation at high spin in the yrast, positive-parity sequences is attributed to the rotation alignment of ${i}_{13/2}$ neutrons and ${h}_{11/2}$ protons. A detailed understanding of the observed features is presented using calculations based on tilted axis cranking covariant density functional theory as well as others with the ultimate cranker code.

Garrett et al. systematically investigated band-crossing frequencies resulting from the rotational alignment of the first pair of i13/2 neutrons (AB) in rare-earth nuclei. In that study, evidence was found for an odd-even neutron number dependence attributed to changes in the strength of neutron pairing correlations. The present paper carries out a similar investigation at higher rotational frequencies for the second pair of aligning i13/2 neutrons (BC). Again, a systematic difference in band-crossing frequencies is observed between odd-N and even-N Er, Yb, Hf, and W nuclei, but in the BC case, it is opposite to the AB neutron-number dependence. These results are discussed in terms of a reduction of neutron pairing correlations at high rotational frequencies and of the effects of Pauli blocking on the pairing field by higher-seniority configurations. Also playing a significant role are the changes in deformation with proton and neutron numbers, the changes in location of single-particle orbitals as a function of quadrupole deformation, and the position of the Fermi surface with regard to the various ω components of the neutron i13/2 shell.

The yields of 42 projectile-like fragments (PLFs) and fission fragments and 36 target-like fragments (TLFs) were measured using off-line $\ensuremath{\gamma}$-ray spectroscopy in a thin target experiment involving the $^{136}\mathrm{Xe}+^{198}\mathrm{Pt}$ reaction. The center of target beam energy was 760.5 MeV $({\mathrm{E}}_{\mathrm{c}.\mathrm{m}.}=450$ MeV). The reported yields are compared with those from previous measurements for this reaction and with predictions of the GRAZING, di-nuclear systems (DNS), and improved quantum molecular dynamics (ImQMD) models. The yields of the TLFs and PLFs are, in general, substantially smaller than those previously observed at a beam energy of 1085 MeV. Neither the GRAZING nor the DNS model correctly describes the measured TLF and PLF yields in this lower- energy reaction but the ImQMD model describes these yields adequately.

Excited states of $^{202}\mathrm{Hg}$ have been studied via the $^{12}\mathrm{C}(^{202}\mathrm{Hg},^{202}\mathrm{Hg}^{*})$ Coulomb excitation reaction at a beam energy of 890 MeV. The $\ensuremath{\gamma}$-ray transitions from the excited states of $^{202}\mathrm{Hg}$ were detected by the Gammasphere array. The intensities of the observed $\ensuremath{\gamma}$ rays determined the relative populations of the excited states which were used to extract the absolute $M1$ and $E2$ transition strength distributions for excited ${2}^{+}$ states of $^{202}\mathrm{Hg}$ up to 2 MeV. The measured absolute $B(M1;{2}_{7}^{+}\ensuremath{\rightarrow}{2}_{1}^{+})$ strength of $0.18(8){\ensuremath{\mu}}_{\mathrm{N}}^{2}$ indicates that the ${2}_{7}^{+}$ level of $^{202}\mathrm{Hg}$ is the main fragment of the proton-neutron mixed-symmetry ${2}_{1,\mathrm{ms}}^{+}$ state. Upper limits for the $F$-spin mixing matrix elements of ${}^{202,204}\mathrm{Hg}$ are determined as well.

Excited states in the neutron-rich 70 Fe nucleus were populated in a one-proton removal reaction from 71 Co projectiles at 87 MeV/nucleon. A new transition was observed with the γ -ray tracking array GRETINA and shown to feed the previously assigned 4+ 1 state. In comparison to reaction theory calculations with shell-model spectroscopic factors, it is argued that the new γ ray possibly originates from the 6+ 1 state. It is further shown that the Doppler-reconstructed γ -ray spectra are sensitive to the very different lifetimes of the 2+ and 4+ states, enabling their approximate measurement. The emerging structure of 70 Fe is discussed in comparison to LNPS-new large-scale shell-model calculations.

As zirconium gains neutrons, its nucleus morphs in shape---changing from a soccer ball to an American football---and researchers have found the exact moment of the transition.

Yrast and near-yrast levels up to an I=17ℏ spin value and a 6-MeV excitation energy have been delineated in the “two-neutron” 210Pb nucleus following deep-inelastic reactions involving 208Pb targets and a number of heavy-ion beams at energies ∼25% above the Coulomb barrier. The level scheme was established on the basis of multifold prompt and delayed coincidence relationships measured with the Gammasphere array. In addition to the previously known states, many new levels were identified. For most of the strongly populated states, spin-parity assignments are proposed on the basis of angular distributions. The reinvestigation of the ν(g9/2)2, 8+ isomeric decay results in the firm identification of the low-energy E2 transitions involved in the 8+→6+→4+ cascade, and in a revised 6+ level half-life of 92(10) ns, nearly a factor of 2 longer than previously measured. Among the newly identified states figure spin I=4–10ℏ levels associated with the νg9/2i11/2 multiplet, as well as yrast states involving νg9/2j15/2, νi11/2j15/2, and ν(j15/2)2 neutron couplings. The highest-spin excitations are understood as 1p−1h core excitations and the yrast population is found to be fragmented to the extent that levels of spin higher than I=17ℏ could not be reached. Four E3 transitions are present in the 210Pb yrast decay; three of these involve the g9/2→j15/2 octupole component, as reflected in the 21(2) and >10 Weisskopf unit enhancements of the B(E3) rates of the first two. The fourth, 16+→13−E3 transition corresponds to the 3− core octupole excitation built on the νi11/2j15/2 state, in analogy to a similar E3 coupling to the νj15/2 level in 209Pb. Shell-model calculations performed for two-neutron states and 1p−1h 208Pb core excitations are in good agreement with the data. Evidence was found for the existence of a hitherto unknown high-spin β-decaying isomer in 210Tl. Shell-model calculations of the 210Tl levels suggest the possibility of a 11+ long-lived, β-decaying state, and the delayed yields observed in various reactions fit rather well with a 210Tl assignment.

The energy levels and γ-ray decay scheme of the positive-parity states in the Tz=12 nucleus As67 have been studied by using the Ca40(Ar36,2αp)As67 reaction at a beam energy of 145 MeV. Two new band structures have been identified which can be connected to the previously known levels. The results for these bands are compared with configuration-dependent cranked Nilsson-Strutinsky calculations. The good level of agreement between theory and experiment suggests that these structures can be interpreted in terms of configurations that involve three g92 particles and that both possess noncollective terminating states.

Excited states in $^{137}\mathrm{Cs}$ have been studied by using the near-barrier, single-proton transfer reaction $^{10}\mathrm{B}(^{136}\mathrm{Xe},\phantom{\rule{4pt}{0ex}}^{9}\mathrm{Be}\ensuremath{\gamma})^{137}\mathrm{Cs}$ in inverse kinematics and performing particle-$\ensuremath{\gamma}$ and particle-$\ensuremath{\gamma}\ensuremath{\gamma}$ coincidence measurements. The low-spin level scheme of $^{137}\mathrm{Cs}$ has been augmented: (i) The expected set of single-proton, seniority $\ensuremath{\upsilon}=1$ states has been delineated in its entirety; (ii) Another member of the $\ensuremath{\upsilon}=3$ proton $0{g}_{7/2}$ multiplet, a low-lying $9/{2}^{+}$ level, has been identified and this set of states now approaches completion; (iii) A second $9/{2}^{+}$ and a candidate $13/{2}^{+}$ level have been observed. The results are discussed in the framework of shell-model calculations in the proton $2s1d0g0h$ shell.

Author(s): Lubna, RS; Tripathi, V; Tabor, SL; Tai, PL; Kravvaris, K; Bender, PC; Volya, A; Bouhelal, M; Chiara, CJ; Carpenter, MP; Janssens, RVF; Lauritsen, T; McCutchan, EA; Zhu, S; Clark, RM; Fallon, P; MacChiavelli, AO; Paschalis, S; Petri, M; Reviol, W; Sarantites, DG | Abstract: Excited states in the neutron-rich isotopes P33 and P34 were populated by the O18+O18 fusion-evaporation reaction at Elab=24 MeV. The Gammasphere array was used along with the Microball particle detector array to detect γ transitions in coincidence with the charged particles emitted from the compound nucleus S36. The use of Microball enabled the selection of the proton emission channel. It also helped in determining the exact position and energy of the emitted proton; this was later employed in kinematic Doppler corrections. 16 new transitions and 13 new states were observed in P33 and 21 γ rays and 20 energy levels were observed in P34 for the first time. The nearly 4π geometry of Gammasphere allowed the measurement of γ-ray angular distributions leading to spin assignments for many states. The experimental observations for both isotopes were interpreted with the help of shell-model calculations using the (0+1)ω PSDPF interaction. The calculations accounted for both the 0p-0h and 1p-1h states reasonably well and indicated that 2p-2h excitations might dominate the higher-spin configurations in both P33 and P34.

Author(s): Jones, MD; MacChiavelli, AO; Wiedeking, M; Bernstein, LA; Crawford, HL; Campbell, CM; Clark, RM; Cromaz, M; Fallon, P; Lee, IY; Salathe, M; Wiens, A; Ayangeakaa, AD; Bleuel, DL; Bottoni, S; Carpenter, MP; Davids, HM; Elson, J; Gorgen, A; Guttormsen, M; Janssens, RVF; Kinnison, JE; Kirsch, L; Larsen, AC; Lauritsen, T; Reviol, W; Sarantites, DG; Siem, S; Voinov, AV; Zhu, S | Abstract: A model-independent technique was used to determine the γ-ray strength function (γSF) of Fe56 down to γ-ray energies less than 1 MeV for the first time with GRETINA using the (p,p′) reaction at 16 MeV. No difference was observed in the energy dependence of the γSF built on 2+ and 4+ final states, supporting the Brink hypothesis. In addition, angular distribution and polarization measurements were performed. The angular distributions are consistent with dipole radiation. The polarization results show a small bias towards magnetic character in the region of the enhancement.

Background: The $^{31}\mathrm{S}(p,\ensuremath{\gamma})\phantom{\rule{0.16em}{0ex}}^{32}\mathrm{Cl}$ reaction becomes important for sulfur production in novae if the $^{31}\mathrm{P}(p,\ensuremath{\alpha})^{28}\mathrm{Si}$ reaction rate is somewhat greater than currently accepted. The rate of the $^{31}\mathrm{S}(p,\ensuremath{\gamma})\phantom{\rule{0.16em}{0ex}}^{32}\mathrm{Cl}$ reaction is uncertain, primarily due to the properties of resonances at ${E}_{\mathrm{c}.\mathrm{m}.}=156$ and 549 keV.Purpose: We precisely determined the excitation energies of states in $^{32}\mathrm{Cl}$ through high-resolution $\ensuremath{\gamma}$ spectroscopy including the two states most important for the $^{31}\mathrm{S}(p,\ensuremath{\gamma})\phantom{\rule{0.16em}{0ex}}^{32}\mathrm{Cl}$ reaction at nova temperatures.Method: Excited states in $^{32}\mathrm{Cl}$ were populated using the $^{10}\mathrm{B}(^{24}\mathrm{Mg},2n)\phantom{\rule{0.16em}{0ex}}^{32}\mathrm{Cl}$ reaction with a $^{24}\mathrm{Mg}$ beam from the ATLAS facility at Argonne National Laboratory. The reaction channel of interest was selected using recoils in the Fragment Mass Analyzer, and precise level energies were determined by detecting $\ensuremath{\gamma}$ rays with Gammasphere.Results: We observed $\ensuremath{\gamma}$ rays from the decay of six excited states in $^{32}\mathrm{Cl}$. The excitation energies for two unbound levels at ${E}_{x}=1738.1$ (6) keV and 2130.5 (10) keV were determined and found to be in agreement with a previous high-precision measurement of the $^{32}\mathrm{S}(^{3}\mathrm{He},t)^{32}\mathrm{Cl}$ reaction [1].Conclusions: An updated $^{31}\mathrm{S}(p,\ensuremath{\gamma})\phantom{\rule{0.16em}{0ex}}^{32}\mathrm{Cl}$ reaction rate is presented. With the excitation energies of important levels firmly established, the dominant uncertainty in the reaction rate at nova temperatures is due to the strength of the resonance corresponding to the 2131-keV state in $^{32}\mathrm{Cl}$.

The Si31 nucleus was produced through the O18(O18, αn) fusion-evaporation reaction at Elab=24MeV. Evaporated α particles from the reaction were detected and identified in the Microball detector array for channel selection. Multiple γ-ray coincidence events were detected in Gammasphere. The energy and angle information for the α particles was used to determine the Si31 recoil kinematics on an event-by-event basis for a more accurate Doppler correction. A total of 22 new states and 52 new γ transitions were observed, including 14 from states above the neutron separation energy. The positive-parity states predicted by the shell-model calculations in the sd model space agree well with experiment. The negative-parity states were compared with shell-model calculations in the psdpf model space with some variations in the N=20 shell gap. The best agreement was found with a shell gap intermediate between that originally used for A≈20 nuclei and that previously adapted for P32,34. This variation suggests the need for a more universal cross-shell interaction.

Excited states in Re186 with spins up to J=12 were investigated in two separate experiments using W186(d,2n) reactions at beam energies of 12.5 and 14.5 MeV. Two- and threefold γ-ray coincidence data were collected using the CAESAR and CAGRA spectrometers, respectively, each composed of Compton-suppressed high-purity germanium detectors. Analysis of the data revealed rotational bands built on several two-quasiparticle intrinsic states, including a long-lived Kπ=(8+) isomer. Configuration assignments were supported by an analysis of in-band properties, such as gK-gR values. The excitation energies of the observed intrinsic states were compared with results from multi-quasiparticle blocking calculations, based on the Lipkin-Nogami pairing approach, that included contributions from the residual proton-neutron interactions.

The calcium isotopes have emerged as a critical testing ground for new microscopically derived shell-model interactions, and a great deal of experimental and theoretical focus has been directed toward this region. We investigate the relative spectroscopic strengths associated with 1f7/2 neutron hole states in Ca47,49 following one-neutron knockout reactions from Ca48,50. The observed reduction of strength populating the 7/21- state in Ca49, as compared to Ca47, is inconsistent with shell-model calculations using both phenomenological interactions such as GXPF1, and interactions derived from microscopically based two- and three-nucleon forces. The result suggests a fragmentation of the l=3 strength to higher-lying states as suggested by the microscopic calculations, but the observed magnitude of the reduction is not reproduced in any shell-model description.

The nucleus ${}^{208}$Pb provides an iconic test of the nuclear shell model because its 82 protons and 126 neutrons are both magic numbers. When excited levels are discovered and characterized, this nucleus provides a means to investigate the mechanisms responsible for the generation of angular momentum and, ultimately, for the development of collectivity. This experiment is a tour de force that reveals extensive new information on ${}^{208}$Pb about high-angular-momentum states, isomeric states, and collective states of octupole nature; thus it serves as a showcase for shell-model descriptions. Many of the states explored show good overall agreement with theory, but others at the highest energies reveal discrepancies, pointing to the need for improved calculations. Above the highest-lying ${28}^{-}$ isomer $\ensuremath{\gamma}$ transitions arising from yet higher spin levels could be identified in two separate experiments as displayed in the figure.

Excited states have been observed for the first time in the neutron-deficient nucleus $^{117}\mathrm{Ba}$ using the recoil-decay tagging technique following the heavy-ion fusion-evaporation reaction $^{64}\mathrm{Zn}$($^{58}\mathrm{Ni}$, 2p3n)$^{117}\mathrm{Ba}$. Prompt $\ensuremath{\gamma}$ rays have been assigned to $^{117}\mathrm{Ba}$ through correlations with $\ensuremath{\beta}$-delayed protons following the decay of $A=117$ recoils. Through the analysis of the $\ensuremath{\gamma}\ensuremath{-}\ensuremath{\gamma}$ coincidence relationships, a high-spin level scheme consisting of two bands has been established in $^{117}\mathrm{Ba}$. Based on the systematics of the level spacings in the neighboring barium isotopes, the two bands are proposed to have $\ensuremath{\nu}{h}_{11/2}[532]5/{2}^{\ensuremath{-}}$ and $\ensuremath{\nu}{d}_{5/2}[413]5/{2}^{+}$ configurations, respectively. The observed band-crossing properties are interpreted in the framework of cranked shell model.

States in $^{209}\mathrm{Tl}$ were populated using a multinucleon transfer reaction with a $^{136}\mathrm{Xe}$ beam impinging on a thick $^{208}\mathrm{Pb}$ target at $E=785$ MeV. The beam was pulsed at 825-ns intervals in order to perform isomer decay spectroscopy. The known ${J}^{\ensuremath{\pi}}=17/{2}^{+}$ isomer in $^{209}\mathrm{Tl}$ was located at 1228(4) keV and measured to have a half-life of ${T}_{1/2}=146(10)$ ns. A second isomer with ${J}^{\ensuremath{\pi}}=13/{2}^{+}$ was found to have ${T}_{1/2}=14(5)$ ns. The previously suggested low-energy X and Y transitions were found to have energies 57(2) and 47(2) keV respectively, while the measurement of conversion coefficients and a new decay path make the spin assignments below the isomers experimentally firm. Correlating the delayed $\ensuremath{\gamma}$ transitions with the prompt beam flash allowed the decay of states above the isomer to be found. The longer-lived isomer represents full alignment of the simplest two-particle, one-hole configuration and illuminates the remarkably weak coupling of the proton hole to the $^{210}\mathrm{Pb}$ core.

Multi-quasiparticle high-K states, several of which are isomeric, were observed in Hf-180 with the Gammasphere array. We determined the lifetimes in the ns-μs range using centroid-shift and decay measurements within a mu s coincidence time window. The configurations of high-K states involve two and four quasiparticles, with states up to Kπ = (18-) established. High-K excitations are found to be progressively more favored with increasing excitation energy. The K quantum number is quite robust up to the highest spins observed, as evidenced by the large values of the reduced hindrance for isomeric decays. Furthermore, rotational bands built on three high-K states are identified, and the measured branching ratios in these sequences enable the assignment of underlying configurations. Multi-quasiparticle calculations using the Lipkin-Nogami approach for pairing, with blocking included, reproduce the observed high-K energies quite well.

The first rotational sequences have been assigned to the odd-odd nucleus $^{168}\mathrm{Re}$. Coincidence relationships of these structures with rhenium x rays confirm the isotopic assignment, while arguments based on the $\ensuremath{\gamma}$-ray multiplicity ($K$-fold) distributions observed with the new bands lead to the mass assignment. Configurations for the two bands were determined through analysis of the rotational alignments of the structures and a comparison of the experimental $B(M1)/B(E2)$ ratios with theory. Tentative spin assignments are proposed for the $\ensuremath{\pi}{h}_{11/2}\ensuremath{\nu}{i}_{13/2}$ band, based on energy level systematics for other known sequences in neighboring odd-odd rhenium nuclei, as well as on systematics seen for the signature inversion feature that is well known in this region. The spin assignment for the $\ensuremath{\pi}{h}_{11/2}\ensuremath{\nu}({h}_{9/2}/{f}_{7/2})$ structure provides additional validation of the proposed spins and configurations for isomers in the $^{176}\mathrm{Au} \ensuremath{\rightarrow} ^{172}\mathrm{Ir}\ensuremath{\rightarrow}^{168}\mathrm{Re} \ensuremath{\alpha}$-decay chain.

The distribution of single-particle strength in 67,69Ni was characterized with one-neutron knockout reactions from intermediate-energy 68,70Ni secondary beams, selectively populating neutron-hole configurations at N = 39 and 41, respectively. The spectroscopic strengths deduced from the measured partial cross sections to the individual final states, as tagged by their γ-ray decays, are used to identify and quantify neutron configurations in the wave functions. While 69Ni compares well to shell-model predictions, the results for 67Ni challenge the validity of current effective shell-model Hamiltonians by revealing discrepancies that cannot be explained so far. These results suggest that our understanding of the low-lying states in the neutron-rich, semi-magic Ni isotopes may be incomplete and requires further investigation on both the experimental and theoretical sides.