1. Competing effects of Mn and Y doping on the low-energy excitations and phase diagram ofLa1−yYyFe1−xMnxAsO0.89F0.11iron-based superconductors
- Author
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R. De Renzi, Toni Shiroka, Sabine Wurmehl, M. Moroni, M. A. Afrassa, A. U. B. Wolter, G. Lamura, R. Kappenberger, Bernd Büchner, Samuele Sanna, and Pietro Carretta
- Subjects
Physics ,Superconductivity ,Condensed matter physics ,02 engineering and technology ,Muon spin spectroscopy ,021001 nanoscience & nanotechnology ,01 natural sciences ,Quantum critical point ,0103 physical sciences ,Content (measure theory) ,010306 general physics ,0210 nano-technology ,Ground state ,Spin (physics) ,Order of magnitude ,Phase diagram - Abstract
Muon spin rotation ($\ensuremath{\mu}\mathrm{SR}$) and $^{19}\mathrm{F}$ nuclear magnetic resonance (NMR) measurements were performed to investigate the effect of Mn for Fe substitutions in ${\mathrm{La}}_{1\ensuremath{-}y}{\mathrm{Y}}_{y}{\mathrm{Fe}}_{1\ensuremath{-}x}{\mathrm{Mn}}_{x}{\mathrm{AsO}}_{0.89}{\mathrm{F}}_{0.11}$ superconductors. While for $y=0$ a very low critical concentration of Mn ($x=0.2%$) is needed to quench superconductivity, as $y$ increases the negative chemical pressure introduced by Y for La substitution stabilizes superconductivity and for $y=20%$ it is suppressed at Mn contents an order of magnitude larger. A magnetic phase arises once superconductivity is suppressed both for $y=0$ and for $y=20%$. Low-energy spin fluctuations give rise to a peak in $^{19}\mathrm{F}$ NMR $1/{T}_{1}$ with an onset well above the superconducting transition temperature and whose magnitude increases with $x$. Also the static magnetic correlations probed by $^{19}\mathrm{F}$ NMR linewidth measurements show a marked increase with Mn content. The disruption of superconductivity and the onset of the magnetic ground state are discussed in the light of the proximity of ${\mathrm{LaFeAsO}}_{0.89}{\mathrm{F}}_{0.11}$ to a quantum critical point.
- Published
- 2016