1. Magnetically ordered and kagome quantum spin liquid states in the Zn-doped claringbullite series
- Author
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M. Georgopoulou, B. Fåk, D. Boldrin, J. R. Stewart, C. Ritter, E. Suard, J. Ollivier, and A. S. Wills
- Subjects
Condensed Matter - Strongly Correlated Electrons ,Strongly Correlated Electrons (cond-mat.str-el) ,FOS: Physical sciences - Abstract
Neutron scattering measurements have been performed on deuterated powder samples of claringbullite and Zn-doped claringbullite (Zn$_x$Cu$_{4-x}$(OD)$_{6}$FCl). At low temperatures, claringbullite Cu$_4$(OD)$_{6}$FCl forms a distorted pyrochlore lattice with long-range magnetic order and spin-wave-like magnetic excitations. Partial Zn doping leads to the nominal ZnCu$_3$(OD)$_{6}$FCl compound, a geometrically frustrated spin-1/2 kagome antiferromagnet that shows no transition to magnetic order down to 1.5 K. The magnetic excitations form a gapless continuum, a signature of fractional excitations in a quantum spin liquid., 8 pages, 5 figures, Supplemental Material
- Published
- 2023
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